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Kunal L. Tiwari

Publications and source records attributed to Kunal L. Tiwari.

7 recordsLinked to original sources

Characterization and Comparison of Energy Relaxation in Fluxonium Qubits

Fluxonium superconducting qubits have demonstrated long coherence times and high single- and two-qubit gate fidelities, making them a favorable building block for superconducting quantum processors. We investigate the dominant limitations to fluxonium qubit energy relaxation time $T_1$ using a set of eight planar, aluminum-on-silicon qubits. We find that a circuit-based model for capacitive dielectric loss best captures the frequency dependence of $T_1$, which we analyze within both a two-level and a six-level energy relaxation model. We convert the measured $T_1$ into an effective capacitive quality factor $Q_\mathrm{C}^{\mathrm{eff}}$ to compare qubits on equal footing, accounting for independently estimated contributions from $1/f$ flux noise and radiative loss to the control and readout circuitry. We apply this methodology to compare qubits from two fabrication processes: a baseline process and one that applies a fluorine-based wet treatment prior to Josephson junction deposition. We resolve a small improvement of (13.8 $\pm$ 8.4$)\%$ in the process mean $Q_\mathrm{C}^{\mathrm{eff}}$, indicating that the fluorine treatment may have reduced loss from the metal-substrate interface, but did not address the primary source of loss in these fluxonium qubits.

quant-ph

A spin-refrigerated cavity quantum electrodynamic sensor

Quantum sensors based on solid-state defects, in particular nitrogen-vacancy (NV) centers in diamond, enable precise measurement of magnetic fields, temperature, rotation, and electric fields. However, the sensitivity of leading NV spin ensemble sensors remains far from the intrinsic spin-projection noise limit. Here we move towards this quantum limit of performance by introducing (i) a cavity quantum electrodynamic (cQED) hybrid system operating in the strong coupling regime, which enables high readout fidelity of an NV ensemble using microwave homodyne detection; (ii) a comprehensive nonlinear model of the cQED sensor operation, including NV ensemble inhomogeneity and optical polarization; and (iii) ``spin refrigeration'' where the optically-polarized spin ensemble sharply reduces the ambient-temperature microwave thermal noise, resulting in enhanced sensitivity. Applying these advances to magnetometry, we demonstrate a broadband sensitivity of 580 fT/$\sqrt{\mathrm{Hz}}$ around 15 kHz in ambient conditions. We then discuss the implications of this model for design of future magnetometers, including devices approaching 12 fT/$\sqrt{\mathrm{Hz}}$ sensitivity. Applications of these techniques extend to the fields of gyroscope and clock technologies.

quant-ph

Tunable skyrmion-skyrmion binding on the surface of a topological insulator

We show that skyrmions on the surface of a magnetic topological insulator may experience an attractive interaction that leads to the formation of a skyrmion-skyrmion bound state. This is in contrast to the case of skyrmions in a conventional chiral ferromagnet, for which the intrinsic interaction is repulsive. The origin of skyrmion binding in our model is the molecular hybridization of topologically protected electronic orbitals associated with each skyrmion. Attraction between the skyrmions can therefore be controlled by tuning a chemical potential that populates/depopulates the lowest-energy molecular orbital. We find that the skyrmion-skyrmion bound state can be made stable, unstable, or metastable depending on the chemical potential, magnetic field, and easy-axis anisotropy of the underlying ferromagnet, resulting in a rich phase diagram. Finally, we discuss the possibility to realize this effect in a recently synthesized Cr doped ${\left(\mathrm{Bi}_{2-y}\mathrm{Sb}_{y}\right)}_{2}\mathrm{Te}_3$ heterostructure.

cond-mat.mes-hall

How optical excitation controls the structure and properties of vanadium dioxide

We combine ultrafast electron diffraction and time-resolved terahertz spectroscopy measurements to unravel the connection between structure and electronic transport properties during the photoinduced insulator-metal transitions in vanadium dioxide. We determine the structure of the metastable monoclinic metal phase, which exhibits anti-ferroelectric charge order arising from a thermally activated, orbital-selective phase transition in the electron system. The relative contribution of this photoinduced monoclinic metal (which has no equilibrium analog) and the photoinduced rutile metal (known from the equilibrium phase diagram) to the time and pump-fluence dependent multi-phase character of the film is established, as is the respective impact of these two distinct phase transitions on the observed changes in terahertz conductivity. Our results represent an important new example of how light can control the properties of strongly correlated materials and elucidate that multi-modal experiements are essential when seeking a detailed connection between ultrafast changes in optical-electronic properties and lattice structure in complex materials.

cond-mat.str-el

Magnetoconductance signatures of chiral domain-wall bound states in magnetic topological insulators

Recent magnetoconductance measurements performed on magnetic topological insulator candidates have revealed butterfly-shaped hysteresis. This hysteresis has been attributed to the formation of gapless chiral domain-wall bound states during a magnetic field sweep. We treat this phenomenon theoretically, providing a link between microscopic magnetization dynamics and butterfly hysteresis in magnetoconductance. Further, we illustrate how a spatially resolved conductance measurement can probe the most striking feature of the domain-wall bound states: their chirality. This work establishes a regime where a definitive link between butterfly hysteresis in longitudinal magneto-conductance and domain-wall bound states can be made. This analysis provides an important tool for the identification of magnetic topological insulators.

cond-mat.mes-hall

A photoinduced metallic phase of monoclinic vanadium dioxide

The complex interplay between several active degrees of freedom (charge, lattice, orbtial and spin order) is thought to determine the electronic properties of many oxides, but the respective role of the various contributions is often extremely difficult to determine. Vanadium dioxide (VO$_2$) is a particularly notorious example. Here we report on combined ultrafast electron diffraction (UED) and infrared transmissivity experiments in which we directly watch and separate the lattice and charge density reorganizations that are associated with the optically-induced semiconductor-metal transition (SMT) in VO$_2$. These studies have uncovered a previously unreported photoinduced transition to a metastable state with the periodic lattice distortion (PLD) characteristic of the insulator intact, but differing by a 1D rearrangement of charge density along the octahedrally coordinated vanadium dimer chains and a transition to metal-like mid IR optical properties. The results demonstrate that UED is capable of following details of both lattice and electronic structural dynamics on the ultrafast timescale.

cond-mat.str-el

Towards equilibration and thermalization between finite quantum systems: The role of dephasing effects and inelastic interactions

We demonstrate the approach towards a Gibbs-like equilibrium state, with a common temperature and a chemical potential, of two finite metallic grains, prepared with a different number of noninteracting electrons, connected by a weak link that is susceptible to incoherent and inelastic processes. By developing an analytic method and by using an exact numerical approach, the quantum time evolution of the electrons in the metallic grains is followed. In the absence of decoherring and inelastic effects, equilibration is never reached. Introducing dephasing effects on the link only, using a dephasing probe, the two quantum systems equilibrate, but do not evolve towards a Gibbs-like state. In contrast, by mimicking inelastic interactions with a voltage probe, the metal pieces evolve towards a common Gibbs-like equilibrium state, with the probe.

cond-mat.mes-hall