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Kyoung-Whan Kim

Publications and source records attributed to Kyoung-Whan Kim.

At least 37 records · Page 2Linked to original sources

Stability and dynamics of in-plane skyrmions in collinear ferromagnets

We study the emergence and dynamics of in-plane skyrmions in collinear ferromagnetic heterostructures. We present a minimal energy model for this class of magnetic textures, determine the crystal symmetries compatible with it and propose material candidates, based on symmetries only, for the observation of these topological solitons. We calculate exact solutions of the energy model for in-plane skyrmions in the absence of dipolar interactions at critical coupling, the latter defined by the relations $H = K$ and $D = \sqrt{AK}$ for the strength of the external magnetic field and the Dzyaloshinskii coupling constant, respectively, with $K$ and $A$ being the anisotropy constant and the exchange stiffness of the material. Through micromagnetic simulations, we demonstrate the possibility of in-plane skyrmion production via i) the motion of domain walls through a geometrical constriction and ii) shedding from a magnetic impurity driven both by spin-transfer torques. In-plane skyrmion dynamics triggered by spin-orbit torques are also investigated analytically and numerically. Our findings point towards the possibility of designing racetracks for in-plane skyrmions, whose speed could be tuned by adjusting the angle between the charge current and the uniform background magnetization; in particular, the speed is maximum for currents parallel to the easy axis and becomes zero for currents transverse to it.

cond-mat.mes-hall↗

Chiral magnetic interlayer coupling in synthetic antiferromagnets

The exchange coupling underlies ferroic magnetic coupling and is thus the key element that governs statics and dynamics of magnetic systems. This fundamental interaction comes in two flavors - symmetric and antisymmetric coupling. While symmetric coupling leads to ferro- and antiferromagnetism, antisymmetric coupling has attracted significant interest owing to its major role in promoting topologically non-trivial spin textures that promise high-speed and energy-efficient devices. So far, the antisymmetric exchange coupling rather short-ranged and limited to a single magnetic layer has been demonstrated, while the symmetric coupling also leads to long-range interlayer exchange coupling. Here, we report the missing component of the long-range antisymmetric interlayer exchange coupling in perpendicularly magnetized synthetic antiferromagnets with parallel and antiparallel magnetization alignments. Asymmetric hysteresis loops under an in-plane field unambiguously reveal a unidirectional and chiral nature of this novel interaction, which cannot be accounted for by existing coupling mechanisms, resulting in canted magnetization alignments. This can be explained by spin-orbit coupling combined with reduced symmetry in multilayers. This new class of chiral interaction provides an additional degree of freedom for engineering magnetic structures and promises to enable a new class of three-dimensional topological structures.

cond-mat.mtrl-sci↗

Prediction of ferroelectricity-driven Berry curvature enabling charge- and spin-controllable photocurrent in tin telluride monolayers

In symmetry-broken crystalline solids, pole structures of Berry curvature (BC) can emerge, and they have been utilized as a versatile tool for controlling transport properties. For example, the monopole component of the BC is induced by the time-reversal symmetry breaking, and the BC dipole arises from a lack of inversion symmetry, leading to the anomalous Hall and nonlinear Hall effects, respectively. Based on first-principles calculations, we show that the ferroelectricity in a tin telluride monolayer produces a unique BC distribution, which offers charge- and spin-controllable photocurrents. Even with the sizable band gap, the ferroelectrically driven BC dipole is comparable to those of small-gap topological materials. By manipulating the photon handedness and the ferroelectric polarization, charge and spin circular photogalvanic currents are generated in a controllable manner. The ferroelectricity in group-IV monochalcogenide monolayers can be a useful tool to control the BC dipole and the nonlinear optoelectronic responses.

cond-mat.mes-hall↗

Intrinsic origin of interfacial second-order magnetic anisotropy in ferromagnet/normal metal heterostructures

Interfacial perpendicular magnetic anisotropy, which is characterized by the first-order (K1) and second-order (K2) anisotropies, is the core phenomenon for nonvolatile magnetic devices. A sizable K2 satisfying a specific condition stabilizes the easy-cone state, where equilibrium magnetization forms at an angle from the film normal. The easy-cone state offers intriguing possibilities for advanced spintronic devices and unique spin textures, such as spin superfluids and easy-cone domain walls. Experimental realization of the easy-cone state requires understanding the origin of K2, thereby enhancing K2. However, previously proposed origins of K2 cannot fully account for experimental results. Here we show experimentally that K2 scales almost linearly with the work-function difference between the Co and X layers in Pt/Co/X heterostructures (X = Pd, Cu, Pt, Mo, Ru, W, and Ta), suggesting the central role of the inversion asymmetry in K2. Our result provides a guideline for enhancing K2 and realizing magnetic applications based on the easy-cone state.

cond-mat.mtrl-sci↗

Spin transparency for an interface of an ultrathin magnet within the spin dephasing length

We examine a modified drift-diffusion formalism to describe spin transport near an ultrathin magnet whose thickness is similar to or less than the spin dephasing length. Most of the previous theories on spin torque assume the transverse component of a injected spin current dephases perfectly thus are fully absorbed into the ferromagnet. However, in the state-of-art multilayer systems under consideration of recent studies, the thicknesses of ferromagnets are on the order of or less than a nanometer, thus one cannot safely assume the spin dephasing to be perfect. To describe the effects of a finite dephasing rate, we adopt the concept of transmitted mixing conductance, whose application to the drift-diffusion formalism has been limited. For a concise description of physical consequences, we introduce an effective spin transparency. Interestingly, for an ultrathin magnet with a finite dephasing rate, the spin transparency can be even enhanced and there arises a non-negligible field-like spin-orbit torque even in the absence of the imaginary part of the spin mixing conductance. The effective spin transparency provides a simple extension of the drift-diffusion formalism, which is accessible to experimentalists analyzing their results.

cond-mat.mes-hall↗

Topological characterization of classical waves: the topological origin of magnetostatic surface spin waves

We propose a topological characterization of Hamiltonians describing classical waves. Applying it to the magnetostatic surface spin waves that are important in spintronics applications, we settle the speculation over their topological origin. For a class of classical systems that includes spin waves driven by dipole-dipole interactions, we show that the topology is characterized by vortex lines in the Brillouin zone in such a way that the symplectic structure of Hamiltonian mechanics plays an essential role. We define winding numbers around these vortex lines and identify them to be the bulk topological invariants for a class of semimetals. Exploiting the bulk-edge correspondence appropriately reformulated for these classical waves, we predict that surface modes appear but not in a gap of the bulk frequency spectrum. This feature, consistent with the magnetostatic surface spin waves, indicates a broader realm of topological phases of matter beyond spectrally gapped ones.

cond-mat.mes-hall↗

Enhanced perpendicular magnetocrystalline anisotropy energy in an artificial magnetic material with bulk spin-momentum coupling

We systematically investigate the perpendicular magnetocrystalline anisotropy (MCA) in Co$-$Pt/Pd-based multilayers. Our magnetic measurement data shows that the asymmetric Co/Pd/Pt multilayer has a significantly larger perpendicular magnetic anisotropy (PMA) energy compared to the symmetric Co/Pt and Co/Pd multilayer samples. We further support this experiment by first principles calculations on the CoPt$_2$, CoPd$_2$, and CoPtPd, which are composite bulk materials that consist of three atomic layers in a unit cell, Pt/Co/Pt, Pd/Co/Pd, Pt/Co/Pd, respectively. By estimating the contribution of bulk spin-momentum coupling to the MCA energy, we show that the CoPtPd multilayer with the symmetry breaking has a significantly larger perpendicular magnetic anisotropy (PMA) energy than the other multilayers that are otherwise similar but lack the symmetry breaking. This observation thus provides an evidence of the PMA enhancement due to the structural inversion symmetry breaking and highlights the asymmetric CoPtPd as the first artificial magnetic material with bulk spin-momentum coupling, which opens a new pathway toward the design of materials with strong PMA.

cond-mat.mtrl-sci↗

Unidirectional Magnon-Driven Domain Wall Motion Due to the Interfacial Dzyaloshinskii-Moriya Interaction

We demonstrate a unidirectional motion of a quasiparticle without an explicit symmetry breaking along the space-time coordinate of the particle motion. This counterintuitive behavior originates from a combined action of two intrinsic asymmetries in the other two directions. We realize this idea with the magnon-driven motion of a magnetic domain wall in thin films with interfacial asymmetry. Contrary to previous studies, the domain wall moves along the same direction regardless of the magnon-flow direction. Our general symmetry analysis and numerical simulation reveal that the odd order contributions from the interfacial asymmetry is unidirectional, which is dominant over bidirectional contributions in the realistic regime. We develop a simple analytic theory on the unidirectional motion, which provides an insightful description of this counterintuitive phenomenon.

cond-mat.mes-hall↗

Asymmetric skyrmion Hall effect in systems with a hybrid Dzyaloshinskii-Moriya interaction

We examine the current-induced dynamics of a skyrmion that is subject to both structural and bulk inversion asymmetry. There arises a hybrid type of Dzyaloshinskii-Moriya interaction (DMI) which is in the form of a mixture of interfacial and bulk DMIs. Examples include crystals with symmetry classes C$_n$ as well as magnetic multilayers composed of a ferromagnet with a noncentrosymmetric crystal and a nonmagnet with strong spin-orbit coupling. As a striking result, we find that, in systems with a hybrid DMI, the spin-orbit-torque-induced skyrmion Hall angle is asymmetric for the two different skyrmion polarities ($\pm 1$ given by out-of-plane core magnetization), even allowing one of them to be tuned to zero. We propose several experimental ways to achieve the necessary straight skyrmion motion (with zero Hall angle) for racetrack memories, even without antiferromagnetic interactions or any interaction with another magnet. Our results can be understood within a simple picture by using a global spin rotation which maps the hybrid DMI model to an effective model containing purely interfacial DMI. The formalism directly reveals the effective spin torque and effective current that result in qualitatively different dynamics. Our work provides a way to utilize symmetry breaking to eliminate detrimental phenomena as hybrid DMI eliminates the skyrmion Hall angle.

cond-mat.mes-hall↗

Roles of chiral renormalization on magnetization dynamics in chiral magnets

In metallic ferromagnets, the interaction between local magnetic moments and conduction electrons renormalizes parameters of the Landau-Lifshitz-Gilbert equation such as the gyromagnetic ratio and the Gilbert damping, and makes them dependent on the magnetic configurations. Although the effects of the renormalization for nonchiral ferromagnets are usually minor and hardly detectable, we show that the renormalization does play a crucial role for chiral magnets. Here the renormalization is chiral and as such we predict experimentally identifiable effects on the phenomenology of magnetization dynamics. In particular, our theory for the self-consistent magnetization dynamics of chiral magnets allows for a concise interpretation of domain wall creep motion. We also argue that the conventional creep theory of the domain wall motion, which assumes Markovian dynamics, needs critical reexamination since the gyromagnetic ratio makes the motion non-Markovian. The non-Markovian nature of the domain wall dynamics is experimentally checkable by the chirality of the renormalization.

cond-mat.mes-hall↗

Spin-orbit torques from interfacial spin-orbit coupling for various interfaces

We use a perturbative approach to study the effects of interfacial spin-orbit coupling in magnetic multilayers by treating the two-dimensional Rashba model in a fully three-dimensional description of electron transport near an interface. This formalism provides a compact analytic expression for current-induced spin-orbit torques in terms of unperturbed scattering coefficients, allowing computation of spin-orbit torques for various contexts, by simply substituting scattering coefficients into the formulas. It applies to calculations of spin-orbit torques for magnetic bilayers with bulk magnetism, those with interface magnetism, a normal metal/ferromagnetic insulator junction, and a topological insulator/ferromagnet junction. It predicts a dampinglike component of spin-orbit torque that is distinct from any intrinsic contribution or those that arise from particular spin relaxation mechanisms. We discuss the effects of proximity-induced magnetism and insertion of an additional layer and provide formulas for in-plane current, which is induced by a perpendicular bias, anisotropic magnetoresistance, and spin memory loss in the same formalism.

cond-mat.mes-hall↗

Simultaneous control of the Dzyaloshinskii-Moriya interaction and magnetic anisotropy in nanomagnetic trilayers

Magneto-optical Kerr effect (MOKE) microscopy measurements of magnetic bubble domains demonstrate that Ar+ irradiation around 100 eV can tune the Dzyaloshinskii-Moriya interaction (DMI) in Pt/Co/Pt trilayers. Varying the irradiation energy and dose changes the DMI sign and magnitude separately from the magnetic anisotropy, allowing tuning of the DMI while holding the coercive field constant. This simultaneous control emphasizes the different physical origins of these effects. To accurately measure the DMI, we propose and apply a physical model for a poorly understood peak in domain wall velocity at zero in-plane field. The ability to tune the DMI with the spatial resolution of the Ar+ irradiation enables new fundamental investigations and technological applications of chiral nanomagnetics.

cond-mat.mtrl-sci↗

Chiral magnetoresistance in Pt/Co/Pt zigzag wires

The Rashba effect leads to a chiral precession of the spins of moving electrons while the Dzyaloshinskii-Moriya interaction (DMI) generates preference towards a chiral profile of local spins. We predict that the exchange interaction between these two spin systems results in a 'chiral' magnetoresistance depending on the chirality of the local spin texture. We observe this magnetoresistance by measuring the domain wall (DW) resistance in a uniquely designed Pt/Co/Pt zigzag wire, and by changing the chirality of the DW with applying an in-plane magnetic field. A chirality-dependent DW resistance is found, and a quantitative analysis shows a good agreement with a theory based on the Rashba model. Moreover, the DW resistance measurement allows us to independently determine the strength of the Rashba effect and the DMI simultaneously, and the result implies a possible correlation between the Rashba effect, the DMI, and the symmetric Heisenberg exchange.

cond-mat.mes-hall↗

Theory of Kondo suppression of spin polarization in nonlocal spin valves

We theoretically analyze contributions from the Kondo effect to the spin polarization and spin diffusion length in all-metal nonlocal spin valves. Interdiffusion of ferromagnetic atoms into the normal metal layer creates a region in which Kondo physics plays a significant role, giving discrepancies between experiment and existing theory. We start from a simple model and construct a modified spin drift-diffusion equation which clearly demonstrates how the Kondo physics not only suppresses the electrical conductivity but even more strongly reduces the spin diffusion length. We also present an explicit expression for the suppression of spin polarization due to Kondo physics in an illustrative regime. We compare this theory to previous experimental data to extract an estimate of the Elliot-Yafet probability for Kondo spin flip scattering of 0.7 $\pm$ 0.4, in good agreement with the value of 2/3 derived in the original theory of Kondo.

cond-mat.mes-hall↗

Perpendicular magnetic anisotropy of two-dimensional Rashba ferromagnets

We compute the magnetocrystalline anisotropy energy within two-dimensional Rashba models. For a ferromagnetic free-electron Rashba model, the magnetic anisotropy is exactly zero regardless of the strength of the Rashba coupling, unless only the lowest band is occupied. For this latter case, the model predicts in-plane anisotropy. For a more realistic Rashba model with finite band width, the magnetic anisotropy evolves from in-plane to perpendicular and back to in-plane as bands are progressively filled. This evolution agrees with first-principles calculations on the interfacial anisotropy, suggesting that the Rashba model captures energetics leading to anisotropy originating from the interface provided that the model takes account of the finite Brillouin zone. The results show that the electron density modulation by doping or an external voltage is more important for voltage-controlled magnetic anisotropy than the modulation of the Rashba parameter.

cond-mat.mes-hall↗

Intrinsic Spin Torque Without Spin-Orbit Coupling

We derive an intrinsic contribution to the non-adiabatic spin torque for non-uniform magnetic textures. It differs from previously considered contributions in several ways and can be the dominant contribution in some models. It does not depend on the change in occupation of the electron states due to the current flow but rather is due to the perturbation of the electronic states when an electric field is applied. Therefore it should be viewed as electric-field-induced rather than current-induced. Unlike previously reported non-adiabatic spin torques, it does not originate from extrinsic relaxation mechanisms nor spin-orbit coupling. This intrinsic non-adiabatic spin torque is related by a chiral connection to the intrinsic spin-orbit torque that has been calculated from the Berry phase for Rashba systems.

cond-mat.mes-hall↗

Chirality from interfacial spin-orbit coupling effects in magnetic bilayers

As nanomagnetic devices scale to smaller sizes, spin-orbit coupling due to the broken structural inversion symmetry at interfaces becomes increasingly important. Here we study interfacial spin-orbit coupling effects in magnetic bilayers using a simple Rashba model. The spin-orbit coupling introduces chirality into the behavior of the electrons and through them into the energetics of the magnetization. In the derived form of the magnetization dynamics, all of the contributions that are linear in the spin-orbit coupling follow from this chirality, considerably simplifying the analysis. For these systems, an important consequence is a correlation between the Dzyaloshinskii-Moriya interaction and the spin-orbit torque. We use this correlation to analyze recent experiments.

cond-mat.mes-hall↗

Self-consistent calculation of spin transport and magnetization dynamics

A spin-polarized current transfers its spin-angular momentum to a local magnetization, exciting current-induced magnetization dynamics. So far, most studies in this field have focused on the direct effect of spin transport on magnetization dynamics, but ignored the feedback from the magnetization dynamics to the spin transport and back to the magnetization dynamics. Although the feedback is usually weak, there are situations when it can play an important role in the dynamics. In such situations, self-consistent calculations of the magnetization dynamics and the spin transport can accurately describe the feedback. This review describes in detail the feedback mechanisms, and presents recent progress in self-consistent calculations of the coupled dynamics. We pay special attention to three representative examples, where the feedback generates non-local effective interactions for the magnetization. Possibly the most dramatic feedback example is the dynamic instability in magnetic nanopillars with a single magnetic layer. This instability does not occur without non-local feedback. We demonstrate that full self-consistent calculations generate simulation results in much better agreement with experiments than previous calculations that addressed the feedback effect approximately. The next example is for more typical spin valve nanopillars. Although the effect of feedback is less dramatic because even without feedback the current can induce magnetization oscillation, the feedback can still have important consequences. For instance, we show that the feedback can reduce the linewidth of oscillations, in agreement with experimental observations. Finally, we consider nonadiabatic electron transport in narrow domain walls. The non-local feedback in these systems leads to a significant renormalization of the effective nonadiabatic spin transfer torque.

cond-mat.mtrl-sci↗