arXiv subjects

Kyung-Jin Lee

Publications and source records attributed to Kyung-Jin Lee.

At least 19 recordsLinked to original sources

arXiv2026

Observation of current-induced orbital quadrupole accumulation

Spintronics and orbitronics rely on current-induced accumulations of magnetic dipoles: spin and orbital angular momentum. However, electronic orbitals inherently carry multipoles beyond the dipole, with the rank-2 orbital quadrupole as the leading term. Here we use polarization-resolved Kerr microscopy to observe current-induced orbital-quadrupole accumulation at the surfaces of Ti and Pt, metals with markedly different spin--orbit-coupling strengths. By separating the symmetric and antisymmetric components of the off-diagonal optical conductivity, we isolate the time-reversal-even quadrupolar response from the conventional time-reversal-odd magnetic-dipolar one, and find that the quadrupolar optical response exceeds the dipolar one in both metals. First-principles analysis of the measured responses indicates that the quadrupole accumulations are of the same order of magnitude in the two metals despite their widely different spin--orbit-coupling strengths, consistent with a previously unidentified channel of charge-to-orbital conversion that does not require spin--orbit coupling. Our findings establish that current-induced orbital polarization is fundamentally multipolar, expanding current-induced phenomena from the dipolar to the multipolar regime and opening a route to electrical control of orbital-ordered phases.

cond-mat.mtrl-sci↗

arXiv2026

Quantum Spin Transfer of Spin-Correlated Electron Pairs

We theoretically investigate quantum spin transfer from spin-correlated conduction-electron pairs to localized spins in a ferromagnet, given that electrons are correlated intrinsically. We show that even spin-singlet pairs and triplet pairs with $m=0$, both carrying no net spin, can transfer finite angular momentum through the quantum fluctuation term inherent to the $sd$ exchange interaction. The amount of transferred spin differs between the singlet and triplet $m=0$ states due to quantum interference. The difference is such that the independent-electron approximation remains valid for spin transfer when injected spin currents are completely incoherent. However, in partially coherent systems, like superconductor/ferromagnet junctions, coherent spin-singlet currents can directly convert into equal-spin triplet currents in generic ferromagnets, without requiring magnetic inhomogeniety or spin-orbit coupling.

cond-mat.mes-hall↗

arXiv2025

Challenges and opportunities in orbitronics

The spin of the electron has been a key enabler to realize spintronics devices that harness the spin degree of freedom beyond conventional charge-based electronics. In addition to spin, electrons have another degree of freedom associated with the angular momentum: orbital angular momentum. While spintronics has evolved fast and spintronics concepts are now used in magnetic sensors and nonvolatile memories, exploiting orbital angular momentum has just started to be studied. Phenomena mediated by orbital angular momentum have led to a new branch of spintronics called orbitronics. This Perspective discusses how orbitronics can constitute the next step in the evolution of spintronics by reviewing the current understandings and experimental results of orbital effects and summarizing the open questions. Prospects and challenges for devices in particular in non-volatile memory are discussed as an applications perspective.

cond-mat.mes-hall↗

arXiv2025

Magnetic Octupole Hall Effect in d-Wave Altermagnets

Order parameters not only characterize symmetry-broken equilibrium phases but also govern transport phenomena in the nonequilibrium regime. Altermagnets, a class of magnetic systems integrating ferromagnetic and antiferromagnetic features, host multipolar orders in addition to dipolar Neel order. In this work, we demonstrate the multipole Hall effect in d-wave altermagnets--a transverse flow of multipole moments induced by an electric field. Using symmetry analysis and linear response theory, we show that the magnetic octupole Hall effect persists even in symmetries where the spin-splitter effect is forbidden and thus provides a robust experimental signature. In addition, we identify a sizable electric quadrupole Hall effect, originating from quadrupole splittings in the band structure. Our results expand the family of Hall effects to include higher-order multipolar responses and establish altermagnets as a versatile platform for exploring multipole transport beyond spin and orbital degrees of freedom.

cond-mat.mtrl-sci↗

arXiv2025

Nonlocal Electrical Detection of Reciprocal Orbital Edelstein Effect

Spin-Orbitronics leverages the spin and orbital degrees of freedom in solids for information processing. The orbital Edelstein effect and orbital Hall effect, where the charge current induces a nonequilibrium orbital angular momentum, offer a promising method to manipulate nanomagnets efficiently using light elements. Despite extensive research, understanding the Onsager reciprocity of orbital transport, fundamentally rooted in the second law of thermodynamics and time-reversal symmetry, remains elusive. In this study, we experimentally demonstrate the Onsager reciprocity of orbital transport in an orbital Edelstein system by utilizing nonlocal measurements. This method enables the precise identification of the chemical potential generated by orbital accumulation, avoiding the limitations associated with local measurements. Remarkably, we observe that the direct and inverse orbital-charge conversion processes produce identical electric voltages, confirming Onsager reciprocity in orbital transport. Additionally, we find that the orbital decay length, approximately 100 nm at room temperature, is independent of Cu thickness and decreases with lowering temperature, revealing a distinct contrast to spin transport behavior. Our findings provide valuable insights into both the reciprocity of the charge-orbital interconversion and the nonlocal correlation of orbital degree of freedom, laying the ground for orbitronics devices with long-range interconnections.

cond-mat.mes-hall↗

arXiv2025

Orbital Pumping Incorporating Both Orbital Angular Momentum and Position

We develop a theory of adiabatic orbital pumping, highlighting qualitative differences from spin pumping. An oscillating magnetic field pumps not only orbital angular momentum current but also orbital angular position current. The latter, which has no spin counterpart, underscores the incompleteness of existing orbital torque theories. Importantly, both types of orbital currents can be detected as transverse electric voltages, which contain considerable second harmonic components unlike in spin pumping. Moreover, orbital currents can be pumped by lattice dynamics that carry phonon angular momentum, implying that orbital currents can, in turn, induce phonon angular momentum. Our work open up new possibilities for generating orbital currents and provides a broader understanding of the interplay between spin, orbital, and phonon dynamics.

cond-mat.mes-hall↗

arXiv2025

Emergence of Giant Magnetic Chirality during Dimensionality Crossover of Magnetic Materials

Chirality, an intrinsic preference for a specific handedness, is a fundamental characteristic observed in nature. In magnetism, magnetic chirality arises from the anti-symmetric Dzyaloshinskii-Moriya interaction in competition with the symmetric Heisenberg exchange interaction. Traditionally, the anti-symmetric interaction has been considered minor relative to the symmetric interaction. In this study, we demonstrate an observation of giant magnetic chirality during the dimensionality crossover of magnetic materials from three-dimensional to two-dimensional. The ratio between the anti-symmetric and symmetric interactions exhibits a reversal in their dominance over this crossover, overturning the traditional consideration. This observation is validated theoretically using a non-local interaction model and tight-binding calculation with distinct pairing schemes for each exchange interaction throughout the crossover. Additional experiments investigating the asphericity of orbital moments corroborate the robustness of our findings. Our findings highlight the critical role of dimensionality in shaping magnetic chirality and offer strategies for engineering chiral magnet states with unprecedented strength, desired for the design of spintronic materials.

cond-mat.mtrl-sci↗

arXiv2024

Orbital diffusion, polarization and swapping in centrosymmetric metals

We propose a general theory of charge, spin, and orbital diffusion based on Keldysh formalism. Our findings indicate that the diffusivity of orbital angular momentum in metals is much lower than that of spin or charge due to the strong orbital intermixing in crystals. Furthermore, our theory introduces the concept of spin-orbit polarization by which a pure orbital (spin) current induces a longitudinal spin (orbital) current, a process as efficient as spin polarization in ferromagnets. Finally, we find that orbital currents undergo momentum swapping, even in the absence of spin-orbit coupling. This theory establishes several key parameters for orbital transport of direct importance to experiments.

cond-mat.mes-hall↗

arXiv2024

Impact of external magnetic fields on STT-MRAM

This application note discusses the working principle of spin-transfer torque magnetoresistive random access memory (STT-MRAM) and the impact that magnetic fields can have on STT-MRAM operation. Sources of magnetic field and typical magnitudes of magnetic fields are given. Based on the magnitude of commonly encountered external magnetic fields, we show below that magnetic immunity of STT-MRAM is sufficient for most uses once the chip is mounted on a printed circuit board (PCB) or inserted in its working environment. This statement is supported by the experience acquired during 60 years of use of magnetic hard disk drives (HDD) including 20 years of HDD with readers comprising magnetic tunnel junctions, 20+ years of use of magnetic field sensors as position encoders in automotive industry and 15+ years of use of MRAM. Mainly during chip handling does caution need to be exercised to avoid exposing the chip to excessively high magnetic fields.

physics.app-ph↗

arXiv2022

Spin current driven by ultrafast magnetization of FeRh

Laser-induced ultrafast demagnetization is an important phenomenon that probes arguably ultimate limits of the angular momentum dynamics in solid. Unfortunately, many aspects of the dynamics remain unclear except that the demagnetization transfers the angular momentum eventually to the lattice. In particular, roles of electron-carried spin current are debated. Here we experimentally probe the spin current in the opposite phenomenon, i.e., laser-induced ultrafast magnetization of FeRh, where the laser pump pulse initiates the angular momentum build-up rather than its dissipation. Using the time-resolved magneto-optical Kerr effect, we directly measure the ultrafast-magnetization-driven spin current in a FeRh/Cu heterostructure. Strong correlation between the spin current and the net magnetization change rate of FeRh is found even though the spin filter effect is negligible in this opposite process. This result implies that the angular momentum build-up is achieved by an angular momentum transfer from the electron bath (supplier) to the magnon bath (receiver) and followed by the spatial transport of angular momentum (spin current) and dissipation of angular momentum to the phonon bath (spin relaxation).

cond-mat.mtrl-sci↗

arXiv2022

Efficient conversion of orbital Hall current to spin current for spin-orbit torque switching

Spin Hall effect, an electric generation of spin current, allows for efficient control of magnetization. Recent theory revealed that orbital Hall effect creates orbital current, which can be much larger than spin Hall-induced spin current. However, orbital current cannot directly exert a torque on a ferromagnet, requiring a conversion process from orbital current to spin current. Here, we report two effective methods of the conversion through spin-orbit coupling engineering, which allows us to unambiguously demonstrate orbital-current-induced spin torque, or orbital Hall torque. We find that orbital Hall torque is greatly enhanced by introducing either a rare-earth ferromagnet Gd or a Pt interfacial layer with strong spin-orbit coupling in Cr/ferromagnet structures, indicating that the orbital current generated in Cr is efficiently converted into spin current in the Gd or Pt layer. Furthermore, we show that the orbital Hall torque can facilitate the reduction of switching current of perpendicular magnetization in spin-orbit-torque-based spintronic devices.

cond-mat.mtrl-sci↗

arXiv2021

The domain-wall motion driven by a rotating field in a ferrimagnet

We theoretically study a ferrimagnetic domain-wall motion driven by a rotating magnetic field. We find that, depending on the magnitude and the frequency of the rotating field, the dynamics of a ferrimagnetic domain wall can be classified into two regimes. First, when the frequency is lower than a certain critical frequency set by the field magnitude, there is a stationary solution for the domain-wall dynamics, where a domain-wall in-plane magnetization rotates in-phase with the external field. The field-induced precession of the domain wall gives rise to the translational motion of the domain wall via the gyrotropic coupling between the domain-wall angle and position. In this so-called phase-locking regime, a domain-wall velocity increases as the frequency increases. Second, when the frequency exceeds the critical frequency, a domain-wall angle precession is not synchronous with the applied field. In this phase-unlocking regime, a domain wall velocity decreases as the frequency increases. Moreover, the direction of the domain-wall motion is found to be reversed across the angular compensation point where the net spin density of the ferrimagnet changes its sign. Our work suggests that the dynamics of magnetic solitons under time-varying biases may serve as platform to study critical phenomena.

cond-mat.mes-hall↗

arXiv2021

Identifying intrinsic and extrinsic mechanisms of anisotropic magnetoresistance with terahertz probes

Identifying the intrinsic and extrinsic origins of magneto-transport in spin-orbit coupled systems has long been a central theme in condensed matter physics. However, it has been elusive owing to the lack of an appropriate experimental tool. In this work, using terahertz time-domain spectroscopy, we unambiguously disentangle the intrinsic and extrinsic contributions to the anisotropic magnetoresistance (AMR) of a permalloy film. We find that the scattering-independent intrinsic contribution to AMR is sizable and is as large as the scattering-dependent extrinsic contribution to AMR. Moreover, the portion of intrinsic contribution to total AMR increases with increasing temperature due to the reduction of extrinsic contribution. Further investigation reveals that the reduction of extrinsic contribution is caused by the phonon/magnon-induced negative AMR. Our result will stimulate further researches on other spin-orbit-interaction-induced phenomena for which identifying the intrinsic and extrinsic contributions is important.

cond-mat.mtrl-sci↗

arXiv2020

Theory of Current-Induced Angular Momentum Transfer Dynamics in Spin-Orbit Coupled Systems

Motivated by the importance of understanding competing mechanisms to current-induced spin-orbit torque in complex magnets, we develop a unified theory of current-induced spin-orbital coupled dynamics. The theory describes angular momentum transfer between different degrees of freedom in solids, e.g., the electron orbital and spin, the crystal lattice, and the magnetic order parameter. Based on the continuity equations for the spin and orbital angular momenta, we derive equations of motion that relate spin and orbital current fluxes and torques describing the transfer of angular momentum between different degrees of freedom. We then propose a classification scheme for the mechanisms of the current-induced torque in magnetic bilayers. Based on our first-principles implementation, we apply our formalism to two different magnetic bilayers, Fe/W(110) and Ni/W(110), which are chosen such that the orbital and spin Hall effects in W have opposite sign and the resulting spin- and orbital-mediated torques can compete with each other. We find that while the spin torque arising from the spin Hall effect of W is the dominant mechanism of the current-induced torque in Fe/W(110), the dominant mechanism in Ni/W(110) is the orbital torque originating in the orbital Hall effect of W. It leads to negative and positive effective spin Hall angles, respectively, which can be directly identified in experiments. This clearly demonstrates that our formalism is ideal for studying the angular momentum transfer dynamics in spin-orbit coupled systems as it goes beyond the "spin current picture" by naturally incorporating the spin and orbital degrees of freedom on an equal footing. Our calculations reveal that, in addition to the spin and orbital torque, other contributions such as the interfacial torque and self-induced anomalous torque within the ferromagnet are not negligible in both material systems.

cond-mat.mes-hall↗

arXiv2020

SU(3) Topology of Magnon-Phonon Hybridization in 2D Antiferromagnets

Magnon-phonon hybrid excitations are studied theoretically in a two-dimensional antiferromagnet with an easy axis normal to the plane. We show that two magnon bands and one phonon band are intertwined by the magnetoelastic coupling through a nontrivial SU(3) topology, which can be intuitively perceived by identifying a skyrmion structure in the momentum space. We develop a continuum theory as the long-wavelength approximation to the tight-binding model, showing our results are insensitive to lattice details and generally applicable to two-dimensional antiferromagnets. The theoretical results can be probed by measuring the thermal Hall conductance as a function of the temperature and the magnetic field. We envision that the magnetoelastic coupling in antiferromagnets can be a promising venue in search of various topological excitations, which cannot be found in magnetic or elastic models alone.

cond-mat.mes-hall↗

arXiv2020

Role of orbital hybridization in anisotropic magnetoresistance

We theoretically and numerically show that longitudinal orbital currents in ferromagnets depend on the magnetization direction, which contribute to the anisotropic magnetoresistance (AMR). This orbital contribution to AMR arises from the momentum-dependent orbital splitting, which is generally present in multi-orbital systems through the orbital anisotropy and the orbital hybridization. We highlight the latter orbital hybridization as an unrecognized origin of AMR and also as a common origin of AMR and orbital Hall effect.

cond-mat.mes-hall↗

arXiv2020

Spin-orbit torque switching of perpendicular magnetization in ferromagnetic trilayers

In ferromagnetic trilayers, a spin-orbit-induced spin current can have a spin polarization of which direction is deviated from that for the spin Hall effect. Recently, magnetization switching in ferromagnetic trilayers has been proposed and confirmed by the experiments. In this work, we theoretically and numerically investigate the switching current required for perpendicular magnetization switching in ferromagnetic trilayers. We confirm that the tilted spin polarization enables field-free deterministic switching at a lower current than conventional spin-orbit torque or spin-transfer torque switching, offering a possibility for high-density and low-power spin-orbit torque devices. Moreover, we provide analytical expressions of the switching current for an arbitrary spin polarization direction, which will be useful to design spin-orbit torque devices and to interpret spin-orbit torque switching experiments.

cond-mat.mtrl-sci↗

arXiv2020

The dynamics of a domain wall in ferrimagnets driven by spin-transfer torque

The spin-transfer-torque-driven (STT-driven) dynamics of a domain wall in an easy-axis rare-earth transition-metal ferrimagnet is investigated theoretically and numerically in the vicinity of the angular momentum compensation point $T_A$, where the net spin density vanishes. The particular focus is given on the unusual interaction of the antiferromagnetic dynamics of a ferrimagnetic domain wall and the adiabatic component of STT, which is absent in antiferromagnets but exists in the ferrimagnets due to the dominant coupling of conduction electrons to transition-metal spins. Specifically, we first show that the STT-induced domain-wall velocity changes its sign across $T_A$ due to the sign change of the net spin density, giving rise to a phenomenon unique to ferrimagnets that can be used to characterize $T_A$ electrically. It is also shown that the frequency of the STT-induced domain-wall precession exhibits its maximum at $T_A$ and it can approach the spin-wave gap at sufficiently high currents. Lastly, we report a numerical observation that, as the current density increases, the domain-wall velocity starts to deviate from the linear-response result, calling for a more comprehensive theory for the domain-wall dynamics in ferrimagnets driven by a strong current.

cond-mat.mes-hall↗