arXiv subjects

L. A. Riley

Publications and source records attributed to L. A. Riley.

At least 19 recordsLinked to original sources

arXiv2026

Observing the effects of numbers of valence nucleons on $0_{gs}^+ \rightarrow 2_1^+$ transitions in deformed nuclei by comparing proton and neutron transition matrix elements

We examined the ratios of neutron and proton transition matrix elements, $M_n/M_p$, for the $0_{gs}^+ \rightarrow 2_1^+$ transitions in 48 even-even stable nuclei with $N>20$ for which electromagnetic matrix elements were compiled by Pritychenko \textit{et al.} and for which high-quality inelastic proton scattering data were available. Several deformed rare earth nuclei have $(M_n/M_p)/(N/Z)$ values significantly below 1.0, which is not consistent with a simple liquid drop picture. However, this phenomenon can be explained using a schematic picture in which $M_p$ reaches a maximum at proton mid-shell ($Z=66$) and $M_n$ reaches its maximum at neutron mid-shell ($N=104$). Several mid-mass vibrational nuclei have $M_n/M_p$ values significantly below $N/Z$, which is not consistent with the expectation that $M_n/M_p = N/Z$ in such nuclei. A shell model investigation of these observations might yield insights about this behavior.

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arXiv2026

Experimental study of $^{53}$Cr via the $(d,p\gamma)$ reaction

Excited states in $^{53}$Cr were studied via the $^{52}$Cr$(d,p\gamma)$ reaction up to the neutron-separation threshold. Proton-$\gamma$ angular correlations and $\gamma$ decay branching ratios were measured in particle-$\gamma$ coincidences between the Super-Enge Split-Pole Spectrograph (SE-SPS) and CeBr$_3$ Array (CeBrA) demonstrator of the John D. Fox Accelerator Laboratory at Florida State University. Previous spin-parity assignments from a $(d,p)$ singles experiment at the SE-SPS are supported and $\gamma$-ray transitions in $^{53}$Cr reported. We firmly assign higher-lying excited states to $^{53}$Cr because overlapping excited states and contaminants could be identified better due to the complementary $\gamma$-decay information. We also correct some of the previously reported excitation energies and present a reanalysis of previously measured $^{52}$Cr$(d,p){}^{53}${Cr} angular distributions guided by the complementary $\gamma$-ray information. Based on this reanalysis, the fragmentation of the neutron $2p_{3/2}$, $2p_{1/2}$, $1f_{5/2}$, $1g_{9/2}$, and $2d_{5/2}$ single-particle strengths is reassessed for $^{53}$Cr. A comparison to the corresponding strengths in $^{55}$Fe is presented.

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arXiv2025

Extraction of neutron-capture cross sections on $^{92}$Zr using the charge-exchange Oslo method

The $^{93}$Nb($t$,$^{3}$He) reaction at 115 MeV/u was studied to demonstrate that nuclear level densities and $\gamma$-ray strength functions can be extracted from charge-exchange reactions at intermediate energies using the Oslo technique. The matrix of excitation energy in $^{93}$Zr, reconstructed from the ($t$,$^{3}$He) reaction, versus the energy of $\gamma$ rays emitted by the excited $^{93}$Zr nuclei, was obtained in an experiment with the S800 Spectrograph operated in coincidence with the GRETINA $\gamma$-ray detector. The extracted level density and $\gamma$-ray strength function obtained by applying the Oslo method to this matrix were used to estimate the $^{92}$Zr($n$,$\gamma$)$^{93}$Zr cross section by combining the new results with other experimental data and theoretical calculations for $E$1 and $M$1 strength functions at higher energies. Good agreement with direct measurements of the $^{92}$Zr($n$,$\gamma$)$^{93}$Zr cross section was found. The contribution from the upbend in the extracted $\gamma$-ray strength function was important to achieve the consistency as the neutron-capture cross section without this contribution is significantly below the direct measurements otherwise. Since charge-exchange reactions at intermediate energies have long been used for extracting Gamow-Teller strengths, the successful demonstration of the charge-exchange Oslo method enables experiments in which ($n$,$\gamma$) cross sections and Gamow-Teller strengths can be measured simultaneously, which is of benefit for astrophysical studies.

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arXiv2025

Determination of proton and neutron contributions to the $0_{g.s.}^+ \rightarrow 2_1^+$ excitations in $^{42}$Si and $^{44}$S using inelastic proton scattering in inverse kinematics and intermediate energy Coulomb excitation

We have measured the $0_{g.s.}^+ \rightarrow 2_1^+$ transition in the neutron rich $N=28$ isotope $^{42}$Si using the probes of intermediate energy Coulomb excitation and inelastic proton scattering in inverse kinematics at the Facility for Rare Isotope Beams with beam particle rates of $\approx 5$ particles/s. The results of these two measurements allowed us to determine $M_n/M_p$, the ratio of the neutron and proton transition matrix elements for the $0_{g.s.}^+ \rightarrow 2_1^+$ transition. In addition, we have measured the $0_{\mathrm{g.s.}}^+ \rightarrow 2_1^+$ transition in the isotone $^{44}$S using inverse kinematics inelastic proton scattering. By comparing the $^{44}$S proton scattering result with a recent intermediate energy Coulomb excitation result on the same transition, we were able to determine $M_n/M_p$ for the $0_{g.s.}^+ \rightarrow 2_1^+$ transition in this nucleus as well. This work strengthens the evidence that $^{42}$Si has a stable quadrupole deformation in its ground state and that $^{44}$S does not. Both conclusions are further supported by shell model calculations carried out with the FSU interaction.

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arXiv2024

Proton removal from $^{73,75}$Br to $^{72,74}$Se at intermediate energies

We report new experimental data for excited states of $^{72,74}$Se obtained from proton removal from $^{73,75}$Br secondary beams on a proton target. The experiments were performed with the Ursinus-NSCL Liquid Hydrogen Target and the combined GRETINA+S800 setup at the Coupled Cyclotron Facility of the National Superconducting Cyclotron Laboratory at Michigan State University. Within uncertainties, the inclusive cross sections for proton removal from $^{73,75}$Br on a proton target are identical suggesting that the same single-particle orbitals contribute to the proton-removal reaction. In addition, details of the partial cross section fragmentation are discussed. The data might suggest that $l = 1, 2, 3$, and 4 angular momentum transfers are important to understand the population of excited states of $^{72,74}$Se in proton removal. Available data for excited states of $^{74}$Ge populated through the $^{75}$As$(d,{}^{3}{\mathrm{He}}){}^{74}$Ge proton-removal reaction in normal kinematics suggest indeed that the $fp$ and $sd$ shell as well as the $1g_{9/2}$ orbital contribute. A comparison to data available for odd-$A$ nuclei supports that the bulk of the spectroscopic strengths could be found at lower energies in the even-even Se isotopes than in, for instance, the even-even Ge isotopes. In addition, the population of high-$J$ states seems to indicate that multi-step processes contribute to proton-removal reactions at intermediate energies in these collective nuclei.

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arXiv2024

Single-Neutron Adding on $^{34}$S

Purpose: Single-neutron adding data was collected in order to determine the distribution of the single-neutron strength of the $0f_{7/2}$, $1p_{3/2}$, $1p_{1/2}$ and $0f_{5/2}$ orbitals outside of $Z=16, N=18$, $^{34}$S. Methods: The $^{34}$S($d$,$p$)$^{35}$S reaction has been measured at 8 MeV/u to investigate cross sections to excited states in $^{35}$S. Outgoing proton yields and momenta were analyzed by the Super-Enge Split-Pole Spectrograph in conjunction with the CeBrA demonstrator located at the John D. Fox Laboratory at Florida State University. Angular distributions were compared with Distorted Wave Born Approximation calculations in order to extract single-neutron spectroscopic overlaps. Results: Spectroscopic overlaps and strengths were determined for states in $^{35}$S up through 6 MeV in excitation energy. Each orbital was observed to have fragmented strength where a single level carried the majority. The single-neutron centroids of the $0f_{7/2}$, $1p_{3/2}$, $1p_{1/2}$ and $0f_{5/2}$ orbitals were determined to be $2360^{+90}_{-40}$ keV, $3280^{+80}_{-50}$ keV, $4780^{+60}_{-40}$ keV, and $\gtrsim7500$ keV, respectively. Conclusion: A previous discrepancy in the literature with respect to distribution of the neutron $1p_{1/2}$ strength was resolved. The integration of the normalized spectroscopic strengths, up to 5.1 MeV in excitation energy, revealed fully-vacant occupancies for the $0f_{7/2}$, $1p_{3/2}$, and $1p_{1/2}$ orbitals, as expected. The spacing in the single-neutron energies highlighted a reduction in the traditional $N=28$ shell-gap, relative to both the $1p$ spin-orbit energy difference ($N=32$) and the lower limit on the $N=34$ shell spacing.

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arXiv2023

The CeBrA demonstrator for particle-$γ$ coincidence experiments at the FSU Super-Enge Split-Pole Spectrograph

We report on a highly selective experimental setup for particle-$γ$ coincidence experiments at the Super-Enge Split-Pole Spectrograph (SE-SPS) of the John D. Fox Superconducting Linear Accelerator Laboratory at Florida State University (FSU) using fast CeBr$_3$ scintillators for $γ$-ray detection. Specifically, we report on the results of characterization tests for the first five CeBr$_3$ scintillation detectors of the CeBr$_3$ Array (CeBrA) with respect to energy resolution and timing characteristics. We also present results from the first particle-$γ$ coincidence experiments successfully performed with the CeBrA demonstrator and the FSU SE-SPS. We show that with the new setup, $γ$-decay branching ratios and particle-$γ$ angular correlations can be measured very selectively using narrow excitation energy gates, which are possible thanks to the excellent particle energy resolution of the SE-SPS. In addition, we highlight that nuclear level lifetimes in the nanoseconds regime can be determined by measuring the time difference between particle detection with the SE-SPS focal-plane scintillator and $γ$-ray detection with the fast CeBrA detectors. Selective excitation energy gates with the SE-SPS exclude any feeding contributions to these lifetimes.

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arXiv2023

$g_{9/2}$ neutron strength in the $N=29$ isotones and the $^{52}$Cr($d,p$)$^{53}$Cr reaction

We performed a measurement of the $^{52}$Cr$(d,p)^{53}$Cr reaction at 16 MeV using the Florida State University Super-Enge Split-Pole Spectrograph (SE-SPS) and observed 26 states. While all of the states observed here had been seen in previous $(d,p)$ experiments, we changed five $L$ assignments from those reported previously and determined $L$ values for nine states that had not had such assignments made previously. The $g_{9/2}$ neutron strength observed in $^{53}$Cr in the present work and in the $N=29$ isotones $^{49}$Ca, $^{51}$Ti, and $^{55}$Fe via $(d,p)$ reactions is much smaller than the sum rule for this strength. Most of the observed $L=4$ strength in these nuclei is located in states near 4 MeV excitation energy. The remaining $g_{9/2}$ strength may be located in the continuum or may be fragmented among many bound states. A covariant density functional theory calculation provides support for the hypothesis that the $g_{9/2}$ neutron orbit is unbound in $^{53}$Cr. The ($α,^3$He) reaction may provide a more sensitive probe for the missing $g_{9/2}$ neutron strength. In addition, particle-$γ$ coincidence experiments may help resolve some remaining questions in this nucleus.

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arXiv2023

Hexadecapole strength in the rare isotopes $^{74,76}$Kr

In the Ge-Sr mass region, isotopes with neutron number $N \leq 40$ are known to feature rapid shape changes with both nucleon number and angular momentum. To gain new insights into their structure, inelastic proton scattering experiments in inverse kinematics were performed on the rare isotopes $^{74,76}$Kr. This work focuses on observables related to the $J^π = 4^+_1$ states of the Kr isotopes and, in particular, on the hexadecapole degree of freedom. By performing coupled-channels calculations, hexadecapole deformation parameters $β_4$ were determined for the $J^π = 4^+_1$ states of $^{74,76}$Kr from inelastic proton scattering cross sections. Two possible coupled-channels solutions were found. A comparison to predictions from nuclear energy density functional theory, employing both non-relativistic and relativistic functionals, clearly favors the large, positive $β_4$ solutions. These $β_4$ values are unambiguously linked to the well deformed prolate configuration. Given the $β_2 - β_4$ trend, established in this work, it appears that $β_4$ values could provide a sensitive measure of the nuclear shell structure.

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arXiv2022

$^{54}$Fe($d$,$p$)$^{55}$Fe and the evolution of single neutron energies in the $N=29$ isotones

A measurement of the $^{54}$Fe($d$,$p$)$^{55}$Fe reaction at 16 MeV was performed using the Florida State University Super-Enge Split-Pole Spectrograph to determine single-neutron energies for the $2p_{3/2}$, $2p_{1/2}$, $1f_{5/2}$, $1g_{9/2}$ and $2d_{5/2}$ orbits. Two states were observed that had not been observed in previous (d, p) measurements. In addition, we made angular momentum transfer, \textit{L}, assignments to four states and changed \textit{L} assignments from previous ($d$, $p$) measurements for nine more states. The spin-orbit splitting between the $2p_{3/2}$ and $2p_{1/2}$ orbits is similar to that in the other $N=29$ isotones and not close to zero as a previous measurement suggested. While the $1f_{5/2}$ single neutron energy is significantly lower in $^{55}$Fe than in $^{51}$Ti, as predicted by a covariant density functional theory calculation, the single-neutron energy for this orbit in $^{55}$Fe is more than 1 MeV higher than the calculation suggests, although it is only 400 keV above the $2p_{1/2}$ orbit. The summed spectroscopic strength we observed for the $1g_{9/2}$ orbit up to the single-neutron separation energy of 9.3 MeV is only 0.3. This is surprising because the $1g_{9/2}$ orbit is predicted by Togashi \textit{et al.} to be located only 5.5 MeV above the $2p_{3/2}$ orbit.

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arXiv2022

Investigation of octupole collectivity near the $A =72$ shape-transitional point

Enhanced octupole collectivity is expected in the neutron-deficient Ge, Se and Kr isotopes with neutron number $N \approx 40$ and has indeed been observed for $^{70,72}$Ge. Shape coexistence and configuration mixing are, however, a notorious challenge for theoretical models trying to reliably predict octupole collectivity in this mass region, which is known to feature rapid shape changes with changing nucleon number and spin of the system. To further investigate the microscopic configurations causing the prolate-oblate-triaxial shape transition at $A \approx 72$ and their influence on octupole collectivity, the rare isotopes $^{72}$Se and $^{74,76}$Kr were studied via inelastic proton scattering in inverse kinematics. While significantly enhanced octupole strength of $\sim 32$ Weisskopf units (W.u.) was observed for $^{72}$Se, only strengths of $\sim 15$ W.u. were observed for $^{74,76}$Kr. In combination with existing data, the new data clearly question a simple origin of enhanced octupole strengths around $N = 40$. The present work establishes two regions of distinct octupole strengths with a sudden strength increase around the $A=72$ shape transitional point.

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arXiv2021

$^{50}$Ti($d$,$p$)$^{51}$Ti, single neutron energies in the $N=29$ isotones and the $N=32$ subshell closure

A measurement of the $^{50}$Ti($d$,$p$)$^{51}$Ti reaction at 16 MeV was performed using a Super Enge Split Pole Spectrograph to measure the magnitude of the $N=32$ subshell gap in Ti. Seven states were observed that had not been observed in previous ($d$,$p$) measurements, and the \textit{L} transfer values for six previously measured states were either changed or measured for the first time. The results were used to determine single neutron energies for the $p_{3/2}$, $p_{1/2}$ and $f_{5/2}$ orbitals. The resulting single neutron energies in $^{51}$Ti confirm the existence of the $N=32$ gap in Ti. These single neutron energies and those from previous measurements in $^{49}$Ca, $^{53}$Cr and $^{55}$Fe are compared to values from a covariant density functional theory calculation.

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arXiv2021

UCGretina GEANT4 Simulation of the GRETINA Gamma-Ray Energy Tracking Array

UCGretina, a GEANT4 simulation of the GRETINA gamma-ray tracking array of highly-segmented high-purity germanium detectors is described. We have developed a model of the array, in particular of the Quad Module and the capsules, that gives good agreement between simulated and measured photopeak efficiencies over a broad range of gamma-ray energies and reproduces the shape of the measured Compton continuum. Both of these features are needed in order to accurately extract gamma-ray yields from spectra collected in in-beam gamma-ray spectroscopy measurements with beams traveling at $v/c \gtrsim 0.3$ at the National Superconducting Cyclotron Laboratory and the Facility for Rare Isotope Beams. In the process of developing the model, we determined that millimeter-scale layers of passive germanium surrounding the active volumes of the simulated crystals must be included in order to reproduce measured photopeak efficiencies. We adopted a simple model of effective passive layers and developed heuristic methods of determining passive-layer thicknesses by comparison of simulations and measurements for a single crystal and for the full array. Prospects for future development of the model are discussed.

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arXiv2020

Inverse-kinematics proton scattering from $^{42,44}$S, $^{41,43}$P and the collapse of the $N=28$ major shell closure

Excited states of the neutron-rich isotopes $^{42,44}$S and $^{41,43}$P have been studied via inverse-kinematics proton scattering from a liquid hydrogen target, using the GRETINA $γ$-ray tracking array to extract inelastic scattering cross sections. Deformation lengths of the $2^+_1$ excitations in $^{42,44}$S have been determined and, when combined with deformation lengths determined with electromagnetic probes, yield the ratio of neutron-to-proton matrix elements $M_n/M_p$ for the $2^+_1$ excitations in these nuclei. The present results for $^{41,43}$P$(p,p')$ are used to compare two shell model interactions, SDPF-U and SDPF-MU. As in a recent study of $^{42}$Si, the present results on $^{41,43}$P favor the SDPF-MU interaction.

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arXiv2018

The structure of 70Fe: Single-particle and collective degrees of freedom

Excited states in the neutron-rich \nuc{70}{Fe} nucleus were populated in a one-proton removal reaction from \nuc{71}{Co} projectiles at 87~MeV/nucleon. A new transition was observed with the $γ$-ray tracking array GRETINA and shown to feed the previously assigned $4^+_1$ state. In comparison to reaction theory calculations with shell-model spectroscopic factors, it is argued that the new $γ$ ray possibly originates from the $6^+_1$ state. It is further shown that the Doppler-reconstructed $γ$-ray spectra are sensitive to the very different lifetimes of the $2^+$ and $4^+$ states, enabling their approximate measurement. The emerging structure of \nuc{70}{Fe} is discussed in comparison to LNPS-new large-scale shell-model calculations.

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arXiv2017

Spectroscopy of $^{54}$Ti and the systematic behavior of low energy octupole states in Ca and Ti isotopes

Excited states of the $N=32$ nucleus $^{54}$Ti have been studied, via both inverse-kinematics proton scattering and one-neutron knockout from $^{55}$Ti by a liquid hydrogen target, using the GRETINA $γ$-ray tracking array. Inelastic proton-scattering cross sections and deformation lengths have been determined. A low-lying octupole state has been tentatively identified in $^{54}$Ti for the first time. A comparison of $(p,p')$ results on low-energy octupole states in the neutron-rich Ca and Ti isotopes with the results of Random Phase Approximation calculations demonstrates that the observed systematic behavior of these states is unexpected.

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arXiv2016

Octupole strength in the neutron-rich calcium isotopes

Low-lying excited states of the neutron-rich calcium isotopes $^{48-52}$Ca have been studied via $γ$-ray spectroscopy following inverse-kinematics proton scattering on a liquid hydrogen target using the GRETINA $γ$-ray tracking array. The energies and strengths of the octupole states in these isotopes are remarkably constant, indicating that these states are dominated by proton excitations.

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arXiv2014

Inverse-kinematics proton scattering on $^{50}$Ca: Determining effective charges using complementary probes

We have performed measurements of the $0_\mathrm{g.s.}^+ \rightarrow 2_1^+$ excitations in the neutron-rich isotopes $^{48,50}$Ca via inelastic proton scattering on a liquid hydrogen target, using the GRETINA $γ$-ray tracking array. A comparison of the present results with those from previous measurements of the lifetimes of the $2_1^+$ states provides us the ratio of the neutron and proton matrix elements for the $0_\mathrm{g.s.}^+ \rightarrow 2_1^+$ transitions. These results allow the determination of the ratio of the proton and neutron effective charges to be used in shell model calculations of neutron-rich isotopes in the vicinity of $^{48}$Ca.

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