arXiv subjects

L. Bougas

Publications and source records attributed to L. Bougas.

8 recordsLinked to original sources

arXiv2019

$\mathcal{P}$,$\mathcal{T}$-odd Faraday rotation on atoms and molecules in intra-cavity absorption spectroscopy as an alternative way to search for the $\mathcal{P}$,$\mathcal{T}$-odd effects in nature

Present limit on the electron electric dipole moment ($e$EDM) is based on the electron spin precession measurement. We propose an alternative approach - observation of the $\mathcal{P}$,$\mathcal{T}$-odd Faraday effect in an external electric field on atoms and molecules using cavity-enhanced polarimetric scheme in combination with molecular (atomic) beam crossing the cavity. Our calculations of the effective electric fields and theoretical simulation of the proposed experiment on Tl and Pb atoms, PbF, YbF, ThO, and YbOH show that the present limit on the $e$EDM can be improved by 6-7 orders of magnitude.

physics.atom-ph↗

arXiv2017

Towards improved measurements of parity violation in atomic ytterbium

We report on progress towards performing precision measurements of parity violation in Yb, in which the theoretical prediction for a strong weak-interaction-induced effect in the 6s^{2} ^{1}S_{0} \rightarrow 5d6s ^{3}D_{1} optical transition at 408 nm has already been confirmed, with a measurement of the effect at the \approx 10 % level of accuracy. With a new atomic-beam apparatus offering enhanced sensitivity, we are aiming at precisely determining the parity violation observable in Yb, which will allow us to probe the distributions of neutrons in different isotopes, investigate physics beyond the Standard Model, as well as to study intra-nucleus weak interactions, through an observation of the anapole moment of Yb nuclei with nonzero spin. We present the experimental principle employed to probe atomic parity violation, describe our new apparatus, and discuss the attained experimental sensitivity as well as the methods for characterizing systematics in these measurements.

physics.atom-ph↗

arXiv2017

Solution nuclear magnetic resonance spectroscopy on a nanostructured diamond chip

We demonstrate nuclear magnetic resonance (NMR) spectroscopy of picoliter-volume solutions with a nanostructured diamond chip. Using optical interferometric lithography, diamond surfaces were nanostructured with dense, high-aspect-ratio nanogratings, enhancing the surface area by more than a factor of 15 over mm^2 regions of the chip. The nanograting sidewalls were doped with nitrogen-vacancy (NV) centers so that more than 10 million NV centers in a (25 micrometer)^2 laser spot are located close enough to the diamond surface (5 nm) to detect the NMR spectrum of 1 pL of fluid lying within adjacent nanograting grooves. The platform was used to perform 1H and 19F NMR spectroscopy at room temperature in magnetic fields below 50 mT. Using a solution of CsF in glycerol, we demonstrate that 4 +/- 2 x 10^12 19F spins in a 1 pL volume, can be detected with a signal-to-noise ratio of 3 in 1 s integration. This represents nearly two orders of magnitude improvement in concentration sensitivity over previous NV and picoliter NMR studies.

cond-mat.mes-hall↗

arXiv2016

Highly spin-polarized deuterium atoms from the UV dissociation of Deuterium Iodide

We report the production of highly spin-polarized Deuterium atoms via photodissociation of deuterium iodide at 270 nm. The velocity distribution of both the deuterium and iodine photodissociation products is performed via velocity mapping slice-imaging. Additionally, the angular momentum polarization of the iodine products is studied using polarization-sensitive ionization schemes. The results are consistent with excitation of the $A^1Π_1$ state followed by adiabatic dissociation. The process produces $\sim$100\% electronically polarized deuterium atoms at the time of dissociation, which is then converted to $\sim 60\%$ nuclear D polarization after $\sim 1.6$ ns. These production times for hyperpolarized deuterium allow collision-limited densities of $\sim 10^{18}$ cm$^{-3}$, which is $\sim 10^6$ times higher than conventional (Stern-Gerlach separation) methods. We discuss how such high-density hyperpolarized deuterium atoms can be combined with laser fusion to measure polarized D-D fusion cross sections.

physics.chem-ph↗

arXiv2014

Towards a new measurement of parity violation in dysprosium

The dysprosium parity violation experiment concluded nearly 17 years ago with an upper limit on weak interaction induced mixing of nearly degenerate, opposite parity states in atomic dysprosium. While that experiment was limited in sensitivity by statistics, a new apparatus constructed in the interim for radio-frequency spectroscopy is expected to provide significant improvements to the statistical sensitivity. Preliminary work from the new PV experiment in dysprosium is presented with a discussion of the current statistical sensitivity and outlook.

physics.atom-ph↗

arXiv2014

Stark shift and parity non-conservation for near-degenerate states of xenon

We identify a pair of near-degenerate states of opposite parity in atomic Xe, the $5p^5 10s \,\, ^2[3/2]_2^o$ at $\rm{E}=94759.927$ cm$^{-1}$ and $5p^5 6f \,\, ^2[5/2]_2$ at $\rm{E}= 94759.935$ cm$^{-1}$, for which parity- and time-odd effects are expected to be enhanced by the small energy separation. We present theoretical calculations which indicate narrow widths for both states and we report a calculated value for the weak matrix element, arising from configuration mixing, of $|W|=2.1$ Hz for $^{132}$Xe. In addition, we measured the Stark effect of the $5p^5\,6f$ $^2[5/2]_{2}$ and $5p^5 \,6f \ ^2[3/2]_2$ ($\rm{E} =94737.121\,\rm{cm}^{-1}$) states. The Stark-shift of the $6f$ states is observed to be negative, revealing the presence of nearby $6g$ states at higher energies, which have not been observed before. The Stark-shift measurements imply an upper limit on the weak matrix element of $|W|\!<\!5$ Hz for the near-degenerate states ($10s \,\, ^2[3/2]_2^o$ and $6f \,\, ^2[5/2]_2$), which is in agreement with the presented calculations.

physics.atom-ph↗

arXiv2013

Fundamentals of Cavity-Enhanced Polarimetry for Parity-Nonconserving Optical Rotation Measurements: Application to Xe, Hg and I

We present the theoretical basis of a cavity-enhanced polarimetric scheme for the measurement of parity-nonconserving (PNC) optical rotation. We discuss the possibility of detecting PNC optical rotation in accessible transitions in metastable Xe and Hg, and ground state I. In particular, the physics of the PNC optical rotation is presented, and we explore the lineshape effects on the expected PNC optical rotation signals. Furthermore, we present an analysis of the eigenpolarizations of the cavity-enhanced polarimeter, which is necessary for understanding the measurement procedure and the ability of employing robust background subtraction procedures using two novel signal reversals. Using recent atomic structure theoretical calculations, we present simulations of the PNC optical rotation signals for all proposed transitions, assuming a range of experimentally feasible parameters. Finally, the possibility of performing sensitive measurements of the nuclear-spin-dependent PNC effects is investigated, for the odd-neutron nuclei $^{129}$Xe and $^{199}$Hg, and the odd-proton nucleus $^{127}$I.

physics.atom-ph↗

arXiv2013

Calculation of parity non-conserving optical rotation in iodine at 1315 nm

We examine the feasibility of a parity non-conserving (PNC) optical rotation experiment for the $^2$P$_{3/2}\rightarrow ^2$P$_{1/2}$ transition of atomic iodine at 1315 nm. The calculated $E1_{\rm PNC}$ to $M1$ amplitude ratio is $R=0.80(16)\times 10^{-8}$. We show that very large PNC rotations (greater than 10 $μ$rad) are obtained for iodine-atom column densities of $\sim 10^{22}$ cm$^{-2}$, which can be produced by increasing the effective interaction pathlength by a factor of $\sim 10^4$ with a high-finesse optical cavity. The simulated signals indicate that measurement of the nuclear anapole moment is feasible, and that a 1% PNC precision measurement should resolve the inconsistency between previous measurements in Cs and Tl.

physics.atom-ph↗