arXiv subjects

L. Bretheau

Publications and source records attributed to L. Bretheau.

16 recordsLinked to original sources

arXiv2026

Fermion parity of an Andreev molecule probed by nonlocal Josephson effect

Fermion parity is a fundamental property of superconducting many-body states. Here, we show that the global fermion parity of a delocalized superconducting state can be detected locally by exploiting the nonlocal Josephson effect. Using a carbon nanotube-based Andreev molecule formed by two coupled quantum-dot Josephson junctions, we observe a pronounced nonlocal Josephson response and demonstrate the formation of delocalized Andreev molecular states extending across both junctions. We further show that changes in the molecular ground-state parity manifest as characteristic $\pi$-phase shifts in the nonlocal response. Supported by a minimal theoretical model, these results identify global fermion parity as an experimentally accessible degree of freedom in hybrid superconducting circuits that can be readily revealed through the nonlocal Josephson effect.

cond-mat.mes-hall↗

arXiv2025

Towards a $\cos(2\varphi)$ Josephson element using aluminum junctions with well-transmitted channels

We introduce a novel method for fabricating all-aluminum Josephson junctions with highly transmitted conduction channels. Such properties are typically associated with structures requiring intricate fabrication processes, such as atomic contacts or hybrid junctions based on semiconducting nanowires and 2D materials. In contrast, our approach relies solely on standard nanofabrication techniques. The resulting devices exhibit a key signature of high-transmission junctions - Multiple Andreev Reflections (MAR) - in their current-voltage characteristics. Furthermore, we propose a straightforward superconducting circuit design based on these junctions, enabling the implementation of a parity-protected qubit.

cond-mat.mes-hall↗

arXiv2025

The carbon nanotube gatemon qubit

Gate-tunable transmon qubits are based on quantum conductors used as weak links within hybrid Josephson junctions. These gatemons have been implemented in just a handful of systems, all relying on extended conductors, namely epitaxial semiconductors or exfoliated graphene. Here we present the coherent control of a gatemon based on a single molecule, a one-dimensional carbon nanotube, which is integrated into a circuit quantum electrodynamics architecture. The measured qubit spectrum can be tuned with a gate voltage and reflects the quantum dot behaviour of the nanotube. Our ultraclean integration, using a hexagonal boron nitride substrate, results in record coherence times of 200ns for carbon nanotube-based qubits. Furthermore, we investigate its decoherence mechanisms, thus revealing a strong gate dependence and identifying charge noise as a limiting factor. On top of positioning carbon nanotubes as contenders for future quantum technologies, our work paves the way for studying microscopic fermionic processes in low-dimensional quantum conductors.

cond-mat.mes-hall↗

arXiv2024

Two-tone spectroscopy of high-frequency quantum circuits with a Josephson emitter

We perform two-tone spectroscopy on quantum circuits, where high-frequency radiation is generated by a voltage-biased superconductor-normal-superconductor Josephson junction and detection is carried out by an ancillary microwave resonator. We implement this protocol on two different systems, a transmon qubit and a $\lambda/4$ resonator. We demonstrate that this two-tone Josephson spectroscopy operates well into the millimeter-wave band, reaching frequencies larger than 80 GHz, and is well-suited for probing highly coherent quantum systems.

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arXiv2024

Josephson junctions based on ultraclean carbon nanotubes

We present a technique for integrating ultraclean carbon nanotubes into superconducting circuits, aiming to realize Josephson junctions based on one-dimensional elementary quantum conductors. This technique primarily involves depositing the nanotube in the final step, thus preserving it from the inherent contaminations of nanofabrication and maintaining contact solely with superconducting electrodes and a crystalline hBN substrate. Through transport measurements performed in both the normal and superconducting states, we demonstrate that our method yields high-quality junctions with Josephson energies suitable for quantum device applications, such as carbon nanotube-based superconducting qubits.

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arXiv2023

Josephson Diode Effect in Andreev Molecules

We propose a new platform for observing the Josephson diode effect: the Andreev molecule. This nonlocal electronic state is hosted in circuits made of two closely spaced Josephson junctions, through the hybridization of the Andreev states. The Josephson diode effect occurs at the level of one individual junction while the other one generates the required time-reversal and spatial-inversion symmetry breaking. We present a microscopic description of this phenomenon based on fermionic Andreev states, focusing on single channels in the short limit, and we compute both supercurrent and energy spectra. We demonstrate that the diode efficiency can be tuned by magnetic flux and the junctions transmissions, and can reach $45~\%$. Going further, by analyzing the Andreev spectra, we demonstrate the key role played by the continuum, which consists of leaky Andreev states and is largely responsible for the critical current asymmetry. On top of proposing an experimentally accessible platform, this work elucidates the microscopic origin of the Josephson diode effect at the level of the fermionic Andreev states.

cond-mat.mes-hall↗

arXiv2017

Observing a quantum Maxwell demon at work

In apparent contradiction to the laws of thermodynamics, Maxwell's demon is able to cyclically extract work from a system in contact with a thermal bath exploiting the information about its microstate. The resolution of this paradox required the insight that an intimate relationship exists between information and thermodynamics. Here, we realize a Maxwell demon experiment that tracks the state of each constituent both in the classical and quantum regimes. The demon is a microwave cavity that encodes quantum information about a superconducting qubit and converts information into work by powering up a propagating microwave pulse by stimulated emission. Thanks to the high level of control of superconducting circuits, we directly measure the extracted work and quantify the entropy remaining in the demon's memory. This experiment provides an enlightening illustration of the interplay of thermodynamics with quantum information.

quant-ph↗

arXiv2016

Using Spontaneous Emission of a Qubit as a Resource for Feedback Control

Persistent control of a transmon qubit is performed by a feedback protocol based on continuous heterodyne measurement of its fluorescence. By driving the qubit and cavity with microwave signals whose amplitudes depend linearly on the instantaneous values of the quadratures of the measured fluorescence field, we show that it is possible to stabilize permanently the qubit in any targeted state. Using a Josephson mixer as a phase-preserving amplifier, it was possible to reach a total measurement efficiency $η$=35%, leading to a maximum of 59% of excitation and 44% of coherence for the stabilized states. The experiment demonstrates multiple-input multiple-output analog Markovian feedback in the quantum regime.

quant-ph↗

arXiv2015

Observing quantum state diffusion by heterodyne detection of fluorescence

A qubit can relax by fluorescence, which prompts the release of a photon into its electromagnetic environment. By counting the emitted photons, discrete quantum jumps of the qubit state can be observed. The succession of states occupied by the qubit in a single experiment, its quantum trajectory, depends in fact on the kind of detector. How are the quantum trajectories modified if one measures continuously the amplitude of the fluorescence field instead? Using a superconducting parametric amplifier, we have performed heterodyne detection of the fluorescence of a superconducting qubit. For each realization of the measurement record, we can reconstruct a different quantum trajectory for the qubit. The observed evolution obeys quantum state diffusion, which is characteristic of quantum measurements subject to zero point fluctuations. Independent projective measurements of the qubit at various times provide a quantitative validation of the reconstructed trajectories. By exploring the statistics of quantum trajectories, we demonstrate that the qubit states span a deterministic surface in the Bloch sphere at each time in the evolution. Additionally, we show that when monitoring fluorescence, coherent superpositions are generated during the decay from excited to ground state. Counterintuitively, measuring light emitted during relaxation can give rise to trajectories with increased excitation probability.

quant-ph↗

arXiv2015

Coherent manipulation of Andreev states in superconducting atomic contacts

Coherent control of quantum states has been demonstrated in a variety of superconducting devices. In all these devices, the variables that are manipulated are collective electromagnetic degrees of freedom: charge, superconducting phase, or flux. Here, we demonstrate the coherent manipulation of a quantum system based on Andreev bound states, which are microscopic quasiparticle states inherent to superconducting weak links. Using a circuit quantum electrodynamics setup we perform single-shot readout of this "Andreev qubit". We determine its excited state lifetime and coherence time to be in the microsecond range. Quantum jumps and parity switchings are observed in continuous measurements. In addition to possible quantum information applications, such Andreev qubits are a testbed for the physics of single elementary excitations in superconductors.

cond-mat.mes-hall↗

arXiv2014

Theory of microwave spectroscopy of Andreev bound states with a Josephson junction

We present a microscopic theory for the current through a tunnel Josephson junction coupled to a non-linear environment, which consists of an Andreev two-level system coupled to a harmonic oscillator. It models a recent experiment [Bretheau, Girit, Pothier, Esteve, and Urbina, Nature (London) 499, 312 (2013)] on photon spectroscopy of Andreev bound states in a superconducting atomic-size contact. We find the eigenenergies and eigenstates of the environment and derive the current through the junction due to inelastic Cooper pair tunneling. The current-voltage characteristic reveals the transitions between the Andreev bound states, the excitation of the harmonic mode that hybridizes with the Andreev bound states, as well as multi-photon processes. The calculated spectra are in fair agreement with the experimental data.

cond-mat.mes-hall↗

arXiv2014

Dynamics of quasiparticle trapping in Andreev levels

We present a theory describing the trapping and untrapping of quasiparticles in the Andreev bound level of a single-channel weak link between two superconductors. We calculate the rates of the transitions between even and odd occupations of the Andreev level induced by absorption and emission of both photons and phonons. We apply the theory to a recent experiment [Phys. Rev. Lett. 106, 257003 (2011)] in which the dynamics of the trapping of quasiparticles in the Andreev levels of superconducting atomic contacts coupled to a Josephson junction was measured. We show that the plasma energy $hν_p$ of the Josephson junction defines a rather abrupt transition between a fast relaxation regime dominated by coupling to photons and a slow relaxation regime dominated by coupling to phonons. With realistic parameters the theory provides a semi-quantitative description of the experimental results.

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arXiv2014

Supercurrent Spectroscopy of Andreev States

We measure the excitation spectrum of a superconducting atomic contact. In addition to the usual continuum above the superconducting gap, the single particle excitation spectrum contains discrete, spin-degenerate Andreev levels inside the gap. Quasiparticle excitations are induced by a broadband on-chip microwave source and detected by measuring changes in the supercurrent flowing through the atomic contact. Since microwave photons excite quasiparticles in pairs, two types of transitions are observed: Andreev transitions, which consists of putting two quasiparticles in an Andreev level, and transitions to odd states with a single quasiparticle in an Andreev level and the other one in the continuum. In contrast to absorption spectroscopy, supercurrent spectroscopy allows detection of long-lived odd states.

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arXiv2013

Exciting Andreev pairs in a superconducting atomic contact

The Josephson effect describes the flow of supercurrent in a weak link, such as a tunnel junction, nanowire, or molecule, between two superconductors. It is the basis for a variety of circuits and devices, with applications ranging from medicine to quantum information. Currently, experiments using Josephson circuits that behave like artificial atoms are revolutionizing the way we probe and exploit the laws of quantum physics. Microscopically, the supercurrent is carried by Andreev pair states, which are localized at the weak link. These states come in doublets and have energies inside the superconducting gap. Existing Josephson circuits are based on properties of just the ground state of each doublet and so far the excited states have not been directly detected. Here we establish their existence through spectroscopic measurements of superconducting atomic contacts. The spectra, which depend on the atomic configuration and on the phase difference between the superconductors, are in complete agreement with theory. Andreev doublets could be exploited to encode information in novel types of superconducting qubits.

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arXiv2012

Superconducting Quantum Point Contacts

We review our experiments on the electronic transport properties of atomic contacts between metallic electrodes, in particular superconducting ones. Despite ignorance of the exact atomic configuration, these ultimate quantum point contacts can be manipulated and well characterized in-situ. They allow performing fundamental tests of the scattering theory of quantum transport. In particular, we discuss the case of the Josephson effect.

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arXiv2011

Evidence for long-lived quasiparticles trapped in superconducting point contacts

We have observed that the supercurrent across phase-biased, highly transmitting atomic size contacts is strongly reduced within a broad phase interval around π. We attribute this effect to quasiparticle trapping in one of the discrete sub-gap Andreev bound states formed at the contact. Trapping occurs essentially when the Andreev energy is smaller than half the superconducting gap Δ, a situation in which the lifetime of trapped quasiparticles is found to exceed 100 \mus. The origin of this sharp energy threshold is presently not understood.

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