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L. Facheris

Publications and source records attributed to L. Facheris.

6 recordsLinked to original sources

Magnetic phase diagram and spin Hamiltonian of antiferromagnet Cs$_2$CoI$_4$

We report comprehensive thermodynamic and neutron scattering measurements on the $S$ = 3/2 antiferromagnet Cs$_2$CoI$_4$, a member of the thoroughly studied family of frustrated magnets Cs$_2MX_4$ ($M$ = Cu, Co, Ru, $X$ = Br, Cl, I, O). Unlike previously studied members, Cs$_2$CoI$_4$ undergoes a structural phase transition, for which we determine the low-temperature crystallographic structure. The resulting symmetry reduction strongly affects both the magnetic exchange interactions and single-ion anisotropy. Despite the large parameter space, we propose a minimal magnetic Hamiltonian that reasonably captures the observed excitation spectrum, analyzed using extended SU(4) linear spin-wave theory.

cond-mat.str-el

Magnetic field-induced phases and spin Hamiltonian in Cs2CoBr4

Magnetic structures and spin excitations are studied across the phase diagram of the geometrically frustrated S = 3/2 quantum antiferromagnet Cs2CoBr4 in magnetic fields applied along the magnetic easy axis, using neutron diffraction, inelastic neutron scattering and THz absorption spectroscopy. The data are analyzed, where appropriate, using extended SU (4) linear spin wave theory. A minimal magnetic Hamiltonian is proposed based on measurements in the high field polarized state. It deviates considerably from the previously considered models. Additional dilatometry experiments highlight the importance of magnetoelastic coupling in this system.

cond-mat.str-el

Confinement of fractional excitations in a triangular lattice antiferromagnet

High-resolution neutron and THz spectroscopies are used to study the magnetic excitation spectrum of Cs$_2$CoBr$_4$, a distorted-triangular-lattice antiferromagnet with nearly XY-type anisotropy. What was previously thought of as a broad excitation continuum [Phys. Rev. Lett. 129, 087201 (2022)] is shown to be a series of dispersive bound states reminiscent of "Zeeman ladders" in quasi-one-dimensional Ising systems. At wave vectors where inter-chain interactions cancel at the Mean Field level, they can indeed be interpreted as bound finite-width kinks in individual chains. Elsewhere in the Brillouin zone their true two-dimensional structure and propagation are revealed.

cond-mat.str-el

Spin Density Wave versus Fractional Magnetization Plateau in a Triangular Antiferromagnet

We report an excellent realization of the highly non-classical incommensurate spin-density wave (SDW) state in the quantum frustrated antiferromagnetic insulator Cs$_2$CoBr$_4$. In contrast to the well-known Ising spin chain case, here the SDW is stabilized by virtue of competing planar in-chain anisotropies and frustrated interchain exchange. Adjacent to the SDW phase is a broad $m = 1/3$ magnetization plateau that can be seen as a commensurate locking of the SDW state into the up-up-down (UUD) spin structure. This represents the first example of long-sought SDW-UUD transition in triangular-type quantum magnets.

cond-mat.str-el

Magnetization plateaux cascade in the frustrated quantum antiferromagnet Cs$_2$CoBr$_4$

We have found an unusual competition of two frustration mechanisms in the 2D quantum antiferromagnet Cs$_2$CoBr$_4$. The key actors are the alternation of single-ion planar anisotropy direction of the individual magnetic Co$^{2+}$ ions, and their arrangement in a distorted triangular lattice structure. In particular, the uniquely oriented Ising-type anisotropy emerges from the competition of easy-plane ones, and for a magnetic field applied along this axis one finds a cascade of five ordered phases at low temperatures. Two of these phases feature magnetization plateaux. The low-field one is supposed to be a consequence of a collinear ground state stabilized by the anisotropy, while the other plateau bears characteristics of an "up-up-down" state exclusive for lattices with triangular exchange patterns. Such coexistence of the magnetization plateaux is a fingerprint of competition between the anisotropy and the geometric frustration in Cs$_2$CoBr$_4$.

cond-mat.str-el

Finite-temperature dynamics and the role of disorder in nearly critical Ni(Cl$_{1-x}$Br$_x$)$_2$$\cdot$4SC(NH$_2$)$_2$

Inelastic neutron scattering is used to investigate the temperature dependence of spin correlations in the 3-dimensional XY antiferromagnet Ni(Cl$_{1-x}$Br$_x$)$_2$$\cdot$4SC(NH$_2$)$_2$, $ x = 0.14(1)$, tuned close to the chemical-composition-induced soft-mode transition. The local dynamic structure factor shows $\hbarω/T$ scaling behavior characteristic of a quantum critical point. The deviation of the measured critical exponent from spin wave theoretical expectations are attributed to disorder. Another effect of disorder is local excitations above the magnon band. Their energy, structure factor and temperature dependence are well explained by simple strong-bond dimers associated with Br-impurity sites.

cond-mat.str-el