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L. G. Sobotka

Publications and source records attributed to L. G. Sobotka.

At least 19 recordsLinked to original sources

Differential cross sections for ${{^{12}\mathrm{C}(n,α_{0})}}$, ${{^{16}\mathrm{O}(n,α_{0})}}$ and ${{^{16}\mathrm{O}(n,α_{1,2,3})}}$ between ${E_n}$ = 7.2 and 10 MeV with an active-target Time Projection Chamber

Data for the ${{^{12}\mathrm{C}(n,α_{0})}}$, ${{^{16}\mathrm{O}(n,α_{0})}}$ and ${{^{16}\mathrm{O}(n,α_{1,2,3})}}$ differential cross sections are important for several different areas of nuclear physics such as understanding neutron transmutation in nuclear reactors. The TexAT Time Projection Chamber was used to measure the differential and angle-integrated cross sections in active-target mode. The chamber was filled with CO$_2$ gas and used a quasi-monoenergetic neutron beam from the $d(d,n)$ reaction at Edwards Accelerator Lab at Ohio University. A comparison between our current and previous results at overlapping energies and angles which showed good agreement in angular dependence and absolute cross section. A broader angular coverage than previous results demonstrated that the integrated cross section for the \po16 reaction deviates from ENDFVIII.0 evaluations. This first instance of neutron-induced measurements with an active-target Time Projection Chamber demonstrates the use of this method for high-quality differential cross section data across a broad angular range, generating good statistics with a relatively low-intensity beam.

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Comparing invariant-mass spectroscopy of 8B with ab initio predictions

Levels in 8B have been investigated experimentally using the invariant-mass technique and compared to ab initio calculations. Data sets obtained using E/A=69-MeV 9C and 13O beams on a Be target have been further analyzed to extend the level scheme of 8B for Ex<10 MeV. New levels were observed in the 2p+6Li, p+3He+alpha, and the p+7Be+gamma exit channels. Momentum correlations between the decay fragments were also investigated in order to deduce the decay pathways and whether the decays are prompt or sequential. This nucleus and its mirror were also investigated in the ab initio symmetry-adapted no-core shell model. Correspondence between the newly observed and predicted levels were made based on the level energy and the decay modes. For positive parity levels with J<=3, all predicted levels can be connected to an experimental counter part (as least tentatively) for Ex<8.4 MeV.

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Triplet of kindred prompt-2p emitters in mass-8 proton-rich nuclei

A triplet of kindred prompt-2p emitters in A=8 nuclei has been demonstrated. Two of these are the ground state of 8C and its isobaric analog state in 8B, both of which are analogs of the halo or thick-skinned nucleus 8He. The third member is the recently found fourth 1+ state in 8B. This new 8B state at E*=8.4 MeV was observed to decay to the ground state of 6Li by 2p emission. Momentum correlations between the decay products indicate that it is not a sequential 2p decay through a 7Be intermediate state, but indicative of prompt 2p emission with correlations similar to those of the other members of the triplet. Ab initio calculations with the symmetry-adapted nocore shell model indicate that these three states have very similar spatial wavefunctions, but with nucleons coupling to different spins, isospins, and isospin projections. The triplet of 2p emitters all have oblate shapes and by stripping two protons equatorially, decay to states which have prolate shapes.

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Deviations from the Isobaric Multiplet Mass Equation due to threshold states

Recent studies have completed the A=16 isospin quintets for states with spin/parity Jπ =0+ and 2+. The dependence of their masses as a function of isospin projection shows evidence for deviations from quadratic behavior indicating isospin violation beyond the expectation from two- body forces. The deviation is most pronounced for the 2+ states. Predictions from the Shell Model Embedded in the Continuum (SMEC) allow us to explain that this isospin violation is associated with a modification of the nuclear structure due to the open-quantum-system nature of the proton- rich members of the quintet. In particular, the 0+ and 2+ states in 16Ne and the 2+ state in 16F are threshold resonances located just above a proton-decay threshold where s-wave coupling to the continuum is expected. The measured deviations of these threshold states from the quadratic behavior of the remaining members of the multiplets makes it possible to obtain information on the magnitude and the energy dependence of the continuum-coupling energy correction. Continuum coupling is also indicated for the ground state of 8C, but this time through p-wave coupling.

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Strong evidence for 9N and the limits of existence of atomic nuclei

The boundaries of the Chart of Nuclides contain exotic isotopes that possess extreme proton-toneutron asymmetries. Here we report on strong evidence of 9N, one of the most exotic proton-rich isotopes where more than one half of its constitute nucleons are unbound. With seven protons and two neutrons, this extremely proton-rich system would represent the first-known example of a ground-state five-proton emitter. The invariant-mass spectrum of its decay products can be fit with two peaks whose energies are consistent with the theoretical predictions of an open-quantum-system approach, however we cannot rule out the possibility that only a single resonance-like peak is present in the spectrum.

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Silicon tracker array for RIB experiments at SAMURAI

This work describes a silicon tracker system developed for experiments with proton-rich radioactive ion beams at the SAMURAI superconducting spectrometer of RIBF at RIKEN. The system is designed for accurate angular reconstruction and atomic number identification of relativistic heavy ions and protons which are simultaneously produced in reactions motivated by studies of proton capture reactions of interest for nuclear astrophysics. The technical characteristics of the tracking array are described in detail as are its performance in two pilot experiments. The physics justification for such a system is also presented.

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Nucleon-nucleon correlations in the extreme oxygen isotopes

There has been an upsurge of interest in two-nucleon decays thanks to the studies of nucleon-nucleon correlations. In our previous work, based on a novel time-dependent three-body approach, we demonstrated that the energy and angular correlations of the emitted nucleons can shed light on the structure of nucleonic pairs formed inside the nucleus. In this work, we apply the new framework to study the decay dynamics and properties of some extreme proton-rich and neutron-rich oxygen isotopes, including two-proton ($2p$) decays of $^{11,12}$O and two-neutron ($2n$) decay of $^{26}$O. Here we show that the low-$\ell$ components of $^{11,12}$O wave functions, which are affected by continuum and configuration-interaction effects, strongly impact decay dynamics and asymptotic correlations. In the calculated wave functions of $^{11,12}$O, diproton and cigarlike structures merge together during the tunneling process and the resulting energy- and angular correlations are very consistent with the experimental data. The asymptotic correlations of the $2n$ decay of $^{26}$O dramatically change as the two-neutron decay energy approaches the zero-energy threshold. The small reported value of $Q_{2n}$ suggests that the $2n$ decay of this nucleus can be understood in terms of the universal phase-space limit.

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Using spin alignment of inelastically-excited fast beams to make spin assignments: the spectroscopy of 13O as a test case

Excited states in 13O were investigated using inelastic scattering of an E/A=69.5-MeV 13O beam off of a 9Be target. The excited states were identified in the invariant-mass spectra of the decay products. Both single proton and sequential two-proton decays of the excited states were examined. For a number of the excited states, the protons were emitted with strong anisotropy where emissions transverse to the beam axis are favored. The measured proton-decay angular distributions were compared to predictions from distorted-wave born-approximation (DWBA) calculations of the spin alignment which was shown to be largely independent of the excitation mechanism. The deduced $^{13}$O level scheme is compared to ab initio no-core shell model with continuum (NCSMC) predictions. The lowest-energy excited states decay isotropically consistent with predictions of strong proton 1s1/2 structure. Above these states in the level scheme, we observed a number of higher-spin states not predicted within the model. Possibly these are associated with rotational bands built on deformed cluster configurations predicted by antisymmetrized molecular dynamics (AMD) calculations. The spin alignment mechanism is shown to be useful for making spin assignments and may have widespread use.

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A Position and Pulse Shape Discriminant p-Terphenyl Detector Module

We present the development of a neutron detector array module made with $\textit{para}$-terphenyl, a bright, fast, n/$γ$ discriminating crystalline organic scintillator. The module is comprised of 2 cm $\times$ 2 cm $\times$ 2 cm $\textit{p}$-terphenyl crystals that have been optically coupled together to create a $\textit{pseudo-bar}$ module. While only relying on two photo detectors, the module is capable of distinguishing interactions between up to eight crystals. Furthermore, the module retains the $\textit{p}$-terphenyl's pulse shape discrimination (PSD) capability. Together this makes the pseudo-bar module a promising position-sensitive neutron detector. Here we present characteristics of the pseudo-bar module - its timing resolution as well as its pulse shape and position discrimination capabilities, and briefly discuss future plans for utilizing an array of pseudo-bar modules in a useful neutron detector system.

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Evidence against the Efimov effect in $^{12}\mathrm{C}$ from spectroscopy and astrophysics

Background: The Efimov effect is a universal phenomenon in physics whereby three-body systems are stabilized via the interaction of an unbound two-body sub-systems. A hypothetical state in $^{12}\mathrm{C}$ at 7.458 MeV excitation energy, comprising of a loose structure of three $α$-particles in mutual two-body resonance, has been suggested in the literature to correspond to an Efimov state in nuclear physics. The existence of such a state has not been demonstrated experimentally. Method: Using the combined data sets from two recent experiments, one with the TexAT TPC to measure $α$-decay and the other with Gammasphere to measure $γ$-decay of states in $^{12}\mathrm{C}$ populated by $^{12}\mathrm{N}$ and $^{12}\mathrm{B}$ $β$-decay respectively, we achieve high sensitivity to states in close-proximity to the $α$-threshold in $^{12}\mathrm{C}$. Results: No evidence of a state at 7.458 MeV is seen in either data set. Using a likelihood method, the 95\% C.L. $γ$-decay branching ratio is determined as a function of the $β$-decay feeding strength relative to the Hoyle state. In parallel, calculations of the triple-alpha reaction rate show the inclusion of the Efimov corresponds to a large increase in the reaction rate around $5 \times 10^{7}$ K. Conclusion: From decay spectroscopy - at the 95\% C.L., the Efimov state cannot exist at 7.458 MeV with any $γ$-decay branching ratio unless the $β$-strength is less than 0.7\% of the Hoyle state. This limit is evaluated for a range of different excitation energies and the results are not favorable for existence of the hypothetical Efimov state in $^{12}\mathrm{C}$. Furthermore, the triple-alpha reaction rate with the inclusion of a state between 7.43 and 7.53 MeV exceeds the rate required for stars to undergo the red giant phase.

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Almost medium-free measurement of the Hoyle state direct-decay component with a TPC

Background: The structure of the Hoyle state, a highly $α$-clustered state at 7.65 MeV in $^{12}\mathrm{C}$, has long been the subject of debate. Understanding if the system comprises of three weakly-interacting $α$-particles in the 0s orbital, known as an $α$-condensate state, is possible by studying the decay branches of the Hoyle state. Purpose: The direct decay of the Hoyle state into three $α$-particles, rather than through the $^{8}\mathrm{Be}$ ground state, can be identified by studying the energy partition of the 3 $α$-particles arising from the decay. This paper provides details on the break-up mechanism of the Hoyle stating using a new experimental technique. Method: By using beta-delayed charged-particle spectroscopy of $^{12}\mathrm{N}$ using the TexAT (Texas Active Target) TPC, a high-sensitivity measurement of the direct 3 $α$ decay ratio can be performed without contributions from pile-up events. Results: A Bayesian approach to understanding the contribution of the direct components via a likelihood function shows that the direct component is $<0.043\%$ at the 95\% confidence level (C.L.). This value is in agreement with several other studies and here we can demonstrate that a small non-sequential component with a decay fraction of about $10^{-4}$ is most likely. Conclusion: The measurement of the non-sequential component of the Hoyle state decay is performed in an almost medium-free reaction for the first time. The derived upper-limit is in agreement with previous studies and demonstrates sensitivity to the absolute branching ratio. Further experimental studies would need to be combined with robust microscopic theoretical understanding of the decay dynamics to provide additional insight into the idea of the Hoyle state as an $α$-condensate.

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Isotopically resolved neutron total cross sections at intermediate energies

The neutron total cross sections $σ_{tot}$ of $^{16,18}$O, $^{58,64}$Ni, $^{103}$Rh, and $^{112,124}$Sn have been measured at the Los Alamos Neutron Science Center (LANSCE) from low to intermediate energies (3 $\leq E_{lab} \leq$ 450 MeV) by leveraging waveform-digitizer technology. The $σ_{tot}$ relative differences between isotopes are presented, revealing additional information about the isovector components needed for an accurate optical-model description away from stability. Digitizer-enabled $σ_{tot}$-measurement techniques are discussed and a series of uncertainty-quantified dispersive optical model (DOM) analyses using these new data is presented, validating the use of the DOM for modeling light systems ($^{16,18}$O) and systems with open neutron shells ($^{58,64}$Ni and $^{112,124}$Sn). The valence-nucleon spectroscopic factors extracted for each isotope reaffirm the usefulness of high-energy proton reaction cross sections for characterizing depletion from the mean-field expectation.

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Systematic Matter and Binding-Energy Distributions from a Dispersive Optical Model Analysis

We present the first systematic nonlocal dispersive optical model analysis using both bound-state and scattering data of $^{16,18}$O, $^{40,48}$Ca, $^{58,64}$Ni, $^{112,124}$Sn, and $^{208}$Pb. In all systems, roughly half the total nuclear binding energy is associated with the most-bound 10% of the total nucleon density. The extracted neutron skins reveal the interplay of asymmetry, Coulomb, and shell effects on the skin thickness. Our results indicate that simultaneous optical model fits of inelastic scattering and structural data on isotopic pairs are effective for constraining asymmetry-dependent nuclear structural quantities otherwise difficult to observe experimentally.

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Particle decays of levels in $^{11,12}$N and $^{12}$O investigated with the invariant-mass method

Particle-decaying states of the light nuclei $^{11,12}$N and $^{12}$O were studied using the invariant-mass method. The decay energies and intrinsic widths of a number of states were measured, and the momentum correlations of three-body decaying states were considered. A second 2$p$-decaying 2$^+$ state of $^{12}$O was observed for the first time, and a higher energy $^{12}$O state was observed in the 4$p$+2$α$ decay channel. This 4$p$+2$α$ channel also contains contributions from fission-like decay paths, including $^6$Be$_{g.s.}$+$^{6}$Be$_{g.s.}$. Analogs to these states in $^{12}$O were found in $^{12}$N in the 2$p$+$^{10}$B and 2$p$+$α$+$^6$Li channels. The momentum correlations for the prompt 2$p$ decay of $^{12}$O$_{g.s.}$ were found to be nearly identical to those of $^{16}$Ne$_{g.s.}$, and the correlations for the new 2$^+$ state were found to be consistent with sequential decay through excited states in $^{11}$N. The momentum correlations for the 2$^+_1$ state in $^{12}$O provide a new value for the $^{11}$N ground-state energy. The states in $^{12}$N/$^{12}$O that belong to the $A$=12 isobaric sextet do not deviate from the quadratic isobaric multiplet mass equation (IMME) form.

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Invariant-mass spectroscopy of $^{14}$O excited states

Excited states in $^{14}$O have been investigated both experimentally and theoretically. Experimentally, these states were produced via neutron-knockout reactions with a fast $^{15}$O beam and the invariant-mass technique was employed to isolate the 1$p$ and 2$p$ decay channels and determine their branching ratios. The spectrum of excited states was also calculated with the Shell Model Embedded in the Continuum that treats bound and scattering states in a unified model. By comparing energies, widths and decay branching patterns, spin and parity assignments for all experimentally observed levels below 8 MeV are made. This includes the location of the second 2$^{+}$ state that we find is in near degeneracy with the third 0$^{+}$ state. An interesting case of sequential 2$p$ decay through a pair of degenerate $^{13}$N excited states with opposite parities was found where the interference between the two sequential decay pathways produces an unusual relative-angle distribution between the emitted protons.

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First observation of unbound $^{11}$O, the mirror of the halo nucleus $^{11}$Li

The structure of the extremely proton-rich nucleus $^{11}_{~8}$O$_3$, the mirror of the two-neutron halo nucleus $^{11}_{~3}$Li$_8$, has been studied experimentally for the first time. Following two-neutron knockout reactions with a $^{13}$O beam, the $^{11}$O decay products were detected after two-proton emission and used to construct an invariant-mass spectrum. A broad peak of width $\sim$3\,MeV was observed. Within the Gamow coupled-channel approach, it was concluded that this peak is a multiplet with contributions from the four-lowest $^{11}$O resonant states: $J^π$=3/2$^-_1$, 3/2$^-_2$, 5/2$^+_1$, and 5/2$^+_2$. The widths and configurations of these states show strong, non-monotonic dependencies on the depth of the $p$-$^9$C potential. This unusual behavior is due to the presence of a broad threshold resonant state in $^{10}$N, which is an analog of the virtual state in $^{10}$Li in the presence of the Coulomb potential. After optimizing the model to the data, only a moderate isospin asymmetry between ground states of $^{11}$O and $^{11}$Li was found.

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Structures and decay properties of extremely proton-rich nuclei $^{11,12}$O

${\rm \bf Background:}$ The recent observation of the unbound nucleus $^{11}$O offers the unique possibility to study how the structure and dynamics of two-proton ($2p$) decay is affected by the removal of one neutron from $^{12}$O, and provides important information on the Thomas-Ehrman effect in the mirror pairs $^{11}_{~8}$O$_3$-$^{11}_{~3}$Li$_8$ and $^{12}_{~8}$O$_4$-$^{12}_{~4}$Be$_8$, which involve the $2p$ emitters $^{11}$O and $^{12}$O. ${\rm \bf Purpose:}$ We investigate how continuum effects impact the structure and decay properties of $^{11}$O and $^{12}$O, and their mirror partners. ${\rm \bf Methods:}$ We solve the three-body core-nucleon-nucleon problem using the Gamow coupled-channel (GCC) method. The GCC Hamiltonian employs a realistic finite-range valence nucleon-nucleon interaction and the deformed cores of $^{9,10}$C, $^{9}$Li, and $^{10}$Be. ${\rm \bf Results:}$ We calculate the energy spectra and decay widths of $^{11}$O and $^{12}$O as well as those of their mirror nuclei. In particular, we investigate the dynamics of the $2p$ decay in the ground state of $^{12}$O by analyzing the evolution of the $2p$ configuration of the emitted protons as well as their angular correlations in the coordinate space. We also show how the analytic structure of the resonant states of $^{10}$Li and $^{10}$N impacts the low-lying states of $^{11}$Li and $^{11}$O. ${\rm \bf Conclusions:}$ We demonstrate that, in both nuclei $^{11}$O and $^{12}$O, there is a competition between direct and "democratic" $2p$ ground-state emission. The broad structure observed in $^{11}$O is consistent with four broad resonances, with the predicted $3/2^-_1$ ground state strongly influenced by the broad threshold resonant state in $^{10}$N, which is an isobaric analog of the antibound (or virtual) state in $^{10}$Li.

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Invariant-mass spectroscopy of $^{18}$Ne, $^{16}$O, and $^{10}$C excited states formed in neutron transfer reactions

Neutron transfer reactions with fast secondary beams of $^{17}$Ne, $^{15}$O, and $^9$C have been studied with the HiRA and CAESAR arrays. Excited states of $^{18}$Ne, $^{16}$O, and $^{10}$C in the continuum have been identified using invariant-mass spectroscopy. The best experimental resolution of these states is achieved by selecting events where the decay fragments are emitted transverse to the beam direction. We have confirmed a number of spin assignments made in previous works for the negative-parity states of $^{18}$Ne. In addition we have found new higher-lying excited states in $^{16}$O and $^{18}$Ne, some of which fission into two ground-state $^8$Be fragments. Finally for $^{10}$C, a new excited state was observed. These transfer reactions were found to leave the remnant of the $^9$Be target nuclei at very high excitation energies and maybe associated with the pickup of a deeply-bound $^9$Be neutron.

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