arXiv subjects

L. J. Sun

Publications and source records attributed to L. J. Sun.

At least 19 recordsLinked to original sources

arXiv2026

Precision $\beta$-delayed charged-particle emission spectroscopy at FRIB: Proof of principle with the $\beta$-decay of $^{25}\mathrm{Si}$

We report on the $\beta$-delayed proton and $\gamma$-ray emission from $^{25}\mathrm{Si}$, measured at the Facility for Rare Isotope Beams (FRIB). Low-energy $^{25}\mathrm{Si}$ ions extracted from the Advanced Cryogenic Gas Stopper were implanted into a thin carbon foil surrounded by a compact, highly segmented array of silicon detector telescopes and two high-purity germanium detectors. This setup provides high-resolution charged-particle spectroscopy, establishing a proof of principle for precision stopped-beam decay studies at FRIB. We reconstruct the $^{25}\mathrm{Si}$ decay scheme, resolving new high-energy proton transitions and determining the feeding to excited states in $^{24}\mathrm{Mg}$. The observation of spectral interference patterns enables firm spin and parity assignments for highly excited states in $^{25}\mathrm{Al}$. The $^{25}\mathrm{Si}$ $\beta$-strength distribution is extracted and compared with large-scale shell-model calculations.

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arXiv2026

Direct Measurement of the $^{59}$Cu$(p,\alpha)^{56}$Ni Excitation Function to Constrain the Ni--Cu Cycle Strength and Its Impact on Explosive Nucleosynthesis

A new direct measurement of the 59Cu(p,a)56Ni excitation function from 2.43-5.88 MeV in the center-of-mass was performed in inverse kinematics using the high-efficiency MUSIC active-target detector at FRIB. This reaction plays a critical role in constraining the strength of the NiCu cycle in different explosive astrophysical scenarios such as Type I X-ray bursts and the nu-p process in neutrino-driven winds after a core-collapse supernova. The newly derived stellar rate is systematically lower than previous estimates, suppressing NiCu cycle recycling in X-ray bursts to below 3% and enhancing nu-p process efficiency throughout the relevant temperature range, potentially extending its effective operation to temperatures as high as T9 = 3.94 (+0.99/-0.85).

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arXiv2026

Detailed Study of the $^{59}$Cu(p,$\alpha)^{56}$Ni Reaction and Constraints on Its Astrophysical Reaction Rate

The $^{59}$Cu$(p,\alpha)^{56}$Ni reaction plays an important role in explosive astrophysical scenarios such as Type I X-ray bursts and the $\nu p$-process in neutrino-driven winds following a core-collapse supernova, where it regulates the flow of nucleosynthesis through the NiCu cycle and the synthesis of heavier nuclei. We present a direct measurement of the $^{59}\mathrm{Cu}(p,\alpha)^{56}\mathrm{Ni}$ excitation function from 2.43--5.88~MeV in the center-of-mass frame, performed in inverse kinematics with the high-efficiency MUSIC active-target detector at FRIB. The angle- and energy-integrated cross sections extend direct measurements to lower energies than previously reported and remove the angular-integration model dependence of earlier work. To extrapolate the rate to astrophysical energies, we constrain the statistical-model description through a systematic optimization of the DEM-3 $\alpha$-optical model potential geometry, and quantify the model-selection uncertainty with a Bayesian model averaging analysis over 96 TALYS combinations. The resulting stellar rate carries a temperature-dependent uncertainty factor of 1.26--1.63 over $T_9 = 0.2$--10 and is systematically lower than the REACLIB evaluation, remaining below the competing $(p,\gamma)$ rate for $T_9 \lesssim 3.94$. These results substantially weaken the inferred NiCu cycle strength and establish the $^{59}$Cu$(p,\gamma)^{60}$Zn rate as the dominant remaining uncertainty.

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arXiv2026

A ground state $^{22}$Al halo is unlikely

We report the decisive resolution of the ground state spin and parity of the proton-dripline nucleus $^{22}$Al, a prime candidate for a proton halo. The resolution stems from the first $β$-delayed charged particle emission experiment in the Gas Stopping Area at the Facility for Rare Isotope Beams (FRIB), leveraging high-intensity, low-energy beams extracted from the Advanced Cryogenic Gas Stopper (ACGS). The pristine beam quality from FRIB and the ACGS enabled a sensitive particle identification technique using thin silicon detectors, allowing for the suppression of the dominant proton background and the first observation of the weak $β$-delayed $α$ transition from the Isobaric Analog State in $^{22}$Mg to the $^{18}$Ne ground state. This observation uniquely fixes the $^{22}$Al ground state as $4^+$. The valence proton is confined by a dominant $d$-wave centrifugal barrier which, combined with the Coulomb repulsion, hinders the tunneling required for halo formation despite the exceptionally low proton separation energy of $^{22}$Al.

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arXiv2025

Extension of the particle x-ray coincidence technique: The lifetimes and branching ratios apparatus

The particle x-ray coincidence technique (PXCT) was originally developed to measure average lifetimes in the $10^{-17}-10^{-15}$~s range for proton-unbound states populated by electron capture (EC). We have designed and built the Lifetimes and Branching Ratios Apparatus (LIBRA) to be used in the stopped-beam area at the Facility for Rare Isotope Beams that extends PXCT to measure lifetimes and decay branching ratios of resonances populated by EC/$β^+$ decay. The first application of LIBRA aims to obtain essential nuclear data from $^{60}$Ga EC/$β^+$ decay to constrain the thermonuclear rates of the $^{59}$Cu$(p,γ)^{60}$Zn and $^{59}$Cu$(p,α)^{56}$Ni reactions, and in turn, the strength of the NiCu nucleosynthesis cycle, which is predicted to significantly impact the modeling of type I x-ray burst light curves and the composition of the burst ashes. Detailed theoretical calculations, Monte Carlo simulations, and performance tests with radioactive sources have been conducted to validate the feasibility of employing LIBRA for the $^{60}$Ga experiment. LIBRA can be utilized to measure most essential ingredients needed for charged-particle reaction rate calculations in a single experiment, in the absence of direct measurements, which are often impractical for radioactive reactants.

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arXiv2025

Object Detection with Deep Learning for Rare Event Search in the GADGET II TPC

In the pursuit of identifying rare two-particle events within the GADGET II Time Projection Chamber (TPC), this paper presents a comprehensive approach for leveraging Convolutional Neural Networks (CNNs) and various data processing methods. To address the inherent complexities of 3D TPC track reconstructions, the data is expressed in 2D projections and 1D quantities. This approach capitalizes on the diverse data modalities of the TPC, allowing for the efficient representation of the distinct features of the 3D events, with no loss in topology uniqueness. Additionally, it leverages the computational efficiency of 2D CNNs and benefits from the extensive availability of pre-trained models. Given the scarcity of real training data for the rare events of interest, simulated events are used to train the models to detect real events. To account for potential distribution shifts when predominantly depending on simulations, significant perturbations are embedded within the simulations. This produces a broad parameter space that works to account for potential physics parameter and detector response variations and uncertainties. These parameter-varied simulations are used to train sensitive 2D CNN object detectors. When combined with 1D histogram peak detection algorithms, this multi-modal detection framework is highly adept at identifying rare, two-particle events in data taken during experiment 21072 at the Facility for Rare Isotope Beams (FRIB), demonstrating a 100% recall for events of interest. We present the methods and outcomes of our investigation and discuss the potential future applications of these techniques.

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arXiv2023

Time Projection Chamber for GADGET II

Background: The established GADGET detection system, designed for measuring weak, low-energy $β$-delayed proton decays, features a gaseous Proton Detector with MICROMEGAS readout for calorimetric particle detection, surrounded by a Segmented Germanium Array for high-resolution prompt $γ$-ray detection. Purpose: To upgrade GADGET's Proton Detector to operate as a compact Time Projection Chamber (TPC) for the detection, 3D imaging and identification of low-energy $β$-delayed single- and multi-particle emissions mainly of interest to astrophysical studies. Method: A new high granularity MM board with 1024 pads has been designed, fabricated, installed and tested. A high-density data acquisition system based on Generic Electronics for TPCs has been installed and optimized to record and process the gas avalanche signals collected on the readout pads. The TPC's performance has been tested using a $^{220}$Rn $α$-particle source and cosmic-ray muons. In addition, decay events in the TPC have been simulated by adapting the ATTPCROOT data analysis framework. Further, a novel application of 2D convolutional neural networks for GADGET II event classification is introduced. Results: The GADGET II TPC is capable of detecting and identifying $α$-particles, as well as measuring their track direction, range, and energy. It has also been demonstrated that the GADGET II TPC is capable of tracking cosmic-ray muons. In addition to being one of the first generation of micro pattern gaseous detectors to utilize a resistive anode applied to low-energy nuclear physics, the GADGET II TPC will also be the first TPC surrounded by a high-efficiency array of high-purity germanium $γ$-ray detectors. \textbf{Conclusions:} The TPC of GADGET II has been designed, fabricated, tested, and is ready for operation at the FRIB for radioactive beam-line experiments.

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arXiv2022

First application of Markov Chain Monte Carlo-based Bayesian data analysis to the Doppler-Shift Attenuation Method

Motivated primarily by the large uncertainties in the thermonuclear rate of the $^{30}$P$(p,γ)^{31}$S reaction that limit our understanding of classical novae, we carried out lifetime measurements of $^{31}$S excited states using the Doppler Shift Lifetimes (DSL) facility at the TRIUMF Isotope Separator and Accelerator (ISAC-II) facility. The $^{31}$S excited states were populated by the $^{3}$He$(^{32}$S$,α)^{31}$S reaction. The deexcitation $γ$ rays were detected by a clover-type high-purity germanium detector in coincidence with the $α$ particles detected by a silicon detector telescope. We have applied modern Markov chain Monte Carlo-based Bayesian methods to perform lineshape analyses of Doppler-shift attenuation method $γ$-ray data for the first time. We have determined the lifetimes of the two lowest-lying $^{31}$S excited states. First experimental upper limits on the lifetimes of four higher-lying states have been obtained. The experimental results were compared to shell-model calculations using five universal $sd$-shell Hamiltonians. Evidence for $γ$ rays originating from the astrophysically important $J^π=3/2^+$, 260-keV $^{30}$P$(p,γ)^{31}$S resonance has also been observed, although strong constraints on the lifetime will require better statistics.

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arXiv2022

$β^{+}$ Gamow-Teller strengths from unstable $^{14}$O via the $(d,{}^2\text{He})$ reaction in inverse kinematics

For the first time, the $(d,{}^2\text{He})$ reaction was successfully used in inverse kinematics to extract the Gamow-Teller transition strength in the $β^{+}$ direction from an unstable nucleus. The nucleus studied was $^{14}$O, and the Gamow-Teller transition strength to $^{14}$N was extracted up to an excitation energy of 22 MeV. The measurement of the $(d,{}^2\text{He})$ reaction in inverse kinematics was made possible by the combination of an active target time projection chamber and a magnetic spectrometer. The data were used to test shell-model and state-of-the-art coupled cluster calculations. Shell-model calculations reproduce the measured Gamow-Teller strength distribution up to about 15 MeV reasonably well, after the application of a phenomenological quenching factor. Coupled-cluster calculation reproduces the full strength distribution well without such quenching, owing to the large model space, the inclusion of strong correlations, and the coupling of the weak interaction to two nucleons through two-body currents. This indicates that such calculations provide a very promising path for answering long-standing questions about the observed quenching of Gamow-Teller strengths in nuclei.

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arXiv2022

Constraining the $^{30}$P($p,γ)^{31}$S reaction rate in ONe novae via the weak, low-energy, $β$-delayed proton decay of $^{31}$Cl

The $^{30}$P$(p,γ)^{31}$S reaction plays an important role in understanding nucleosynthesis of $A\geq 30$ nuclides in oxygen-neon novae. The Gaseous Detector with Germanium Tagging was used to measure $^{31}$Cl $β$-delayed proton decay through the key $J^π=3/2^{+}$, 260-keV resonance. The intensity $I^{260}_{βp} = 8.3^{+1.2}_{-0.9} \times 10^{-6}$ represents the weakest $β$-delayed, charged-particle emission ever measured below 400 keV, resulting in a proton branching ratio of $Γ_p / Γ= 2.5^{+0.4}_{-0.3} \times 10^{-4}$. By combining this measurement with shell-model calculations for $Γ_γ$ and past work on other resonances, the total $^{30}$P$(p,γ)^{31}$S rate has been determined with reduced uncertainty. The new rate has been used in hydrodynamic simulations to model the composition of nova ejecta, leading to a concrete prediction of $^{30}$Si/$^{28}$Si excesses in presolar nova grains and the calibration of nuclear thermometers.

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arXiv2021

$^{25}$Si $β^+$-decay spectroscopy

$β$-decay spectroscopy provides valuable information on exotic nuclei and a stringent test for nuclear theories beyond the stability line. To search for new $β$-delayed protons and $γ$ rays of $^{25}$Si to investigate the properties of $^{25}$Al excited states. $^{25}$Si $β$ decays were measured by using the Gaseous Detector with Germanium Tagging system at the National Superconducting Cyclotron Laboratory. The protons and $γ$ rays emitted in the decay were detected simultaneously. A Monte Carlo method was used to model the Doppler broadening of $^{24}$Mg $γ$-ray lines caused by nuclear recoil from proton emission. Shell-model calculations using two newly developed universal \textit{sd}-shell Hamiltonians, USDC and USDI, were performed. The most precise $^{25}$Si half-life to date has been determined. A new proton branch at 724(4)~keV and new proton-$γ$-ray coincidences have been identified. Three $^{24}$Mg $γ$-ray lines and eight $^{25}$Al $γ$-ray lines are observed for the first time in $^{25}$Si decay. The first measurement of the $^{25}$Si $β$-delayed $γ$ ray intensities through the $^{25}$Al unbound states is reported. All the bound states of $^{25}$Al are observed to be populated in the $β$ decay of $^{25}$Si. Several inconsistencies between the previous measurements have been resolved, and new information on the $^{25}$Al level scheme is provided. An enhanced decay scheme has been constructed and compared to the mirror decay of $^{25}$Na and the shell-model calculations. The measured excitation energies, $γ$-ray and proton branchings, log~$ft$ values, and Gamow-Teller transition strengths for the states of $^{25}$Al populated in the $β$ decay of $^{25}$Si are in good agreement with the shell-model calculations, offering gratifyingly consistent insights into the fine nuclear structure of $^{25}$Al.

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arXiv2020

RC-chain: Reputation-based Crowdsourcing Blockchain for Vehicular Networks

As the commercial use of 5G technologies has grown more prevalent, smart vehicles have become an efficient platform for delivering a wide array of services directly to customers. The vehicular crowdsourcing service (VCS), for example, can provide immediate and timely feedback to the user regarding real-time transportation information. However, different sources can generate spurious information towards a specific service request in the pursuit of profit. Distinguishing trusted information from numerous sources is the key to a reliable VCS platform. This paper proposes a solution to this problem called "RC-chain", a reputation-based crowdsourcing framework built on a blockchain platform (Hyperledger Fabric). We first establish the blockchain-based platform to support the management of crowdsourcing trading and user-reputation evaluating activities. A reputation model, the Trust Propagation \& Feedback Similarity (TPFS), then calculates the reputation values of participants and reveals any malicious behavior accordingly. Finally, queueing theory is used to evaluate the blockchain-based platform and optimize the system performance. The proposed framework was deployed on the IBM Hyperledger Fabric platform to observe its real-world running time, effectiveness, and overall performance.

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arXiv2020

First Penning trap mass measurement of $^{36}$Ca

Isobaric quintets provide the best test of the isobaric multiplet mass equation (IMME) and can uniquely identify higher order corrections suggestive of isospin symmetry breaking effects in the nuclear Hamiltonian. The Generalized IMME (GIMME) is a novel microscopic interaction theory that predicts an extension to the quadratic form of the IMME. Only the $A=20, 32$ $T=2$ quintets have the exotic $T_z = -2$ member ground state mass determined to high-precision by Penning trap mass spectrometry. In this work, we establish $A=36$ as the third high-precision $T=2$ isobaric quintet with the $T_z = -2$ member ground state mass measured by Penning trap mass spectrometry and provide the first test of the predictive power of the GIMME. A radioactive beam of neutron-deficient $^{36}$Ca was produced by projectile fragmentation at the National Superconducting Cyclotron Laboratory. The beam was thermalized and the mass of $^{36}$Ca$^+$ and $^{36}$Ca$^{2+}$ measured by the Time of Flight - Ion Cyclotron Resonance method in the LEBIT 9.4 T Penning trap. We measure the mass excess of $^{36}$Ca to be ME$ = -6483.6(56)$ keV, an improvement in precision by a factor of 6 over the literature value. The new datum is considered together with evaluated nuclear data on the $A=36$, $T=2$ quintet. We find agreement with the quadratic form of the IMME given by isospin symmetry, but only coarse qualitative agreement with predictions of the GIMME. A total of three isobaric quintets have their most exotic members measured by Penning trap mass spectrometry. The GIMME predictions in the $T = 2$ quintet appear to break down for $A = 32$ and greater.

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arXiv2020

Determination of the cluster-decay branching ratio from a near-threshold molecular state in $^{10}$Be

A puzzle has long existed for the $α$-cluster content in the near-threshold 7.54 MeV state of $^{10}$Be. A new measurement was conducted to measure the cluster-decay partial width of this state, using the reaction $\rm{^9Be}(\rm{^9Be}, \rm{^{10}Be}^{*} \rightarrow α+ \rm{^6He})\rm{^8Be}$ at 45 MeV beam energy. Special measures were taken to reduce the strong near-threshold background. The neutron-decay strength was also obtained based on the three-fold coincident measurement. A cluster-decay branching ratio of $(4.04 \pm 1.26)\times 10^{-4}$ is obtained, resulting in a reasonably large $α$-cluster spectroscopic factor. The present work confirms the formation of the $σ$-bond molecular rotational band headed by the 6.18 MeV state in $^{10}$Be.

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arXiv2019

Fine structure in the $α$ decay of $^{223}$U

Fine structure in the $α$ decay of $^{223}$U was observed in the fusion-evaporation reaction $^{187}$Re($^{40}$Ar, p3n) by using fast digital pulse processing technique. Two $α$-decay branches of $^{223}$U feeding the ground state and 244 keV excited state of $^{219}$Th were identified by establishing the decay chain $^{223}$U $\xrightarrow{α_{1}}$ $^{219}$Th $\xrightarrow{α_{2}}$ $^{215}$Ra $\xrightarrow{α_{3}}$ $^{211}$Rn. The $α$-particle energy for the ground-state to ground-state transition of $^{223}$U was determined to be 8993(17) keV, 213 keV higher than the previous value, the half-life was updated to be 62$^{+14}_{-10}$ $μ$s. Evolution of nuclear structure for $N$ = 131 even-$Z$ isotones from Po to U was discussed in the frameworks of nuclear mass and reduced $α$-decay width, a weakening octupole deformation in the ground state of $^{223}$U relative to its lighter isotones $^{219}$Ra and $^{221}$Th was suggested.

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arXiv2019

Experimentally well-constrained masses of $^{27}$P and $^{27}$S: Implications for studies of explosive binary systems

The mass of $^{27}$P was predicted to impact the X-ray burst (XRB) model predictions of burst light curves and the composition of the burst ashes. To address the uncertainties and inconsistencies in the reported $^{27}$P masses in literature, a wealth of information has been extracted from the $β$-decay spectroscopy of the drip-line nucleus $^{27}$S. We determine the most precise mass excess of $^{27}$P to date to be $-659(9)$~keV, which is 63~keV (2.3$σ$) higher than the AME2016 recommended value of $-722(26)$~keV. The experimentally unknown mass excess of $^{27}$S was estimated to be 17030(400)~keV in AME2016, and we constrain this mass to be 17678(77)~keV based on the measured $β$-delayed two-proton energy. In the temperature region of $(0.06-0.3)$~GK, the $^{26}$Si$(p,γ)^{27}$P reaction rate determined in this work is significantly lower than the rate recommended in the reaction rate libraries, up to two orders of magnitude around 0.1~GK. The impact of these newly determined masses and well-constrained rate on the modeling of the explosive astrophysical scenarios has been explored by hydrodynamic nova and post-processing XRB models. No substantial change was found in the nova contribution to the synthesis of galactic $^{26}$Al or in the XRB energy generation rate, but we found that the calculated abundances of $^{26}$Al and $^{26}$Si at the last stage of XRB are increased by a factor of 2.4. We also conclude that $^{27}$S is not a significant waiting point in the rapid proton capture process.

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arXiv2019

Simultaneous measurement of beta-delayed proton and gamma emission of $^{26}$P for $^{25}$Al($p,γ$)$^{26}$Si reaction rate

$β$ decay of $^{26}$P was used to populate the astrophysically important $E_x=$5929.4(8) keV $J^π=3{^+}$ state of $^{26}$Si. Both $β$-delayed proton at 418(8) keV and gamma ray at 1742(2) keV emitted from this state were measured simultaneously for the first time with corresponding absolute intensities of 11.1(12)\% and 0.59(44)\%, respectively. Besides, shell model calculations with weakly bound effects were performed to investigate the decay properties of other resonant states and a spin-parity of $4^+$ rather than $0^+$ was favored for the $E_x=$5945.9(40) keV state. Combining the experimental results and theoretical calculations, $^{25}$Al($p,γ$)$^{26}$Si reaction rate in explosive hydrogen burning environments was calculated and compared with previous studies.

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arXiv2019

Beta-decay spectroscopy of $^{27}$S

Background: Beta-decay spectroscopy provides valuable nuclear physics input for thermonuclear reaction rates of astrophysical interest and stringent test for shell-model theories far from the stability line. Purpose: The available decay properties of proton drip-line nucleus $^{27}$S is insufficient to constrain the properties of the key resonance in $^{26}$Si$(p,γ)^{27}$P reaction rate and probe the possible isospin asymmetry. The decay scheme of $^{27}$S is complicated and far from being understood, which has motivated but also presented challenges for our experiment. Method: The $^{27}$S ions were implanted into a double-sided silicon strip detector array surrounded by the high-purity germanium detectors, where the $β$-delayed protons and $γ$ rays were measured simultaneously. Results: The improved spectroscopic properties including the precise half-life of $^{27}$S, the excitation energies, $β$-decay branching ratios, log~$ft$ values, and $B$(GT) values for the states of $^{27}$P populated in the $β$ decay of $^{27}$S were measured and compared to the $^{27}$Mg mirror states and the shell-model calculations. The present work has expanded greatly on the previously established decay scheme of $^{27}$S. Conclusions: The precise proton-separation energy of $^{27}$P, the energy and the ratio between $γ$ and proton partial widths of the $3/2^+$ resonance were obtained, thereby determining the $^{26}$Si$(p,γ)^{27}$P reaction rate based mainly on experimental constraints. The first evidence for the observation of a large isospin asymmetry for the mirror decays of $^{27}$S and $^{27}$Na is also provided. The experimental spectroscopic information can be reproduced by the shell-model calculation taking the weakly bound effect of the proton $1s_{1/2}$ orbit into account.

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