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L. Kondic

Publications and source records attributed to L. Kondic.

At least 19 recordsLinked to original sources

On the fractal dimension of non-Newtonian Hele-Shaw flow subject to Saffman-Taylor instability

We introduce a discrete numerical method based on the diffusion-limited aggregation (DLA) approach to simulate two-fluid Hele-Shaw flow subject to the Saffman-Taylor interfacial instability, in the case where the displaced fluid is non-Newtonian. Focusing on fluids for which the most relevant non-Newtonian aspect of the thin-gap flow is shear-thinning, we introduce a history-dependent aspect into the algorithm, modeling shear-rate-dependent fluid viscosity. The main finding is that the morphology of the emerging patterns, characterized by the fractal dimension, is modified in a nontrivial manner by the shear-thinning nature of the displaced fluid. In particular, we consistently find that shear-thinning leads to the formation of patterns characterized by a smaller fractal dimension, compared to the corresponding Newtonian fluid.

physics.flu-dyn

Modeling the dynamics of an oil drop driven by a surface acoustic wave in the underlying substrate

We present a theoretical study, supported by simulations and experiments, on the spreading of a silicone oil drop under MHz-frequency surface acoustic wave (SAW) excitation in the underlying solid substrate. Our time-dependent theoretical model uses the long wave approach and considers interactions between fluid dynamics and acoustic driving. While similar methods have analyzed micron-scale oil and water film dynamics under SAW excitation, acoustic forcing was linked to boundary layer flow, specifically Schlichting and Rayleigh streaming, and acoustic radiation pressure. For the macroscopic drops in this study, acoustic forcing arises from Reynolds stress variations in the liquid due to changes in the intensity of the acoustic field leaking from the SAW beneath the drop and the viscous dissipation of the leaked wave. Contributions from Schlichting and Rayleigh streaming are negligible in this case. Both experiments and simulations show that after an initial phase where the oil drop deforms to accommodate acoustic stress, it accelerates, achieving nearly constant speed over time, leaving a thin wetting layer. Our model indicates that the steady speed of the drop results from the quasi-steady shape of its body. The drop speed depends on drop size and SAW intensity. Its steady shape and speed are further clarified by a simplified traveling wave-type model that highlights various physical effects. Although the agreement between experiment and theory on drop speed is qualitative, the results' trend regarding SAW amplitude variations suggests that the model realistically incorporates the primary physical effects driving drop dynamics.

physics.flu-dyn

Intruder in a two-dimensional granular system: statics and dynamics of force networks in an experimental system experiencing stick-slip dynamics

In quasi-two-dimensional experiments with photoelastic particles confined to an annular region, an intruder constrained to move in a circular path halfway between the annular walls experiences stick-slip dynamics. We discuss the response of the granular medium to the driven intruder, focusing on the evolution of the force network during sticking periods. Because the available experimental data does not include precise information about individual contact forces, we use an approach developed in our previous work (Basak et al, J. Eng. Mechanics (2021)) based on networks constructed from measurements of the integrated strain magnitude on each particle. These networks are analyzed using topological measures based on persistence diagrams, revealing that force networks evolve smoothly but in a nontrivial manner throughout each sticking period, even though the intruder and granular particles are stationary. Characteristic features of persistence diagrams show identifiable changes as a slip is approaching, indicating the existence of slip precursors. Key features of the dynamics are similar for granular materials composed of disks or pentagons, but some details are consistently different. In particular, we find significantly larger fluctuations of the measures computed based on persistence diagrams, and therefore of the underlying networks, for systems of pentagonal particles.

cond-mat.soft

Properties of Interaction Networks in Compressed Two and Three Dimensional Particulate Systems

We consider two (2D) and three (3D) dimensional granular systems exposed to compression, and ask what is the influence of the number of physical dimensions on the properties of the interaction networks that spontaneously form as these systems evolve. The study is carried out based on discrete element simulations of frictional disks in 2D and spheres in 3D. The main finding is that both the number of physical dimensions and the type of particle-particle interaction influence significantly the properties of interaction networks. These networks play an important role in bridging the microscale (particle size) and macroscale (system size), thus both aspects (the interaction model and dimensionality) are carefully considered. Our work uses a combination of tools and techniques, including percolation study, statistical analysis, as well as algebraic topology-based techniques. In many instances we find that different techniques and measures provide complementary information that, when combined, allow for gaining better insight into the properties of interaction networks.

cond-mat.soft

Instabilities of a thin liquid film in a funnel

We explore flow of a completely wetting fluid in a funnel, with particular focus on contact line instabilities at the fluid front. While the flow in a funnel may be related to a number of other flow configurations as limiting cases, understanding its stability is complicated due to the presence of additional azimuthal curvature, as well as due to convergent flow effects imposed by the geometry. Convergent nature of the flow leads to thickening of the film, therefore influencing its stability properties. In this work, we analyze these stability properties by combining physical experiments, asymptotic modeling, self-similar type of analysis and numerical simulations. We show that appropriate long-wave based model supported by the input from experiments, simulations and linear stability analysis origination from the flow down an incline plane provides a basic insight allowing to understand the development of contact line instability and emerging lengthscales.

physics.flu-dyn

Effects of spatially-varying substrate anchoring on instabilities and dewetting of thin Nematic Liquid Crystal films

Partially wetting nematic liquid crystal (NLC) films on substrates are unstable to dewetting-type instabilities due to destablizing solid/NLC interaction forces. These instabilities are modified by the nematic nature of the films, which influences the effective solid/NLC interaction. In this work, we focus on the influence of imposed substrate anchoring on the instability development. The analysis is carried out within a long-wave formulation based on the Leslie-Ericksen description of NLC films. Linear stability analysis of the resulting equations shows that some features of the instability, such as emerging wavelengths, may not be influenced by the imposed substrate anchoring. Going further into the nonlinear regime, considered via large-scale GPU-based simulations, shows however that nonlinear effects may play an important role, in particular in the case of strong substrate anchoring anisotropy. Our simulations show that instability of the film develops in two stages: the first stage involves formation of ridges that are perpendicular to the local anchoring direction; and the second involves breakup of these ridges and formation of drops, whose final distribution is influenced by the anisotropy imposed by the substrate. Finally, we show that imposing more complex substrate anisotropy patterns allows us to reach basic understanding of the influence of substrate-imposed defects in director orientation on the instability evolution.

cond-mat.soft

Energy dissipation in sheared wet granular assemblies

Energy dissipation in sheared dry and wet granulates is considered in the presence of an externally applied confining pressure. Discrete element simulations reveal that for sufficiently small confining pressures, the energy dissipation is dominated by the effects related to the presence of cohesive forces between the particles. The residual resistance against shear can be quantitatively explained by a combination of two effects arising in a wet granulate: i) enhanced friction at particle contacts in the presence of attractive capillary forces, and ii) energy dissipation due to the rupture and reformation of liquid bridges. Coulomb friction at grain contacts gives rise to an energy dissipation which grows linearly with increasing confining pressure, for both dry and wet granulates. Because of a lower Coulomb friction coefficient in the case of wet grains, as the confining pressure increases the energy dissipation for dry systems is faster than for wet ones.

cond-mat.soft

Granular Response to Impact: Topology of the Force Networks

Impact of an intruder on granular matter leads to formation of mesoscopic force networks seen particularly clearly in the recent experiments carried out with photoelastic particles, e.g., Clark et al., Phys. Rev. Lett., 114 144502 (2015). These force networks are characterized by complex structure and evolve on fast time scales. While it is known that total photoelastic activity in the granular system is correlated with the acceleration of the intruder, it is not known how the structure of the force network evolves during impact, and if there is a dominant features in the networks that can be used to describe intruder's dynamics. Here, we use topological tools, in particular persistent homology, to describe these features. Persistent homology allows quantification of both structure and time evolution of the resulting force networks. We find that there is a clear correlation of the intruder's dynamics and some of the topological measures implemented. This finding allows us to discuss which properties of the force networks are most important when attempting to describe intruder's dynamics. Regarding temporal evolution of the networks, we are able to define the upper bound on the relevant time scale on which the networks evolve.

cond-mat.soft

A numerical approach for the direct computation of flows including fluid-solid interaction: modeling contact angle, film rupture, and dewetting

In this paper, we present a computationally efficient method for including fluid-solid interactions into direct numerical simulations of the Navier-Stokes equations. This method is found to be as powerful as our earlier formulation [J. Comp. Phys., vol. 249: 243 (2015)], while outperforming the earlier method in terms of computational efficiency. The performance and efficacy of the presented method are demonstrated by computing contact angles of droplets at equilibrium. Furthermore, we study the instability of films due to destabilizing fluid-solid interactions, and discuss the influence of contact angle and inertial effects on film breakup. In particular, direct simulation results show an increase in the final characteristic length scales when compared to the predictions of a linear stability analysis, suggesting significant influence of nonlinear effects. Our results also show that emerging length scales differ, depending on a number of physical dimensions considered.

physics.flu-dyn

Structure of force networks in tapped particulate systems of disks and pentagons (Part 2): Persistence analysis

In the companion paper~\cite{paper1}, we use classical measures based on force probability density functions (PDFs), as well as Betti numbers (quantifying the number of components, related to force chains, and loops), to describe the force networks in tapped systems of disks and pentagons. In the present work, we focus on the use of persistence analysis, that allows to describe these networks in much more detail. This approach allows not only to describe, but also to quantify the differences between the force networks in different realizations of a system, in different parts of the considered domain, or in different systems. We show that persistence analysis clearly distinguishes the systems that are very difficult or impossible to differentiate using other means. One important finding is that the differences in force networks between disks and pentagons are most apparent when loops are considered: the quantities describing properties of the loops may differ significantly even if other measures (properties of components, Betti numbers, or force PDFs) do not distinguish clearly the investigated systems.

physics.data-an

Structure of force networks in tapped particulate systems of disks and pentagons (Part 1): Clusters and Loops

The force network of a granular assembly, defined by the contact network and the corresponding contact forces, carries valuable information about the state of the packing. Simple analysis of these networks based on the distribution of force strengths is rather insensitive to the changes in preparation protocols or to the types of particles. In this paper we consider two dimensional simulations of tapped systems built from frictional disks and pentagons, and study the structure of the force networks of granular packings by considering network's topology as force thresholds are varied. We show that the number of clusters and loops observed in the force networks as a function of the force threshold are markedly different for disks and pentagons if the tangential contact forces are considered, whereas they are surprisingly similar for the network defined by the normal forces. In particular, the results indicate that, overall, the force network is more heterogeneous for disks than for pentagons. Additionally, we show that the states obtained by tapping with different intensities that display similar packing fraction are difficult to distinguish based on simple topological invariants.

cond-mat.soft

Percolation and jamming transitions in particulate systems with and without cohesion

We consider percolation and jamming transitions for particulate systems exposed to compression. For the systems built of particles interacting by purely repulsive forces in addition to friction and viscous damping, it is found that these transitions are influenced by a number of effects, and in particular by the compression rate. In a quasi-static limit, we find that for the considered type of interaction between the particles, percolation and jamming transitions coincide. For cohesive systems, however, or for any system exposed to even slow dynamics, the differences between the considered transitions are found and quantified.

cond-mat.soft

Role of Thermal Fluctuations in Nonlinear Thin Film Dewetting

The spontaneous formation of droplets via dewetting of a thin fluid film from a solid substrate allows for materials nanostructuring, under appropriate experimental control. While thermal fluctuations are expected to play a role in this process, their relevance has remained poorly understood, particularly during the nonlinear stages of evolution. Within a stochastic lubrication framework, we show that thermal noise speeds up and substantially influences the formation and evolution of the droplet arrangement. As compared with their deterministic counterparts, for a fixed spatial domain, stochastic systems feature a smaller number of droplets, with a larger variability in sizes and space distribution. Finally, we discuss the influence of stochasticity on droplet coarsening for very long times.

cond-mat.soft

Capillary focusing close to a topographic step: Shape and instability of confined liquid filaments

Step-emulsification is a microfluidic technique for droplet generation which relies on the abrupt decrease of confinement of a liquid filament surrounded by a continuous phase. A striking feature of this geometry is the transition between two distinct droplet breakup regimes, the "step-regime" and "jet-regime", at a critical capillary number. In the step-regime, small and monodisperse droplets break off from the filament directly at a topographic step, while in the jet-regime a jet protrudes into the larger channel region and large plug-like droplets are produced. We characterize the breakup behavior as a function of the filament geometry and the capillary number and present experimental results on the shape and evolution of the filament for a wide range of capillary numbers in the jet-regime. We compare the experimental results with numerical simulations. Assumptions based on the smallness of the depth of the microfluidic channel allow to reduce the governing equations to the Hele-Shaw problem with surface tension. The full nonlinear equations are then solved numerically using a volume-of-fluid based algorithm. The computational framework also captures the transition between both regimes, offering a deeper understanding of the underlying breakup mechanism.

physics.flu-dyn

Quantifying force networks in particulate systems

We present mathematical models based on persistent homology for analyzing force distributions in particulate systems. We define three distinct chain complexes: digital, position, and interaction, motivated by different capabilities of collecting experimental or numerical data, e.g. digital images, location of the particles, and normal forces between particles, respectively. We describe how algebraic topology, in particular, homology allows one to obtain algebraic representations of the geometry captured by these complexes. To each complexes we define an associated force network from which persistent homology is computed. Using numerical data obtained from molecular dynamics simulations of a system of particles being slowly compressed we demonstrate how persistent homology can be used to compare the geometries of the force distributions in different granular systems. We also discuss the properties of force networks as a function of the underlying complexes, and hence, as a function of the type of experimental or numerical data provided.

cond-mat.soft

Numerical simulation of ejected molten metal-nanoparticles liquefied by laser irradiation: Interplay of geometry and dewetting

Metallic nanoparticles, liquefied by fast laser irradiation, go through a rapid change of shape attempting to minimize their surface energy. The resulting nanodrops may be ejected from the substrate when the mechanisms leading to dewetting are sufficiently strong, as in the experiments involving gold nanoparticles [Habenicht et al., Science 309, 2043 (2005)]. We use a direct continuum-level approach to accurately model the process of liquid nanodrop formation and the subsequent ejection from the substrate. Our computations show a significant role of inertial effects and an elaborate interplay of initial geometry and wetting properties: e.g., we can control the direction of ejection by prescribing appropriate initial shape and/or wetting properties. The basic insight regarding ejection itself can be reached by considering a simple effective model based on an energy balance. We validate our computations by comparing directly with the experiments specified above involving the length scales measured in hundreds of nanometers, and with molecular dynamics simulations on much shorter scales measured in tens of atomic diameters, as in [M. Fuentes-Cabrera et al., Phys. Rev. E 83, 041603 (2011)]. The quantitative agreement, in addition to illustrating how to controlling particle ejection, shows utility of continuum-based simulation in describing dynamics on nanoscale quantitatively, even in a complex setting as considered here.

physics.flu-dyn

Thin films flowing down inverted substrates: Three dimensional flow

We study contact line induced instabilities for a thin film of fluid under destabilizing gravitational force in three dimensional setting. In the previous work (Phys. Fluids, {\bf 22}, 052105 (2010)), we considered two dimensional flow, finding formation of surface waves whose properties within the implemented long wave model depend on a single parameter, $D=(3Ca)^{1/3}\cotα$, where $Ca$ is the capillary number and $α$ is the inclination angle. In the present work we consider fully 3D setting and discuss the influence of the additional dimension on stability properties of the flow. In particular, we concentrate on the coupling between the surface instability and the transverse (fingering) instabilities of the film front. We furthermore consider these instabilities in the setting where fluid viscosity varies in the transverse direction. It is found that the flow pattern strongly depends on the inclination angle and the viscosity gradient.

physics.flu-dyn

Monte Carlo and MD Modeling of Density Relaxation by Tapping

The density relaxation phenomenon is modeled using both Monte Carlo and dissipative MD simulations to investigate the effects of regular taps applied to a vessel having a planar floor filled with monodisperse spheres. Results suggest the existence of a critical tap intensity that depends on the mass overburden, which produces a maximum bulk solids fraction. We find that the mechanism responsible for the relaxation phenomenon is evolving quasi-ordered packing structure propagating upwards from the plane floor.

cond-mat.dis-nn