arXiv subjects

L. Lalanne

Publications and source records attributed to L. Lalanne.

16 recordsLinked to original sources

arXiv2026

Evolution of Spectroscopic Factors in Neutron-deficient $p$-shell Nuclei in connection with Short-Range Correlations

We report an uncertainty-controlled determination of neutron-removal spectroscopic factors in the neutron-deficient $p$-shell nuclei $^{12}\mathrm{C}$, $^{10}\mathrm{C}$, $^{9}\mathrm{C}$, and $^{8}\mathrm{B}$, all measured under uniform conditions through exclusive ground-state-to-ground-state $(p,d)$ reactions at about 50 MeV/nucleon in a liquid hydrogen target at the GANIL/LISE facility. The deuterons were detected in the highly-segmented MUST2 detector placed at forward angles and the excitation energy was reconstructed by the missing mass method. Several transitions, including a new state in $^7\mathrm{B}$, were observed. Differential cross sections, which display an $L=1$ pattern for all nuclei, were fitted with 416 sets of uncertainty-quantified optical-model potential parameters and considering various single-particle bound-state wavefunctions to derive $C^2S$ values. The ratio between experimental and shell-model calculated values, $R_S$, is found to be slightly decreasing as a function of increasing proton to neutron separation energy asymmetry $\Delta S$, with a slope of $-0.0049(36)_{\rm stat}(13)_{\rm omp}(8)_{\rm s.p.}$. The observed trend is compatible with the phenomenological expectation that the short-range correlation effect on $C^2S$ increases with the degree of nucleon minority. The present data set delivers a high-precision benchmark that will tightly constrain future microscopic descriptions of short-range correlations in asymmetric nuclei.

nucl-ex↗

arXiv2026

Energies and lifetimes of the 9p and 10p excited states in atomic francium

We present the first measurement of 9p 2P1/2,3/2 and 10p 2P1/2,3/2 excited levels absolute wavenumbers and radiative lifetime in francium. We used the Collinear Resonance Ionization Spectroscopy (CRIS) technique, applied on a beam of 221Fr atoms. Prior to this work, no experimental data existed for francium p-states with n > 8. The results provide a precision experimental test of relativistic coupled-cluster theory for the heaviest alkali, showing good agreement for lifetimes and relative excitation energies, despite a residual global offset in absolute energies.

physics.atom-ph↗

arXiv2026

Direct transfer to $^{46,48}$K as a survey of the $\pi(s_{1/2})$$-\nu(sdpf)$ interaction

The collapse of the canonical $N=28$ magic number in nuclei with $Z<20$ has drawn significant interest as it relates to the emergence of an island of inversion centered on $^{42}$Si and $^{44}$S. In particular, interactions between the $\pi s_{1/2}$ orbital -- empty in $^{42}$Si and full in $^{44}$S -- and the neutron orbitals just above and below the $N=28$ gap are expected to be critical in this region, but remain relatively unexplored. In this paper, we expand upon the results of our previous study of the direct transfer reaction $^{47}$K(d,p$\gamma$)$^{48}$K [C.\,J.~Paxman \textit{et al.}, Phys. Rev. Lett. 134, 162504 (2025)] with the results of the complementary $^{47}$K(d,t$\gamma$)$^{46}$K reaction. Through this study, we present a comprehensive scan of the interaction between the critical $\pi s_{1/2}$ orbital and a broad range of neutron orbitals spanning nearly two full shells. We identify several discrepancies between the experimental results and state-of-the-art shell model calculations, which suggest a deficiency of the shell model to fully capture the complex proton configuration mixing in this region, highlighting a significant challenge for single-particle descriptions of the island of inversion.

nucl-ex↗

arXiv2025

Observation of the distribution of nuclear magnetization in a molecule

Rapid progress in the experimental control and interrogation of molecules, combined with developments in precise calculations of their structure, are enabling new opportunities in the investigation of nuclear and particle physics phenomena. Molecules containing heavy, octupole-deformed nuclei such as radium are of particular interest for such studies, offering an enhanced sensitivity to the properties of fundamental particles and interactions. Here, we report precision laser spectroscopy measurements and theoretical calculations of the structure of the radioactive radium monofluoride molecule, $^{225}$Ra$^{19}$F. Our results allow fine details of the short-range electron-nucleus interaction to be revealed, indicating the high sensitivity of this molecule to the distribution of magnetization, currently a poorly constrained nuclear property, within the radium nucleus. These results provide a direct and stringent test of the description of the electronic wavefunction inside the nuclear volume, highlighting the suitability of these molecules to investigate subatomic phenomena.

nucl-ex↗

arXiv2025

$^{61}$Cr as a Doorway to the N = 40 Island of Inversion

This paper reports on the measurement of the ground-state spin and nuclear magnetic dipole moment of $^{61}$Cr. The radioactive ion beam was produced at the CERN-ISOLDE facility and was probed using high-resolution resonance ionization laser spectroscopy with the CRIS apparatus. The present ground-state spin measurement $I = \frac{1}{2}$, differing from the previously adopted $I =(\frac{5}{2})$, has significant consequences on the interpretation of existing beta decay data and nuclear structure in the region. The structure and shape of $^{61}$Cr is interpreted with state-of-the-art Large-Scale Shell Model and Discrete-Non-Orthogonal Shell Model calculations. From the measured magnetic dipole moment $μ(^{61}$Cr$)=+0.539(7)~μ_N$ and the theoretical findings, its configuration is understood to be driven by 2 particle - 2 hole neutron excitations with an unpaired $1p_{1/2}$ neutron. This establishes the western border of the $N=40$ Island Of Inversion (IoI), characterized by 4 particle - 4 hole neutron components. We discuss the shape evolution along the Cr isotopic chain as a quantum phase transition at the entrance of the $N=40$ IoI.

nucl-ex↗

arXiv2025

Laser spectroscopy and CP-violation sensitivity of actinium monofluoride

The apparent invariance of the strong nuclear force under combined charge conjugation and parity (CP) remains an open question in modern physics. Precision experiments with heavy atoms and molecules can provide stringent constraints on CP violation via searches for effects due to permanent electric dipole moments and other CP-odd properties in leptons, hadrons, and nuclei. Radioactive molecules have been proposed as highly sensitive probes for such searches, but experiments with most such molecules have so far been beyond technical reach. Here we report the first production and spectroscopic study of a gas-phase actinium molecule, $^{227}$AcF. We observe the predicted strongest electronic transition from the ground state, which is necessary for efficient readout in searches of symmetry-violating interactions. Furthermore, we perform electronic- and nuclear-structure calculations for $^{227}$AcF to determine its sensitivity to various CP-violating parameters, and find that a realistic, near-term experiment with a precision of 1 mHz would improve current constraints on the CP-violating parameter hyperspace by three orders of magnitude. Our results thus highlight the potential of $^{227}$AcF for exceptionally sensitive searches of CP violation.

physics.atom-ph↗

arXiv2025

Probing exotic cross-shell interactions at N=28 with single-neutron transfer on 47K

We present the first measurement of the $^{47}$K($d,pγ$)$^{48}$K transfer reaction, performed in inverse kinematics using a reaccelerated beam of $^{47}$K. The level scheme of $^{48}$K has been greatly extended with nine new bound excited states identified and spectroscopic factors deduced. Detailed comparisons with SDPF-U and SDPF-MU shell-model calculations reveal a number of discrepancies with these results, and a preference for SDPF-MU is found. Intriguingly, an apparent systematic overestimation of spectroscopic factors and a poor reproduction of the energies for 1$^-$ states suggests that the mixing between the $πs^{\,\,\,1}_{1/2} d^{\,\,\,4}_{3/2}$ and $πs^{\,\,\,2}_{1/2} d^{\,\,\,3}_{3/2}$ proton configurations in $^{48}$K is not correctly described using current interactions, challenging our descriptions of light $N=28$ nuclei.

nucl-ex↗

arXiv2024

Pinning down electron correlations in RaF via spectroscopy of excited states and high-accuracy relativistic quantum chemistry

We report the spectroscopy of the 14 lowest excited electronic states in the radioactive molecule radium monofluoride (RaF). The observed excitation energies are compared with fully relativistic state-of-the-art Fock-space coupled cluster (FS-RCC) calculations, which achieve an agreement of >=99.64% (within ~12 meV) with experiment for all states. Guided by theory, a firm assignment of the angular momentum and term symbol is made for 10 states and a tentative assignment for 4 states. The role of high-order electron correlation and quantum electrodynamics effects in the excitation energy of excited states is studied, found to be important for all states. Establishing the simultaneous accuracy and precision of calculations is an important step for research at the intersection of particle, nuclear, and chemical physics, including searches of physics beyond the Standard Model, for which RaF is a promising probe.

physics.atom-ph↗

arXiv2024

Ionization potential of radium monofluoride

The ionization potential (IP) of radium monofluoride (RaF) was measured to be 4.969(2)[10] eV, revealing a relativistic enhancement in the series of alkaline earth monofluorides. The results are in agreement with a relativistic coupled-cluster prediction of 4.969[7] eV, incorporating up to quantum electrodynamics corrections. Using the same computational methodology, an improved calculation for the dissociation energy ($D_{0}$) of 5.54[5] eV is presented. This confirms that radium monofluoride joins the small group of diatomic molecules for which $D_{0}>\mathrm{IP}$, paving the way for precision control and interrogation of its Rydberg states.

physics.atom-ph↗

arXiv2024

Radiative lifetime of the A 2Π1/2 state in RaF with relevance to laser cooling

The radiative lifetime of the $A$ $^2 Π_{1/2}$ (v=0) state in radium monofluoride (RaF) is measured to be 35(1) ns. The lifetime of this state and the related decay rate $Γ= 2.86(8) \times 10^7$ $s^{-1}$ are of relevance to the laser cooling of RaF via the optically closed $A$ $^2 Π_{1/2} \leftarrow X$ $^2Σ_{1/2}$ transition, which makes the molecule a promising probe to search for new physics. RaF is found to have a comparable photon-scattering rate to homoelectronic laser-coolable molecules. Thanks to its highly diagonal Franck-Condon matrix, it is expected to scatter an order of magnitude more photons than other molecules when using just 3 cooling lasers, before it decays to a dark state. The lifetime measurement in RaF is benchmarked by measuring the lifetime of the $8P_{3/2}$ state in Fr to be 83(3) ns, in agreement with literature.

physics.atom-ph↗

arXiv2023

N=16 magicity revealed at the proton drip-line through the study of 35Ca

The last proton bound calcium isotope $^{35}$Ca has been studied for the first time, using the $^{37}$Ca($p, t$)$^{35}$Ca two neutron transfer reaction. The radioactive $^{37}$Ca nuclei, produced by the LISE spectrometer at GANIL, interacted with the protons of the liquid hydrogen target CRYPTA, to produce tritons $t$ that were detected in the MUST2 detector array, in coincidence with the heavy residues Ca or Ar. The atomic mass of $^{35}$Ca and the energy of its first 3/2$^+$ state are reported. A large $N=16$ gap of 4.61(11) MeV is deduced from the mass measurement, which together with other measured properties, makes $^{36}$Ca a doubly-magic nucleus. The $N = 16$ shell gaps in $^{36}$Ca and $^{24}$O are of similar amplitude, at both edges of the valley of stability. This feature is discussed in terms of nuclear forces involved, within state-of-the-art shell model calculations. Even though the global agreement with data is quite convincing, the calculations underestimate the size of the $N = 16$ gap in 36Ca by 840(110) keV.

nucl-ex↗

arXiv2022

The structure of $^{36}$Ca under the Coulomb magnifying glass

Detailed spectroscopy of the neutron-deficient nucleus $^{36}$Ca was obtained up to 9 MeV using the $^{37}$Ca($p$,$d$)$^{36}$Ca and the $^{38}$Ca($p$,$t$)$^{36}$Ca transfer reactions. The radioactive nuclei, produced by the LISE spectrometer at GANIL, interacted with the protons of the liquid Hydrogen target CRYPTA, to produce light ejectiles (the deuteron $d$ or triton $t$) that were detected in the MUST2 detector array, in coincidence with the heavy residues %identified by a zero degree detection system. %States have been measured up to 9 MeV. Our main findings are: i) a similar shift in energy for the 1$^+_1$ and 2$^+_1$ states by about -250 keV, as compared to the mirror nucleus $^{36}$S, ii) the discovery of an intruder 0$^+_2$ state at 2.83(13) MeV, which appears below the first 2$^+$ state, in contradiction with the situation in $^{36}$S, and iii) a tentative 0$^+_3$ state at 4.83(17) MeV, proposed to exhibit a bubble structure with two neutron vacancies in the 2s$_{1/2}$ orbit. The inversion between the 0$^+_2$ and 2$^+_1$ states is due to the large mirror energy difference (MED) of -516(130) keV for the former. This feature is reproduced by Shell Model (SM) calculations, using the $sd$-$pf$ valence space, predicting an almost pure intruder nature for the 0$^+_2$ state, with two protons (neutrons) being excited across the $Z$=20 magic closure in $^{36}$Ca ($^{36}$S). This mirror system has the largest MEDs ever observed, if one excludes the few cases induced by the effect of the continuum.

nucl-ex↗

arXiv2021

Narrow resonances in the continuum of the unbound nucleus $^{15}$F

The structure of the unbound $^{15}$F nucleus is investigated using the inverse kinematics resonant scattering of a radioactive $^{14}$O beam impinging on a CH$_2$ target. The analysis of $^{1}$H($^{14}$O,p)$^{14}$O and $^{1}$H($^{14}$O,2p)$^{13}$N reactions allowed the confirmation of the previously observed narrow $1/2^{-}$ resonance, near the two-proton decay threshold, and the identification of two new narrow 5/2$^{-}$ and 3/2$^{-}$ resonances. The newly observed levels decay by 1p emission to the ground of $^{14}$O, and by sequential 2p emission to the ground state (g.s.) of $^{13}$N via the $1^-$ resonance of $^{14}$O. Gamow shell model (GSM) analysis of the experimental data suggests that the wave functions of the 5/2$^{-}$ and 3/2$^{-}$ resonances may be collectivized by the continuum coupling to nearby 2p- and 1p- decay channels. The observed excitation function $^{1}$H($^{14}$O,p)$^{14}$O and resonance spectrum in $^{15}$F are well reproduced in the unified framework of the GSM.

nucl-ex↗

arXiv2021

Evaluation of the $^{35}$K($p$,$γ$)$^{36}$Ca reaction rate using the $^{37}$Ca($p$,$d$)$^{36}$Ca transfer reaction

A recent sensitivity study has shown that the $^{35}$K$(p,γ)^{36}$Ca reaction is one of the ten $(p,γ)$ reaction rates that could significantly impact the shape of the calculated X-ray burst light curve. In this work, we propose to reinvestigate the $^{35}$K$(p,γ)^{36}$Ca reaction rate, as well as related uncertainties, by determining the energies and decay branching ratios of $^{36}$Ca levels, within the Gamow window, in the 0.5 to 2 GK X-ray burst temperature range. These properties were studied using the one neutron pick-up transfer reaction $^{37}$Ca$(p,d)^{36}$Ca in inverse kinematics using a radioactive beam of $^{37}$Ca at 48 MeV nucleon$^{-1}$. The experiment performed at GANIL, used the liquid Hydrogen target CRYPTA, the MUST2 detector array for the detection of the light charged particles and a zero degree detection system for the outgoing heavy ions. The atomic mass of $^{36}$Ca is confirmed and new resonances have been proposed together with their proton decay branching ratios. This spectroscopic information, used in combination with recent theoretical predictions for the $γ$-width, were used to calculate the $^{35}$K$(p,γ)^{36}$Ca reaction rate. The recommended rate of the present work was obtain within a uncertainty factor of 2 at 1 sigma. This is consistent, with the previous estimate in the X-ray burst temperature range. A large increase of the reaction rate was found at higher temperatures due to two newly discovered resonances. The $^{35}$K$(p,γ)^{36}$Ca thermonuclear reaction rate is now well constrained by the present work in a broad range of temperatures. Our results show that the $^{35}$K$(p,γ)^{36}$Ca reaction does not affect the shape of the X-ray burst light curve, and that it can be removed from the list of the few influential proton radiative captures reactions having a strong impact on the light curve.

nucl-ex↗

arXiv2021

The MUGAST-AGATA-VAMOS campaign : set-up and performance

The MUGAST-AGATA-VAMOS set-up at GANIL combines the MUGAST highly-segmented silicon array with the state-of-the-art AGATA array and the large acceptance VAMOS spectrometer. The mechanical and electronics integration copes with the constraints of maximum efficiency for each device, in particular γ-ray transparency for the silicon array. This complete set-up offers a unique opportunity to perform exclusive measurements of direct reactions with the radioactive beams from the SPIRAL1 facility. The performance of the set-up is described through its commissioning and two examples of transfer reactions measured during the campaign. High accuracy spectroscopy of the nuclei of interest, including cross-sections and angular distributions, is achieved through the triple-coincidence measurement. In addition, the correction from Doppler effect of the γ-ray energies is improved by the detection of the light particles and the use of two-body kinematics and a full rejection of the background contributions is obtained through the identification of heavy residues. Moreover, the system can handle high intensity beams (up to 108 pps). The particle identification based on the measurement of the time-of-flight between MUGAST and VAMOS and the reconstruction of the trajectories is investigated.

physics.ins-det↗

arXiv2021

Probing nuclear forces beyond the nuclear drip line: The cases of $^{16}$F and $^{15}$F

The unbound proton-rich nuclei $^{16}$F and $^{15}$F are investigated experimentally and theoretically. Several experiments using the resonant elastic scattering method were performed at GANIL with radioactive beams to determine the properties of the low lying states of these nuclei. Strong asymmetry between $^{16}$F-$^{16}$N and $^{15}$F-$^{15}$C mirror nuclei is observed. The strength of the $nucleon-nucleon$ effective interaction involving the loosely bound proton in the $s_{1/2}$ orbit is significantly modified with respect to their mirror nuclei $^{16}$N and $^{15}$C. The reduction of the effective interaction is estimated by calculating the interaction energies with a schematic zero-range force. It is found that, after correcting for the effects due to changes in the radial distribution of the single-particle wave functions, the mirror symmetry of the $n-p$ interaction is preserved between $^{16}$F and $^{16}$N, while a difference of 63\% is measured between the $p-p$ versus $n-n$ interactions in the second excited state of $^{15}$F and $^{15}$C nuclei. Several explanations are proposed.

nucl-ex↗