arXiv subjects

L. M. Robledo

Publications and source records attributed to L. M. Robledo.

At least 37 records · Page 2Linked to original sources

arXiv2023

Beyond-mean-field description of octupolarity in dysprosium isotopes with the Gogny-D1M energy density functional

The emergence and stability of (static) octupole deformation effects in Dy isotopes from dripline to dripline ($72 \le N \le 142$) is analyzed in this paper using mean-field and beyond-mean-field techniques often used for this purpose. We find static octupole deformations at the Hartree-Fock-Bogoliubov (HFB) level with the Gogny D1M force for $N \approx 134$ isotopes, while nuclei with $N \approx 88$ exhibit reflection-symmetric ground states. It is shown that, given the softness found in the mean-field and parity-projected potential energy surfaces along the octupole direction, neither of these two levels of approximation is suficcient to extract conclusions about the (permanent and/or vibrational) nature of octupole dynamic in Dy isotopes. From the analysis of the collective wave functions as well as the excitation energies of the first negative-parity states and $B(E3)$ strengths, obtained within the framework of a two-dimensional symmetry-conserving generator coordinate method (2D-GCM), it is concluded that the increased octupole collectivity in Dy isotopes with $N \approx 88$ and $N \approx 134$ is a vibrational-like effect that is not directly related to permanent mean-field octupole deformation in the considered nuclei. A pronounced suppression of the $B(E1)$ strengths is predicted for isotopes with $N \approx 82$ and $N \approx 126$. The comparison of results obtained with other parametrizations, show the robustness of the predicted trends with respect to the underlying Gogny energy density functional.

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arXiv2023

Hexadecapole axial collectivity in the rare earth region, a beyond mean field study

Hexadecapole collectivity and its interplay with quadrupole degrees of freedom is studied in an axial symmetry preserving framework based on the Hartree Fock Bogoliubov (HFB) plus generator coordinate method (GCM). Results are obtained for several even-even isotopes of Sm and Gd with various parametrizations of the Gogny force. The analysis of the results indicates the strong coupling between the quadrupole and hexadecapole degrees of freedom. The first two excited states are vibrational in character in most of the cases. The impact of prolate-oblate shape mixing in the properties of hexadecapole states is analyzed.

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arXiv2023

Least action description of dynamic pairing correlations in the fission of Curium and Californium isotopes based on the Gogny energy density functional

The impact of dynamic pairing correlations and their interplay with Coulomb antipairing effects on the systematic of the spontaneous fission half-lives for the nuclei $^{240-250}$Cm and $^{240-250}$Cf is analyzed, using a hierarchy of approximations based on the parametrization D1M of the Gogny energy density functional (EDF). First, the constrained Hartree-Fock-Bogoliubov (HFB) approximation is used to compute deformed mean-field configurations, zero-point quantum corrections and collective inertias either by using the Slater approximation to Coulomb exchange and neglecting Coulomb antipairing or by fully considering the exchange and pairing channels of the Coulomb interaction. Next, the properties of the {\it{least action}} and {\it{least energy}} fission paths are compared. In the {\it{least action}} case, pairing is identified as the relevant degree of freedom in order to minimize the action entering the Wentzel-Kramers-Brillouin (WKB) approximation to the tunneling probability through the fission barrier. Irrespective of the treatment of Coulomb exchange and antipairing, it is shown that the {\it{least action}} path obtained taking into account the pairing degree of freedom leads to stronger pairing correlations that significantly reduce the spontaneous fission half-lives $t_{SF}$ improving thereby the comparison with the experiment by several orders of magnitude. It is also shown that the Coulomb antipairing effect is, to a large extent, washed out by the {\it{least action}} procedure and therefore the $t_{SF}$ values obtained by the two different treatments of the Coulomb exchange and pairing are of similar quality.

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arXiv2022

Simultaneous description of $β$ decay and low-lying structure of neutron-rich even- and odd-mass Rh and Pd nuclei

The low-energy structure and $β$ decay properties of neutron-rich even- and odd-mass Pd and Rh nuclei are studied using a mapping framework based on the nuclear density functional theory and the particle-boson coupling scheme. Constrained Hartree-Fock-Bogoliubov calculations using the Gogny-D1M energy density functional are performed to obtain microscopic inputs to determine the interacting-boson Hamiltonian employed to describe the even-even core Pd nuclei. The mean-field calculations also provide single-particle energies for the odd systems, which are used to determine essential ingredients of the particle-boson interactions for the odd-nucleon systems, and of the Gamow-Teller and Fermi transition operators. The potential energy surfaces obtained for even-even Pd isotopes as well as the spectroscopic properties for the even- and odd-mass systems suggest a transition from prolate deformed to $γ$-unstable and to nearly-spherical shapes. The predicted $β$ decay $\log{ft}$ values are shown to be sensitive to the details of the wave functions for the parent and daughter nuclei, and therefore serve as a stringent test of the employed theoretical approach.

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arXiv2022

The finite range simple effective interaction including tensor terms

The prediction of single particle level crossing phenomenon between $2p_{3/2}$ and $1f_{5/2}$ orbitals in $Ni$- and $Cu$-isotopic chains by the finite range simple effective interaction without requiring the tensor part is discussed. In this case the experimentally observed crossing could be studied as a function of nuclear matter incompressibility, $K(ρ_0)$. The estimated crossing for the neutron number $N$=46 could be reproduced by the equation of state corresponding to $K(ρ_0)$=240 MeV. However, the observed proton gaps between the $1h_{11/2}$ and $1g_{7/2}$ shells in $Sn$ and $Sb$ isotopic chain, and the neutron gaps between the $1i_{13/2}$ and $1h_{9/2}$ shells in $N$=82 isotones, as well as the shell closure properties at $N$=28 require explicit consideration of a tensor part as the central contribution is not enough to initiate the required level splittings.

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arXiv2022

Operator overlaps in harmonic oscillator bases with different oscillator lengths

We apply a formalism recently developed to carry out Generator Coordinate Method calculations using a set of Hartree- Fock- Bogoliubov wave functions, where each of the members of the set can be expanded in an arbitrary basis. In this paper it is assumed that the HFB wave functions are expanded in Harmonic Oscillator (HO) bases with different oscillator lengths. General expressions to compute the required matrix elements of arbitrary operators are given. The application of the present formalism to the case of fission is illustrated with an example.

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arXiv2022

Formulation of the Generator Coordinate Method with arbitrary bases

The existing formalism used to compute the operator overlaps necessary to carry out generator coordinate method calculations using a set of Hartree- Fock- Bogoliubov wave functions, is generalized to the case where each of the HFB states are expanded in different arbitrary bases spanning different sub-space of the Hilbert space.

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arXiv2021

Quadrupole-octupole coupling and the evolution of collectivity in neutron-deficient Xe, Ba, Ce, and Nd isotopes

The evolution of quadrupole and octupole collectivity in neutron-deficient Xe, Ba, Ce, and Nd nuclei near the "octupole magic" neutron number $N=56$ is investigated within the mapped $sdf$-IBM framework. Microscopic input is obtained via quadrupole and octupole constrained Hartree-Fock-Bogoliubov calculations, based on the parametrization D1M of the Gogny energy density functional. Octupole-deformed mean-field ground states are predicted for Ba and Ce isotopes near $N=56$. Excitation energies of positive- and negative-parity states as well as electric transition rates are computed with wave functions resulting from the diagonalization of the mapped IBM Hamiltonian. The parameters of the Hamiltonian are determined via the mapping of the mean-field potential energy surfaces onto the expectation value of the Hamiltonian in the condensate state of the $s$, $d$, and $f$ bosons. Enhanced octupolarity is predicted for Xe, Ba, and Ce isotopes near $N=56$. The shape/phase transition from octupole-deformed to strongly quadrupole-deformed near $N=60$ is analyzed in detail.

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arXiv2021

Evolution of octupole deformation and collectivity in neutron-rich lanthanides

The onset of octupole deformation and its impact on related spectroscopic properties is studied in even-even neutron-rich lanthanide isotopes Xe, Ba, Ce, and Nd with neutron number $86\leqslant N\leqslant 94$. Microscopic input comes from the Hartree-Fock-Bogoliubov approximation with constrains on the axially symmetric quadrupole and octupole operators using the Gogny-D1M interaction. At the mean-field level, reflection asymmetric ground states are predicted for isotopes with neutron number around $N=88$. Spectroscopic properties are studied by diagonalizing the interacting boson model Hamiltonian, with the parameters obtained via the mapping of the mean-field potential energy surface onto the expectation value of the Hamiltonian in the $s$, $d$, and $f$ boson condensate state. The results obtained for low-energy positive- and negative-parity excitation spectra as well as the electric dipole, quadrupole, and octupole transition probabilities indicate the onset of pronounced octupolarity for $Z\approx 56$ and $N\approx 88$ nuclei.

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arXiv2021

Scission configuration in the self-consistent calculations with neck constraint

The calculations of the potential energy surface are essential in the theoretical description of the fission process. In the constrained self-consistent approach, the smooth evolution of nuclear shape is described from the ground state until a very elongated one with a narrow neck. In all microscopic calculations, the rupture of the neck at scission is associated with a substantial change of nuclear matter density distribution and rapid energy decrease. In this paper, we show that there is no discontinuity of the potential energy surface at scission when multi-constrained calculations are applied with the neck constraint. An early rupture of the neck at lower quadrupole and octupole moments is discussed as competitive with the conventional fission path. We discuss the neck properties in the scission configuration. We find that the neck radius in the asymmetric fission mode cannot decrease below 2 fm, and the nuclear matter density cannot decrease below the saturation density. In the compact fission mode, nuclear density may go down to half of the saturation density before the rupture of the neck.

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arXiv2021

Symmetry restoration in mean-field approaches

The mean-field approximation based on effective interactions or density functionals plays a pivotal role in the description of finite quantum many-body systems that are too large to be treated by ab initio methods. Some examples are strongly interacting medium and heavy mass atomic nuclei and mesoscopic condensed matter systems. In this approach, the linear Schrodinger equation for the exact many-body wave function is mapped onto a non-linear density-dependent one-body potential problem. This approximation, not only provides computationally very simple solutions even for systems with many particles, but due to the non-linearity, it also allows for obtaining solutions that break essential symmetries of the system, often connected with phase transitions. In this way, additional correlations are subsumed in the system. However, the mean-field approach suffers from the drawback that the corresponding wave functions do not have sharp quantum numbers and, therefore, many results cannot be compared directly with experimental data. In this article, we discuss general group-theory techniques to restore the broken symmetries, and provide detailed expressions on the restoration of translational, rotational, spin, isospin, parity and gauge symmetries, where the latter corresponds to the restoration of the particle number. In order to avoid the numerical complexity of exact projection techniques, various approximation methods available in the literature are examined. Applications of the projection methods are presented for simple nuclear models, realistic calculations in relatively small configuration spaces, nuclear energy density functional theory, as well as in other mesoscopic systems. Further, unresolved problems in the application of the symmetry restoration methods to the energy density functional theories are highlighted in the present work.

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arXiv2021

The N=50 and Z=28 shell closure revisited

Recent experiments performed in neutron-rich copper isotopes have revealed a crossing in the nucleus $^{75}$Cu between the $3/2^-$ and $5/2^-$ levels, which correspond to the ground-state and the first excited state in isotopes with mass number below $A =75$. Due to the strong single-particle character of these states, this scenario can be investigated through the analysis of the proton spectrum provided by mean-field models in nickel isotopes with neutron numbers between $N$=40 and $N$=50. In this work we show that the aforementioned crossing is mainly driven by the mean-field provided by the effective nucleon-nucleon and spin-orbit interactions. We also analyze the impact of the tensor interaction, and find that in some mean-field models it is essential to reproduce the crossing of the 2$p_{3/2}$ and 1$f_{5/2}$ proton single-particle levels, as in the case of the SAMi-T Skyrme force and the D1M Gogny interaction, whereas in other cases, as for example the SLy5 Skyrme force, a reasonable tensor force appears to be unable to modify the mean-field enough to reproduce this level crossing. Finally, in the calculations performed with the so-called simple effective interaction (SEI), it is shown that the experimental data in nickel and copper isotopes considered in this work can be explained satisfactorily without any explicit consideration of the tensor interaction.

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arXiv2021

Microscopic description of quadrupole-octupole coupling in neutron-rich actinides and superheavy nuclei with the Gogny-D1M energy density functional

The interplay between quadrupole and octupole degrees of freedom is discussed in a series of neutron-rich actinides and superheavy nuclei with $92 \le$ Z $\le 110$ and $186 \le$ N $\le 202$. In addition to the static Hartree-Fock-Bogoliubov approach, dynamical beyond-mean-field correlations are taken into account via both parity restoration and symmetry-conserving Generator Coordinate Method calculations based on the Gogny-D1M energy density functional. Physical properties such as correlation energies, negative-parity excitation energies as well as reduced transition probabilities $B(E1)$ and $B(E3)$ are discussed in detail. It is shown that, for the studied nuclei, the quadrupole-octupole coupling is weak and to a large extent the properties of negative parity states can be reasonably well described in terms of the octupole degree of freedom alone.

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arXiv2021

Quadrupole-octupole coupling and the onset of octupole deformation in actinides

The evolution of quadrupole and octupole collectivity and their coupling is investigated in a series of even-even isotopes of the actinide Ra, Th, U, Pu, Cm, and Cf with neutron number in the interval $130\leqslant N\leqslant 150$. The Hartree-Fock-Bogoliubov approximation, based on the parametrization D1M of the Gogny energy density functional, is employed to generate potential energy surfaces depending upon the axially-symmetric quadrupole and octupole shape degrees of freedom. The mean-field energy surface is then mapped onto the expectation value of the $sdf$ interacting-boson-model Hamiltonian in the boson condensate state as to determine the strength parameters of the boson Hamiltonian. Spectroscopic properties related to the octupole degree of freedom are produced by diagonalizing the mapped Hamiltonian. Calculated low-energy negative-parity spectra, $B(E3;3^{-}_{1}\to 0^{+}_{1})$ reduced transition rates, and effective octupole deformation suggest that the transition from nearly spherical to stable octupole-deformed, and to octupole vibrational states occurs systematically in the actinide region.

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arXiv2020

Octupole correlations in light actinides from the interacting boson model based on the Gogny energy density functional

The quadrupole-octupole coupling and the related spectroscopic properties have been studied for the even-even light actinides $^{218-238}$Ra and $^{220-240}$Th. The Hartree-Fock-Bogoliubov approximation, based on the Gogny-D1M energy density functional, has been employed as a microscopic input, i.e., to obtain (axially symmetric) mean-field potential energy surfaces as functions of the quadrupole and octupole deformation parameters. The mean-field potential energy surfaces have been mapped onto the corresponding bosonic potential energy surfaces using the expectation value of the $sdf$ Interacting Boson Model (IBM) Hamiltonian in the boson condensate state. The strength parameters of the $sdf$-IBM Hamiltonian have been determined via this mapping procedure. The diagonalization of the mapped IBM Hamiltonian provides energies for positive- and negative-parity states as well as wave functions which are employed to obtain transitional strengths. The results of the calculations compare well with available data from Coulomb excitation experiments and point towards a pronounced octupole collectivity around $^{224}$Ra and $^{226}$Th.

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arXiv2020

Description of the multidimensional potential energy surface in fission of $^{252}$Cf and $^{258}$No

The microscopic studies on nuclear fission require the evaluation of the potential energy surface as a function of the collective coordinates. A reasonable choice of constraints on multipole moments should be made to describe the topography of the surface completely within a reasonable amount of computing time. We present a detailed analysis of fission barriers in the self-consistent Hartree-Fock-Bogoliubov approach with the D1S parametrization of the Gogny nucleon-nucleon interaction. Two heavy isotopes representing different spontaneous fission modes - $^{252}$Cf (asymmetric) and $^{258}$No (bimodal) - have been chosen for the analysis. We have shown the existence of complicated structures on the energy surface that can not be fully described in two-dimensional calculations. We analyze apparent problems that can be encountered in this type of calculations: multiple solutions for given constraints and transitions between various potential energy surfaces. We present possible solutions on how to deal with these issues.

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arXiv2020

Microscopic description of quadrupole-octupole coupling in actinides with the Gogny-D1M energy density functional

The interplay between quadrupole and octupole degrees of freedom is discussed in a series of U, Pu, Cm and Cf isotopes both at the mean-field level and beyond. In addition to the static Hartree-Fock-Bogoliubov approach, dynamical beyond-mean-field correlations are taken into account via both parity restoration and symmetry-conserving Generator Coordinate Method calculations based on the parametrization D1M of the Gogny energy density functional. Physical properties such as correlation energies, negative-parity excitation energies as well as reduced transition probabilities $B(E1)$ and $B(E3)$ are discussed in detail and compared with the available experimental data. It is shown that, for the studied nuclei, the quadrupole-octupole coupling is weak and to a large extent the properties of negative parity states can be reasonably well described in terms of the octupole degree of freedom alone.

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arXiv2020

Microscopic description of fission in superheavy nuclei with the parametrization D1M$^{*}$ of the Gogny energy density functional

The constrained Hartree-Fock-Bogoliubov approximation, based on the recent parametrization D1M$^{*}$ of the Gogny energy density functional, is used to describe fission in 435 superheavy nuclei. The Gogny-D1M$^{*}$ parametrization is benchmarked against available experimental data on inner and second barrier heights, excitation energies of the fission isomers and half-lives in a selected set of Pu, Cm, Cf, Fm, No, Rf, Sg, Hs and Fl nuclei. Results are also compared with those obtained with the Gogny-D1M energy density functional. A detailed study of the minimal energy fission paths is carried out for isotopic chains with atomic numbers 100 $\le$ Z $\le$ 126 including very neutron-rich sectors up to around 4 MeV from the two-neutron driplines. Single-particle energies, ground state deformations, pairing correlations, two-nucleon separation energies and barrier heights are also discussed. In addition to fission paths, the constrained Hartree-Fock-Bogoliubov framework provides collective masses and zero-point quantum rotational and vibrational energies. Those quantities are building blocks within the Wentzel-Kramer-Brillouin formalism employed to evaluate the systematic of the spontaneous fission half-lives t$_\mathrm{SF}$. The competition between spontaneous fission and $α$-decay is studied, through the computation of the $α$-decay half-lives t$_\mathrmα$ using a parametrization of the Viola-Seaborg formula. From the comparison with the available experimental data and the results obtained with other theoretical approaches, it is concluded that D1M$^{*}$ represents a reasonable starting point to describe fission in heavy and superheavy nuclei.

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