arXiv subjects

L. Ma

Publications and source records attributed to L. Ma.

At least 37 records · Page 2Linked to original sources

arXiv2023

Optoelectronic properties of one-dimensional molecular chains simulated by a tight-binding model

Studying optical properties of organic materials is important due to the rapid development of organic light-emitting diodes, solar cells, and photon detectors. Here for the first time we have performed tight-binding calculations for singlet excitons, in combination with first-principles calculations of the excited states in molecular dimers, to describe the optical properties of a zinc-phthalocyanine one-dimensional molecular chain. We have included the intra-molecule and charge-transfer excitations and the coupling between them. Our calculations have successfully interpreted a body of experimental UV-Vis optical spectra of transition-metal phthalocyanines. Compared with the previous ab initio calculations for a molecular dimer, the optical absorptions at the split peaks of the Q-bands can be comparable, which indicates the importance of the coupling between the intra-molecular and charge-transfer excitons.

cond-mat.mes-hall↗

arXiv2022

Final results on the $0νββ$ decay half-life limit of $^{100}$Mo from the CUPID-Mo experiment

The CUPID-Mo experiment to search for 0$νββ$ decay in $^{100}$Mo has been recently completed after about 1.5 years of operation at Laboratoire Souterrain de Modane (France). It served as a demonstrator for CUPID, a next generation 0$νββ$ decay experiment. CUPID-Mo was comprised of 20 enriched Li$_2$$^{100}$MoO$_4$ scintillating calorimeters, each with a mass of $\sim$ 0.2 kg, operated at $\sim$20 mK. We present here the final analysis with the full exposure of CUPID-Mo ($^{100}$Mo exposure of 1.47 kg$\times$yr) used to search for lepton number violation via 0$νββ$ decay. We report on various analysis improvements since the previous result on a subset of data, reprocessing all data with these new techniques. We observe zero events in the region of interest and set a new limit on the $^{100}$Mo 0$νββ$ decay half-life of $T^{0ν}_{1/2} > 1.8 \times 10^{24}$ year (stat.+syst.) at 90% CI. Under the light Majorana neutrino exchange mechanism this corresponds to an effective Majorana neutrino mass of $\left < (0.28$--$0.49)$ eV, dependent upon the nuclear matrix element utilized.

nucl-ex↗

arXiv2022

Deep underground laboratory measurement of $^{13}$C($α$,$n$)$^{16}$O in the Gamow windows of the $s$- and $i$-processes

The $^{13}$C($α$,$n$)$^{16}$O reaction is the main neutron source for the slow-neutron-capture (s-) process in Asymptotic Giant Branch stars and for the intermediate (i-) process. Direct measurements at astrophysical energies in above-ground laboratories are hindered by the extremely small cross sections and vast cosmic-ray induced background. We performed the first consistent direct measurement in the range of $E_{\rm c.m.}=$0.24 MeV to 1.9 MeV using the accelerators at the China Jinping Underground Laboratory (CJPL) and Sichuan University. Our measurement covers almost the entire i-process Gamow window in which the large uncertainty of the previous experiments has been reduced from 60\% down to 15\%, eliminates the large systematic uncertainty in the extrapolation arising from the inconsistency of existing data sets, and provides a more reliable reaction rate for the studies of the s- and i-processes along with the first direct determination of the alpha strength for the near-threshold state.

nucl-ex↗

arXiv2022

An Energy-dependent Electro-thermal Response Model of CUORE Cryogenic Calorimeter

The Cryogenic Underground Observatory for Rare Events (CUORE) is the most sensitive experiment searching for neutrinoless double-beta decay ($0νββ$) in $^{130}\text{Te}$. CUORE uses a cryogenic array of 988 TeO$_2$ calorimeters operated at $\sim$10 mK with a total mass of 741 kg. To further increase the sensitivity, the detector response must be well understood. Here, we present a non-linear thermal model for the CUORE experiment on a detector-by-detector basis. We have examined both equilibrium and dynamic electro-thermal models of detectors by numerically fitting non-linear differential equations to the detector data of a subset of CUORE channels which are well characterized and representative of all channels. We demonstrate that the hot-electron effect and electric-field dependence of resistance in NTD-Ge thermistors alone are inadequate to describe our detectors' energy dependent pulse shapes. We introduce an empirical second-order correction factor in the exponential temperature dependence of the thermistor, which produces excellent agreement with energy-dependent pulse shape data up to 6 MeV. We also present a noise analysis using the fitted thermal parameters and show that the intrinsic thermal noise is negligible compared to the observed noise for our detectors.

physics.ins-det↗

arXiv2022

New measurement of double beta decays of $^{100}$Mo to excited states of $^{100}$Ru with the CUPID-Mo experiment

The CUPID-Mo experiment, located at Laboratoire Souterrain de Modane (France), was a demonstrator experiment for CUPID. It consisted of an array of 20 Li$_2^{100}$MoO$_4$ (LMO) calorimeters each equipped with a Ge light detector (LD) for particle identification. In this work, we present the result of a search for two-neutrino and neutrinoless double beta decays of $^{100}$Mo to the first 0$^+$ and $2^+$ excited states of $^{100}$Ru using the full CUPID-Mo exposure (2.71 kg$\times$yr of LMO). We measure the half-life of $2νββ$ decay to the $0^{+}_1$ state as $T_{1/2}^{2ν\rightarrow 0_1^+}=7.5\pm 0.8 \ \text{(stat.)} \ ^{+ 0.4}_{-0.3} \ \text{(syst.)} )\times 10^{20} \ \mathrm{yr}$. The bolometric technique enables measurement of the electron energies as well as the gamma rays from nuclear de-excitation and this allows us to set new limits on the two-neutrino decay to the $2_1^+$ state of $T^{2ν\rightarrow 2_1^+}_{1/2}>4.4\times 10^{21} \ \mathrm{yr} \ \text{(90 % c.i.)}$ and on the neutrinoless modes of $T_{1/2}^{0ν\rightarrow 2_1^+}>2.1\times10^{23} \ \mathrm{yr}\ \text{(90 % c.i.)}$, $T_{1/2}^{0ν\rightarrow 0_1^+}>1.2\times10^{23} \ \mathrm{yr}\ \text{(90 % c.i.)}$. Information on the electrons spectral shape is obtained which allows us to make the first comparison of the single state (SSD) and higher state (HSD) $2νββ$ decay models for the $0_1^+$ excited state of $^{100}$Ru.

nucl-ex↗

arXiv2022

Search for Neutrinoless $β^+EC$ Decay of $^{120}$Te with CUORE

CUORE is a large scale cryogenic experiment searching for neutrinoless double beta decay ($0νββ$) in $^{130}$Te. The CUORE detector is made of natural tellurium, providing the possibility of rare event searches on isotopes other than $^{130}$Te. In this work we describe a search for neutrinoless positron emitting electron capture ($0νβ^+EC$) decay in $^{120}$Te with a total TeO$_2$ exposure of 355.7 kg $\cdot$ yr, corresponding to 0.2405 kg $\cdot$ yr of $^{120}$Te. Albeit $0 νββ$ with two final state electrons represents the most promising channel, the emission of a positron and two 511-keV $γ$s make $0νβ^+EC$ decay signature extremely clear. To fully exploit the potential offered by the detector modularity we include events with different topology and perform a simultaneous fit of five selected signal signatures. Using blinded data we extract a median exclusion sensitivity of $3.4 \cdot 10^{22}$ yr at 90% Credibility Interval (C.I.). After unblinding we find no evidence of $0νβ^+EC$ signal and set a 90% C.I. Bayesian lower limit of $2.9 \cdot 10^{22}$ yr on $^{120}$Te half-life. This result improves by an order of magnitude the existing limit from the combined analysis of CUORE-0 and Cuoricino.

nucl-ex↗

arXiv2022

Cosmogenic background study for a 100Mo-based bolometric demonstration experiment at China JinPing underground Laboratory

We perform simulation study for a 10-kg $^{100}$Mo-based bolometeric demonstration experiment for neutrinoless double-beta decay ($0νββ$) search at China JinPing underground Laboratory (CJPL). Cosmogenic production of radionuclides in $^{100}$Mo-enriched lithium molybdate crystals and copper components of the detector system are studied using Geant4 toolkit based on the simulated cosmic ray data from the CRY library. Background energy spectra of the cosmogenic radionuclides including $^{56}$Co, $^{82}$Rb and $^{88}$Y which are harmful for the $^{100}$Mo-based $0νββ$ experiment are investigated. We then evaluate the total cosmogenic background level in the $^{100}$Mo $0νββ$ search energy region of interest (ROI) for the demonstration experiment. After one year of cooling down underground, the residual background contribution is found to be 1.8$\times$10$^{-6}$ cts/kg/keV/yr and 3.3$\times$10$^{-4}$ cts/kg/keV/yr from crystals and copper components, respectively. Furthermore, underground cosmogenic activation of copper and lithium molybdate crystal is calculated based on the simulation spectra of neutron and proton in CJPL. The underground cosmogenic background is found to be negligible in the ROI.

physics.ins-det↗

arXiv2022

Fourfold anisotropic magnetoresistance of L1$_0$ FePt due to relaxation time anisotropy

Experimental measurements show that the angular dependence of the anisotropic magnetoresistance (AMR) in L1$_0$ ordered FePt epitaxial films on the current orientation and magnetization direction is a superposition of the corresponding dependences of twofold and fourfold symmetries. The twofold AMR exhibits a strong dependence on the current orientation, whereas the fourfold term only depends on the magnetization direction in the crystal and is independent of the current orientation. First-principles calculations reveal that the fourfold AMR arises from the relaxation time anisotropy due to the variation of the density of states near the Fermi energy under rotation of the magnetization. This relaxation time anisotropy is a universal property in ferromagnetic metals and determines other anisotropic physical properties that are observable in experiment.

cond-mat.mtrl-sci↗

arXiv2022

Search for Majorana neutrinos exploiting millikelvin cryogenics with CUORE

The possibility that neutrinos may be their own antiparticles, unique among the known fundamental particles, arises from the symmetric theory of fermions proposed by Ettore Majorana in 1937. Given the profound consequences of such Majorana neutrinos, among which is a potential explanation for the matter-antimatter asymmetry of the universe via leptogenesis, the Majorana nature of neutrinos commands intense experimental scrutiny globally; one of the primary experimental probes is neutrinoless double beta ($0 νββ$) decay. Here we show results from the search for $0 νββ$ decay of $^{130}$Te, using the latest advanced cryogenic calorimeters with the CUORE experiment. CUORE, operating just 10 millikelvin above absolute zero, has pushed the state of the art on three frontiers: the sheer mass held at such ultra-low temperatures, operational longevity, and the low levels of ionising radiation emanating from the cryogenic infrastructure. We find no evidence for $0 νββ$ decay and set a lower bound of $T_{1/2}^{0 ν} > 2.2 \times 10^{25}$ years at a 90% credibility interval. We discuss potential applications of the advances made with CUORE to other fields such as direct dark matter, neutrino and nuclear physics searches and large-scale quantum computing, which can benefit from sustained operation of large payloads in a low-radioactivity, ultra-low temperature cryogenic environment.

nucl-ex↗

arXiv2022

Toward CUPID-1T

Current experiments to search for broken lepton-number symmetry through the observation of neutrinoless double-beta decay ($0\mathrm{νββ}$) provide the most stringent limits on the Majorana nature of neutrinos and the effective Majorana neutrino mass ($m_{ββ}$). The next-generation experiments will focus on the sensitivity to the $0\mathrm{νββ}$ half-life of $\mathcal{O}(10^{27}$--$10^{28}$~years$)$ and $m_{ββ}\lesssim15$~meV, which would provide complete coverage of the so-called Inverted Ordering region of the neutrino mass parameter space. By taking advantage of recent technological breakthroughs, new, future calorimetric experiments at the 1-ton scale can increase the sensitivity by at least another order of magnitude, exploring the large fraction of the parameter space that corresponds to the Normal neutrino mass ordering. In case of a discovery, such experiments could provide important insights toward a new understanding of the mechanism of $0\mathrm{νββ}$. We present here a series of projects underway that will provide advancements in background reduction, cryogenic readout, and physics searches beyond $0\mathrm{νββ}$, all moving toward the next-to-next generation CUPID-1T detector.

nucl-ex↗

arXiv2022

Optimization of the first CUPID detector module

CUPID will be a next generation experiment searching for the neutrinoless double $β$ decay, whose discovery would establish the Majorana nature of the neutrino. Based on the experience achieved with the CUORE experiment, presently taking data at LNGS, CUPID aims to reach a background free environment by means of scintillating Li$_{2}$$^{100}$MoO$_4$ crystals coupled to light detectors. Indeed, the simultaneous heat and light detection allows us to reject the dominant background of $α$ particles, as proven by the CUPID-0 and CUPID-Mo demonstrators. In this work we present the results of the first test of the CUPID baseline module. In particular, we propose a new optimized detector structure and light sensors design to enhance the engineering and the light collection, respectively. We characterized the heat detectors, achieving an energy resolution of (5.9 $\pm$ 0.2) keV FWHM at the $Q$-value of $^{100}$Mo (about 3034 keV). We studied the light collection of the baseline CUPID design with respect to an alternative configuration which features gravity-assisted light detectors' mounting. In both cases we obtained an improvement in the light collection with respect to past measures and we validated the particle identification capability of the detector, which ensures an $α$ particle rejection higher than 99.9%, fully satisfying the requirements for CUPID.

physics.ins-det↗

arXiv2022

Spectrum Sharing for Secrecy Performance Enhancement in D2D-enabled UAV Networks

With the assistance of device-to-device (D2D) communications, unmanned aerial vehicle (UAV) networks are anticipated to support widespread applications in the fifth generation (5G) and beyond wireless systems, by providing seamless coverage, flexible deployment, and high channel rate. However, the networks face significant security threats from malicious eavesdroppers due to the inherent broadcast and openness nature of wireless channels. To ensure secure communications of such networks, physical layer security is a promising technique, which utilizes the randomness and noise of wireless channels to enhance secrecy performance. This article investigates physical layer security performance via spectrum sharing in D2D-enabled UAV networks. We first present two typical network architectures where each UAV serves as either a flying base station or an aerial user equipment. Then, we propose a spectrum sharing strategy to fully exploit interference incurred by spectrum reuse for improving secrecy performance. We further conduct two case studies to evaluate the spectrum sharing strategy in these two typical network architectures, and also show secrecy performance gains compared to traditional spectrum sharing strategy. Finally, we discuss some future research directions in D2D-enabled UAV networks.

cs.NI↗

arXiv2021

Search for Double-Beta Decay of $\mathrm{^{130}Te}$ to the $0^+$ States of $\mathrm{^{130}Xe}$ with CUORE

The CUORE experiment is a large bolometric array searching for the lepton number violating neutrino-less double beta decay ($0νββ$) in the isotope $\mathrm{^{130}Te}$. In this work we present the latest results on two searches for the double beta decay (DBD) of $\mathrm{^{130}Te}$ to the first $0^{+}_2$ excited state of $\mathrm{^{130}Xe}$: the $0νββ$ decay and the Standard Model-allowed two-neutrinos double beta decay ($2νββ$). Both searches are based on a 372.5 kg$\times$yr TeO$_2$ exposure. The de-excitation gamma rays emitted by the excited Xe nucleus in the final state yield a unique signature, which can be searched for with low background by studying coincident events in two or more bolometers. The closely packed arrangement of the CUORE crystals constitutes a significant advantage in this regard. The median limit setting sensitivities at 90\% Credible Interval (C.I.) of the given searches were estimated as $\mathrm{S^{0ν}_{1/2} = 5.6 \times 10^{24} \: \mathrm{yr}}$ for the ${0νββ}$ decay and $\mathrm{S^{2ν}_{1/2} = 2.1 \times 10^{24} \: \mathrm{yr}}$ for the ${2νββ}$ decay. No significant evidence for either of the decay modes was observed and a Bayesian lower bound at $90\%$ C.I. on the decay half lives is obtained as: $\mathrm{(T_{1/2})^{0ν}_{0^+_2} > 5.9 \times 10^{24} \: \mathrm{yr}}$ for the $0νββ$ mode and $\mathrm{(T_{1/2})^{2ν}_{0^+_2} > 1.3 \times 10^{24} \: \mathrm{yr}}$ for the $2νββ$ mode. These represent the most stringent limits on the DBD of $^{130}$Te to excited states and improve by a factor $\sim5$ the previous results on this process.

nucl-ex↗

arXiv2021

Novel technique for the study of pile-up events in cryogenic bolometers

Precise characterization of detector time resolution is of crucial importance for next-generation cryogenic-bolometer experiments searching for neutrinoless double-beta decay, such as CUPID, in order to reject background due to pile-up of two-neutrino double-beta decay events. In this paper, we describe a technique developed to study the pile-up rejection capability of cryogenic bolometers. Our approach, which consists of producing controlled pile-up events with a programmable waveform generator, has the benefit that we can reliably and reproducibly control the time separation and relative energy of the individual components of the generated pile-up events. The resulting data allow us to optimize and benchmark analysis strategies to discriminate between individual and pile-up pulses. We describe a test of this technique performed with a small array of detectors at the Laboratori Nazionali del Gran Sasso, in Italy; we obtain a 90% rejection efficiency against pulser-generated pile-up events with rise time of ~15ms down to time separation between the individual events of about 2ms.

physics.ins-det↗

arXiv2021

Measurement of the 2$νββ$ Decay Half-life of $^{130}$Te with CUORE

We measured two-neutrino double beta decay of $^{130}$Te using an exposure of 300.7 kg$\cdot$yr accumulated with the CUORE detector. Using a Bayesian analysis to fit simulated spectra to experimental data, it was possible to disentangle all the major background sources and precisely measure the two-neutrino contribution. The half-life is in agreement with past measurements with a strongly reduced uncertainty: $T^{2ν}_{1/2} = 7.71^{+0.08}_{-0.06}\mathrm{(stat.)}^{+0.12}_{-0.15}\mathrm{(syst.)}\times10^{20}$ yr. This measurement is the most precise determination of the $^{130}$Te 2$νββ$ decay half-life to date.

nucl-ex↗

arXiv2021

Long-range Rydberg-atom-ion molecules of Rb and Cs

We propose a novel type of Rydberg dimer, consisting of a Rydberg-state atom bound to a distant positive ion. The molecule is formed through long-range electric-multipole interaction between the Rydberg atom and the point-like ion. We present potential energy curves (PECs) that are asymptotically connected with Rydberg $nP$- or $nD$-states of rubidium or cesium. The PECs exhibit deep, long-range wells which support many vibrational states of Rydberg-atom-ion molecules (RAIMs). We consider photo-association of RAIMs in both the weak and the strong optical-coupling regimes between initial and Rydberg states of the neutral atom. Experimental considerations for the realization of RAIMs are discussed.

physics.atom-ph↗

arXiv2021

New Limit for Neutrinoless Double-Beta Decay of $^{100}$Mo from the CUPID-Mo Experiment

The CUPID-Mo experiment at the Laboratoire Souterrain de Modane (France) is a demonstrator for CUPID, the next-generation ton-scale cryogenic $0νββ$ experiment. It consists of a 4.2 kg array of 20 enriched Li$_{2}$$^{100}$MoO$_4$ scintillating bolometers to search for the lepton number violating process of $0νββ$ decay in $^{100}$Mo. With more than one year of operation (2.16 kg$\times$yr of physics data), no event in the region of interest and hence no evidence for $0νββ$ is observed. We report a new limit on the half-life of $0νββ$ decay in $^{100}$Mo of $T_{1/2} > 1.5 \times 10^{24}\,$yr at 90 % C.I. The limit corresponds to an effective Majorana neutrino mass $\langle m_{ββ} \rangle$ $<$ (0.31--0.54)$\,$eV, dependent on the nuclear matrix element in the light Majorana neutrino exchange interpretation.

nucl-ex↗

arXiv2021

Pulse Shape Discrimination in CUPID-Mo using Principal Component Analysis

CUPID-Mo is a cryogenic detector array designed to search for neutrinoless double-beta decay ($0νββ$) of $^{100}$Mo. It uses 20 scintillating $^{100}$Mo-enriched Li$_2$MoO$_4$ bolometers instrumented with Ge light detectors to perform active suppression of $α$ backgrounds, drastically reducing the expected background in the $0νββ$ signal region. As a result, pileup events and small detector instabilities that mimic normal signals become non-negligible potential backgrounds. These types of events can in principle be eliminated based on their signal shapes, which are different from those of regular bolometric pulses. We show that a purely data-driven principal component analysis based approach is able to filter out these anomalous events, without the aid of detector response simulations.

physics.data-an↗