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L. Maisel Licerán

Publications and source records attributed to L. Maisel Licerán.

4 recordsLinked to original sources

Theory of exciton-exciton interactions in crystalline systems

Excitons are bound electron-hole pairs in semiconductors whose interactions influence optical properties and determine their collective behavior and emergent correlated phases. Despite the theoretical and experimental significance of these phenomena, a microscopic theory of exciton-exciton interactions that takes into account the full composite nature of these quasiparticles is lacking. Here, we present a general theory of exciton-exciton interactions that builds upon our previous publication [Physical Review B 113, 155440 (2026)], which applied only to conventional semiconductors with weak band hybridization. By contrast, the theory presented here is valid in virtually any crystalline semiconducting system and can be applied to the study of biexciton formation and correlated excitonic phases in systems where band topology, quantum geometry, and moiré effects play a significant role. In addition to the analytical theory, we also present results in simple systems with flat bands with a nontrivial quantum metric and show that the biexcitonic spectrum differs strongly from that in the case without quantum geometry. Our theory paves the way for accurate quantitative calculations of biexciton spectra and excitonic many-body phases in modern condensed-matter systems.

cond-mat.mes-hall↗

Correlated phases of moat-band excitons in two dimensions

We study dilute two-dimensional systems of interacting excitons with a moat dispersion, whose ground-state manifold consists of a set of discrete or continuously degenerate energy minima. At low densities and in the presence of contact interactions, it is known that the bosons can undergo statistical transmutation and give rise to a chiral spin liquid. Here, we show that long-range interactions such as those expected in excitonic systems introduce a rich competition between the chiral spin liquid and different kinds of Bose-Einstein condensates. The moat dispersion can favor Bose-Einstein condensation into states occupying multiple momenta, leading to inhomogeneous and supersolid phases with a highly anisotropic superfluid response. We demonstrate that a proper $T$-matrix renormalization of the exciton-exciton interaction is essential for describing these phases and show that they can arise even from purely repulsive interactions. This formalism is employed to obtain the phase diagram of competing homogeneous and stripe condensates with the chiral spin liquid in an electron-hole bilayer model. In addition, we show how the $T$ matrix enters the familiar Gross-Pitaevskii framework and map out extended phase diagrams within a pseudopotential approximation. We place our findings in the context of real excitonic systems by discussing the roles of finite lifetimes, disorder, band-structure warping, and nonzero temperatures. We conclude that moat bands can drive Bose-Einstein condensation and supersolidity already at weak coupling, in contrast to the case of a standard parabolic dispersion.

cond-mat.quant-gas↗

Unconventional excitonic insulators in two-dimensional topological materials

Bound electron-hole pairs in semiconductors known as excitons can form a coherent state at low temperatures akin to a BCS condensate. The resulting phase is known as the excitonic insulator and has superfluid properties. Here we theoretically study the excitonic insulator in a pair of recently proposed two-dimensional candidate materials with nontrivial band topology. Contrary to previous works, we include interaction channels that violate the individual electron and hole number conservations. These are on equal footing with the number-conserving processes due to the substantial overlap of Wannier orbitals of different bands, which cannot be exponentially localized due to the nontrivial Chern numbers of the latter. Their inclusion is crucial to determine the symmetry of the electron-hole pairing, and by performing mean-field calculations at nonzero temperatures we find that the order parameter in these systems is a chiral $d$-wave. We discuss the nontrivial topology of this unconventional state and discuss some properties of the associated Berezinskii-Kosterlitz-Thouless transition. In particular, we argue that here it becomes a smooth crossover and estimate the associated temperature to lie between 50 K and 75 K on realistic substrates, over an order of magnitude larger than in the number-conserving approximation where $s$-wave pairing is favored. Our results highlight the interplay between topology at the single-particle level and long-range interactions, motivating further research in systems where both phenomena coexist.

cond-mat.str-el↗

Topological Wannier excitons in bismuth chalcogenide nanosheets I: Single-particle properties

We analyze the topology and dispersion of bulk Wannier excitons in nanosheets of topological insulators in the family of bismuth chalcogenides. Our main finding is that excitons also inherit the topology of the electronic bands, quantified by the skyrmion winding numbers of the constituent electron and hole pseudospins as a function of the total exciton momentum. We furthermore show that every $s$-wave exciton state consists of a quartet with a degenerate and quadratically dispersing nonchiral doublet, and a chiral doublet with one linearly dispersing mode as in transition metal dichalcogenides. We also demonstrate the existence of topological edge states of chiral excitons arising from the bulk-boundary correspondence.

cond-mat.mes-hall↗