arXiv subjects

L. Patthey

Publications and source records attributed to L. Patthey.

At least 55 records · Page 3Linked to original sources

arXiv2009

Renormalization of Bulk Magnetic Electron States at High Binding Energies

The quasiparticle dynamics of electrons in a magnetically ordered state is investigated by high-resolution angle-resolved photoemission of Ni(110) at 10 K. The self-energy is extracted for high binding energies reaching up to 500 meV, using a Gutzwiller calculation as a reference frame for correlated quasiparticles. Significant deviations exist in the 300 meV range, as identified on magnetic bulk bands for the first time. The discrepancy is strikingly well described by a self-energy model assuming interactions with spin excitations. Implications relating to different electron-electron correlation regimes are discussed.

cond-mat.str-el↗

arXiv2009

First observation of spin-helical Dirac fermions and topological phases in undoped and doped Bi2Te3 demonstrated by spin-ARPES spectroscopy

Electron systems that possess light-like dispersion relations or the conical Dirac spectrum, such as graphene and bismuth, have recently been shown to harbor unusual collective states in high magnetic fields. Such states are possible because their light-like electrons come in spin pairs that are chiral,which means that their direction of propagation is tied to a quantity called pseudospin that describes their location in the crystal lattice. An emerging direction in quantum materials research is the manipulation of atomic spin-orbit coupling to simulate the effect of a spin dependent magnetic field,in attempt to realize novel spin phases of matter. This effect has been proposed to realize systems consisting of unpaired Dirac cones that are helical, meaning their direction of propagation is tied to the electron spin itself, which are forbidden to exist in graphene or bismuth. The experimental existence of topological order can not be determined without spin-resolved measurements. Here we report a spin-and angle-resolved photoemission study of the hexagonal surface of the Bi2Te3 and Bi{2-x}MnxTe3 series, which is found to exhibit a single helical Dirac cone that is fully spin-polarized. Our observations of a gap in the bulk spin-degenerate band and a spin-resolved surface Dirac node close to the chemical potential show that the low energy dynamics of Bi2Te3 is dominated by the unpaired spin-helical Dirac modes. Our spin-texture measurements prove the existence of a rare topological phase in this materials class for the first time, and suggest its suitability for novel 2D Dirac spin device applications beyond the chiral variety or traditional graphene.

cond-mat.mes-hall↗

arXiv2009

Anisotropic dressing of charge-carriers in the electron-doped cuprate superconductor Sm(1.85)Ce(0.15)CuO(4) from angle-resolved photoemission measurements

Angle-resolved photoemission measurements on the electron-doped cuprate Sm(1.85)Ce(0.15)CuO(4) evidence anisotropic dressing of charge-carriers due to many-body interactions. Most significantly, the scattering rate along the zone boundary saturates for binding energies larger than ~200 meV, while along the diagonal direction it increases nearly linearly with the binding energy in the energy range ~150-500 meV. These results indicate that many-body interactions along the diagonal direction are strong down to the bottom of the band, while along the zone-bounday they become very weak at energies above ~200 meV.

cond-mat.supr-con↗

arXiv2009

Collective spin excitations in a quantum spin ladder probed by high-resolution Resonant Inelastic X-ray Scattering

We investigate magnetic excitations in the spin-ladder compound Sr$_{14}$Cu$_{24}$O$_{41}$ using high-resolution Cu $L_3$-edge Resonant Inelastic X-ray Scattering (RIXS). Our findings demonstrate that RIXS couples to collective spin excitations from a quantum spin-liquid ground state. In contrast to Inelastic Neutron Scattering (INS), the RIXS cross section changes only moderately over the entire Brillouin Zone (BZ), revealing a high sensitivity also at small momentum transfers. The two-triplon energy gap is found to be $100\pm 30$ meV. Our results are supported by calculations within an effective Hubbard model for a finite-size cluster.

cond-mat.str-el↗

arXiv2008

Spectroscopic evidence for preformed Cooper pairs in the pseudogap phase of cuprates

Angle-resolved photoemission on underdoped La$_{1.895}$Sr$_{0.105}$CuO$_4$ reveals that in the pseudogap phase, the dispersion has two branches located above and below the Fermi level with a minimum at the Fermi momentum. This is characteristic of the Bogoliubov dispersion in the superconducting state. We also observe that the superconducting and pseudogaps have the same d-wave form with the same amplitude. Our observations provide direct evidence for preformed Cooper pairs, implying that the pseudogap phase is a precursor to superconductivity.

cond-mat.supr-con↗

arXiv2008

Spontaneous exciton condensation in 1T-TiSe2: a BCS-like approach

Recently strong evidence has been found in favor of a BCS-like condensation of excitons in 1\textit{T}-TiSe$_2$. Theoretical photoemission intensity maps have been generated by the spectral function calculated within the excitonic condensate phase model and set against experimental angle-resolved photoemission spectroscopy data. Here, the calculations in the framework of this model are presented in detail. They represent an extension of the original excitonic insulator phase model of Jérome \textit{et al.} [Phys. Rev. {\bf 158}, 462 (1967)] to three dimensional and anisotropic band dispersions. A detailed analysis of its properties and further comparison with experiment are also discussed

cond-mat.str-el↗

arXiv2008

The coherent {\it d}-wave superconducting gap in underdoped La$_{2-x}$Sr$_{x}$CuO$_4$ as studied by angle-resolved photoemission

We present angle-resolved photoemission spectroscopy (ARPES) data on moderately underdoped La$_{1.855}$Sr$_{0.145}$CuO$_4$ at temperatures below and above the superconducting transition temperature. Unlike previous studies of this material, we observe sharp spectral peaks along the entire underlying Fermi surface in the superconducting state. These peaks trace out an energy gap that follows a simple {\it d}-wave form, with a maximum superconducting gap of 14 meV. Our results are consistent with a single gap picture for the cuprates. Furthermore our data on the even more underdoped sample La$_{1.895}$Sr$_{0.105}$CuO$_4$ also show sharp spectral peaks, even at the antinode, with a maximum superconducting gap of 26 meV.

cond-mat.supr-con↗

arXiv2008

The electronic structure of La$_{1-x}$Sr$_{x}$MnO$_{3}$ thin films and its $T_c$ dependence as studied by angle-resolved photoemission

We present angle-resolved photoemission spectroscopy results for thin films of the three-dimensional manganese perovskite La$_{1-x}$Sr$_{x}$MnO$_{3}$. We show that the transition temperature ($T_c$) from the paramagnetic insulating to ferromagnetic metallic state is closely related to details of the electronic structure, particularly to the spectral weight at the ${\bf k}$-point, where the sharpest step at the Fermi level was observed. We found that this ${\bf k}$-point is the same for all the samples, despite their different $T_c$. The change of $T_c$ is discussed in terms of kinetic energy optimization. Our ARPES results suggest that the change of the electronic structure for the samples having different transition temperatures is different from the rigid band shift.

cond-mat.str-el↗

arXiv2008

Pseudogap-driven Hall effect sign reversal

We present a calculation of the Hall coefficient in 2H-TaSe2 and 2H-Cu0.2NbS2 relied on the photoemission data and compare the results to transport observations. The approach, based on the solution of the semiclassical Boltzmann equation in the isotropic tau-approximation yields high-temperature Hall coefficient consistent with the one measured directly. Taking into account the opening of the pseudogap and redistribution of the spectral weight, recently observed in angle resolved photoemission spectra of 2H-TaSe2, allows us to reproduce the temperature dependence of the Hall coefficient including prominent sign change with no adjustable parameters.

cond-mat.supr-con↗

arXiv2008

Non-monotonic pseudo-gap in high-Tc cuprates

The mechanism of high temperature superconductivity is not resolved for so long because the normal state of cuprates is not yet understood. Here we show that the normal state pseudo-gap exhibits an unexpected non-monotonic temperature dependence, which rules out the possibility to describe it by a single mechanism such as superconducting phase fluctuations. Moreover, this behaviour, being remarkably similar to the behaviour of the charge ordering gap in the transition-metal dichalcogenides, completes the correspondence between these two classes of compounds: the cuprates in the PG state and the dichalcogenides in the incommensurate charge ordering state reveal virtually identical spectra of one-particle excitations as function of energy, momentum and temperature. These results suggest that the normal state pseudo-gap, which was considered to be very peculiar to cuprates, seems to be a general complex phenomenon for 2D metals. This may not only help to clarify the normal state electronic structure of 2D metals but also provide new insight into electronic properties of 2D solids where the metal-insulator and metal-superconductor transitions are considered on similar basis as instabilities of particle-hole and particle-particle interaction, respectively.

cond-mat.supr-con↗

arXiv2007

The electronic structure of La$_{1.48}$Nd$_{0.4}$Sr$_{0.12}$CuO$_4$ probed by high- and low-energy angle-resolved photoelectron spectroscopy: evolution with probing depth

We present angle-resolved photoelectron spectroscopy data probing the electronic structure of the Nd-substituted high-$T_c$ cuprate La$_{1.48}$Nd$_{0.4}$Sr$_{0.12}$CuO$_4$ (Nd-LSCO). Data have been acquired at low and high photon energies, $hν$ = 55 and 500 eV, respectively. Earlier comparable low-energy studies of La$_{1.4-x}$Nd$_{0.6}$Sr$_{x}$CuO$_4$ ($x = 0.10, 0.12, 0.15$) have shown strongly suppressed photoemission intensity, or absence thereof, in large parts of the Brillouin zone. Contrary to these findings we observe spectral weight at all points along the entire Fermi surface contour at low and high photon energies. No signs of strong charge modulations are found. At high photon energy, the Fermi surface shows obvious differences in shape as compared to the low-energy results presented here and in similar studies. The observed difference in shape and the high bulk-sensitivity at this photon energy suggest intrinsic electronic structure differences between the surface and bulk regions.

cond-mat.str-el↗

arXiv2007

Non-gapped Fermi surfaces, quasiparticles and the anomalous temperature dependence of the near-$E_F$ electronic states in the CMR oxide La$_{2-2x}$Sr$_{1+2x}$Mn$_2$O$_7$ with $x=0.36$

After years of research into colossal magnetoresistant (CMR) manganites using bulk techniques, there has been a recent upsurge in experiments directly probing the electronic states at or near the surface of the bilayer CMR materials La$_{2-2x}$Sr$_{1+2x}$Mn$_2$O$_7$ using angle-resolved photoemission or scanning probe microscopy. Here we report new, temperature dependent, angle resolved photoemission data from single crystals with a doping level of $x=0.36$. The first important result is that there is no sign of a pseudogap in the charge channel of this material for temperatures below the Curie temperature $T_C$. The second important result concerns the temperature dependence of the electronic states. The temperature dependent changes in the Fermi surface spectra both at the zone face and zone diagonal regions in $k$-space indicate that the coherent quasiparticle weight disappears for temperatures significantly above $T_C$, and that the $k$-dependence of the T-induced changes in the spectra invalidate an interpretation of these data in terms of the superposition of a `universal' metallic spectrum and an insulating spectrum whose relative weight changes with temperature. In this sense, our data are not compatible with a phase separation scenario.

cond-mat.str-el↗

arXiv2007

Direct observation of strong correlations near the band insulator regime of Bi misfit cobaltates

We present the first angle-resolved photoemission (ARPES) measurement of Fermi Surface in the "misfit" cobaltate [Bi2Ba2O4].[CoO2]~2. This compound contains the same triangular Co planes as Na cobaltates, but in a different 3D environment. Our data establish the similarity of their electronic structure. We propose that the peculiar lineshape of all cobaltates is of the "peak-dip-hump" type, due to strong many-body effects. We detect a progressive transfer of spectral weight from the quasiparticle feature near Ef to a broad hump in misfit phases where Ba is replaced by Sr or Ca. This indicates stronger many-body interactions in proximity of the band insulator regime, which we attribute to the presence of unusual magnetic excitations.

cond-mat.str-el↗

arXiv2007

Pseudogap and charge density waves in two dimensions

An interaction between electrons and lattice vibrations (phonons) results in two fundamental quantum phenomena in solids: in three dimensions it can turn a metal into a superconductor whereas in one dimension it can turn a metal into an insulator. In two dimensions (2D) both superconductivity and charge-density waves (CDW) are believed to be anomalous. In superconducting cuprates, critical transition temperatures are unusually high and the energy gap may stay unclosed even above these temperatures (pseudogap). In CDW-bearing dichalcogenides the resistivity below the transition can decrease with temperature even faster than in the normal phase and a basic prerequisite for the CDW, the favourable nesting conditions (when some sections of the Fermi surface appear shifted by the same vector), seems to be absent. Notwithstanding the existence of alternatives to conventional theories, both phenomena in 2D still remain the most fascinating puzzles in condensed matter physics. Using the latest developments in high-resolution angle-resolved photoemission spectroscopy (ARPES) here we show that the normal-state pseudogap also exists in one of the most studied 2D examples, dichalcogenide 2H-TaSe2, and the formation of CDW is driven by a conventional nesting instability, which is masked by the pseudogap. Our findings reconcile and explain a number of unusual, as previously believed, experimental responses as well as disprove many alternative theoretical approaches. The magnitude, character and anisotropy of the 2D-CDW pseudogap are intriguingly similar to those seen in superconducting cuprates.

cond-mat.supr-con↗

arXiv2007

Evidence for an excitonic insulator phase in 1T-TiSe$_{2}$

We present a new high-resolution angle-resolved photoemission study of 1\textit{T}-TiSe$_{2}$ in both, its room-temperature, normal phase and its low-temperature, charge-density wave phase. At low temperature the photoemission spectra are strongly modified, with large band renormalisations at high-symmetry points of the Brillouin zone and a very large transfer of spectral weight to backfolded bands. A theoretical calculation of the spectral function for an excitonic insulator phase reproduces the experimental features with very good agreement. This gives strong evidence in favour of the excitonic insulator scenario as a driving force for the charge-density wave transition in 1\textit{T}-TiSe$_{2}$.

cond-mat.str-el↗

arXiv2007

Disentangling surface and bulk photoemission using circularly polarized light

We show that in the angle resolved photoemission spectroscopy (ARPES) near-surface induced fields can be useful for disentangling the surface and bulk related emission. The jump of the dielectric function at the interface results in a nonzero term $\operatorname{div}\textbf{A}$ in the photoemission matrix element. The term happens to be significant approximately within the first unit cell and leads to the circular dichroism for the states localized therein. As an example we use ARPES spectra of an YBa$_2$Cu$_3$O$_{7-δ}$ crystal to distinguish between the overdoped surface related component and its bulk counterparts.

cond-mat.supr-con↗

arXiv2006

When low- and high-energy electronic responses meet in cuprate superconductors

The existence of coherent quasiparticles near the Fermi energy in the low temperature state of high-temperature superconductors has been well established by angle-resolved photoemission spectroscopy (ARPES). This technique directly probes the momentum-resolved electronic excitation spectrum of the CuO$_2$ planes. We present a study of close to optimally doped La$_{1.83}$Sr$_{0.17}$CuO$_4$ in the superconducting state and report an abrupt change in the quasiparticle spectral function, as we follow the dispersion of the ARPES signal from the Fermi energy up to 0.6 eV. The interruption in the quasiparticle dispersion separates coherent quasiparticle peaks at low energies from broad incoherent excitations at high energies. We find that the boundary between these low-energy and high-energy features exhibits a cosine-shaped momentum dependence, reminiscent of the superconducting d-wave gap. Further intriguing similarities between characteristics of the incoherent excitations and quasiparticle properties (lifetime, Fermi arcs) suggest a close relation between the electronic response at high and low energies in cuprate superconductors.

cond-mat.supr-con↗

arXiv2006

Coexistence of metallicity and superconductivity in adjacent bilayers of a high-Tc superconductor

Experimental studies of the electronic structure remain the basic means for understanding the nature of high-temperature superconductivity (HTSC) and testing relevant theoretical models. Appreciable contributions to establish the overall picture in HTSC have recently been made by investigations on the charge dynamics in BSCCO (ref. 1) and the spin dynamics in YBCO, using Angle Resolved Photoemission Spectroscopy (ARPES) and Inelastic Neutron Scattering (INS), respectively. Concentration of each of these techniques on a "suitable" compound turns out to be a barrier on the way to a crucial quantitative test allowing to support or discard spin fluctuations (interaction between the charge and spin degrees of freedom) as a possible origin for the pairing in doped cuprates. Here we solve the long-standing puzzle of ARPES on YBCO by showing that the photoelectron spectrum of YBCO generally includes two components: One from the topmost anomalously overdoped metallic CuO2 bilayer and the other from the next superconducting bilayer that retains the bulk properties. Our findings clearly show the opening of a large superconducting gap and, for the first time, demonstrate the anisotropic renormalization in the bulk component of YBCO, supporting the universality of these effects for different cuprate families. With our study we re-open this cuprate family for new systematic ARPES investigations.

cond-mat.supr-con↗