arXiv subjects

L. Pierre

Publications and source records attributed to L. Pierre.

8 recordsLinked to original sources

arXiv2023

Finite-temperature phase transitions in $S=1/2$ three-dimensional Heisenberg magnets from high-temperature series expansions

Many frustrated spin models on three-dimensional (3D) lattices are currently being investigated, both experimentally and theoretically, and develop new types of long-range orders in their respective phase diagrams. They present finite-temperature phase transitions, most likely in the Heisenberg 3D universality class. However, the combination between the 3D character and frustration makes them hard to study. We present here several methods derived from high-temperature series expansions (HTSEs), which give exact coefficients directly in the thermodynamic limit up to a certain order; for several 3D lattices, supplementary orders than in previous literature are reported for the HTSEs. We introduce an interpolation method able to describe thermodynamic quantities at $T > T_c$, which we use here to reconstruct the magnetic susceptibility and the specific heat and to extract universal and non-universal quantities (for example critical exponents, temperature, energy, entropy, and other parameters related to the phase transition). While the susceptibility associated with the order parameter is not usually known for more exotic long-range orders, the specific heat is indicative of a phase transition for any kind of symmetry breaking. We present examples of applications on ferromagnetic and antiferromagnetic models on various 3D lattices and benchmark our results whenever possible.

cond-mat.str-el↗

arXiv2021

Logarithmic divergent specific heat from high-temperature series expansions: application to the two-dimensional XXZ Heisenberg model

We present an interpolation method for the specific heat $c_v(T)$, when there is a phase transition with a logarithmic singularity in $c_v$ at a critical temperature $T=T_c$. The method uses the fact that $c_v$ is constrained both by its high temperature series expansion, and just above $T_c$ by the type of singularity. We test our method on the ferro and antiferromagnetic Ising model on the two-dimensional square, triangular, honeycomb, and kagome lattices, where we find an excellent agreement with the exact solutions. We then explore the XXZ Heisenberg model, for which no exact results are available.

cond-mat.str-el↗

arXiv2008

Chirality and $Z_2$ vortices in an Heisenberg spin model on the kagomé lattice

The phase diagram of the classical \jj model on the \kag lattice is investigated using extensive \mc simulations. In a realistic range of parameters, this model has a low-temperature chiral-ordered phase without long-range spin order. We show that the critical transition marking the destruction of chiral order is preempted by the first order proliferation of \Zdeux point defects. The core energy of these vortices appears to vanish when approaching the T=0 phase boundary, where both \Zdeux defects and gapless magnons contribute to disordering the system at very low temperature. This situation might be typical of a large class of frustrated magnets. Possible relevance for real materials is also discussed.

cond-mat.str-el↗

arXiv2003

Determination of the exchange energies in Li2VOSiO4 from a high-temperature series analysis of the square lattice J1-J2 Heisenberg model

We present a high-temperature expansion (HTE) of the magnetic susceptibility and specific heat data of Melzi et al. on Li2VOSiO4 [Phys. Rev. B 64, 024409 (2001)]. The data are very well reproduced by the J1-J2 Heisenberg model on the square lattice with exchange energies J1=1.25+-0.5 K and J2=5.95+-0.2 K. The maximum of the specific heat Cv^{max}(T_{max}) is obtained as a function J2/J1 from an improved method based on HTE.

cond-mat.str-el↗

arXiv1998

First excitations of the spin 1/2 Heisenberg antiferromagnet on the kagomé lattice

We study the exact low energy spectra of the spin 1/2 Heisenberg antiferromagnet on small samples of the kagomé lattice of up to N=36 sites. In agreement with the conclusions of previous authors, we find that these low energy spectra contradict the hypothesis of Néel type long range order. Certainly, the ground state of this system is a spin liquid, but its properties are rather unusual. The magnetic ($ΔS=1$) excitations are separated from the ground state by a gap. However, this gap is filled with nonmagnetic ($ΔS=0$) excitations. In the thermodynamic limit the spectrum of these nonmagnetic excitations will presumably develop into a gapless continuum adjacent to the ground state. Surprisingly, the eigenstates of samples with an odd number of sites, i.e. samples with an unsaturated spin, exhibit symmetries which could support long range chiral order. We do not know if these states will be true thermodynamic states or only metastable ones. In any case, the low energy properties of the spin 1/2 Heisenberg antiferromagnet on the kagomé lattice clearly distinguish this system from either a short range RVB spin liquid or a standard chiral spin liquid. Presumably they are facets of a generically new state of frustrated two-dimensional quantum antiferromagnets.

cond-mat.stat-mech↗

arXiv1997

Order versus Disorder in the Quantum Heisenberg Antiferromagnet on the Kagom{é} lattice: an approach through exact spectra analysis

A group symmetry analysis of the low lying levels of the spin-1/2 kagomé Heisenberg antiferromagnet is performed for small samples up to N=27. This approach allows to follow the effect of quantum fluctuations when the sample size increases. The results contradict the scenario of ``order by disorder'' which has been advanced on the basis of large S calculations. A large enough second neighbor ferromagnetic exchange coupling is needed to stabilize the $\sqrt 3 \times \sqrt 3$ pattern: the finite size analysis indicates a quantum critical transition at a non zero coupling.

cond-mat.str-el↗

arXiv1995

$J_1-J_2$ quantum Heisenberg antiferromagnet on the triangular lattice: a group symmetry analysis of order by disorder

On the triangular lattice, for $J_2/J_1$ between $1/8$ and $1$, the classical Heisenberg model with first and second neighbor interactions presents four-sublattice ordered ground-states. Spin-wave calculations of Chubukov and Jolicoeur\cite{cj92} and Korshunov\cite{k93} suggest that quantum fluctuations select amongst these states a colinear two-sublattice order. From theoretical requirements, we develop the full symmetry analysis of the low lying levels of the spin-1/2 Hamiltonian in the hypotheses of either a four or a two-sublattice order. We show on the exact spectra of periodic samples ($N=12,16$ and $28$) how quantum fluctuations select the colinear order from the four-sublattice order.

cond-mat↗

arXiv1994

Exact spectra, spin susceptibilities and order parameter of the quantum Heisenberg antiferromagnet on the triangular lattice

Exact spectra of periodic samples are computed up to $ N=36 $. Evidence of an extensive set of low lying levels, lower than the softest magnons, is exhibited. These low lying quantum states are degenerated in the thermodynamic limit; their symmetries and dynamics as well as their finite-size scaling are strong arguments in favor of Néel order. It is shown that the Néel order parameter agrees with first-order spin-wave calculations. A simple explanation of the low energy dynamics is given as well as the numerical determinations of the energies, order parameter and spin susceptibilities of the studied samples. It is shown how suitable boundary conditions, which do not frustrate Néel order, allow the study of samples with $ N=3p+1 $ spins. A thorough study of these situations is done in parallel with the more conventional case $ N=3p $.

cond-mat↗