arXiv subjects

L. Roso

Publications and source records attributed to L. Roso.

At least 19 recordsLinked to original sources

arXiv2023

Towards direct spatial and intensity characterization of ultra-high intensity laser pulses using ponderomotive scattering of free electrons

Spatial distributions of electrons ionized and scattered from ultra-low pressure gases are proposed and experimentally demonstrated as a method to directly measure the intensity of an ultra-high intensity laser pulse. Analytic models relating the peak scattered electron energy to the peak laser intensity are derived and compared to paraxial Runge-Kutta simulations highlighting two models suitable for describing electrons scattered from weakly paraxial beams ($f_{\#}>5$) for intensities in the range of $10^{18}-10^{21}$Wcm$^{-2}$. Scattering energies are shown to be dependant on gas species emphasizing the need for specific gases for given intensity ranges. Direct measurements of the laser intensity at full power of two laser systems is demonstrated both showing a good agreement between indirect methods of intensity measurement and the proposed method. One experiment exhibited the role of spatial aberrations in the scattered electron distribution motivating a qualitative study on the effect. We propose the use of convolutional neural networks as a method for extracting quantitative information of the spatial structure of the laser at full power. We believe the presented technique to be a powerful tool that can be immediately implemented in many high-power laser facilities worldwide.

physics.plasm-ph↗

arXiv2020

A quasi-monoenergetic short time duration compact proton source for probing high energy density states of matter

We report on the development of a highly directional, narrow energy band, short time duration proton beam operating at high repetition rate, suitable for measurements of stopping power in high energy density plasmas as well as other applications. The protons are generated with an ultrashort-pulse laser interacting with a solid target and converted to a pencil-like narrow-band beam using a compact magnet-based energy selector. We experimentally demonstrate the production of a proton beam with an energy of 500 keV and energy spread well below 10%, and a pulse duration of 260 ps. The energy loss of this beam is measured in a 2 $μ$m thick solid Mylar target and found to be in within 1% of theoretical predictions. The short time duration of the proton pulse makes it particularly well suited for applications involving the probing of highly transient plasma states produced in laser-matter interaction experiments, in particular measurements of proton stopping power.

physics.plasm-ph↗

arXiv2019

Towards an in situ, full-power gauge of the focal-volume intensity of petawatt-class lasers

About 50 years ago, Sarachick and Schappert [Phys. Rev. D. 1, 2738 (1970)] showed that relativistic Thomson scattering leads to wavelength shifts that are proportional to the laser intensity. About 28 years later Chen et al. [Nature 396, 653 (1998)] used these shifts to estimate their laser intensity near 10^18 W/cm^2. More recently there have been several theoretical studies aimed at exploiting nonlinear Thomson scattering as a tool for direct measurement of intensities well into the relativistic regime. We present the first quantitative study of this approach for intensities between 10^18 and 10^19 W/cm^2. We show that the spectral shifts are in reasonable agreement with estimates of the peak intensity extracted from images of the focal area obtained at reduced power. Finally, we discuss the viability of the approach, its range of usefulness and how it might be extended to gauge intensities well in excess of 10^19 W/cm^2.

physics.plasm-ph↗

arXiv2019

A 2D scintillator based proton detector for HRR experiments

We present a scintillator based detector able to measure both spatial and energy information at High repetition rate (HRR) with a relatively simple design. It has been built at the Center of Pulsed Laser (CLPU) in Salamanca and tested in the proton accelerator at the Centro de Micro-Analisis de Materiales (CMAM) in Madrid. The detector has been demonstrated to work in HRR mode by reproducing the performance of the radiochromic film detector. It represents a new class of on-line detectors for Laser-plasma physics experiments in the new emerging High Power and HRR laser systems.

physics.ins-det↗

arXiv2018

Development of an adjustable Kirkpatrick-Baez microscope for laser driven x-ray sources at CLPU

A promising prototype of a highly adjustable Kirkpatrick-Baez (KB) microscope has been designed, built and tested in a number of laser driven x-ray experiments using the high power (200TW) VEGA-2 laser system of the Spanish Centre for Pulsed Lasers (CLPU). The presented KB version consists of two, perpendicularly mounted, 500μm thick Silicon wafers, coated with a few tens of nm layer of Platinum unlike the conventional, coated, millimetre thick glass substrates, affording more bending flexibility and large adjustment range. According to simulations, and based on total external reflection, this KB offers a broad-band multi-keV reflection spectra, allowing more spectral tunablity than conventional Bragg crystals. In addition to be vacuum compatible, the prototype is characterised by a relatively small size (21cm x 31cm x 27cm) and permits remote control and modification of both the radius of curvature (down to 10m) and the grazing incidence angle (up to 60mrad). A few examples of focusing performance tests, limitations and experimental campaign results are discussed.

physics.ins-det↗

arXiv2018

Generation of high energy laser-driven electron and proton sources with the 200 TW system VEGA 2 at the Centro de Laseres Pulsados

The Centro de Laseres Pulsados in Salamanca Spain has recently started operation phase and the first User access period on the 6 J 30 fs 200 TW system (VEGA 2) already started at the beginning of 2018. In this paper we report on two commissioning experiments recently performed on the VEGA 2 system in preparation for the user campaign. VEGA 2 system has been tested in different configurations depending on the focusing optics and targets used. One configuration (long focal length f=130 cm) is for under-dense laser-matter interaction where VEGA 2 is focused onto a low density gas-jet generating electron beams (via laser wake field acceleration mechanism) with maximum energy up to 500 MeV and an X-ray betatron source with a 10 keV critical energy. A second configuration (short focal length f=40 cm) is for over-dense laser-matter interaction where VEGA 2 is focused onto an 5 microns thick Al target generating a proton beam with a maximum energy of 10 MeV and average energy of 7-8 MeV and temperature of 2.5 MeV. In this paper we present preliminary experimental results.

physics.plasm-ph↗

arXiv2018

Reevaluation of radiation reaction and consequences for light-matter interactions at the nanoscale

In the context of electromagnetism and nonlinear optical interactions damping is generally introduced as a phenomenological, viscous term that dissipates energy, proportional to the temporal derivative of the polarization. Here, we follow the radiation reaction method presented in [G. W. Ford and R. F. O'Connell, Phys. Lett. A, 157, 217 (1991)], which applies to non-relativistic electrons of finite size, to introduce an explicit reaction force in the Newtonian equation of motion, and derive a hydrodynamic equation that offers new insight on the influence of damping in generic plasmas, metal-based and/or dielectric structures. In these settings, we find new damping-dependent linear and nonlinear source terms that suggest the damping coefficient is proportional to the local charge density, and nonlocal contributions that stem from the spatial derivative of the magnetic field and discuss the conditions that could modify both linear and nonlinear electromagnetic responses.

physics.optics↗

arXiv2018

High-order harmonic generation driven by inhomogeneous plasmonics fields spatially bounded: influence on the cut-off law

We study high-order harmonic generation (HHG) in model atoms driven by plasmonic-enhanced fields. These fields result from the illumination of plasmonic nanostructures by few-cycle laser pulses. We demonstrate that the spatial inhomogeneous character of the laser electric field, in a form of Gaussian-shaped functions, leads to an unexpected relationship between the HHG cutoff and the laser wavelength. Precise description of the spatial form of the plasmonic-enhanced field allows us to predict this relationship. We combine the numerical solutions of the time-dependent Schrödinger equation (TDSE) with the plasmonic-enhanced electric fields obtained from 3D finite element simulations. We additionally employ classical simulations to supplement the TDSE outcomes and characterize the extended HHG spectra by means of their associated electron trajectories. A proper definition of the spatially inhomogeneous laser electric field is instrumental to accurately describe the underlying physics of HHG driven by plasmonic-enhanced fields. This characterization opens new perspectives for HHG control with various experimental nano-setups

physics.atom-ph↗

arXiv2017

X-ray emission from a liquid curtain jet when irradiated by femtosecond laser pulses

Laser-based sources of ionizing radiation have attracted a considerable attention in the last years for their broad potential applications. However the stability and robustness of such sources is still an issue that needs to be addressed. Aiming to solve such problems, we propose a source that uses a liquid jet -rather than a solid- as a target for the production of X-rays. Liquid jets offer always a clean surface for every laser shot which represent a clear advantage over solids. In this work, we present an experimental characterization of the X-ray emission of such targets, and study the efficiency of the process when two temporally delayed pulses are used. According to the obtained results, the X-ray yield is comparable with commonly used targets.

physics.plasm-ph↗

arXiv2016

Emergence of a higher energy structure in strong field ionization with inhomogeneous electric fields

Studies of strong field ionization have historically relied on the strong field approximation, which neglects all spatial dependence in the forces experienced by the electron after ionization. More recently, the small spatial inhomogeneity introduced by the long-range Coulomb potential has been linked to a number of important features in the photoelectron spectrum, such as Coulomb asymmetry, Coulomb focusing, and the low energy structure (LES). Here, we demonstrate by combined quantum and classical simulations that a small time-varying spatial dependence in the laser electric field creates a prominent higher energy peak at energies above the "classical cut-off" for direct electrons. This higher energy structure (HES) originates from direct electrons ionized near the peak of a single half-cycle of the laser pulse. The HES is separated from all other ionization events (providing sub-cycle resolution) and is highly sensitive to the carrier envelope phase (CEP). The large accumulation of electrons with tuneable energy suggests a promising method for creating a localized source of electron pulses of attosecond duration using tabletop laser technology.

physics.atom-ph↗

arXiv2016

Attosecond physics at the nanoscale

Recently two emerging areas of research, attosecond and nanoscale physics, have started to come together. Attosecond physics deals with phenomena occurring when ultrashort laser pulses, with duration on the femto- and sub-femtosecond time scales, interact with atoms, molecules or solids. The laser-induced electron dynamics occurs natively on a timescale down to a few hundred or even tens of attoseconds, which is comparable with the optical field. On the other hand, the second branch involves the manipulation and engineering of mesoscopic systems, such as solids, metals and dielectrics, with nanometric precision. Although nano-engineering is a vast and well-established research field on its own, the merger with intense laser physics is relatively recent. In this article we present a comprehensive experimental and theoretical overview of physics that takes place when short and intense laser pulses interact with nanosystems, such as metallic and dielectric nanostructures. In particular we elucidate how the spatially inhomogeneous laser induced fields at a nanometer scale modify the laser-driven electron dynamics. Consequently, this has important impact on pivotal processes such as ATI and HHG. The deep understanding of the coupled dynamics between these spatially inhomogeneous fields and matter configures a promising way to new avenues of research and applications. Thanks to the maturity that attosecond physics has reached, together with the tremendous advance in material engineering and manipulation techniques, the age of atto-nano physics has begun, but it is in the initial stage. We present thus some of the open questions, challenges and prospects for experimental confirmation of theoretical predictions, as well as experiments aimed at characterizing the induced fields and the unique electron dynamics initiated by them with high temporal and spatial resolution.

physics.atom-ph↗

arXiv2016

Laser-based X-ray and electron source for X-ray fluorescence studies

In this work we present a modification to conventional X-rays fluorescence using electrons as excitation source, and compare it with the traditional X-ray excitation for the study of pigments. For this purpose we have constructed a laser-based source capable to produce X-rays as well as electrons. Because of the large penetration depth of X-rays, the collected fluorescence signal is a combination of several material layers of the artwork under study. However electrons are stopped in the first layers allowing therefore a more superficial analysis. We show that the combination of both excitation sources can provide extremely valuable information about the structure of the artwork.

physics.ins-det↗

arXiv2015

Determination of the species generated in atmospheric-pressure laser-induced plasmas by mass spectrometry techniques

We present temporal information obtained by mass spectrometry techniques about the evolution of plasmas generated by laser filamentation in air. The experimental setup used in this work allowed us to study not only the dynamics of the filament core but also of the energy reservoir that surrounds it. Furthermore, valuable insights about the chemistry of such systems like the photofragmentation and/or formation of molecules were obtained. The interpretation of the experimental results are supported by PIC (particle in cell) simulations.

physics.plasm-ph↗

arXiv2015

Carrier-wave Rabi flopping signatures in high-order harmonic generation for alkali atoms

We present the first theoretical investigation of carrier-wave Rabi flopping in real atoms by employing numerical simulations of high-order harmonic generation (HHG) in alkali species. Given the short HHG cutoff, related to the low saturation intensity, we concentrate on the features of the third harmonic of sodium (Na) and potassium (K) atoms. For pulse areas of 2$π$ and Na atoms, a characteristic unique peak appears, which, after analyzing the ground state population, we correlate with the conventional Rabi flopping. On the other hand, for larger pulse areas, carrier-wave Rabi flopping occurs, and is associated with a more complex structure in the third harmonic. These new characteristics observed in K atoms indicate the breakdown of the area theorem, as was already demonstrated under similar circumstances in narrow band gap semiconductors.

physics.atom-ph↗

arXiv2014

High-order harmonic generation at high laser intensities beyond the tunnel regime

We present studies of high-order harmonic generation (HHG) at laser intensities well above saturation. We use driving laser pulses which present a particular electron dynamics in the turn-on stage. Our results predict an increasing on the harmonic yield, after an initial dropping, when the laser intensity is increased. This fact contradicts the general belief of a progressive degradation of the harmonic emission at ultrahigh intensities. We have identified a particular set of trajectories which emerges in the turn-on stage of these singular laser pulses, responsible of the unexpected growth on the harmonic efficiency at this high intensity regime. Our study combines two complementary approaches: classical analysis and full quantum mechanical calculations resulting from the numerical integration of the 3-dimensional time-dependent Schrödinger equation complemented with the time-frequency analysis.

physics.atom-ph↗

arXiv2013

Electron momentum distributions and photoelectron spectra of atoms driven by intense spatially inhomogeneous field

We use three dimensional time-dependent Schrödinger equation (3D--TDSE) to calculate angular electron momentum distributions and photoelectron spectra of atoms driven by spatially inhomogeneous fields. An example for such inhomogeneous fields is the locally enhanced field induced by resonant plasmons, appearing at surfaces of metallic nanoparticles, nanotips and gold bow-tie shape nanostructures. Our studies show that the inhomogeneity of the laser electric field plays an important role in the above threshold ionization process in the tunneling regime, causing significant modifications to the electron momentum distributions and photoelectron spectra, while its effects in the multiphoton regime appear to be negligible. Indeed, through tunneling ATI process, one can obtain higher energy electrons as well as high degree of asymmetry in the momentum space map. In this study we consider near infrared laser fields with intensities in the mid-$10^{14}$ W/cm$^{2}$ range and we use linear approximation to describe their spatial dependence. We show that in this case it is possible to drive electrons with energies in the near-keV regime. Furthermore, we study how the carrier envelope phase influences the emission of ATI photoelectrons for few-cycle pulses. Our quantum mechanical calculations are fully supported by their classical counterparts.

physics.atom-ph↗

arXiv2012

Beyond Carbon K-edge harmonic emission using spatial and temporal synthesized laser field

We present numerical simulations of high-order harmonic generation in helium using a temporally synthesised and spatially non-homogeneous strong laser field. The combination of temporal and spatial laser field synthesis results in a dramatic cut-off extension far beyond the usual semiclassical limit. Our predictions are based on the convergence of three complementary approaches: resolution of the three dimensional Time Dependent Schrödinger Equation, time-frequency analysis of the resulting dipole moment and classical trajectories extraction. Employing a combination of temporally and spatially synthesised laser field provides coherent XUV photons beyond the carbon K-edge which is of high interest for initiating inner-shell dynamics and study time-resolved intra-molecular attosecond spectroscopy.

physics.optics↗

arXiv2010

Dipole spectrum structure of non-resonant non-pertubative driven two-level atoms

We analize the dipole spectrum of a two-level atom excited by a non-resonant intense monochromatic field, under the electric dipole approximation and beyond the rotating wave approximation. We show that the apparently complex spectral structure can be completely described by two families: harmonic frequencies of the driving field and field-induced nonlinear fluorescence. Our formulation of the problem provides quantitative laws for the most relevant spectral features: harmonic ratios and phases, non-perturbative Stark shift, and frequency limits of the harmonic plateau. In particular, we demonstrate the locking of the harmonic phases at the wings of the plateau opening the possibility of ultra-short pulse generation through harmonic filtering.

physics.optics↗