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L. Smejkal

Publications and source records attributed to L. Smejkal.

5 recordsLinked to original sources

Altermagnetic spintronics

The research landscape of magnetism has been recently enriched by the discovery of altermagnetism. It is an unconventional phase of matter characterized by a d-wave (or higher even-parity-wave) collinear compensated spin ordering, which enables strongly spin-polarized currents in the absence of magnetization, and features fast spin dynamics. Simultaneously, on the applied magnetism front, spintronic memories based on conventional ferromagnets are currently turning from a niche to a mass produced integrated-circuit technology as they start to complement semiconductors on advanced-node microprocessor chips. Our review connects these two rapidly developing science and technology fields by discussing how the unique signatures of altermagnetism can impact the functionality and scalability of future spintronic devices. As a reference, we first briefly recall the merits and physical limitations of the present ferromagnetic spintronic technology, and of proof-of-concept spintronic devices based on conventional collinear antiferromagnets and non-collinear compensated magnets. The main part of the review then focuses on physical concepts of the altermagnetic spintronics, and its potential interplay with ferroelectricity or superconductivity. We conclude with an outlook on the nascent experimental research of altermagnetic spintronics, and on the role of relativistic phenomena.

cond-mat.mtrl-sci

Altermagnetism: an unconventional spin-ordered phase of matter

The Pauli exclusion principle combined with interactions between fermions is a basic mechanism across condensed-matter systems giving rise to a spontaneous breaking of the spin-space rotation symmetry of spin-ordered phases. Ferromagnetism is a conventional manifestation of spin ordering which leads to numerous applications, e.g., in spintronic information technologies. Altermagnetism, whose recent discovery was largely motivated by spintronics, stands apart from conventional magnetism in the sense that it spontaneously breaks not only spin-space but also real-space rotation symmetries, while it preserves a symmetry combining spin-space and real-space rotations. This is realized on crystals by a collinear compensated ordering of spins with a characteristic d, g or i-wave symmetry. Our Perspective goes beyond the theory of spin arrangements on crystals by connecting altermagnetism to basic notions in condensed matter physics. Specifically, we reflect on the analogies and distinctions of altermagnetism as compared to superfluid 3He and theories of spin ordering in the momentum space generated by other higher-partial-wave instabilities of a Fermi-liquid. On one hand, all these physical systems have in common the extraordinary combination of spontaneous breaking of spin-space and real-space rotation symmetries. On the other hand, we point out that there are key differences, both at the symmetry level and, particularly, at the level of microscopic mechanisms of ordering. These explain the comparatively large abundance, robustness and utility of altermagnetism, as predicted by the symmetry-classification of spin arrangements on crystals and ab initio calculations, and supported by initial experiments.

cond-mat.mtrl-sci

Observation of time-reversal symmetry breaking in the band structure of altermagnetic RuO$_2$

Altermagnets are an emerging third elementary class of magnets. Unlike ferromagnets, their distinct crystal symmetries inhibit magnetization while, unlike antiferromagnets, they promote strong spin polarization in the band structure. The corresponding unconventional mechanism of timereversal symmetry breaking without magnetization in the electronic spectra has been regarded as a primary signature of altermagnetism, but has not been experimentally visualized to date. We directly observe strong time-reversal symmetry breaking in the band structure of altermagnetic RuO$_2$ by detecting magnetic circular dichroism in angle-resolved photoemission spectra. Our experimental results, supported by ab initio calculations, establish the microscopic electronic-structure basis for a family of novel phenomena and functionalities in fields ranging from topological matter to spintronics, that are based on the unconventional time-reversal symmetry breaking in altermagnets.

cond-mat.mtrl-sci

Band structure of CuMnAs probed by optical and photoemission spectroscopy

Tetragonal phase of CuMnAs progressively appears as one of the key materials for antiferromagnetic spintronics due to efficient current-induced spin-orbit torques whose existence can be directly inferred from crystal symmetry. Theoretical understanding of spintronic phenomena in this material, however, relies on the detailed knowledge of electronic structure (band structure and corresponding wave functions) which has so far been tested only to a limited extent. We show that AC permittivity (obtained from ellipsometry) and UV photoelectron spectra agree with density functional calculations. Together with the x-ray diffraction and precession electron diffraction tomography, our analysis confirms recent theoretical claim [Phys.Rev.B 96, 094406 (2017)] that copper atoms occupy lattice positions in the basal plane of the tetragonal unit cell.

cond-mat.mtrl-sci

Room-temperature spin-orbit torque in NiMnSb

Materials that crystalize in diamond-related lattices, with Si and GaAs as their prime examples, are at the foundation of modern electronics. Simultaneoulsy, the two atomic sites in the unit cell of these crystals form inversion partners which gives rise to relativistic non-equilibrium spin phenomena highly relevant for magnetic memories and other spintronic devices. When the inversion-partner sites are occupied by the same atomic species, electrical current can generate local spin polarization with the same magnitude and opposite sign on the two inversion-partner sites. In CuMnAs, which shares this specific crystal symmetry of the Si lattice, the effect led to the demonstration of electrical switching in an antiferromagnetic memory at room temperature. When the inversion-partner sites are occupied by different atoms, a non-zero global spin-polarization is generated by the applied current which can switch a ferromagnet, as reported at low temperatures in the diluted magnetic semiconductor (Ga,Mn)As. Here we demonstrate the effect of the global current-induced spin polarization in a counterpart crystal-symmetry material NiMnSb which is a member of the broad family of magnetic Heusler compounds. It is an ordered high-temperature ferromagnetic metal whose other favorable characteristics include high spin-polarization and low damping of magnetization dynamics. Our experiments are performed on strained single-crystal epilayers of NiMnSb grown on InGaAs. By performing all-electrical ferromagnetic resonance measurements in microbars patterned along different crystal axes we detect room-temperature spin-orbit torques generated by effective fields of the Dresselhaus symmetry. The measured magnitude and symmetry of the current-induced torques are consistent with our relativistic density-functional theory calculations.

cond-mat.mtrl-sci