arXiv subjects

L. Snyder

Publications and source records attributed to L. Snyder.

9 recordsLinked to original sources

arXiv2024

Remeasurement of the $^{239}$Pu(n,f)/$^{235}$U(n,f) Cross-Section Ratio with the NIFFTE fission Time Projection Chamber Using Vapor-deposited Targets

The NIFFTE fission Time Projection Chamber (fissionTPC) has been used to measure the $^{239}$Pu(n,f)/$^{235}$U(n,f) cross-section ratio for neutron-induced fission in the range of 0.1 - 100 MeV, with high precision. A white neutron source was provided by the Los Alamos Neutron Science Center, where the experiment was conducted as a remeasurement to evaluate a roughly 2% discrepancy of the previous fissionTPC results with ENDF/B-VIII.0. A detailed accounting of measurement uncertainties was performed, based on the fissionTPC's novel ability to provide three-dimensional reconstruction of fission-fragment ionization profiles. Current results obtained using a vapor-deposited, highly uniform $^{239}$Pu target, in comparison to the measurement published in 2021, where a $^{239}$Pu electroplated target was used, are presented and discussed. The remeasurement presented here is in agreement with the previous fissionTPC result within measurement uncertainties.

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arXiv2021

Measurement of the $^{239}$Pu(n,f)/$^{235}$U(n,f) Cross-Section Ratio with the NIFFTE fission Time Projection Chamber

The $^{239}$Pu(n,f)/$^{235}$U(n,f) cross-section ratio has been measured with the fission Time Projection Chamber (fissionTPC) from 100 keV to 100 MeV. The fissionTPC provides three-dimensional reconstruction of fission-fragment ionization profiles, allowing for a precise quantification of measurement uncertainties. The measurement was performed at the Los Alamos Neutron Science Center which provides a pulsed white source of neutrons. The data are recommended to be used as a cross-section ratio shape. A discussion of the status of the absolute normalization and comparisons to ENDF evaluations and previous measurements is included.

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arXiv2021

Measurement of material isotopics and atom number ratio with alpha-particle spectroscopy for the NIFFTE fission Time Projection Chamber actinide target

We present the results of a measurement of isotopic concentrations and atomic number ratio of a double-sided actinide target with alpha-spectroscopy and mass spectrometry. The double-sided actinide target, with primarily Pu-239 on one side and U-235 on the other, was used in the fission Time Projection Chamber (fissionTPC) for a measurement of the neutron-induced fission cross-section ratio between the two isotopes. The measured atomic number ratio is intended to provide an absolute normalization of the measured fission cross-section ratio. The Pu-239/U-235 atom number ratio was measured with a combination of mass spectrometry and alpha-spectroscopy with a planar silicon detector with uncertainties of less than 1%.

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arXiv2020

Neutron Induced Fission Fragment Angular Distributions, Anisotropy, and Linear Momentum Transfer Measured with the NIFFTE Fission Time Projection Chamber

The Neutron Induced Fission Fragment Tracking Experiment (NIFFTE) collaboration has performed measurements with a fission time projection chamber (fissionTPC) to study the fission process by reconstructing full three-dimensional tracks of fission fragments and other ionizing radiation. The amount of linear momentum imparted to the fissioning nucleus by the incident neutron can be inferred by measuring the opening angle between the fission fragments. Using this measured linear momentum, fission fragment angular distributions can be converted to the center-of-mass frame for anisotropy measurements. Angular anisotropy is an important experimental observable for understanding the quantum mechanical state of the fissioning nucleus and vital to determining detection efficiency for cross section measurements. Neutron linear momentum transfer to fissioning $^{235}$U, $^{238}$U, and $^{239}$Pu and fission fragment angular anisotropy of $^{235}$U and $^{238}$U as a function of neutron energies in the range 130 keV--250 MeV are presented.

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arXiv2019

Fission Fragment Angular Anisotropy in Neutron-Induced Fission of $^{235}$U Measured with a Time Projection Chamber

Fission fragment angular distributions can provide an important constraint on fission theory, improving predictive fission codes, and are a prerequisite for a precise ratio cross section measurement. Available anisotropy data is sparse, especially at neutron energies above 5 MeV. For the first time, a three-dimensional tracking detector is employed to study fragment emission angles and provide a direct measurement of angular anisotropy. The Neutron Induced Fission Fragment Tracking Experiment (NIFFTE) collaboration has deployed the fission time projection chamber (fissionTPC) to measure nuclear data with unprecedented precision. The fission fragment anisotropy of $^{235}$U has been measured over a wide range of incident neutron energies from 180 keV to 200 MeV; a careful study of the systematic uncertainties complement the data.

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arXiv2019

1H(n,el) as a Cross Section Reference in a White Source Neutron Beam With the fissionTPC

We provide a quantitative description of a method to measure neutron-induced fission cross sections in ratio to elastic hydrogen scattering in a white-source neutron beam with the fission Time Projection Chamber. This detector has measured precision fission cross section ratios using actinide references such as $^{235}$U(n,f) and $^{238}$U(n,f). However, by employing a more precise reference such as the H(n,el) cross section there is the potential to further reduce the evaluation uncertainties of the measured cross sections. In principle the fissionTPC could provide a unique measurement by simultaneously measuring both fission fragments and proton recoils over a large solid angle. We investigate one method with a hydrogenous gas target and with the neutron energy determined by the proton recoil kinematics. This method enables the measurement to be performed in a white-source neutron beam and with the current configuration of the fissionTPC. We show that while such a measurement is feasible in the energy range of 0.5 MeV to $\sim$10 MeV, uncertainties on the proton detection efficiency and the neutron energy resolution do not allow us to preform a fission ratio measurement to the desired precision. Utilizing either a direct measurement of the neutron time-of-flight for the recoil proton or a mono-energetic neutron source or some combination of both would provide a path to a sub-percent precision measurement.

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arXiv2018

Measurement of the normalized $^{238}$U(n,f)/$^{235}$U(n,f) cross section ratio from threshold to 30 MeV with the fission Time Projection Chamber

The normalized $^{238}$U(n,f)/$^{235}$U(n,f) cross section ratio has been measured using the NIFFTE fission Time Projection Chamber from the reaction threshold to $30$~MeV. The fissionTPC is a two-volume MICROMEGAS time projection chamber that allows for full three-dimensional reconstruction of fission-fragment ionization profiles from neutron-induced fission. The measurement was performed at the Los Alamos Neutron Science Center, where the neutron energy is determined from neutron time-of-flight. The $^{238}$U(n,f)/$^{235}$U(n,f) ratio reported here is the first cross section measurement made with the fissionTPC, and will provide new experimental data for evaluation of the $^{238}$U(n,f) cross section, an important standard used in neutron-flux measurements. Use of a development target in this work prevented the determination of an absolute normalization, to be addressed in future measurements. Instead, the measured cross section ratio has been normalized to ENDF/B-VIII.$β$5 at 14.5 MeV.

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arXiv2014

A Time Projection Chamber for High Accuracy and Precision Fission Cross Section Measurements

The fission Time Projection Chamber (fissionTPC) is a compact (15 cm diameter) two-chamber MICROMEGAS TPC designed to make precision cross section measurements of neutron-induced fission. The actinide targets are placed on the central cathode and irradiated with a neutron beam that passes axially through the TPC inducing fission in the target. The 4$π$ acceptance for fission fragments and complete charged particle track reconstruction are powerful features of the fissionTPC which will be used to measure fission cross sections and examine the associated systematic errors. This paper provides a detailed description of the design requirements, the design solutions, and the initial performance of the fissionTPC.

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arXiv2013

Targets for Precision Measurements

The general properties needed in targets (sources) for high precision, high accuracy measurements are reviewed. The application of these principles to the problem of developing targets for the Fission TPC is described. Longer term issues, such as the availability of actinide materials, improved knowledge of energy losses and straggling and the stability of targets during irradiation are also discussed.

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