arXiv subjects

L. Szunyogh

Publications and source records attributed to L. Szunyogh.

At least 19 recordsLinked to original sources

arXiv2024

THz spin-wave excitations in the transverse conical phase of BiFeO$_3$

Although BiFeO$_3$ is one of the most studied multiferroic materials, recent magnetization and neutron scattering studies have revealed a new magnetic phase in this compound - the transverse conical phase. To study the collective spin excitations of this phase, we performed THz spectroscopy in magnetic fields up to 17 T at and above room temperature. We observed five spin-wave branches in the magnetic phase with long wavelength conical modulation. Using a numerical spin dynamics model we found two kinds of excitations with magnetic moments oscillating either along or perpendicular to the static fields. Remarkably, we detected strong directional dichroism, an optical manifestation of the magnetoelectric effect, for two spin-wave modes of the conical phase. According to our experiments, the stability of the conical state is sensitive to the magnetic field history and it can become (meta)stable at or close to zero magnetic field, which may allow exploiting its magnetoelectric properties at room temperature.

cond-mat.mtrl-sci↗

arXiv2021

Exceptional sign changes of the non-local spin Seebeck effect in antiferromagnetic hematite

Low power spintronic devices based on the propagation of pure magnonic spin currents in antiferromagnetic insulator materials offer several distinct advantages over ferromagnetic components including higher frequency magnons and a stability against disturbing external magnetic fields. In this work, we make use of the insulating antiferromagnetic phase of iron oxide, the mineral hematite $α$-Fe$_2$O$_3$ to investigate the long distance transport of thermally generated magnonic spin currents. We report on the excitation of magnons generated by the spin Seebeck effect, transported both parallel and perpendicular to the antiferromagnetic easy-axis under an applied magnetic field. Making use of an atomistic hematite toy model, we calculate the transport characteristics from the deviation of the antiferromagnetic ordering from equilibrium under an applied field. We resolve the role of the magnetic order parameters in the transport, and experimentally we find significant thermal spin transport without the need for a net magnetization.

cond-mat.mtrl-sci↗

arXiv2019

Damping in Ru/Co-based multilayer films with large Dzyaloshinskii-Moriya interaction

Recent development of the magnetic material engineering led to achievement of the systems with a high interfacial Dzyaloshinskii-Moriya interaction (DMI). As a result, the formation of non-collinear magnetic soliton states or nonreciprocal spin wave dynamics is achievable. Typically used materials are based on bi-layers Heavy Metal/Ferromagnet, e.g., Pt/Co. These layers are characterized not only by a strong DMI, but also by the spin pumping effect and the resulting relatively large damping. Here, we show that the considerable interfacial DMI can be also present in bi-layers based on Ru/Co, characterized with low spin pumping effect and low damping. It is therefore a good candidate for the dynamical studies and implementations of chiral DMI. It is demonstrated by theoretical calculations that the value of DMI can be strongly affected and controlled by the strain of the lattice. We show a systematic experimental and theoretical comparison of magnetic material parameters between Pt/Co and Ru/Co bi-layers as a deserving candidate for spintronic and spin-orbitronic applications.

cond-mat.mtrl-sci↗

arXiv2018

Magnetism of a Co monolayer on Pt(111) capped by overlayers of $5d$ elements: a spin-model study

Using first-principles calculations, we study the magnetic properties of a Co monolayer on a Pt(111) surface with a capping monolayer of selected $5d$ elements (Re, Os, Ir, Pt and Au). First we determine the tensorial exchange interactions and magnetic anisotropies characterizing the Co monolayer for all considered systems. We find a close relationship between the magnetic moment of the Co atoms and the nearest-neighbor isotropic exchange interaction, which is attributed to the electronic hybridization between the Co and the capping layers, in spirit of the Stoner picture of ferromagnetism. The Dzyaloshinskii-Moriya interaction is decreased for all overlayers compared to the uncapped Co/Pt(111) system, while even the sign of the Dzyaloshinskii-Moriya interaction changes in case of the Ir overlayer. We conclude that the variation of the Dzyaloshinskii-Moriya interaction is well correlated with the change of the magnetic anisotropy energy and of the orbital moment anisotropy. The unique influence of the Ir overlayer on the Dzyaloshinskii-Moriya interaction is traced by scaling the strength of the spin--orbit coupling of the Ir atoms in Ir/Co/Pt(111) and by changing the Ir concentration in the Au$_{1-x}$Ir$_{x}$/Co/Pt(111) system. Our spin dynamics simulations indicate that the magnetic ground state of Re/Co/Pt(111) thin film is a spin spiral with a tilted normal vector, while the other systems are ferromagnetic.

cond-mat.mtrl-sci↗

arXiv2017

Role of temperature-dependent spin model parameters in ultra-fast magnetization dynamics

In the spirit of multi-scale modelling magnetization dynamics at elevated temperature is often simulated in terms of a spin model where the model parameters are derived from first principles. While these parameters are mostly assumed temperature-independent and thermal properties arise from spin fluctuations only, other scenarios are also possible. Choosing bcc Fe as an example, we investigate the influence of different kinds of model assumptions on ultra-fast spin dynamics, where following a femtosecond laser pulse a sample is demagnetized due to a sudden rise of the electron temperature. While different model assumptions do not affect the simulational results qualitatively, their details do depend on the nature of the modelling.

cond-mat.mtrl-sci↗

arXiv2016

Domain wall profiles in Co/Ir$_n$/Pt(111) ultrathin films: influence of the Dzyaloshinskii-Moriya interaction

We perform a study of domain walls in Co/Ir$_n$/Pt(111) (n = 0,1,...,6) films by a combined approach of first-principles calculations and spin dynamics simulations. We determine the tensorial exchange interactions and the magnetic anisotropies for the Co overlayer in both FCC and HCP geometries, depending on the number of Ir buffer layers. We find strong ferromagnetic nearest-neighbor isotropic exchange interactions between the Co atoms and an out-of-plane magnetic anisotropy for the films in FCC geometry. Our simulations show that the magnetic domain walls are of Néel type, and their rotational sense (chirality) is changed upon the insertion of an Ir buffer layer as compared to the pristine Co/Pt(111) system. Our spin dynamics simulations indicate a twisting of the spins with respect to the planar domain wall profile on the triangular lattice. We discuss this domain wall twisting using symmetry arguments and in terms of an appropriate micromagnetic continuum model considering extra energy terms compared to the available literature.

cond-mat.mes-hall↗

arXiv2015

Improved efficiency of heat generation in nonlinear dynamics of magnetic nanoparticles

The deterministic Landau-Lifshitz-Gilbert equation has been used to investigate the nonlinear dynamics of magnetization and the specific loss power in magnetic nanoparticles with uniaxial anisotropy driven by a rotating magnetic field. We propose a new type of applied field, which is "simultaneously rotating and alternating", i.e. the direction of the rotating external field changes periodically. We show that a more efficient heat generation by magnetic nanoparticles is possible with this new type of applied field and we suggest its possible experimental realization in cancer therapy which requires the enhancement of loss energies.

cond-mat.mes-hall↗

arXiv2015

Band bending at the surface of Bi$_2$Se$_3$ studied from first principles

The band bending (BB) effect on the surface of the second-generation topological insulators implies a serious challenge to design transport devices. The BB is triggered by the effective electric field generated by charged impurities close to the surface and by the inhomogeneous charge distribution of the occupied surface states. Our self-consistent calculations in the Korringa-Kohn-Rostoker framework showed that in contrast to the bulk bands, the spectrum of the surface states is not bent at the surface. In turn, it is possible to tune the energy level of the Dirac point via the deposited surface dopants. In addition, the electrostatic modifications induced by the charged impurities on the surface induce long range oscillations in the charge density. For dopants located beneath the surface, however, these oscillations become highly suppressed. Our findings are in good agreement with recent experiments, however, our results indicate that the concentration of the surface doping cannot be estimated from the energy shift of the Dirac cone within the scope of the effective continuous model for the protected surface states.

cond-mat.mes-hall↗

arXiv2015

Universal distribution of magnetic anisotropy of impurities in ordered and disordered nano-grains

We examine the distribution of the magnetic anisotropy (MA) experienced by a magnetic impurity embedded in a metallic nano-grain. As an example of a generic magnetic impurity with partially filled $d$-shell, we study the case of $d^{1}$ impurities imbedded into ordered and disordered Au nano-grains, described in terms of a realistic band structure. Confinement of the electrons induces a magnetic anisotropy that is large, and can be characterized by 5 real parameters, coupling to the quadrupolar moments of the spin. In ordered (spherical) nano-grains, these parameters exhibit symmetrical structures and reflect the symmetry of the underlying lattice, while for disordered grains they are randomly distributed and, - for stronger disorder, - their distribution is found to be characterized by random matrix theory. As a result, the probability of having small magnetic anisotropies $K_L$ is suppressed below a characteristic scale $Δ_E$, which we predict to scale with the number of atoms $N$ as $Δ_E\sim 1/N^{3/2}$. This gives rise to anomalies in the specific heat and the susceptibility at temperatures $T\sim Δ_E$ and produces distinct structures in the magnetic excitation spectrum of the clusters, that should be possible to detect experimentally.

cond-mat.mes-hall↗

arXiv2015

Magnetic correlations beyond the Heisenberg model in an Fe monolayer on Rh(001)

Motivated by a recent experimental observation of a complex magnetic structure [Takada et al. 2013 J. Magn. Magn. Mater. 329 95] we present a theoretical study of the magnetic structure of an Fe monolayer deposited on Rh(001). We use a classical spin Hamiltonian with parameters obtained from ab initio calculations and go beyond the usual anisotropic Heisenberg model by including isotropic biquadratic interactions. Zero-temperature Landau--Lifshitz--Gilbert spin dynamics simulations lead to a complex collinear spin configuration that, however, contradicts experimental finding. We thus conclude that higher order multi-spin interactions are likely needed to account for the magnetic ordering of the system.

cond-mat.mes-hall↗

arXiv2014

Non-collinear Magnetic Configurations at Finite Temperature in Thin Films

The finite-temperature magnetism of a monolayer on a bcc (110) surface was examined using a model Hamiltonian containing ferromagnetic or antiferromagnetic exchange interactions, Dzyaloshinsky-Moriya interactions and easy-axis on-site anisotropy. We examined the competition between the collinear ground state parallel to the easy axis and the spin spiral state in the plane perpendicular to this axis preferred by the Dzyaloshinsky-Moriya interaction. Using approximative methods to calculate the magnon spectrum at finite temperatures, it was found that even if the ground state is collinear, increasing the Dzyaloshinsky-Moriya interaction strongly decreases the critical temperature where this collinear order disappears. Using atomistic spin dynamics simulations it was found that at this critical temperature the system transforms into the non-collinear state. Including external magnetic field helps stabilising the ferromagnetic state. An effect due to the finite size of the magnetic monolayer was included in the model by considering a different value for the anisotropy at the edges of the monolayer. This effect was shown to stabilize the spin spiral state by fixing the phase at the ends of the stripe.

cond-mat.str-el↗

arXiv2014

Formation of magnetic skyrmions with tunable properties in PdFe bilayer deposited on Ir(111)

We perform an extensive study of the spin-configurations in a PdFe bilayer on Ir(111) in terms of ab initio and spin-model calculations. We use the spin-cluster expansion technique to obtain spin model parameters, and solve the Landau-Lifshitz-Gilbert equations at zero temperature. In particular, we focus on effects of layer relaxations and the evolution of the magnetic ground state in external magnetic field. In the absence of magnetic field, we find a spin-spiral ground state, while applying external magnetic field skyrmions are generated in the system. Based on energy calculations of frozen spin configurations with varying magnetic field we obtain excellent agreement for the phase boundaries with available experiments. We find that the wave length of spin-spirals and the diameter of skyrmions decrease with increasing inward Fe layer relaxation which is correlated with the increasing ratio of the nearest-neighbor Dzyaloshinskii-Moriya interaction and the isotropic exchange coupling, $D/J$. Our results also indicate that the applied field needed to stabilize the skyrmion lattice increases when the diameter of individual skyrmions decreases. Based on our observations, we suggest that the formation of the skyrmion lattice can be tuned by small structural modification of the thin film.

cond-mat.mtrl-sci↗

arXiv2014

Langevin spin dynamics based on ab initio calculations: numerical schemes and applications

A method is proposed to study the finite-temperature behaviour of small magnetic clusters based on solving the stochastic Landau-Lifshitz-Gilbert equations, where the effective magnetic field is calculated directly during the solution of the dynamical equations from first principles instead of relying on an effective spin Hamiltonian. Different numerical solvers are discussed in the case of a one-dimensional Heisenberg chain with nearest-neighbour interactions. We performed detailed investigations for a monatomic chain of ten Co atoms on top of Au(001) surface. We found a spiral-like ground state of the spins due to Dzyaloshinsky-Moriya interactions, while the finite-temperature magnetic behaviour of the system was well described by a nearest-neighbour Heisenberg model including easy-axis anisotropy.

cond-mat.mtrl-sci↗

arXiv2014

Metallic magnetism at finite temperatures studied by relativistic disordered moment description: Theory and applications

We develop a self-consistent relativistic disordered local moment (RDLM) scheme aimed at describing finite temperature magnetism of itinerant metals from first principles. Our implementation in terms of the Korringa--Kohn--Rostoker multiple scattering theory and the coherent potential approximation allows to relate the orientational distribution of the spins to the electronic structure, thus a self-consistent treatment of the distribution is possible. We present applications for bulk bcc Fe, L1$_0$-FePt and FeRh ordered in the CsCl structure. The calculations for Fe show significant variation of the local moments with temperature, whereas according to the mean field treatment of the spin fluctuations the Curie temperature is overestimated. The magnetic anisotropy of FePt alloys is found to depend strongly on intermixing between nominally Fe and Pt layers, and it shows a power-law behavior as a function of magnetization for a broad range of chemical disorder. In case of FeRh we construct a lattice constant vs. temperature phase diagram and determine the phaseline of metamagnetic transitions based on self-consistent RDLM free energy curves.

cond-mat.mtrl-sci↗

arXiv2014

Spin-correlations and magnetic structure in an Fe monolayer on 5d transition metal surfaces

We present a detailed first principles study on the magnetic structure of an Fe monolayer on different surfaces of 5d transition metals. We use the spin-cluster expansion technique to obtain parameters of a spin model, and predict the possible magnetic ground state of the studied systems by employing the mean field approach and in certain cases by spin dynamics calculations. We point out that the number of shells considered for the isotropic exchange interactions plays a crucial role in the determination of the magnetic ground state. In the case of Ta substrate we demonstrate that the out-of-plane relaxation of the Fe monolayer causes a transition from ferromagnetic to antiferromagnetic ground state. We examine the relative magnitude of nearest neighbour Dzyaloshinskii-Moriya (D) and isotropic (J) exchange interactions in order to get insight into the nature of magnetic pattern formations. For the Fe/Os(0001) system we calculate a very large D/J ratio, correspondingly, a spin spiral ground state. We find that, mainly through the leading isotropic exchange and Dzyaloshinskii-Moriya interactions, the inward layer relaxation substantially influences the magnetic ordering of the Fe monolayer. For the Fe/Re(0001) system characterized by large antiferromagnetic interactions we also determine the chirality of the $120^{\circ}$ Néel-type ground state.

cond-mat.mtrl-sci↗

arXiv2014

Fluctuating local moments, itinerant electrons and the magnetocaloric effect: the compositional hypersensitivity of FeRh

We describe an ab-initio Disordered Local Moment Theory for materials with quenched static compositional disorder traversing first order magnetic phase transitions. It accounts quantitatively for metamagnetic changes and the magnetocaloric effect. For perfect stoichiometric B2-ordered FeRh, we calculate the transition temperature of the ferromagnetic-antiferromagnetic transition to be $T_t =$ 495K and a maximum isothermal entropy change in 2 Tesla of $|ΔS|= 21.1$ J~K$^{-1}$~kg$^{-1}$. A large (40\%) component of $|ΔS|$ is electronic. The transition results from a fine balance of competing electronic effects which is disturbed by small compositional changes - e.g. swapping just 2\% Fe of `defects' onto the Rh sublattice makes $T_t$ drop by 290K. This hypersensitivity explains the narrow compositional range of the transition and impurity doping effects.

cond-mat.mtrl-sci↗

arXiv2013

Relativistic and thermal effects on the magnon spectrum of a ferromagnetic monolayer

A spin model including magnetic anisotropy terms and Dzyaloshinsky-Moriya interactions is studied for the case of a ferromagnetic monolayer with C2v symmetry like Fe/W(110). Using the quasiclassical stochastic Landau-Lifshitz-Gilbert equations, the magnon spectrum of the system is derived using linear response theory. The Dzyaloshinsky-Moriya interaction leads to asymmetry in the spectrum, while the anisotropy terms induce a gap. It is shown that in the presence of lattice defects, both the Dzyaloshinsky-Moriya interactions and the two-site anisotropy lead to a softening of the magnon energies. Two methods are developed to investigate the magnon spectrum at finite temperatures. The theoretical results are compared to atomistic spin dynamics simulations and a good agreement is found between them.

cond-mat.str-el↗

arXiv2013

Exchange Bias driven by Dzyaloshinskii-Moriya interactions

The exchange bias effect in compensated IrMn3/Co(111) system is studied using multiscale modeling from "ab initio" to atomistic calculations. We evaluate numerically the out-of-plane hysteresis loops of the bi-layer for different thickness of the ferromagnetic layer. The results show the existence of a perpendicular exchange bias field and an enhancement of the coercivity of the system. In order to elucidate the possible origin of the exchange bias, we analyze the hysteresis loops of a selected bi-layer by tuning the different contributions to the exchange interactions across the interface. Our results indicate that the exchange bias is primarily induced by the Dzyaloshinskii-Moriya interactions, while the coercivity is increased mainly due to a spin-flop mechanism.

cond-mat.mtrl-sci↗