arXiv subjects

L. Thulliez

Publications and source records attributed to L. Thulliez.

15 recordsLinked to original sources

arXiv2026

Results on $^{235}$U(n$_{\mathrm{th}}$,f) isotopic fission yields using prompt and delayed gamma rays at the FIPPS spectrometer of the ILL

We present preliminary results from a measurement campaign conducted with the FIPPS $γ$-ray spectrometer at the ILL using an active target made of $^{235}$U dissolved in a liquid scintillator. Prompt $γ$ rays were used to extract absolute, independent isotopic fission yields. We obtained yields for a selected set of well-produced even-even nuclei from the $^{235}$U(n$_{\mathrm{th}}$,f) reaction and compared them with JEFF-3.3 evaluated data. This included the doubly magic nucleus $^{132}$Sn, for which we observed a pronounced deficit (about a factor 7) with respect to JEFF-3.3. Using the FIFRELIN fission fragment de-excitation code, we interpreted this discrepancy as evidence that $^{132}$Sn is mainly produced in its ground state at scission or after neutron evaporation. Delayed $γ$ rays recorded in the same experiment were also analysed. No deviation was found in the beta decay of $^{132}$Sn compared to the nuclear database. However, an excess of about a 40% was found in the $β$ decay of $^{90}$Kr, which may originate from an overestimated ground-state feeding of $^{90}$Rb in the evaluated data.

nucl-ex↗

arXiv2025

Observation of two nuclear recoil peaks induced by neutron capture on Al2O3

We report the observation of two nuclear recoil peaks induced by neutron capture on aluminum in a cryogenic Al$_2$O$_3$ detector developed by the NUCLEUS collaboration for the detection of reactor neutrinos via coherent elastic neutrino-nucleus (CEvNS) process. Data collected at the Technical University of Munich in 2024 with a $^{252}$Cf source reveal a main recoil line at 1145 eV from single-$γ$ de-excitation of $^{28}$Al and a newly observed structure near 575 eV originating from several two-$γ$ cascades. The latter constitutes the first direct measurement of a nuclear recoil line induced by multi-$γ$ cascades. It is predicted by our simulations when the recoiling nucleus has time to stop before the emission of the next $γ$-ray in the cascade. These results demonstrate the potential performance of the CRAB (Calibration Recoil for Accurate Bolometry) method for in situ nuclear recoil calibration and highlight the importance of accurately modeling recoil stopping and nuclear de-excitation times in cryogenic detectors of CEvNS and dark matter interactions.

physics.ins-det↗

arXiv2025

Neutron production with a 10 kW HiCANS based on SATELIT, a CEA-Saclay target with liquid lithium

High-Current Accelerator-driven Neutron Sources (HiCANS) are currently under development across Europe to address the shortage of medium-scale neutron sources, as many research nuclear reactors have been decommissioned over the past several years. At CEA-Saclay, a HiCANS has been developed utilizing the IPHI accelerator, which delivers a 3 MeV proton beam with a current of up to 100 mA, and the CEA-Saclay liquid lithium target named SATELIT. In 2024-2025, a successful experimental campaign was conducted, during which a 10 kW proton beam was directed at the liquid lithium target for nearly 100 h to generate neutrons via the 7Li(p,n)7Be nuclear reaction. Throughout the experimental campaign, a total deposited beam power of 840~kW.h was accumulated, including two continuous operational days exceeding 11 h each. A polyethylene moderator coupled with SATELIT enabled the extraction of a thermal neutron beam, with a flux measured at 1.4 m from the extraction point exceeding $10^6$ n.cm$^{-2}$.s$^{-1}$, which is sufficient for numerous neutron applications. The next step for the long-term operation of this facility involves developing strategies to mitigate the radiological concerns associated with the accumulation of 7Be within the system. Overall, this work demonstrates that such facilities can play a significant role in the future of medium-scale neutron sources in Europe.

physics.acc-ph↗

arXiv2025

The CRAB facility at the TU Wien TRIGA reactor: status and related physics program

The CRAB (Calibrated nuclear Recoils for Accurate Bolometry) project aims to precisely characterize the response of cryogenic detectors to sub-keV nuclear recoils of direct interest for coherent neutrino-nucleus scattering and dark matter search experiments. The CRAB method relies on the radiative capture of thermal neutrons in the target detector, resulting in a nuclear recoil with a well-defined energy. We present a new experimental setup installed at the TRIGA Mark-II reactor at Atominstitut (Vienna), providing a low intensity beam of thermal neutrons sent to the target cryogenic detector mounted inside a wet dilution refrigerator Kelvinox 100. A crown of BaF$_2$ detectors installed outside the dewar enables coincident detection of the high-energy $γ$ escaping the target crystal after neutron capture. After the presentation of all components of the setup we report the analysis of first commissioning data with a CaWO$_4$ detector of the \NUCLEUS experiment. They show stable operation of the cryostat and detectors on a week-scale. Due to an energy resolution currently limited to 20 eV we use neutron beam induced events at high energy, in the 10 to 100 keV range, to demonstrate the excellent agreement between the data and simulation and the accurate understanding of external background. Thanks to these data we also propose an updated decay scheme of the low-lying excited states of $^{187}$W. Finally, we present the first evidence of neutron-capture induced coincidences between $γ$-detectors and a cryogenic detector. These promising results pave the way for an extensive physics program with various detector materials, like CaWO$_4$, Al$_2$O$_3$, Ge and Si.

physics.ins-det↗

arXiv2024

First simultaneous measurement of the gamma-ray and neutron emission probabilities in inverse kinematics at a heavy-ion storage ring

The probabilities for gamma-ray and particle emission as a function of the excitation energy of a decaying nucleus are valuable observables for constraining the ingredients of the models that describe the de-excitation of nuclei near the particle emission threshold. These models are essential in nuclear astrophysics and applications. In this work, we have for the first time simultaneously measured the gamma-ray and neutron emission probabilities of 208Pb. The measurement was performed in inverse kinematics at the Experimental Storage Ring (ESR) of the GSI/FAIR facility, where a 208Pb beam interacted through the 208Pb(p,p') reaction with a hydrogen gas jet target. Instead of detecting the gamma-rays and neutrons emitted by 208Pb, we detected the heavy beam-like residues produced after gamma and neutron emission. These heavy residues were fully separated by a dipole magnet of the ESR and were detected with outstanding efficiencies. The comparison of the measured probabilities with model calculations has allowed us to test and select different descriptions of the gamma-ray strength function and the nuclear level density available in the literature.

nucl-ex↗

arXiv2024

First measurement of the neutron-emission probability with a surrogate reaction in inverse kinematics at a heavy-ion storage ring

Neutron-induced reaction cross sections of short-lived nuclei are imperative to understand the origin of heavy elements in stellar nucleosynthesis and for societal applications, but their measurement is extremely complicated due to the radioactivity of the targets involved. One way of overcoming this issue is to combine surrogate reactions with the unique possibilities offered by heavy-ion storage rings. In this work, we describe the first surrogate-reaction experiment in inverse kinematics, which we successfully conducted at the Experimental Storage Ring (ESR) of the GSI/FAIR facility, using the 208Pb(p,p') reaction as a surrogate for neutron capture on 207Pb. Thanks to the outstanding detection efficiencies possible at the ESR, we were able to measure for the first time the neutron-emission probability as a function of the excitation energy of 208Pb. We have used this probability to select different descriptions of the gamma-ray strength function and nuclear level density, and provide reliable results for the neutron-induced radiative capture cross section of 207Pb at energies for which no experimental data exist.

nucl-ex↗

arXiv2024

Improvement of Geant4 Neutron-HP package: Unresolved Resonance Region description with Probability Tables

Whether for shielding applications or for criticality safety studies, solving the neutron transport equation with good accuracy requires to take into account the resonant structure of cross sections in part of the Unresolved Resonance Region (URR). In this energy range even if the resonances can no longer be resolved experimentally, neglecting them can lead to significant numerical biases, namely in flux-based quantities. In Geant4, low energy neutrons are transported using evaluated nuclear data libraries handled by the Neutron High-Precision (Neutron-HP) package. In the version 11.01.p02 of the code, the URR can only be described by average smooth cross sections that do not take into account the statistical resonant structure of the cross sections. To overcome this shortcoming, the treatment of the URR with the use of the probability table method has been implemented in Geant4 and successfully validated with the reference Monte Carlo neutron transport codes MCNP6 (version 6.2) and Tripoli-4 (version 12). These developments will be taken into account in the next release of Geant4. All the validations of Geant4 have been performed with probability tables generated from both the NJOY and CALENDF pre-processing tools. Therefore Geant4 now has this unique feature to study the relative impact of the strategies involved during the production of probability table by the two pre-processing codes. This has been used to show that self-shielding is important also for inelastic cross sections in the example of 238U. The tool to generate probability tables usable by Geant4 either from NJOY or from CALENDF is made available on a dedicated GitLab repository and will be included in Geant4.

physics.comp-ph↗

arXiv2023

Observation of a nuclear recoil peak at the 100 eV scale induced by neutron capture

Coherent elastic neutrino-nucleus scattering and low-mass Dark Matter detectors rely crucially on the understanding of their response to nuclear recoils. We report the first observation of a nuclear recoil peak at around 112 eV induced by neutron capture. The measurement was performed with a CaWO$_4$ cryogenic detector from the NUCLEUS experiment exposed to a $^{252}$Cf source placed in a compact moderator. The measured spectrum is found in agreement with simulations and the expected peak structure from the single-$γ$ de-excitation of $^{183}$W is identified with 3 $σ$ significance. This result demonstrates a new method for precise, in-situ, and non-intrusive calibration of low-threshold experiments.

nucl-ex↗

arXiv2023

Study of collision and $γ$-cascade times following neutron-capture processes in cryogenic detectors

The emission of $γ$-rays after a neutron capture in a cryogenic detector can generate mono-energetic nuclear recoils in the sub-keV regime, of direct interest for the calibration of Dark Matter and Coherent Elastic Neutrino Nucleus Scattering experiments. Here we show that accurate predictions of the nuclear recoil spectra induced by neutron captures require taking into account the interplay between the development in time of the de-excitation $γ$-cascade of the target nucleus and that of the associated atomic collisions in matter. We present detailed simulations coupling the FIFRELIN code for the description of the $γ$-cascades and the IRADINA code for the modelling of the fast atomic movements in matter. Nuclear recoil spectra are predicted, and made available to the community, for concrete cases of Al$_2$O$_3$, Si, Ge and CaWO$_4$ crystals exposed to a low intensity beam of thermal neutrons. We find that timing effects cause new calibration peaks to emerge in the recoil spectra and also impact the shape of the continuous recoil distribution. We discuss how they could give access to a rich physics program, spanning the accurate study of the response of cryogenic detectors in the sub-keV range, tests of solid state physics simulations and tests of nuclear models.

physics.ins-det↗

arXiv2023

Improvement of Geant4 Neutron-HP package: Doppler broadening of the neutron elastic scattering kernel and cross sections

Whether it is for shielding applications or for safety criticality studies, numerically solving the neutron transport equation with a good accuracy requires to precisely estimate the Doppler broadened elastic scattering kernel in the thermal and epithermal energy range of neutrons travelling in a free gas. In Geant4, low energy neutrons are transported using evaluated data libraries handled by the Neutron High-Precision (Neutron-HP) package. Version 11.00.p03 of the code features in particular the Doppler broadened elastic scattering kernel, provided by the so-called 'Sampling of the Velocity of the Target' (SVT) method. However this latter fails for resonant heavy nuclei such as 238U and can severely impact the solving of the Boltzmann equation in fissile media. To overcome this shortcoming, the Doppler Broadened Rejection Correction (DBRC) method has been implemented in Geant4 and successfully validated with the reference Monte Carlo neutron transport code Tripoli4 (version 11). This development will be taken into account in the next release of the code. The cross section Doppler broadening process, which is performed on-the-fly, is also carefully investigated and ways to improve it on a simulation-by-simulation basis are presented. All the validations have been performed with an automated benchmark tool which has been designed to support the quality assurance of the Geant4 Neutron-HP package. This tool is currently available on an ad hoc Gitlab repository and will be included in Geant4.

physics.comp-ph↗

arXiv2023

TOUCANS: a versatile Monte Carlo neutron transport code based on Geant4

This paper reports the development of TOUCANS, a new Monte Carlo neutron transport code fully written using the Geant4 toolkit. It aims at modeling complex systems easily and rapidly, thanks to a simple key-value input file. While its main focus is the transport of low energy neutrons -- below 20 MeV -- using evaluated cross-section libraries, it also takes advantage of the state-of-the-art capabilities offered by Geant4 regarding the modeled cross-sections for practically all particles at all energies. Hence it gives access to non-specialists to a wide variety of applications involving different particles, such as for instance the simulation of compact accelerator based neutron sources (CANS) which initially motivated its development. It leverages on recent implementations performed within Geant4 to provide both shielding calculation capabilities (using Adaptive Multilevel Splitting, which is a fully automated variance reduction technique) and criticality calculation capabilities (to estimate the keff of a multiplicative system). It also benefits from a tight coupling with CADMesh to readily import CAD models, with NCrystal to extend the support of thermal neutron transport to crystals, with FIFRELIN to increase compound nucleus de-excitation accuracy, and with FUNZ to provide to the user parametric simulation capabilities (such as multi-objective algorithms, calculation of Pareto sets, etc). Thanks to recent improvements of the neutron physics within the Geant4 Neutron-HP package, the TOUCANS code can be considered on-par with industrial neutron transport codes such as Tripoli-4 or MCNP in term of neutron physics accuracy. Its sources should be released soon amongst Geant4 advanced examples.

physics.acc-ph↗

arXiv2022

Improved FIFRELIN de-excitation model for neutrino applications

The precise modeling of the de-excitation of Gd isotopes is of great interest for experimental studies of neutrinos using Gd-loaded organic liquid scintillators. The FIFRELIN code was recently used within the purposes of the STEREO experiment for the modeling of the Gd de-excitation after neutron capture in order to achieve a good control of the detection efficiency. In this work, we report on the recent additions in the FIFRELIN de-excitation model with the purpose of enhancing further the de-excitation description. Experimental transition intensities from EGAF database are now included in the FIFRELIN cascades, in order to improve the description of the higher energy part of the spectrum. Furthermore, the angular correlations between γ rays are now implemented in FIFRELIN, to account for the relative anisotropies between them. In addition, conversion electrons are now treated more precisely in the whole spectrum range, while the subsequent emission of X rays is also accounted for. The impact of the aforementioned improvements in FIFRELIN is tested by simulating neutron captures in various positions inside the STEREO detector. A repository of up-to-date FIFRELIN simulations of the Gd isotopes is made available for the community, with the possibility of expanding for other isotopes which can be suitable for different applications.

hep-ex↗

arXiv2021

Calibration of nuclear recoils at the 100 eV scale using neutron capture

The development of low-threshold detectors for the study of coherent elastic neutrino-nucleus scattering and for the search for light dark matter necessitates methods of low-energy calibration. We suggest this can be provided by the nuclear recoils resulting from the $γ$ emission following thermal neutron capture. In particular, several MeV-scale single-$γ$ transitions induce well-defined nuclear recoil peaks in the 100 eV range. Using the FIFRELIN code, complete schemes of $γ$-cascades for various isotopes can be predicted with high accuracy to determine the continuous background of nuclear recoils below the calibration peaks. We present a comprehensive experimental concept for the calibration of CaWO$_4$ and Ge cryogenic detectors at a research reactor. For CaWO$_4$ the simulations show that two nuclear recoil peaks at 112.5 eV and 160.3 eV should be visible above background simply in the spectrum of the cryogenic detector. Then we discuss how the additional tagging for the associated $γ$ increases the sensitivity of the method and extends its application to a wider energy range and to Ge cryogenic detectors.

physics.ins-det↗

arXiv2021

Stopping power of fission fragments in thin Mylar and nickel foils

The energy loss of heavy ions in thin Mylar and nickel foils was measured accurately using fission fragments from $^{239}Pu(n_{th},f)$, mass and energy separated by the Lohengrin separator at ILL. The detection setup, placed at the focal plane of the Lohengrin separator enabled to measure precisely the kinetic energy difference of selected fragments after passing through the sample. From these data, the stopping powers in Mylar and nickel layers were extracted and compared to calculations. Whereas large deviations are observed with SRIM-2013 for Mylar, fairly good agreements are obtained with the semi-empirical approach of Knyazheva et al. and the calculations contained within the DPASS database. In nickel, SRIM-2013 and Knyazheva model are in agreement with our data within about 10 %, while large deviations are observed with DPASS. We used our data to provide updated parameters for the Knyazheva et al. model and rescale DPASS database for nickel and Mylar.

nucl-ex↗

arXiv2019

Improved STEREO simulation with a new gamma ray spectrum of excited gadolinium isotopes using FIFRELIN

The STEREO experiment measures the electron antineutrino spectrum emitted in a research reactor using the inverse beta decay reaction on H nuclei in a gadolinium loaded liquid scintillator. The detection is based on a signal coincidence of a prompt positron and a delayed neutron capture event. The simulated response of the neutron capture on gadolinium is crucial for the comparison with data, in particular in the case of the detection efficiency. Among all stable isotopes, $^{155}$Gd and $^{157}$Gd have the highest cross sections for thermal neutron capture. The excited nuclei after the neutron capture emit gamma rays with a total energy of about 8 MeV. The complex level schemes of $^{156}$Gd and $^{158}$Gd are a challenge for the modeling and prediction of the deexcitation spectrum, especially for compact detectors where gamma rays can escape the active volume. With a new description of the Gd(n,$γ$) cascades obtained using the FIFRELIN code, the agreement between simulation and measurements with a neutron calibration source was significantly improved in the STEREO experiment. A database of ten millions of deexcitation cascades for each isotope has been generated and is now available for the user.

physics.ins-det↗