arXiv subjects

L. Varriano

Publications and source records attributed to L. Varriano.

14 recordsLinked to original sources

arXiv2026

Precision Mass Measurements of \textsuperscript{130}Te, \textsuperscript{130}Sn, and Their Impact on Models for R-Process Nucleosynthesis

The astrophysical rapid neutron capture nucleosynthesis process (r-process) remains an active area of research due to the fact that it occurs in extreme conditions and involves reactions with exotic nuclei that are difficult to study experimentally. For the first time using the Phase-Imaging Ion Cyclotron Resonance (PI-ICR) technique, we measured the mass excesses of \textsuperscript{130}Te, \textsuperscript{130}Sn, and \textsuperscript{130}Sn\textsuperscript{m} with the Canadian Penning Trap (CPT). Our results show good agreement with previous Penning trap values obtained using the Time-of-Flight Ion Cyclotron Resonance (TOF-ICR) and the Fourier Transform Ion Cyclotron Resonance (FT-ICR) techniques, while being twice as precise for \textsuperscript{130}Sn. These new mass excesses were added to a SkyNet network calculation to determine their impact on r-process abundances and to find the best astrophysical conditions to reproduce the Solar System r-process abundance pattern. Finally, by treating lighter and heavier elements separately, we assess the relative frequency of events producing elements in a cold versus a hot r-process scenario.

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arXiv2026

Precise Mass Measurement of the $^{149}$La-$^{149}$Ce-$^{149}$Pr isobaric chain

Penning trap mass measurements of $^{149}$La, $^{149}$Ce, and $^{149}$Pr were performed with the Canadian Penning Trap (CPT) at the CARIBU facility of Argonne National Laboratory using the phase-imaging ion-cyclotron-resonance technique. The resulting mass excess of $^{149}$La differs by 221 keV from a recent JYFLTRAP measurement, resulting in a significant change in the profile of the two-neutron separation energy for that isotopic chain. The mass excesses of $^{149}$Ce and $^{149}$Pr are determined with an eight-fold improvement in precision compared to previous time-of-flight ion-cyclotron-resonance measurements; the $^{149}$Ce value is consistent with AME2020, while the $^{149}$Pr mass excess is lower by 17.5 keV. The mass excesses of $^{149}$La and $^{149}$Pr reported in this work have been confirmed recently by a measurement with a multi-reflection time-of-flight mass spectrometer coupled to a $\beta$-time of flight detector at RIKEN, providing further validation of the present results.

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arXiv2025

Exploration for Astromers near $^{132}$Sn with the Canadian Penning Trap

Nuclear isomers can have significant impacts on astrophysical nucleosynthesis processes, with recent efforts demonstrating that the population of isomeric states with different half-lives may require separate treatment in reaction networks to accurately capture the differences in heating or in identifiable electromagnetic signals. Several potential so-called ``astromers'' in tin and antimony isotopes near doubly-magic $^{132}$Sn were identified and direct mass measurements of their ground and isomeric states were performed with the Canadian Penning Trap at Argonne National Laboratory's CARIBU facility, and their impact on astrophysical reaction rates and in reaction networks calculated. It was found that $^{129g,m}$Sn, with measured mass excesses of $-80 593.2(25)$ keV and $-80 557.4(25)$ keV, respectively, and an excitation energy of $35.8(35)$ keV, behaves as an astromer during neutron capture in the $i$-process and in the $r$-process.

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arXiv2025

Astrophysical significance of the isomer $^{119m}$Ag demonstrated through direct mass measurement

The abundance of elements heavier than iron produced via the astrophysical rapid-neutron capture process depends sensitively on the atomic mass of the involved nuclei as well as the behavior of a few special types of nuclear isomers called astromers. High-precision mass measurements of $^{119}$Cd, $^{119}$Ag and their respective isomeric states have been performed with the Phase Imaging-Ion Cyclotron Resonance (PI-ICR) method with a precision of $\delta m/m \approx 10^{-8}$ using the Canadian Penning Trap (CPT). The ground state mass excess, as well as the excitation energy, agrees with recent Penning Trap measurements from JYFLTRAP. Network calculations using these new measurements revealed that, contrary to previous expectations, $^{119m}$Ag behaves as an astromer which significantly affects the population of $^{119}$Ag.

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arXiv2024

Mass measurements of neutron-rich nuclides using the Canadian Penning Trap to inform predictions in the $r$-process rare-earth peak region

Studies aiming to determine the astrophysical origins of nuclei produced by the rapid neutron capture process ($r$ process) rely on nuclear properties as inputs for simulations. The solar abundances can be used as a benchmark for such calculations, with the $r$-process rare-earth peak (REP) around mass number ($A$) 164 being of special interest due to its presently unknown origin. With the advancement of rare isotope beam production over the last decade and improvement in experimental sensitivities, many of these REP nuclides have become accessible for measurement. Masses are one of the most critical inputs as they impact multiple nuclear properties, namely the neutron-separation energies, neutron capture rates, $\beta$-decay rates, and $\beta$-delayed neutron emission probabilities. In this work, we report masses of 20 neutron-rich nuclides (along the Ba, La, Ce, Pr, Nd, Pm, Gd, Dy and Ho isotopic chains) produced at the CAlifornium Rare Isotope Breeder Upgrade (CARIBU) facility at Argonne National Laboratory. The masses were measured with the Canadian Penning trap (CPT) mass spectrometer using the Phase-Imaging Ion-Cyclotron-Resonance (PI-ICR) technique. We then use these new masses along with previously published CPT masses to inform predictions for a Markov Chain Monte Carlo (MCMC) procedure aiming to identify the astrophysical conditions consistent with both solar data and mass measurements. We show that the MCMC responds to this updated mass information, producing refined results for both mass predictions and REP abundances.

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arXiv2024

Precise Mass Measurement of the Longest Odd-Odd Chain of \boldmath $1^+$ Ground States

Precise mass measurements of the ground and isomeric states of the odd-odd $^{108, 110, 112, 114, 116}$Rh were performed using the Canadian Penning Trap at Argonne National Laboratory, showing good agreement with recent JYFLTRAP measurements. A new possible isomeric state of $^{114}$Rh was also observed. These isotopes are part of the longest odd-odd chain of identical ground-state spin-parity assignment of 1$^+$, spanning $^{104-118}$Rh, despite being in a region of deformation. Realistic phenomenological mean-field calculations using ``universal'' Wood-Saxon Hamiltonian were performed, which explained this phenomenon for the first time. In addition, multi-quasiparticle blocking calculations were performed to study the configuration of low-lying states in the odd-odd Rh nuclei, elucidating anomalous isomeric yield ratio observed for $^{114}$Rh.

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arXiv2024

Investigating the effects of precise mass measurements of Ru and Pd isotopes on machine learning mass modeling

Atomic masses are a foundational quantity in our understanding of nuclear structure, astrophysics and fundamental symmetries. The long-standing goal of creating a predictive global model for the binding energy of a nucleus remains a significant challenge, however, and prompts the need for precise measurements of atomic masses to serve as anchor points for model developments. We present precise mass measurements of neutron-rich Ru and Pd isotopes performed at the Californium Rare Isotope Breeder Upgrade facility at Argonne National Laboratory using the Canadian Penning Trap mass spectrometer. The masses of $^{108}$Ru, $^{110}$Ru and $^{116}$Pd were measured to a relative mass precision $\delta m/m \approx 10^{-8}$ via the phase-imaging ion-cyclotron-resonance technique, and represent an improvement of approximately an order of magnitude over previous measurements. These mass data were used in conjunction with the physically interpretable machine learning (PIML) model, which uses a mixture density neural network to model mass excesses via a mixture of Gaussian distributions. The effects of our new mass data on a Bayesian-updating of a PIML model are presented.

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arXiv2024

Direct cross-section measurement of the weak r-process 88Sr({\alpha},n)91Zr reaction in {\nu}-driven winds of core collapse supernovae

About half of the heavy elements beyond iron are known to be produced by the rapid neutron capture process, known as r-process. However, the astrophysical site producing the r-process is still uncertain. Chemical abundances observed in several cosmic sites indicate that different mechanisms should be at play. For instance, the abundances around silver measured in a subset of metal-poor stars indicate the presence of a weak r-process. This process may be active in neutrino-driven winds of core collapse supernovae where (${\alpha}$,n) reactions dominate the synthesis of Z ~ 40 elements in the expelled materials. Scarcely measured, the rates of (${\alpha}$,n) reactions are determined from statistical Hauser-Feshbach calculations with ${\alpha}$-optical-model potentials, which are still poorly constrained. The uncertainties of the (${\alpha}$,n) reaction rates therefore make a significant contribution to the uncertainties of the abundances determined from stellar modeling. In this work, the $^{88}$Sr(${\alpha}$,n)$^{91}$Zr reaction which impacts the weak r-process abundances has been probed at astrophysics energy for the first time; directly measuring the total cross sections at astrophysical energies of 8.37 - 13.09 MeV in the center of mass (3.8 - 7.5 GK). Two measurements were performed at ATLAS with the electrically-segmented ionization chamber MUSIC, in inverse kinematics, while following the active target technique. The cross sections of this ${\alpha}$-induced reaction on $^{88}$Sr, located at the shell closure N = 50, have been found to be lower than expected, by a factor of 3, despite recent statistical calculations validated by measurements on neighboring nuclei. This result encourages more experimental investigations of (${\alpha}$,n) reactions, at N = 50 and towards the neutron-rich side, to further test the predictive power and reliability of such calculations.

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arXiv2023

Precise Mass Measurements of $A=133$ Isobars with the Canadian Penning Trap: Resolving the $Q_{\beta^-}$ anomaly at $^{133}$Te

We report precision mass measurements of $^{133}$Sb, $^{133g,m}$Te, and $^{133g,m}$I, produced at CARIBU at Argonne National Laboratory's ATLAS facility and measured using the Canadian Penning Trap mass spectrometer. These masses clarify an anomaly in the $^{133}$Te $\beta$-decay. The masses reported in the 2020 Atomic Mass Evaluation (M. Wang et al., 2021) produce $Q_{\beta^-}(^{133}$Te)=2920(6) keV; however, the highest-lying $^{133}$I level populated in this decay is observed at $E_i=2935.83(15)$ keV, resulting in an anomalous $Q_{\beta^{-}}^{i}=-16(6)$~keV. Our new measurements give $Q_{\beta^-}(^{133}\text{Te})=2934.8(11)$ keV, a factor of five more precise, yielding $Q{_\beta^i}=-1.0(12)$~keV, a 3$\sigma$ shift from the previous results. This resolves this anomaly, but indicates further anomalies in our understanding of the structure of this isotope.

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arXiv2023

The Beta-decay Paul Trap Mk IV: Design and commissioning

The Beta-decay Paul Trap is an open-geometry, linear trap used to measure the decays of $^8$Li and $^8$B to search for a tensor contribution to the weak interaction. In the latest $^8$Li measurement of Burkey et al. (2022), $\beta$ scattering was the dominant experimental systematic uncertainty. The Beta-decay Paul Trap Mk IV reduces the prevalence of $\beta$ scattering by a factor of 4 through a redesigned electrode geometry and the use of glassy carbon and graphite as electrode materials. The trap has been constructed and successfully commissioned with $^8$Li in a new data campaign that collected 2.6 million triple coincidence events, an increase in statistics by 30% with 4 times less $\beta$ scattering compared to the previous $^8$Li data set.

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arXiv2022

Improved Limit on Tensor Currents in the Weak Interaction from $^8$Li $\beta$ Decay

The electroweak interaction in the Standard Model (SM) is described by a pure vector-axial-vector structure, though any Lorentz-invariant component could contribute. In this work, we present the most precise measurement of tensor currents in the low-energy regime by examining the $\beta$-$\bar{\nu}$ correlation of trapped $^{8}$Li ions with the Beta-decay Paul Trap. We find $a_{\beta\nu} = -0.3325 \pm 0.0013_{stat} \pm 0.0019_{syst}$ at $1\sigma$ for the case of coupling to right-handed neutrinos $(C_T=-C_T')$, which is consistent with the SM prediction.

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arXiv2021

Experimental Search for Neutron to Mirror Neutron Oscillations as an Explanation of the Neutron Lifetime Anomaly

An unexplained $>4\,\sigma$ discrepancy persists between "beam" and "bottle" measurements of the neutron lifetime. A new model proposed that conversions of neutrons $n$ into mirror neutrons $n'$, part of a dark mirror sector, can increase the apparent neutron lifetime by $1\%$ via a small mass splitting $\Delta{m}$ between $n$ and $n'$ inside the 4.6 T magnetic field of the National Institute of Standards and Technology Beam Lifetime experiment. A search for neutron conversions in a 6.6 T magnetic field was performed at the Spallation Neutron Source which excludes this explanation for the neutron lifetime discrepancy.

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arXiv2021

Impact of clustering on the $^8$Li $\beta$ decay and recoil form factors

We place unprecedented constraints on recoil corrections in the $\beta$ decay of $^8$Li, by identifying a strong correlation between them and the $^8$Li ground state quadrupole moment in large-scale ab initio calculations. The results are essential for improving the sensitivity of high-precision experiments that probe the weak interaction theory and test physics beyond the Standard Model (BSM). In addition, our calculations predict a $2^+$ state of the $\alpha+\alpha$ system that is energetically accessible to $\beta$ decay but has not been observed in the experimental $^8$Be energy spectrum, and has an important effect on the recoil corrections and $\beta$ decay for the $A=8$ systems. This state and an associated $0^+$ state are notoriously difficult to model due to their cluster structure and collective correlations, but become feasible for calculations in the ab initio symmetry-adapted no-core shell-model framework.

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arXiv2020

New high-sensitivity searches for neutrons converting into antineutrons and/or sterile neutrons at the European Spallation Source

The violation of Baryon Number, $\mathcal{B}$, is an essential ingredient for the preferential creation of matter over antimatter needed to account for the observed baryon asymmetry in the universe. However, such a process has yet to be experimentally observed. The HIBEAM/NNBAR %experiment program is a proposed two-stage experiment at the European Spallation Source (ESS) to search for baryon number violation. The program will include high-sensitivity searches for processes that violate baryon number by one or two units: free neutron-antineutron oscillation ($n\rightarrow \bar{n}$) via mixing, neutron-antineutron oscillation via regeneration from a sterile neutron state ($n\rightarrow [n',\bar{n}'] \rightarrow \bar{n}$), and neutron disappearance ($n\rightarrow n'$); the effective $\Delta \mathcal{B}=0$ process of neutron regeneration ($n\rightarrow [n',\bar{n}'] \rightarrow n$) is also possible. The program can be used to discover and characterise mixing in the neutron, antineutron, and sterile neutron sectors. The experiment addresses topical open questions such as the origins of baryogenesis, the nature of dark matter, and is sensitive to scales of new physics substantially in excess of those available at colliders. A goal of the program is to open a discovery window to neutron conversion probabilities (sensitivities) by up to three orders of magnitude compared with previous searches. The opportunity to make such a leap in sensitivity tests should not be squandered. The experiment pulls together a diverse international team of physicists from the particle (collider and low energy) and nuclear physics communities, while also including specialists in neutronics and magnetics.

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