arXiv subjects

L. X. Yang

Publications and source records attributed to L. X. Yang.

At least 55 records · Page 3Linked to original sources

arXiv2011

Electronic identification of the actual parental phase of KxFe2-ySe2 superconductor and its intrinsic mesoscopic phase separation

While the parent compounds of the cuprate high temperature superconductors (high-Tc's) are Mott insulators, the iron-pnictide high-Tc's are in the vicinity of a metallic spin density wave (SDW) state, which highlights the difference between these two families. However, insulating parent compounds were identified for the newly discovered KxFe2-ySe2. This raises an intriguing question as to whether the iron-based high-Tc's could be viewed as doped Mott insulators like the cuprates. Here we report angle-resolved photoemission spectroscopy (ARPES) evidence of two insulating and one semiconducting phases of KxFe2-ySe2, and the mesoscopic phase separation between the superconducting/semiconducting phase and the insulating phases. The insulating phases are characterized by the depletion of electronic states over a 0.5 eV window below the chemical potential, giving a compelling evidence for the presence of Mott-like physics. The charging effects and the absence of band folding in the superconducting/semiconducting phase further prove that the static magnetic and vacancy orders are not related to the superconductivity. Instead, the electronic structure of the superconducting phase is much closer to the semiconducting phase, indicating the superconductivity is likely developed by doping the semiconducting phase rather than the insulating phases.

cond-mat.supr-con↗

arXiv2011

Electronic structure of BaNi$_2$As$_2$

BaNi$_2$As$_2$, with a first order phase transition around 131 K, is studied by the angle-resolved photoemission spectroscopy. The measured electronic structure is compared to the local density approximation calculations, revealing similar large electronlike bands around $\bar{M}$ and differences along $\barΓ$-$\bar{X}$. We further show that the electronic structure of BaNi$_2$As$_2$ is distinct from that of the sibling iron pnictides. Particularly, there is no signature of band folding, indicating no collinear SDW related magnetic ordering. Moreover, across the strong first order phase transition, the band shift exhibits a hysteresis, which is directly related to the significant lattice distortion in BaNi$_2$As$_2$.

cond-mat.supr-con↗

arXiv2011

Pressure induced Superconductivity in Topological Compound Bi2Te3

Bi2Te3 compound has been theoretically predicted (1) to be a topological insulator, and its topologically non-trivial surface state with a single Dirac cone has been observed in photoemission experiments (2). Here we report that superconductivity (Tc^~3K) can be induced in Bi2Te3 as-grown single crystal (with hole-carriers) via pressure. The first-principles calculations show that the electronic structure under pressure remains to be topologically nontrivial, and the Dirac-type surface states can be well distinguished from bulk states at corresponding Fermi level. The proximity effect between superconducting bulk states and Dirac-type surface state could generate Majorana fermions on the surface. We also discuss the possibility that the bulk state could be a topological superconductor.

cond-mat.supr-con↗

arXiv2010

Heavily electron-doped electronic structure and isotropic superconducting gap in AxFe2Se2 (A=K,Cs)

The low energy band structure and Fermi surface of the newly discovered superconductor, AxFe2Se2 (A=K,Cs), have been studied by angle-resolved photoemission spectroscopy. Compared with iron pnictide superconductors, AxFe2Se2 (A=K,Cs) is the most heavily electron-doped with Tc~30 K. Only electron pockets are observed with an almost isotropic superconducting gap of ~10.3 meV, while there is no hole Fermi surface near the zone center, which indicates the inter-pocket hopping or Fermi surface nesting is not a necessary ingredient for the unconventional superconductivity in iron-based superconductors. Thus, the sign changed s$_\pm$ pairing symmetry, a leading candidate proposed for iron-based superconductors, becomes conceptually irrelevant in describing the superconducting state here. A more conventional s-wave pairing is a better description.

cond-mat.supr-con↗

arXiv2010

Out-of-plane momentum and symmetry dependent superconducting gap in Ba0.6K0.4Fe2As2

The three-dimensional band structure and superconducting gap of Ba0.6K0.4Fe2As2 are studied with high-resolution angle-resolved photoemission spectroscopy. In contrast to previous results, we have identified three hole-like Fermi surfaces near the zone center with sizable out-of-plane or kz dispersion. The superconducting gap on certain Fermi surface shows significant kz-dependence. Moreover, we found that the superconducting gap sizes are different at the same Fermi momentum for two bands with different spatial symmetries (one odd, one even). Our results provide further information on the rich superconducting gap structure in iron pnictides, and a distinct test for theories.

cond-mat.supr-con↗

arXiv2010

Surface and bulk electronic structures of LaOFeAs studied by angle resolved photoemission spectroscopy

The electronic structure of LaOFeAs, a parent compound of iron-arsenic superconductors, is studied by angleresolved photoemission spectroscopy. By examining its dependence on photon energy, polarization, sodium dosing and the counting of Fermi surface volume, both the bulk and the surface contributions are identified. We find that a bulk band moves toward high binding energies below structural transition, and shifts smoothly across the spin density wave transition by about 25 meV. Our data suggest the band reconstruction may play a crucial role in the spin density wave transition, and the structural transition is driven by the short range magnetic order. For the surface states, both the LaO-terminated and FeAs-terminated components are revealed. Certain small band shifts are verified for the FeAs-terminated surface states in the spin density wave state, which is a reflection of the bulk electronic structure reconstruction. Moreover, sharp quasiparticle peaks quickly rise at low temperatures, indicating of drastic reduction of the scattering rate. A kink structure in one of the surface band is shown to be possibly related to the electron-phonon interactions.

cond-mat.supr-con↗

arXiv2010

Strong correlation and massive spectral-weight redistribution induced spin density wave in a-Fe1.06Te

The electronic structure of a-Fe1.06Te is studied with angle-resolved photoemission spectroscopy. We show that there is substantial spectral weight around Gamma and X, and lineshapes are intrinsically incoherent in the paramagnetic state. The magnetic transition is characterized by a massive spectral-weight transfer over an energy range as large as the band width, which even exhibits a hysteresis loop that marks the strong first order transition. Coherent quasiparticles emerge in the magnetically ordered state due to decreased spin fluctuations, which account for the change of transport properties from insulating behavior to metallic behavior. Our observation demonstrates that Fe1.06Te distinguishes itself from other iron-based systems with more local characters and much stronger interactions among different degrees of freedom, and how a spin density wave is formed in the presence of strong correlation.

cond-mat.supr-con↗

arXiv2010

Electronic structure reconstruction: the driving force behind the magnetic and structural transitions in NaFeAs

The electronic structure of NaFeAs is studied with angle resolved photoemission spectroscopy on high quality single crystals. Large portions of the band structure start to shift around the structural transition temperature, and smoothly evolve as the temperature lowers through the spin density wave transition. Moreover, band folding due to magnetic order emerges around structural transition. Our observation provides direct evidence that the structural and magnetic transitions share the same origin, and are both driven by the electronic structure reconstruction in Fe-based superconductors, instead of Fermi surface nesting.

cond-mat.supr-con↗

arXiv2009

Out of plane effect on the superconductivity of Sr2-xBaxCuO3+y with Tc up to 98K

A series of new Sr2-xBaxCuO3+y (0 x 0.6) superconductors were prepared using high-pressure and high-temperature synthesis. A Rietveld refinement based on powder x-ray diffraction confirms that the superconductors crystallize in the K2NiF4-type structure of a space group I4/mmm similar to that of La2CuO4 but with partially occupied apical oxygen sites. It is found that the superconducting transition temperature Tc of this Ba substituted Sr2CuO3+y superconductor with constant carrier doping level, i.e., constant d, is controlled not only by order/disorder of apical-O atoms but also by Ba content. Tcmax =98 K is achieved in the material with x=0.6 that reaches the record value of Tc among the single-layer copper oxide superconductors, and is higher than Tc=95K of Sr2CuO3+y with optimally ordered apical-O atoms. There is Sr-site disorder in Sr2-xBaxCuO3+y which might lead to a reduction of Tc. The result indicates that another effect surpasses the disorder effect that is related either to the increased in-plane Cu-O bond length or to elongated apical-O distance due to Ba substitution with larger cation size. The present experiment demonstrates that the optimization of local geometry out of the Cu-O plane can dramatically enhance Tc in the cuprate superconductors.

cond-mat.supr-con↗

arXiv2008

The superconductivity at 18 K in LiFeAs system

A new iron arsenide superconducting system LiFeAs was found that crystallizes into a tetragonal structure with space group P4/nmm. The superconductivity with Tc up to 18 K was observed in the compounds. This simple 111 type layered iron arsenide superconductor can be viewed as an analogue of the infinite layer structure of copper oxides.

cond-mat.supr-con↗

arXiv2008

Primary role of the barely occupied states in the charge density wave formation of NbSe2

NbSe2 is a prototypical charge-density-wave (CDW) material, whose mechanism remains mysterious so far. With angle resolved photoemission spectroscopy, we mapped out the CDW gap and recovered the long-lost nesting condition over a large broken-honeycomb region in the Brillouin zone, which consists of six saddle band point regions with high density of states (DOS), and large regions away from Fermi surface with negligible DOS at the Fermi energy. We show that the major contributions to the CDW come from these barely occupied states rather than the saddle band points. Our findings not only resolve a long standing puzzle, but also overthrow the conventional wisdom that CDW is dominated by regions with high DOS.

cond-mat.str-el↗

arXiv2008

Electronic structure and exotic exchange splitting in spin-density-wave states of BaFe$_2$As$_2$

The magnetic properties in the parent compounds are often intimately related to the microscopic mechanism of superconductivity. Here we report the first direct measurements on the electronic structure of a parent compound of the newly discovered iron-based superconductor, BaFe$_2$As$_2$, which provides a foundation for further studies. We show that the energy of the spin density wave (SDW) in BaFe$_2$As$_2$ is lowered through exotic exchange splitting of the band structure, rather than Fermi surface nesting of itinerant electrons. This clearly demonstrates that a metallic SDW state could be solely induced by interactions of local magnetic moments, resembling the nature of antiferromagnetic order in cuprate parent compounds.

cond-mat.supr-con↗

arXiv2008

Doping-insensitive density-of-states suppression in polycrystalline iron-based superconductor SmO$_{1-x}$F$_{x}$FeAs

We investigated the temperature dependence of the density-of-states in the iron-based superconductor SmO_1-xF_xFeAs (x=0, 0.12, 0.15, 0.2) with high resolution angle-integrated photoemission spectroscopy. The density-of-states suppression is observed with decreasing temperature in all samples, revealing two characteristic energy scales (10meV and 80meV). However, no obvious doping dependence is observed. We argue that the 10meV suppression is due to an anomalously doping-independent normal state pseudogap, which becomes the superconducting gap once in the superconducting state; and alert the possibility that the 80meV-scale suppression might be an artifact of the polycrystalline samples.

cond-mat.supr-con↗

arXiv2008

Angle integrated photoemission study of SmO$_{0.85}$F$_{0.15}$FeAs

The electronic structure of the new superconductor, SmO$_{1-x}$F$_x$FeAs ($x=0.15$), has been studied by angle-integrated photoemission spectroscopy. Our data show a sharp feature very close to the Fermi energy, and a relative flat distribution of the density of states between 0.5 eV and 3 eV binding energy, which agrees best with band structure calculations considering an antiferromagnetic ground state. No noticeable gap opening was observed at 12 Kelvin below the superconducting transition temperature, indicating the existence of large ungapped regions in the Brillouin zone.

cond-mat.supr-con↗

arXiv2008

Superconducting coherence peak in the electronic excitations of a single layer cuprate superconductor $Bi_2 Sr_{1.6} La_{0.4} Cu O_{6+δ}$

Angle resolved photoemission spectroscopy study is reported on a high quality optimally doped Bi2Sr1.6La0.4CuO6+delta high Tc superconductor. In the antinodal region with maximal d-wave gap, the symbolic superconducting coherence peak, which has been widely observed in multi-CuO2-layer cuprate superconductors, is unambiguously observed in a single layer system. The associated peak-dip separation is just about 19 meV, which is much smaller than its counterparts in multi-layered compounds, but correlates with the energy scales of spin excitations in single layer cuprates.

cond-mat.supr-con↗

arXiv2007

Evolution of the Electronic Structure of 1T-CuxTiSe2

The electronic structure of a new charge-density-wave/ superconductor system, 1T-CuxTiSe2, has been studied by photoemission spectroscopy. A correlated semiconductor band structure is revealed for the undoped case. With Cu doping, the charge density wave is suppressed by the raising of the chemical potential, while the superconductivity is enhanced by the enhancement of the density of states. Moreover, the strong scattering at high doping might be responsible for the suppression of superconductivity in that regime.

cond-mat.str-el↗

arXiv2007

A novel mechanism of charge density wave in a transition metal dichalcogenide

Charge density wave, or CDW, is usually associated with Fermi surfaces nesting. We here report a new CDW mechanism discovered in a 2H-structured transition metal dichalcogenide, where the two essential ingredients of CDW are realized in very anomalous ways due to the strong-coupling nature of the electronic structure. Namely, the CDW gap is only partially open, and charge density wavevector match is fulfilled through participation of states of the large Fermi patch, while the straight FS sections have secondary or negligible contributions.

cond-mat.str-el↗

arXiv2006

Enhancement of the superconducting critical temperature of Sr2CuO3+d up to 95K by ordering dopant atoms

We address the question of whether the superconducting transition temperature (Tc) of high-Tc cuprates is enhanced when randomly distributed dopant atoms form an ordered array in the charge reservoir layers. This study is possible for the Sr2CuO3+d superconductor with K2NiF4-type structure in which oxygen atoms only partially occupy the apical sites next to the CuO2 planes and act as hole-dopants. We show that remarkable Tc enhancement up to 95K in this mono CuO2 layered HTS is associated with the apical oxygen ordering, not to the hole concentration change. The result points a route toward further enhancement of Tc in cuprate superconductors.

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