arXiv subjects

L. Yao

Publications and source records attributed to L. Yao.

26 records · Page 2Linked to original sources

arXiv2018

Measurement of the normalized $^{238}$U(n,f)/$^{235}$U(n,f) cross section ratio from threshold to 30 MeV with the fission Time Projection Chamber

The normalized $^{238}$U(n,f)/$^{235}$U(n,f) cross section ratio has been measured using the NIFFTE fission Time Projection Chamber from the reaction threshold to $30$~MeV. The fissionTPC is a two-volume MICROMEGAS time projection chamber that allows for full three-dimensional reconstruction of fission-fragment ionization profiles from neutron-induced fission. The measurement was performed at the Los Alamos Neutron Science Center, where the neutron energy is determined from neutron time-of-flight. The $^{238}$U(n,f)/$^{235}$U(n,f) ratio reported here is the first cross section measurement made with the fissionTPC, and will provide new experimental data for evaluation of the $^{238}$U(n,f) cross section, an important standard used in neutron-flux measurements. Use of a development target in this work prevented the determination of an absolute normalization, to be addressed in future measurements. Instead, the measured cross section ratio has been normalized to ENDF/B-VIII.$β$5 at 14.5 MeV.

nucl-ex↗

arXiv2014

A Time Projection Chamber for High Accuracy and Precision Fission Cross Section Measurements

The fission Time Projection Chamber (fissionTPC) is a compact (15 cm diameter) two-chamber MICROMEGAS TPC designed to make precision cross section measurements of neutron-induced fission. The actinide targets are placed on the central cathode and irradiated with a neutron beam that passes axially through the TPC inducing fission in the target. The 4$π$ acceptance for fission fragments and complete charged particle track reconstruction are powerful features of the fissionTPC which will be used to measure fission cross sections and examine the associated systematic errors. This paper provides a detailed description of the design requirements, the design solutions, and the initial performance of the fissionTPC.

physics.ins-det↗

arXiv2014

The Excitation Energy Dependence of the Total Kinetic Energy Release in 235U(n,f)

The total kinetic energy release in the neutron induced fission of $^{235}$U was measured (using white spectrum neutrons from LANSCE) for neutron energies from E$_{n}$ = 3.2 to 50 MeV. In this energy range the average post-neutron total kinetic energy release drops from 167.4 $\pm$ 0.7 to 162.1 $\pm$ 0.8 MeV, exhibiting a local dip near the second chance fission threshold. The values and the slope of the TKE vs. E$_{n}$ agree with previous measurements but do disagree (in magnitude) with systematics. The variances of the TKE distributions are larger than expected and apart from structure near the second chance fission threshold, are invariant for the neutron energy range from 11 to 50 MeV. We also report the dependence of the total excitation energy in fission, TXE, on neutron energy.

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arXiv2014

Measurement of the Survival Probabilities for Hot Fusion Reactions

We have studied the fission-neutron emission competition in highly excited $^{274}$Hs (Z=108) (where the fission barrier is due to shell effects) formed by a hot fusion reaction. Matching cross bombardments ($^{26}$Mg + $^{248}$Cm and $^{25}$Mg + $^{248}$Cm) were used to identify the properties of first chance fission of $^{274}$Hs. A Harding-Farley analysis of the fission neutrons emitted in the $^{25,26}$Mg + $^{248}$Cm was performed to identify the pre- and post-scission components of the neutron multiplicities in each system. ($Γ$$_{n}$/$Γ$$_{t}$) for the first chance fission of $^{274}$Hs (E$^{\ast}$ = 63 MeV) is 0.89 $\pm$ 0.13, i.e., $\sim$ 90 $%$ of the highly excited nuclei survive.The high value of that survival probability is due to dissipative effects during de-excitation. A proper description of the survival probabilities of excited superheavy nuclei formed in hot fusion reactions requires consideration of both dynamic and static (shell-related) effects.

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arXiv2013

Measurement of the Fusion Probability, PCN, for Hot Fusion Reactions

Background: The cross section for forming a heavy evaporation residue in fusion reactions depends on the capture cross section, the fusion probability, PCN, i.e., the probability that the projectile-target system will evolve inside the fission saddle point to form a completely fused system rather than re-separating (quasifission), and the survival of the completely fused system against fission. PCN is the least known of these quantities. Purpose: To measure PCN for the reaction of 101.2 MeV 18O, 147.3 MeV 26Mg, 170.9 MeV 30Si and 195.3 MeV 36S with 197Au. Methods: We measured the fission fragment angular distributions for these reactions and used the formalism of Back to deduce the fusion-fission and quasifission cross sections. From these quantities we deduced PCN for each reaction. Results: The values of PCN for the reaction of 101.2 MeV 18O, 147.3 MeV 26Mg, 170.9 MeV 30Si and 195.3 MeV 36S with 197Au are 0.66, 1.00, 0.06, 0.13, respectively. Conclusions: The new measured values of PCN agree roughly with the semi-empirical system- atic dependence of PCN upon fissility for excited nuclei.

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arXiv2013

Targets for Precision Measurements

The general properties needed in targets (sources) for high precision, high accuracy measurements are reviewed. The application of these principles to the problem of developing targets for the Fission TPC is described. Longer term issues, such as the availability of actinide materials, improved knowledge of energy losses and straggling and the stability of targets during irradiation are also discussed.

physics.ins-det↗

arXiv2013

The interaction of 11Li with 208Pb

Background: 11Li is one of the most studied halo nuclei. The fusion of 11Li with 208Pb has been the subject of a number of theoretical studies with widely differing predictions, ranging over four orders of magnitude, for the fusion excitation function. Purpose: To measure the excitation function for the 11Li + 208Pb reaction. Methods: A stacked foil/degrader assembly of 208Pb targets was irradiated with a 11Li beam producing center of target beam energies from above barrier to near barrier energies (40 to 29 MeV). The intensity of the 11Li beam (chopped) was 1250 p/s and the beam on-target time was 34 hours. The alpha-decay of the stopped evaporation residues was detected in a alpha-detector array at each beam energy in the beam-off period (the beam was on for <= 5 ns and then off for 170 ns). Results: The 215At evaporation residues were associated with the fusion of 11Li with 208Pb. The 213,214At evaporation residues were formed by the breakup of 11Li into 9Li + 2n, with the 9Li fusing with 208Pb. The 214At evaporation residue appears to result from a "quasi-breakup" process. Conclusions: Most of 11Li + 208Pb interactions lead to breakup with a small fraction (<= 11%) leading to complete fusion.

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arXiv2012

d0 Ferromagnetic Interface Between Non-magnetic Perovskites

We use computational and experimental methods to study d0 ferromagnetism at a charge- imbalanced interface between two perovskites. In SrTiO3/KTaO3 superlattice calculations, the charge imbalance introduces holes in the SrTiO3 layer, inducing a d0 ferromagnetic half-metallic 2D electron gas at the interface oxygen 2p orbitals. The charge imbalance overrides doping by vacancies at realistic concentrations. Varying the constituent materials shows ferromagnetism to be a gen- eral property of hole-type d0 perovskite interfaces. Atomically sharp epitaxial d0 SrTiO3/KTaO3, SrTiO3 /KNbO3 and SrTiO3 /NaNbO3 interfaces are found to exhibit ferromagnetic hysteresis at room temperature. We suggest the behavior is due to high density of states and exchange coupling at the oxygen t1g band in comparison with the more studied d band t2g symmetry electron gas.

cond-mat.mtrl-sci↗