arXiv subjects

L. Yuan

Publications and source records attributed to L. Yuan.

At least 19 recordsLinked to original sources

arXiv2025

Catalight -- an open source automated photocatalytic reactor package illustrated through plasmonic acetylene hydrogenation

An open-source and modular Python package, Catalight, is developed and demonstrated to automate (photo)catalysis measurements. (Photo)catalysis experiments require studying several parameters to evaluate performance, including temperature, gas flow rate and composition, illumination power, and spectral profile. Catalight orchestrates measurements over this complicated parameter space and systematically stores, analyzes, and visualizes the resulting data. To showcase the capabilities of Catalight, we perform an automated apparent activation barrier measurement of acetylene hydrogenation over a plasmonic AuPd catalyst on Al2O3 support, simultaneously varying laser power, wavelength, and temperature in a multi-day experiment controlled by a simple Python script. Our chemical results unexpectedly show an increased activation barrier upon light excitation, contrary to previous findings for other plasmonic reactions and catalysts. We show that the reaction rate order with respect to both acetylene and hydrogen is unchanged upon illumination, suggesting that molecular surface coverage is not changing under light excitation. By analyzing the inhomogeneity of the laser induced heating, we attribute these results to a partial photothermal effect combined with a photochemical/hot electron driven mechanism. Our findings highlight the capabilities of a new experiment automation tool; explore the photocatalytic mechanism for an industrially relevant reaction; and identify systematic sources of error in canon photocatalysis experimental procedures.

physics.chem-ph↗

arXiv2023

Revisiting the Properties of GW190814 and Its Formation History

GW190814 was reported during LIGO's and Virgo's third observing run with the most asymmetric component masses (a $\sim 23$ $M_{\odot}$ black hole and a $\sim2.6$ $M_{\odot}$ compact object). Under the assumption that this event is a binary black hole (BBH) merger formed through the isolated binary evolution channel, we reanalyze the publicly released data of GW190814 with the modified astrophysical priors on the effective spin $χ_{\rm eff}$, and further explore its formation history using detailed binary modeling. We show that GW190814 is likely to have been formed through the classical common envelope channel. Our findings show that the properties inferred using the modified astrophysical priors are consistent with those inferred by the uniform priors. With the newly-inferred properties of GW190814, we perform detailed binary evolution of the immediate progenitor of the BBH (namely a close binary system composed of a BH and a helium star) in a large parameter space, taking into account mass-loss, internal differential rotation, supernova kicks, and tidal interactions between the helium star and the BH companion. Our findings show that GW190814-like events could be formed in limited initial conditions just after the common envelope phase: a $\sim 23$ $M_{\odot}$ BH and a helium star of $M_{\rm ZamsHe}$ $\sim$ 8.5 $M_{\odot}$ at solar metallicity ($\sim$ 7.5 $M_{\odot}$ at 10\% solar metallicity) with an initial orbital period at around 1.0 day. Additionally, the inferred low spin of the secondary indicates that the required metallicity for reproducing GW190814-like events should not be too low (e.g., Z $\gtrsim$ 0.1 $Z_{\odot}$).

astro-ph.HE↗

arXiv2022

Evidence for the singly Cabibbo-suppressed decay $\Omega^0_c\to\Xi^-\pi^+$ and search for $\Omega^0_c\to\Xi^-K^+$ and $\Omega^-K^+$ decays at Belle

Using a data sample of 980 fb$^{-1}$ collected with the Belle detector at the KEKB asymmetric-energy $e^+e^-$ collider, we study for the first time the singly Cabibbo-suppressed decays $\Omega^0_c\to\Xi^{-}\pi^{+}$ and $\Omega^-K^+$ and the doubly Cabibbo-suppressed decay $\Omega^0_c\to \Xi^- K^{+}$. Evidence for an $\Omega^0_c$ signal in the $\Omega^0_c\to\Xi^-\pi^+$ mode is reported with a significance of $4.5\sigma$ including systematic uncertainties. The ratio of branching fractions to the normalization mode $\Omega_c^0\to \Omega^-\pi^+$ is measured to be $${\cal B}(\Omega_{c}^{0} \to \Xi^{-} \pi ^{+} )/{\cal B}(\Omega_c^0\to \Omega^-\pi^+)=0.253\pm 0.053({\rm stat.})\pm 0.030({\rm syst.}).$$ No significant signals of $\Omega^0_c\to\Xi^-K^+$ and $\Omega^-K^+$ modes are found. The upper limits at $90\%$ confidence level on ratios of branching fractions are determined to be $${\cal B}(\Omega_{c}^{0} \to \Xi^{-} K ^{+})/{\cal B}(\Omega_c^0\to \Omega^-\pi^+) < 0.070$$ and $${\cal B}(\Omega_{c}^{0} \to \Omega^{-}K^{+})/{\cal B}(\Omega_c^0\to \Omega^-\pi^+) < 0.29.$$

hep-ex↗

arXiv2022

Scintillation yield from electronic and nuclear recoils in superfluid $^4$He

Superfluid $^4$He is a promising target material for direct detection of light ($<$ 1 GeV) dark matter. Possible signal channels available for readout in this medium include prompt photons, triplet excimers, and roton and phonon quasiparticles. The relative yield of these signals has implications for the sensitivity and discrimination power of a superfluid $^4$He dark matter detector. Using a 16~cm$^3$ volume of 1.75~K superfluid $^4$He read out by six immersed photomultiplier tubes, we measured the scintillation from electronic recoils ranging between 36.3 and 185 keV$_\mathrm{ee}$, yielding a mean signal size of $1.25^{+0.03}_{-0.03}$~phe/keV$_\mathrm{ee}$, and nuclear recoils from 53.2 to 1090 keV$_\mathrm{nr}$. We compare the results of our relative scintillation yield measurements to an existing semiempirical model based on helium-helium and electron-helium interaction cross sections. We also study the behavior of delayed scintillation components as a function of recoil type and energy, a further avenue for signal discrimination in superfluid $^4$He.

physics.ins-det↗

arXiv2021

Measurement of the EMC effect in light and heavy nuclei

Inclusive electron scattering from nuclear targets has been measured to extract the nuclear dependence of the inelastic cross section in Hall C at the Thomas Jefferson National Accelerator facility. Results are presented for 2H, 3He, 4He, 9B, 12C, 63Cu and 197Au at an incident electron beam energy of 5.77 GeV for a range of momentum transfer from Q^2 = 2 to 7 (GeV/c)^2. These data improve the precision of the existing measurements of the EMC effect in the nuclear targets at large x, and allow for more detailed examinations of the A dependence of the EMC effect.

nucl-ex↗

arXiv2021

Spectroscopy of $A=9$ hyperlithium by the $(e,e^{\prime}K^{+})$ reaction

Missing mass spectroscopy with the $(e,e^{\prime}K^{+})$ reaction was performed at Jefferson Laboratory's Hall C for the neutron rich $Λ$ hypernucleus $^{9}_Λ{\rm Li}$. The ground state energy was obtained to be $B_Λ^{\rm g.s.}=8.84\pm0.17^{\rm stat.}\pm0.15^{\rm sys.}~{\rm MeV}$ by using shell model calculations of a cross section ratio and an energy separation of the spin doublet states ($3/2^{+}_1$ and $5/2^{+}_1$). In addition, peaks that are considered to be states of [$^{8}{\rm Li}(3^{+})\otimes s_Λ=3/2^{+}_{2}, 1/2^{+}$] and [$^{8}{\rm Li}(1^{+})\otimes s_Λ=5/2^{+}_{2}, 7/2^{+}$] were observed at $E_Λ({\rm no.~2})=1.74\pm0.27^{\rm stat.}\pm0.11^{\rm sys.}~{\rm MeV}$ and $E_Λ({\rm no.~3})=3.30\pm0.24^{\rm stat.}\pm0.11^{\rm sys.}~{\rm MeV}$, respectively. The $E_Λ({\rm no.~3})$ is larger than shell model predictions by a few hundred keV, and the difference would indicate that a ${\rm ^{5}He}+t$ structure is more developed for the $3^{+}$ state than those for the $2^{+}$ and $1^{+}$ states in a core nucleus $^{8}{\rm Li}$ as a cluster model calculation suggests.

nucl-ex↗

arXiv2019

Precision Measurements of $A_1^n$ in the Deep Inelastic Regime

We have performed precision measurements of the double-spin virtual-photon asymmetry $A_1$ on the neutron in the deep inelastic scattering regime, using an open-geometry, large-acceptance spectrometer. Our data cover a wide kinematic range $0.277 \leq x \leq 0.548$ at an average $Q^2$ value of 3.078~(GeV/c)$^2$, doubling the available high-precision neutron data in this $x$ range. We have combined our results with world data on proton targets to extract the ratio of polarized-to-unpolarized parton distribution functions for up quarks and for down quarks in the same kinematic range. Our data are consistent with a previous observation of an $A_1^n$ zero crossing near $x=0.5$. We find no evidence of a transition to a positive slope in $(Δd + Δ\bar{d})/(d + \bar{d})$ up to $x=0.548$.

nucl-ex↗

arXiv2018

Experimental techniques and performance of $Λ$-hypernuclear spectroscopy with the $(e,e^{\prime}K^{+})$ reaction

The missing-mass spectroscopy of $Λ$ hypernuclei via the $(e,e^{\prime}K^{+})$ reaction has been developed through experiments at JLab Halls A and C in the last two decades. For the latest experiment, E05-115 in Hall C, we developed a new spectrometer system consisting of the HKS and HES; resulting in the best energy resolution ($E_Λ \simeq0.5$-MeV FWHM) and $B_Λ$ accuracy ($B_Λ\leq0.2$ MeV) in $Λ$-hypernuclear reaction spectroscopy. This paper describes the characteristics of the $(e,e^{\prime}K^{+})$ reaction compared to other reactions and experimental methods. In addition, the experimental apparatus, some of the important analyses such as the semi-automated calibration of absolute energy scale, and the performance achieved in E05-115 are presented.

physics.ins-det↗

arXiv2016

Refinement on non-hydrostatic shallow granular flow model in a global Cartesian coordinate system

Current shallow granular flow models suited to arbitrary topography can be divided into two types, those formulated in bed-fitted curvilinear coordinates, and those formulated in global Cartesian coordinates. The shallow granular flow model of Denlinger and Iverson \cite{Denlinger2004} and the Boussinesq-type shallow granular flow theory of Castro-Orgaz \emph{et al}. \cite{Castro2014} are formulated in a Cartesian coordinate system (with $z$ vertical), and both account for the effect of nonzero vertical acceleration on depth-averaged momentum fluxes and stress states. In this paper, we first reformulate the vertical normal stress of Castro-Orgaz \emph{et al}. \cite{Castro2014} in a quadratic polynomial in the relative elevation $η$. This form allows for analytical depth integration of the vertical normal stress. We then calculate the basal normal stress based on the basal friction law and scaling analysis. These calculations, plus certain constitutive relations, lead to a refined full non-hydrostatic shallow granular flow model, which is further rewritten in a form of Boussinesq-type water wave equations for future numerical studies. In the present numerical study, we apply the open-source code TITAN2D to numerical solution of a low-order version of the full model involving only a mean vertical acceleration correction term. To cure the numerical instability associated with discretization of the enhanced gravity, we propose an approximate formula for the enhanced gravity by utilizing the hydrostatic pressure assumption in the bed normal direction. Numerical calculations are conducted for several test cases involving steep slopes. Comparison with a bed-fitted model shows that even the simplified non-hydrostatic Cartesian model can be used to simulate shallow granular flows over arbitrary topography.

physics.geo-ph↗

arXiv2016

Spectroscopy of the neutron-rich hypernucleus $^{7}_Λ$He from electron scattering

The missing mass spectroscopy of the $^{7}_Λ$He hypernucleus was performed, using the $^{7}$Li$(e,e^{\prime}K^{+})^{7}_Λ$He reaction at the Thomas Jefferson National Accelerator Facility Hall C. The $Λ$ binding energy of the ground state (1/2$^{+}$) was determined with a smaller error than that of the previous measurement, being $B_Λ$ = 5.55 $\pm$ 0.10(stat.) $\pm$ 0.11(sys.) MeV. The experiment also provided new insight into charge symmetry breaking in p-shell hypernuclear systems. Finally, a peak at $B_Λ$ = 3.65 $\pm$ 0.20(stat.) $\pm$ 0.11(sys.) MeV was observed and assigned as a mixture of 3/2$^{+}$ and 5/2$^{+}$ states, confirming the "gluelike" behavior of $Λ$, which makes an unstable state in $^{6}$He stable against neutron emission.

nucl-ex↗

arXiv2016

Measurements of $d_{2}^{n}$ and $A_{1}^{n}$: Probing the neutron spin structure

We report on the results of the E06-014 experiment performed at Jefferson Lab in Hall A, where a precision measurement of the twist-3 matrix element $d_2$ of the neutron ($d_{2}^{n}$) was conducted. This quantity represents the average color Lorentz force a struck quark experiences in a deep inelastic electron scattering event off a neutron due to its interaction with the hadronizing remnants. This color force was determined from a linear combination of the third moments of the spin structure functions $g_1$ and $g_2$ on $^{3}$He after nuclear corrections had been applied to these moments. The kinematics included two average $Q^{2}$ bins of $3.2$ GeV$^{2}$ and $4.3$ GeV$^{2}$, and Bjorken-$x$ $0.25 \leq x \leq 0.90$ covering the DIS and resonance regions. We found $d_2^n$ to be small and negative for $ = 3.2$ GeV$^{2}$, and smaller for $ = 4.3$ GeV$^{2}$, consistent with a lattice QCD calculation. The twist-4 matrix element $f_{2}^{n}$ was extracted by combining our $d_{2}^{n}$ with the world data on $Γ_{1}^{n} = \int_{0}^{1} g_{1}^{n} dx$. We found $f_{2}^{n}$ to be roughly an order of magnitude larger than $d_{2}^{n}$. Utilizing the extracted $d_{2}^{n}$ and $f_{2}^{n}$ data, we separated the color force into its electric and magnetic components, $F_{E}^{y,n}$ and $F_{B}^{y,n}$, and found them to be equal and opposite in magnitude, in agreement with instanton model predictions but not with those from QCD sum rules. Additionally, we have extracted the neutron virtual photon-nucleon asymmetry $A_{1}^{n}$, the structure function ratio $g_{1}^{n}/F_{1}^{n}$, and the quark ratios $(Δu + Δ\bar{u})/(u + \bar{u})$ and $(Δd + Δ\bar{d})/(d + \bar{d})$. These results were found to be consistent with DIS world data and with the prediction of the constituent quark model but at odds with those of perturbative QCD at large $x$.

nucl-ex↗

arXiv2016

Measurements of the Separated Longitudinal Structure Function F_L from Hydrogen and Deuterium Targets at Low Q^2

Structure functions, as measured in lepton-nucleon scattering, have proven to be very useful in studying the quark dynamics within the nucleon. However, it is experimentally difficult to separately determine the longitudinal and transverse structure functions, and consequently there are substantially less data available for the longitudinal structure function in particular. Here we present separated structure functions for hydrogen and deuterium at low four--momentum transfer squared, Q^2< 1 GeV^2, and compare these with parton distribution parameterizations and a k_T factorization approach. While differences are found, the parameterizations generally agree with the data even at the very low Q^2 scale of the data. The deuterium data show a smaller longitudinal structure function, and smaller ratio of longitudinal to transverse cross section R, than the proton. This suggests either an unexpected difference in R for the proton and neutron or a suppression of the gluonic distribution in nuclei.

nucl-ex↗

arXiv2016

High Resolution Spectroscopic Study of $^{10}_Λ$Be

Spectroscopy of a $^{10}_Λ$Be hypernucleus was carried out at JLab Hall C using the $(e,e^{\prime}K^{+})$ reaction. A new magnetic spectrometer system (SPL+HES+HKS), specifically designed for high resolution hypernuclear spectroscopy, was used to obtain an energy spectrum with a resolution of 0.78 MeV (FWHM). The well-calibrated spectrometer system of the present experiment using the $p(e,e^{\prime}K^{+})Λ,Σ^{0}$ reactions allowed us to determine the energy levels, and the binding energy of the ground state peak (mixture of 1$^{-}$ and 2$^{-}$ states) was obtained to be B$_Λ$=8.55$\pm$0.07(stat.)$\pm$0.11(sys.) MeV. The result indicates that the ground state energy is shallower than that of an emulsion study by about 0.5 MeV which provides valuable experimental information on charge symmetry breaking effect in the $ΛN$ interaction.

nucl-ex↗

arXiv2014

The experiments with the High Resolution Kaon Spectrometer at JLab Hall C and the new spectroscopy of ${}^{12}_Λ\text{B}$ hypernuclei

Since the pioneering experiment, E89-009 studying hypernuclear spectroscopy using the $(e,e^{\prime}K^+)$ reaction was completed, two additional experiments, E01-011 and E05-115, were performed at Jefferson Lab. These later experiments used a modified experimental design, the "tilt method", to dramatically suppress the large electromagnetic background, and allowed for a substantial increase in luminosity. Additionally, a new kaon spectrometer, HKS (E01-011), a new electron spectrometer, HES, and a new splitting magnet were added to produce precision, high-resolution hypernuclear spectroscopy. These two experiments, E01-011 and E05-115, resulted in two new data sets, producing sub-MeV energy resolution in the spectra of ${}^{7}_Λ\text{He}$, ${}^{12}_Λ\text{B}$ and ${}^{28}_Λ\text{Al}$ and ${}^{7}_Λ\text{He}$, ${}^{10}_Λ\text{Be}$, ${}^{12}_Λ\text{B}$ and ${}^{52}_Λ\text{V}$. All three experiments obtained a ${}^{12}_Λ\text{B}$, spectrum, which is the most characteristic $p$-shell hypernucleus and is commonly used for calibration. Independent analyses of these different experiments demonstrate excellent consistency and provide the clearest level structure to date of this hypernucleus as produced by the $(e,e^{\prime}K^+)$ reaction. This paper presents details of these experiments, and the extraction and analysis of the observed ${}^{12}_Λ\text{B}$ spectrum.

nucl-ex↗

arXiv2014

A Precision Measurement of the Neutron Twist-3 Matrix Element $d_2^n$: Probing Color Forces

Double-spin asymmetries and absolute cross sections were measured at large Bjorken $x$ (0.25 $ \le x \le $ 0.90), in both the deep-inelastic and resonance regions, by scattering longitudinally polarized electrons at beam energies of 4.7 and 5.9 GeV from a transversely and longitudinally polarized $^3$He target. In this dedicated experiment, the spin structure function $g_2$ on $^3$He was determined with precision at large $x$, and the neutron twist-three matrix element $d_2^n$ was measured at $\left< Q^2\right>$ of 3.21 and 4.32 GeV$^2$/$c^2$, with an absolute precision of about $10^{-5}$. Our results are found to be in agreement with lattice QCD calculations and resolve the disagreement found with previous data at $\left< Q^2\right> =$ 5 GeV$^2$/$c^2$. Combining $d_2^n$ and a newly extracted twist-four matrix element, $f_2^n$, the average neutron color electric and magnetic forces were extracted and found to be of opposite sign and about 30 MeV/fm in magnitude.

nucl-ex↗

arXiv2013

Direct Measurements of the Lifetime of Heavy Hypernuclei

The lifetime of a Lambda particle embedded in a nucleus (hypernucleus) decreases from that of free Lambda decay due to the opening of the Lambda N to NN weak decay channel. However, it is generally believed that the lifetime of a hypernucleus attains a constant value (saturation) for medium to heavy hypernuclear masses, yet this hypothesis has been difficult to verify. The present paper reports a direct measurement of the lifetime of medium-heavy hypernuclei produced with a photon-beam from Fe, Cu, Ag, and Bi targets. The recoiling hypernuclei were detected by a fission fragment detector using low-pressure multi-wire proportional chambers. The experiment agrees remarkably well with the only previously-measured single-species heavy-hypernucleus lifetime, that of Fe56_Lambda at KEK, and has significantly higher precision. The experiment disagrees with the measured lifetime of an unknown combination of heavy hypernuclei with 180<A<225 and, with a small statistical and systematic uncertainty, strongly favors the expected saturation of the lifetime decrease.

nucl-ex↗

arXiv2013

Measurement of R = sigma_L / sigma_T and the Separated Longitudinal and Transverse Structure Functions in the Nucleon Resonance Region

We report on a detailed study of longitudinal strength in the nucleon resonance region, presenting new results from inclusive electron-proton cross sections measured at Jefferson Lab Hall C in the four-momentum transfer range 0.2 < Q^2 < 5.5 GeV^2. The data have been used to accurately perform 167 Rosenbluth-type longitudinal / transverse separations. The precision R = sigma_L / sigma_T data are presented here, along with the first separate values of the inelastic structure functions F_1 and F_L in this regime. The resonance longitudinal component is found to be significant, both in magnitude and in the existence of defined mass peaks. Additionally, quark-hadron duality is here observed above Q^2 = 1 GeV^2 in the separated structure functions independently.

nucl-ex↗

arXiv2012

Observation of the Helium 7 Lambda hypernucleus by the (e,e'K+) reaction

An experiment with a newly developed high-resolution kaon spectrometer (HKS) and a scattered electron spectrometer with a novel configuration was performed in Hall C at Jefferson Lab (JLab). The ground state of a neutron-rich hypernucleus, He 7 Lambda, was observed for the first time with the (e,e'K+) reaction with an energy resolution of ~0.6 MeV. This resolution is the best reported to date for hypernuclear reaction spectroscopy. The he 7 Lambda binding energy supplies the last missing information of the A=7, T=1 hypernuclear iso-triplet, providing a new input for the charge symmetry breaking (CSB) effect of ΛN potential.

nucl-ex↗