arXiv subjects

Lara Benfatto

Publications and source records attributed to Lara Benfatto.

At least 37 records · Page 2Linked to original sources

arXiv2022

Many-body Green's function approach to lattice thermal transport

Recent progress in understanding thermal transport in complex crystals has highlighted the prominent role of heat conduction mediated by interband tunneling processes, which emerge between overlapping phonon bands (i.e. with energy differences smaller than their broadenings). These processes have recently been described in different ways, relying on the Wigner or Green-Kubo formalism, leading to apparently different results which question the definition of the heat-current operator. Here, we implement a full quantum approach based on the Kubo formula, elucidating analogies and differences with the recently introduced Wigner or Green-Kubo formulations, and extending the description of thermal transport to the overdamped regime of atomic vibrations, where the phonon quasiparticle picture breaks down. We rely on first-principles calculations on complex crystals with ultralow conductivity to compare numerically the thermal conductivity obtained within the aforementioned approaches, showing that at least in the quasiparticle regime the differences are negligible for practical applications.

cond-mat.mtrl-sci↗

arXiv2022

Contribution of Collective Excitations to Third Harmonic Generation in Multiband Superconductors: the case of MgB$_2$

Multiband superconductors can host collective excitations with marked differences with respect to their single-band counterpart. We first study the spectrum of collective amplitude fluctuations in a clean two-bands superconductor, showing that the spectral weight of the Higgs mode rapidly deviates from the naive extension of the single band case as the interband coupling is turned on. These results are then used to critically analyze the non-linear optical response in MgB$_2$, providing an explanation for the apparently contradictory results of recent experiments, pointing towards a selective relevance either of the Leggett mode or of the amplitude fluctuations at twice the lower gap. By using exact numerical simulations and realistic estimate of disorder we compute the relative contribution of the quasiparticle, amplitude and phase fluctuations to the non-linear optical response. We show that at low pumping frequency only the resonance at twice the smaller gap emerges, as due to the BCS response, while the Leggett mode dominates only in a narrow range of higher pumping frequencies matching its low-temperature value. Our findings provide a fresh perspective on the potential of non-linear THz spectroscopy to detect collective modes in other multiband systems, as e.g. iron-based superconductors.

cond-mat.supr-con↗

arXiv2022

Boltzmann electronic dc transport in multiorbital weakly-disordered crystals

Motivated by the increasing number of systems featuring multiple bands at low energy, we address the Boltzmann approach to transport in a multiband weakly disordered noninteracting crystal subject to a small electric field. In general, the multiband structure leads to a considerable complication of the Boltzmann equation. Indeed, even in the presence of elastic impurity scattering, one needs to compute for each band and momentum the dressed velocities, which account for scattering events. Here we provide a semianalytical solution to the Boltzmann equation that reduces such a challenging numerical task to the much simpler numerical computation of a small tensor whose dimension is set by the number of bands at the Fermi level. This approach further allows us to discuss the interplay of symmetry and disorder for different impurity types, including those originating from random-matrix Wigner ensembles. As an example of application, we consider the 2D isotropic Rashba metal and we discuss, in a full analytical fashion, how different types of disorders may break the exactness of the relaxation-time approximation and induce transport anisotropy, and may allow one to identify the presence of spin-orbit coupling as deviations of the conductivity from the Drude behavior.

cond-mat.mes-hall↗

arXiv2022

THz non-linear optical response in cuprates: predominance of the BCS response over the Higgs mode

Recent experiments with strong THz fields in unconventional cuprates superconductors have clearly evidenced an increase of the non-linear optical response below the superconducting critical temperature Tc. As in the case of conventional superconductors, a theoretical estimate of the various effects contributing to the non-linear response is needed in order to interpret the experimental findings. Here we report a detailed quantitative analysis of the non-linear THz optical kernel in cuprates within a realistic model, accounting for the band structure and disorder level appropriate for these systems. We show that the BCS quasiparticle response is the dominant contribution for cuprates, and its polarization dependence accounts very well for the third-harmonic generation measurements. On the other hand, the polarization dependence of the THz Kerr effect is only partly captured by our calculations, suggesting the presence of additional effects when the system is probed using light pulses with different central frequencies.

cond-mat.supr-con↗

arXiv2021

Transport signatures of fragile-glass dynamics in the melting of the two-dimensional vortex lattice

In two-dimensional (2D) systems, the melting from a solid to an isotropic liquid can occur via an intermediate phase that retains orientational order. However, in 2D superconducting vortex lattices, the effect of orientational correlations on transport, and their interplay with disorder remain open questions. Here we study a 2D weakly pinned vortex system in amorphous MoGe films over an extensive range of temperatures ($\bm{T}$) and perpendicular magnetic fields ($\bm{H}$) using linear and nonlinear transport measurements. We find that, at low fields, the resistivity obeys the Vogel-Fulcher-Tamman (VFT) form, $\bm{ρ(T)\propto\exp[-{W}(H)/(T-T_0(H))]}$, characteristic of fragile glasses. As $\bm{H}$ increases, $\bm{T_0(H)}$ is suppressed to zero, and a standard vortex liquid behavior consistent with a $\bm{T=0}$ superconducting transition is observed. Our findings, supported also by simulations, suggest that the presence of orientational correlations gives rise to a heterogeneous dynamics responsible for the VFT behavior. The effects of quenched disorder become dominant at high $\bm{H}$, where a crossover to a strong-glass behavior is observed. This is a new insight into the dynamics of melting in 2D systems with competing orders.

cond-mat.supr-con↗

arXiv2021

Uniformly frustrated XY model: strengthening of the vortex lattice by intrinsic disorder

In superconducting films, the role of intrinsic disorder is typically to compete with superconductivity by fragmenting the global phase coherence and lowering the superfluid density. Nonetheless, when a transverse magnetic field is applied to the system and an Abrikosov vortex lattice forms, the presence of disorder can actually strengthen the superconducting state against thermal fluctuations. By means of Monte Carlo simulations on the uniformly frustrated XY model in two dimensions, we show that while for weak pinning the superconducting critical temperature $T_c$ increases with the applied field $H$, for strong enough pinning the experimental decreasing dependence between $T_c$ and $H$ is recovered with a resulting more robust vortex lattice.

cond-mat.supr-con↗

arXiv2020

Lattice contribution to the unconventional charge density wave transition in $2H$-NbSe$_2$: a non-equilibrium optical approach

The complex Fermi surfaces of transition-metal dichalcogenides (TMDCs) challenge the standard Peierls-instability-driven charge-density-wave (CDW) formation. Recently, evidence has been accumulating of a prominent role of ionic thermal fluctuations, which frozen out below $T_{CDW}$ inducing a periodic lattice distortion (PLD). We focus on $2H$-NbSe$_2$, displaying a quasi-commensurate CDW below $T_{CDW}$ $\approx$33 K, and use time-resolved optical spectroscopy (TR-OS) to detect and disentangle the electronic and lattice degrees of freedom. We reveal a fingerprint of the ordered phase at h$ν$ $\sim$1 eV: at $T_{CDW}$, a divergent relaxation timescale and a sign-change of the differential reflectivity indicate that CDW gap opening and PLD formation occur at the same temperature. However, we show that these effects can be decoupled under moderate photoexcitation, forming a long-lived state in which the electronic order is destroyed, but the lattice distortion is not. Our results and computations suggest an unconventional CDW mechanims in $2H$-NbSe$_2$, highlighting the dominant role of the lattice in driving the ordered-phase formation.

cond-mat.str-el↗

arXiv2020

Interplay of spin waves and vortices in the 2D XY model at small vortex-core energy

The Berezinskii-Kosterlitz-Thouless (BKT) mechanism describes universal vortex unbinding in many two-dimensional systems, including the paradigmatic XY model. However, most of these systems present a complex interplay between excitations at different length scales that complicates theoretical calculations of nonuniversal thermodynamic quantities. These difficulties may be overcome by suitably modifying the initial conditions of the BKT flow equations to account for noncritical fluctuations at small length scales. In this work, we perform a systematic study of the validity and limits of this two-step approach by constructing optimised initial conditions for the BKT flow. We find that the two-step approach can accurately reproduce the results of Monte-Carlo simulations of the traditional XY model. In order to systematically study the interplay between vortices and spin-wave excitations, we introduce a modified XY model with increased vortex fugacity. We present large-scale Monte-Carlo simulations of the spin stiffness and vortex density for this modified XY model and show that even at large vortex fugacity, vortex unbinding is accurately described by the nonperturbative functional renormalisation group.

cond-mat.str-el↗

arXiv2020

Non-linear Terahertz Driving of Plasma Waves in Layered Cuprates

The hallmark of superconductivity is the rigidity of the quantum-mechanical phase of electrons, responsible for superfluid behavior and Meissner effect. The strength of the phase stiffness is set by the Josephson coupling, which is strongly anisotropic in layered superconducting cuprates. So far, THz light pulses have been efficiently used to achieve non-linear control of the out-of-plane Josephson plasma mode, whose frequency scale lies in the THz range. However, the high-energy in-plane plasma mode has been assumed to be insensitive to THz pumping. Here, we show that THz driving of both low-frequency and high-frequency plasma waves is possible via a general two-plasmon excitation mechanism. The anisotropy of the Josephson couplings leads to marked differences in the thermal effects among the out-of-plane and in-plane response, consistently with the experiments. Our results link the observed survival of the in-plane THz non-linear driving above $T_c$ to enhanced fluctuating effects in the phase stiffness in cuprates, paving the way to THz impulsive control of phase rigidity in unconventional superconductors.

cond-mat.supr-con↗

arXiv2020

Destruction of superconductivity through phase fluctuations in ultrathin a-MoGe films

We investigate the evolution of superconductivity with decreasing film thickness in ultrathin amorphous MoGe (a-MoGe) films using a combination of sub-Kelvin scanning tunneling spectroscopy, magnetic penetration depth measurements and magneto-transport measurements. We observe that superconductivity is strongly affected by quantum and classical phase fluctuations for thickness below 5 nm. The superfluid density is strongly suppressed by quantum phase fluctuations at low temperatures and evolves towards a linear-T dependence at higher temperatures. This is associated with a rapid decrease in the superconducting transition temperature, Tc, and the emergence of a pronounced pseudogap above Tc. These observations suggest that at strong disorder the destruction of superconductivity follows a Bosonic route where the global superconducting state is destroyed by phase fluctuations even though the pairing amplitude remains finite.

cond-mat.supr-con↗

arXiv2019

Theory of coherent oscillations detection in THz pump-probe spectroscopy: from phonons to electronic collective modes

Time-resolved spectroscopies using intense THz pulses appear as a promising tool to address collective electronic excitations in condensed matter. In particular recent experiments showed the possibility to selectively excite collective modes emerging across a phase transition, as it is the case for superconducting and charge-density-wave (CDW) systems. One possible signature of these excitations is the emergence of coherent oscillations of the differential probe field in pump-probe protocols. While the analogy with the case of phonon modes suggests that the basic underlying mechanism should be a sum-frequency stimulated Raman process, a general theoretical scheme able to describe the experiments and to define the relevant optical quantity is still lacking. Here we provide this scheme by showing that coherent oscillations as a function of the pump-probe time delay can be linked to the convolution in the frequency domain between the squared pump field and a Raman-like non-linear optical kernel. This approach is applied and discussed in few paradigmatic examples: ordinary phonons in an insulator, and collective charge and Higgs fluctuations across a superconducting and a CDW transition. Our results not only account very well for the existing experimental data in a wide variety of systems, but they also offer an useful perspective to design future experiments in emerging materials.

cond-mat.str-el↗

arXiv2019

Raman response in the nematic phase of FeSe

Raman experiments on bulk FeSe revealed that the low-frequency part of $B_{1g}$ Raman response $R_{B_{1g}}$, which probes nematic fluctuations, rapidly decreases below the nematic transition at $T_n \sim 85$K. Such behavior is usually associated with the gap opening and at a first glance is inconsistent with the fact that FeSe remains a metal below $T_n$, with sizable hole and electron pockets. We argue that the drop of $R_{B_{1g}}$ in a nematic metal comes about because the nematic order drastically changes the orbital content of the pockets and makes them nearly mono-orbital. In this situation $B_{1g}$ Raman response gets reduced by the same vertex corrections that enforce charge conservation. The reduction holds at low frequencies and gives rise to gap-like behavior of $R_{B_{1g}}$, in full agreement with the experimental data.

cond-mat.str-el↗

arXiv2019

Anisotropy of the DC conductivity due to orbital-selective spin fluctuations in the nematic phase of iron superconductors

We study the dc conductivity of iron-based superconductors within the orbital-selective spin fluctuation scenario. Within this approach, the anisotropy of spin fluctuations below the spin-nematic transition at T$_S$ is also responsible for the orbital ordering, induced by nematic self-energy corrections to the quasiparticle dispersion. As a consequence, the anisotropy of the dc conductivity below T$_S$ is determined not only by the anisotropy of the scattering rates as expected within a spin-nematic scenario, but also by the modification of the Fermi velocity due to the orbital reconstruction. More interestingly, it turns out that these two effects contribute to the dc-conductivity anisotropy with opposite signs. By using realistic band-structure parameters we compute the conductivity anisotropy for both 122 and FeSe compounds, discussing the possible origin of the different dc-conductivity anisotropy observed experimentally in these two families of iron-based superconductors.

cond-mat.supr-con↗

arXiv2019

Giant Effective charges and Piezoelectricity in Gapped Graphene

Since the first realization of reversible charge doping in graphene via field-effect devices, it has become evident how the induction a gap could further enhance its potential for technological applications. Here we show that the gap opening due to a sublattice symmetry breaking has also a profound impact on the polar response of graphene. By combining ab-initio calculations and analytical modelling we show that for realistic band-gap values ($Δ\lesssim 0.5$ eV) the piezoelectric coefficient and the Born effective charge of graphene attain a giant value, independent on the gap. In particular the piezoelectric coefficient per layer of gapped mono- and bilayer graphene is three times larger than that of a large-gap full polar insulator as hexagonal Boron Nitride (h-BN) monolayer, and 30\% larger than that of a polar semiconductor as MoS$_2$. This surprising result indicates that piezoelectric acoustic-phonons scattering can be relevant to model charge transport and charge-carrier relaxation in gated bilayer graphene. The independence of the piezoelectric coefficient and of the Born effective charge on the gap value follows from the connection between the polar response and the valley Chern number of gapped Dirac electrons, made possible by the effective gauge-field description of the electron-lattice/strain coupling in these systems. In the small gap limit, where the adiabatic ab-initio approximation fails, we implement analytically the calculation of the dynamical effective charge, and we establish a universal relation between the complex effective charge and the so-called Fano profile of the phonon optical peak. Our results provide a general theoretical framework to understand and compute the polar response in narrow-gap semiconductors, but may also be relevant for the contribution of piezoelectric scattering to the transport properties in Dirac-like systems.

cond-mat.mtrl-sci↗

arXiv2018

Disordered XY model: effective medium theory and beyond

We study the effect of uncorrelated random disorder on the temperature dependence of the superfluid stiffness in the two-dimensional classical XY model. By means of a perturbative expansion in the disorder potential, equivalent to the T-matrix approximation, we provide an extension of the effective-medium-theory result able to describe the low-temperature stiffness, and its separate diamagnetic and paramagnetic contributions. These analytical results provide an excellent description of the Monte Carlo simulations for two prototype examples of uncorrelated disorder. Our findings offer an interesting perspective on the effects of quenched disorder on longitudinal phase fluctuations in two-dimensional superfluid systems.

cond-mat.supr-con↗

arXiv2018

Melting of the vortex lattice through intermediate hexatic fluid in a-MoGe thin film

The hexatic fluid refers to a phase in between a solid and a liquid which has short range positional order but quasi-long range orientational order. In the celebrated theory of Berezinskii, Kosterlitz and Thouless and subsequently refined by Halperin, Nelson and Young, it was predicted that a 2-dimensional hexagonal solid can melt in two steps: first, through a transformation from a solid to a hexatic fluid which retains quasi long range orientational order and then from a hexatic fluid to an isotropic liquid. In this paper, using a combination of real space imaging and transport measurements we show that the 2-dimensional vortex lattice in a-MoGe thin film follows this sequence of melting as the magnetic field is increased. Identifying the signatures of various transitions on the bulk transport properties of the superconductor, we construct a vortex phase diagram for a two dimensional superconductor.

cond-mat.supr-con↗

arXiv2018

Orbital mismatch boosting nematic instability in iron-based superconductors

We derive the effective action for the collective spin modes in iron-based superconductors. We show that, due to the orbital-selective nature of spin fluctuations, the magnetic and nematic instabilities are controlled by the degrees of orbital nesting between electron and hole pockets. Within a prototypical three-pockets model the hole-electron orbital mismatch is found to boost spin-nematic order. This explains the enhancement of the nematic order in FeSe as compared to 122 compounds, and its suppression under pressure, where the emergence of the second hole pocket compensates the orbital mismatch of the three-pockets configuration.

cond-mat.supr-con↗

arXiv2018

BKT universality class in the presence of correlated disorder

The correct detection of the Berezinskii-Kosterlitz-Thouless (BKT) transition in quasi-two-dimensional superconductors still remains a controversial issue. Its main signatures, indeed, are often at odds with the theoretical expectations. In a recent work\cite{me} we have shown that the presence of spatially correlated disorder plays a key role in this sense being it the reason underlying the experimentally-observed smearing of the universal superfluid-density jump. In the present paper, we closely investigate the effects of correlated disorder on the BKT transition, addressing specifically the issue whether it changes or not the BKT universality class.

cond-mat.supr-con↗