SearcharxivSearch

arXiv subjects

Larry Aagesen

Publications and source records attributed to Larry Aagesen.

2 recordsLinked to original sources

Development of a Model for Irradiation-Assisted Grain Growth for Nanocrystalline UO2

In this work, we have developed a model for irradiation-assisted grain growth in nanocrystalline UO$_2$ using the MARMOT code. We include the impact of irradiation on UO$_2$ grain growth by coupling a phase field grain growth model with a heat conduction simulation that features a random heat source representing thermal spikes. Our model parameters have been calibrated against experimental measurements at 300 K. The calibrated model predicts grain growth in an irradiated UO$_2$ thin film that compares well with experimental data at 50 K. These results suggest that thermal spikes are the major cause of the irradiation-assisted grain growth observed in the UO$_2$ experiments. They also indicate that irradiation-assisted grain growth is only significant with average grain sizes less than 35 nm, and thus can be neglected when considering fuel performance of typical UO$_2$ fuel pellets.

cond-mat.mtrl-sci

Impact of grain boundary and surface diffusion on predicted fission gas bubble behavior and release in UO$_2$ fuel

In this work, we quantify the impact of grain boundary (GB) and surface diffusion on fission gas bubble evolution and fission gas release in UO$_2$ nuclear fuel using simulations with a hybrid phase field/cluster dynamics model. We begin with a comprehensive literature review of uranium vacancy and xenon atom diffusivity in UO$_2$ through the bulk, along GBs, and along surfaces. In our model we represent fast GB and surface diffusion using a heterogeneous diffusivity that is a function of the order parameters that represent bubbles and grains. We find that the GB diffusivity directly impacts the rate of gas release via GB transport, and that the GB diffusivity is likely below 10$^4$ times the lower value from Olander and van Uffelen (2001). We also find that the surface diffusivity impacts bubble coalescence and mobility, and that the bubble surface diffusivity is likely below $10^{-4}$ times the value from Zhou and Olander (1984).

physics.comp-ph