arXiv subjects

Lars Bojer Madsen

Publications and source records attributed to Lars Bojer Madsen.

104 records · Page 6Linked to original sources

arXiv2006

Symmetry of carrier-envelope phase difference effects in strong-field, few-cycle ionization of atoms and molecules

In few-cycle pulses, the exact value of the carrier-envelope phase difference (CEPD) has a pronounced influence on the ionization dynamics of atoms and molecules. We show that for atoms in circularly polarized light, a change in the CEPD is mapped uniquely to an overall rotation of the system, and results for arbitrary CEPD are obtained by rotation of the results from a single calculation with fixed CEPD. For molecules this is true only for linear molecules aligned parallel with the propagation direction of the field. The effects of CEPD are classified as geometric or non-geometric. The observations are exemplified by strong-field calculations on hydrogen.

physics.atom-ph↗

arXiv2006

High-harmonic generation from arbitrarily oriented diatomic molecules including nuclear motion and field-free alignment

We present a theoretical model of high-harmonic generation from diatomic molecules. The theory includes effects of alignment as well as nuclear motion and is used to predict results for N$_2$, O$_2$, H$_2$ and D$_2$. The results show that the alignment dependence of high-harmonics is governed by the symmetry of the highest occupied molecular orbital and that the inclusion of the nuclear motion in the theoretical description generally reduces the intensity of the harmonic radiation. We compare our model with experimental results on N$_2$ and O$_2$, and obtain very good agreement.

physics.atom-ph↗

arXiv2006

Strong-field ionization of atoms and molecules: The two-term saddle point method

We derive an analytical formula for the ionization rate of neutral atoms and molecules in a strong monochromatic field. Our model is based on the strong-field approximation with transition amplitudes calculated by an extended saddle point method. We show that the present two-term saddle point method reproduces even complicated structures in angular resolved photo electron spectra.

physics.atom-ph↗

arXiv2006

Entanglement between remote continuous variable quantum systems: effects of transmission loss

We study the effects of losses on the entanglement created between two separate atomic gases by optical probing and homodyne detection of the transmitted light. The system is well-described in the Gaussian state formulation. Analytical results quantifying the degree of entanglement between the two gases are derived and compared with the entanglement in a pair of light pulses generated by an EPR source. For low (high) transmission losses the highest degree of entanglement is obtained by probing with squeezed (antisqueezed) light. In an asymmetric setup where light is only sent one way through the atomic samples, we find that the logarithmic negativity of entanglement attains a constant value $-\log_2(N)$ with $N=1/3$ irrespectively of the loss along the transmission line.

quant-ph↗

arXiv2006

Fidelities for transformations of unknown quantum states

We present a general theoretical formalism to compute the fidelity of transformations of unknown quantum states. We then focus on the case of Gaussian transformations of continuous variable quantum systems, where, for the case of a Gaussian distribution of displaced coherent states, the theory is readily tractable by a covariance matrix formalism. We present analytical results for recently implemented teleportation and memory storage protocols for continuous variables.

quant-ph↗

arXiv2006

Molecular orbitals and strong-field approximation

V.I. Usachenko and S.-I. Chu [Phys. Rev. A {\bf 71}, 063410 (2005)] discuss the molecular strong-field approximation in the velocity gauge formulation and indicate that some of our earlier velocity gauge calculations are inaccurate. Here we comment on the results of Usachenko and Chu. First, we show that the molecular orbitals used by Usachenko and Chu do not have the correct symmetry, and second, that it is an oversimplification to describe the molecular orbitals in terms of just a single linear combination of two atomic orbitals. Finally, some values for the generalized Bessel function are given for comparison.

physics.atom-ph↗

arXiv2005

Vibrational excitation of diatomic molecular ions in strong-field ionization of diatomic molecules

A model based on the strong-field and Born-Oppenheimer approximations qualitatively describes the distribution over vibrational states formed in a diatomic molecular ion following ionization of the neutral molecule by intense laser pulses. Good agreement is found with a recent experiment [X. Urbain et al., Phys. Rev. Lett. 92, 163004 (2004)]. In particular, the observed deviation from a Franck-Condon-like distribution is reproduced. Additionally, we demonstrate control of the vibrational distribution by a variation of the peak intensity or a change of frequency of the laser pulse.

physics.atom-ph↗

arXiv2005

Gaussian State Description of Squeezed Light

We present a Gaussian state description of squeezed light generated in an optical parametric oscillator. Using the Gaussian state description we describe the dynamics of the system conditioned on homodyne detection on the output field. Our theory shows that the output field is squeezed only if observed for long enough times or by a detector with finite bandwidth. As an application of the present approach we consider the use of finite bandwidth squeezed light together with a sample of spin-polarized atoms to estimate a magnetic field.

quant-ph↗

arXiv2005

Pyramidal Atoms: Berylliumlike Hollow States

Based on the idea that four excited electrons arrange themselves around the nucleus in the corners of a pyramid in order to minimize their mutual repulsion, we present an analytical model of quadruply excited states. The model shows excellent comparison with ab initio results and provides a clear physical picture of the intrinsic motion of the four electrons. The model is used to predict configuration-mixing fractions and spectra of these highly correlated states.

physics.atom-ph↗

arXiv2005

Strong-field ionization of diatomic molecules and companion atoms: strong-field approximation and tunneling theory including nuclear motion

We present a detailed comparison of strong-field ionization of diatomic molecules and their companion atoms with nearly equal ionization potentials. We perform calculations in the length and velocity gauge formulations of the molecular strong-field approximation and with the molecular tunneling theory, and in both cases we consider effects of nuclear motion. A comparison of our results with experimental data shows that the length gauge strong-field approximation gives the most reliable predictions.

physics.atom-ph↗

arXiv2004

Influence of molecular symmetry on strong-field ionization: Studies on ethylene, benzene, fluorobenzene, and chlorofluorobenzene

Using the molecular strong-field approximation we consider the effects of molecular symmetry on the ionization of molecules by a strong, linearly polarized laser pulse. Electron angular distributions and total ionization yields are calculated as a function of the relative orientation between the molecule and the laser polarization. Our studies focus on ethylene (C$_2$H$_4$), benzene (C$_6$H$_6$), fluorobenzene (C$_6$H$_5$F), and ortho chlorofluorobenzene (1,2 C$_6$H$_4$ClF), the molecules representing four different point groups. The results are compared with experiments, when available, and with the molecular tunneling theory appropriately extended to non-linear polyatomic molecules. Our investigations show that the orientational dependence of ionization yields is primarily determined by the nodal surface structure of the molecular orbitals.

physics.atom-ph↗

arXiv2004

Magnetometry with entangled atomic samples

We present a theory for the estimation of a scalar or a vector magnetic field by its influence on an ensemble of trapped spin polarized atoms. The atoms interact off-resonantly with a continuous laser field, and the measurement of the polarization rotation of the probe light, induced by the dispersive atom-light coupling, leads to spin-squeezing of the atomic sample which enables an estimate of the magnetic field which is more precise than that expected from standard counting statistics. For polarized light and polarized atoms, a description of the non-classical components of the collective spin angular momentum for the atoms and the collective Stokes vectors of the light-field in terms of effective gaussian position and momentum variables is practically exact. The gaussian formalism describes the dynamics of the system very effectively and accounts explicitly for the back-action on the atoms due to measurement and for the estimate of the magnetic field. Multi-component magnetic fields are estimated by the measurement of suitably chosen atomic observables and precision and efficiency is gained by dividing the atomic gas in two or more samples which are entangled by the dispersive atom-light interaction.

quant-ph↗

arXiv2004

Spin squeezing and precision probing with light and samples of atoms in the gaussian approximation

We consider an ensemble of trapped atoms interacting with a continuous wave laser field. For sufficiently polarized atoms and for a polarized light field, we may approximate the non-classical components of the collective spin angular momentum operator for the atoms and the Stokes vectors of the field by effective position and momentum variables for which we assume a gaussian state. Within this approximation, we present a theory for the squeezing of the atomic spin by polarization rotation measurements on the probe light. We derive analytical expressions for the squeezing with and without inclusion of the noise effects introduced by atomic decay and by photon absorption. The theory is readily adapted to the case of inhomogeneous light-atom coupling [A. Kuzmich and T.A.B. Kennedy, Phys. Rev. Lett. Vol. 92, 030407 (2004)]. As a special case, we show how to formulate the theory for an optically thick sample by slicing the gas into pieces each having only small photon absorption probability. Our analysis of a realistic probing and measurement scheme shows that it is the maximally squeezed component of the atomic gas that determines the accuracy of the measurement.

quant-ph↗

arXiv2004

Estimation of a classical parameter with gaussian probes: magnetometry with collective atomic spins

We present a theory for the estimation of a classical magnetic field by an atomic sample with a gaussian distribution of collective spin components. By incorporating the magnetic field and the probing laser field as quantum variables with gaussian distributions on equal footing with the atoms, we obtain a very versatile description which is readily adapted to include probing with squeezed light, dissipation and loss and additional measurement capabilities on the atomic system.

quant-ph↗