arXiv subjects

Lars S. Madsen

Publications and source records attributed to Lars S. Madsen.

17 recordsLinked to original sources

arXiv2026

Practical Limits on Integrated Squeezers

Recent experiments have demonstrated the successful generation and detection of moderately squeezed vacuum states with integrated photonics. However, in order to benefit from the reduced noise of highly squeezed light, many different noise sources must be mitigated. Here, we quantify the fundamental limits these noise sources impose on squeezing measurements and find surprising generality across different platforms and designs. We combine these different limitations into a simple model that provides practical guidance for the design and benchmarking of next-generation integrated squeezed-light systems.

quant-ph↗

arXiv2021

Dynamic polarizability of macromolecules for single-molecule optical biosensing

The structural dynamics of macromolecules is important for most microbiological processes, from protein folding to the origins of neurodegenerative disorders. Noninvasive measurements of these dynamics are highly challenging. Recently, optical sensors have been shown to allow noninvasive time-resolved measurements of the dynamic polarizability of single-molecules. Here we introduce a method to efficiently predict the dynamic polarizability from the atomic configuration of a given macromolecule. This provides a means to connect the measured dynamic polarizability to the underlying structure of the molecule, and therefore to connect temporal measurements to structural dynamics. To illustrate the methodology we calculate the change in polarizability as a function of time based on conformations extracted from molecular dynamics simulations and using different conformations of motor proteins solved crystalographically. This allows us to quantify the magnitude of the changes in polarizablity due to thermal and functional motions.

physics.bio-ph↗

arXiv2020

Quantum correlations overcome the photodamage limits of light microscopy

State-of-the-art microscopes use intense lasers that can severely disturb biological processes, function and viability. This introduces hard limits on performance that only quantum photon correlations can overcome. Here we demonstrate this absolute quantum advantage, achieving signal-to-noise beyond the photodamage-free capacity of conventional microscopy. We achieve this in a coherent Raman microscope, which we use to image molecular bonds within a cell with both quantum-enhanced contrast and sub-wavelength resolution. This allows the observation of nanoscale biological structures that would otherwise not be resolved. Coherent Raman microscopes allow highly selective biomolecular finger-printing in unlabelled specimens, but photodamage is a major roadblock for many applications. By showing that this roadblock can be overcome, our work provides a path towards order-of-magnitude improvements in both sensitivity and imaging speed.

physics.optics↗

arXiv2020

Ultrafast viscosity measurement with ballistic optical tweezers

Viscosity is an important property of out-of-equilibrium systems such as active biological materials and driven non-Newtonian fluids, and for fields ranging from biomaterials to geology, energy technologies and medicine. However, noninvasive viscosity measurements typically require integration times of seconds. Here we demonstrate a four orders-of-magnitude improvement in speed, down to twenty microseconds, with uncertainty dominated by fundamental thermal noise for the first time. We achieve this using the instantaneous velocity of a trapped particle in an optical tweezer. To resolve the instantaneous velocity we develop a structured-light detection system that allows particle tracking with megahertz bandwidths. Our results translate viscosity from a static averaged property, to one that may be dynamically tracked on the timescales of active dynamics. This opens a pathway to new discoveries in out-of-equilibrium systems, from the fast dynamics of phase transitions, to energy dissipation in motor molecule stepping, to violations of fluctuation laws of equilibrium thermodynamics.

cond-mat.soft↗

arXiv2020

A Quantum Heat Machine from Fast Optomechanics

We consider a thermodynamic machine in which the working fluid is a quantized harmonic oscillator that is controlled on timescales that are much faster than the oscillator period. We find that operation in this `fast' regime allows access to a range of quantum thermodynamical behaviors that are otherwise inaccessible, including heat engine and refrigeration modes of operation, quantum squeezing, and transient cooling to temperatures below that of the cold bath. The machine involves rapid periodic squeezing operations and could potentially be constructed using pulsed optomechanical interactions. The prediction of rich behavior in the fast regime opens up new possibilities for quantum optomechanical machines and quantum thermodynamics.

quant-ph↗

arXiv2019

The sounds of science: a symphony for many instruments and voices

This paper is a celebration of the frontiers of science. Goodenough, the maestro who transformed energy usage and technology through the invention of the lithium ion battery, opens the programme, reflecting on the ultimate limits of battery technology. This applied theme continues through the subsequent pieces on energy related topics (the sodium ion battery and artificial fuels, by Mansson) and the ultimate challenge for 3 dimensional printing the eventual production of life, by Atala. A passage by Alexander follows, reflecting on a related issue: How might an artificially produced human being behave? Next comes a consideration of consiousness and free will by Allen and Lidstrom. Further voices and new instruments enter as Bowen, Mauranyapin and Madsen discuss whether dynamical processes of single molecules might be observed in their native state. The exploitation of chaos in science and technology, applications of Bose Einstein condensates and a consideration of the significance of entropy follow in pieces by Reichl, Rasel and Allen, respectively. Katsnelson and Koonin then discuss the potential generalisation of thermodynamic concepts in the context of biological evolution. Entering with the music of the cosmos, Yasskin discusses whether we might be able to observe torsion in the geometry of the universe. The crescendo comes with the crisis of singularities, their nature and whether they can be resolved through quantum effects, in the composition of Coley. The climax is Krenn, Melvin and Zeilinger consideration of how computer code can be autonomously surprising and creative. In a harmonious counterpoint, Yampolskiy concludes that such code is not yet able to take responsibility for coauthoring a paper.

physics.pop-ph↗

arXiv2019

Quantum noise limited nanoparticle detection with exposed-core fiber

Label-free biosensors are important tools for clinical diagnostics and for studying biology at the single molecule level. The development of optical label-free sensors has allowed extreme sensitivity, but can expose the biological sample to photodamage. Moreover, the fragility and complexity of these sensors can be prohibitive to applications. To overcome these problems, we develop a quantum noise limited exposed-core fiber sensor providing robust platform for label-free biosensing with a natural path toward microfluidic integration. We demonstrate the detection of single nanoparticles down to 25 nm in radius with optical intensities beneath known biophysical damage thresholds.

quant-ph↗

arXiv2018

Complete elimination of information leakage in continuous-variable quantum communication channels

In all lossy communication channels realized to date, information is inevitably leaked to a potential eavesdropper. Here we present a communication protocol that does not allow for any information leakage to a potential eavesdropper in a purely lossy channel. By encoding information into a restricted Gaussian alphabet of squeezed states we show, both theoretically and experimentally, that the Holevo information between the eavesdropper and the intended recipient can be exactly zero in a purely lossy channel while minimized in a noisy channel. This result is of fundamental interest, but might also have practical implications in extending the distance of secure quantum key distribution.

quant-ph↗

arXiv2018

Quantum enhanced optomechanical magnetometry

The resonant enhancement of both mechanical and optical response in microcavity optomechanical devices allows exquisitely sensitive measurements of stimuli such as acceleration, mass and magnetic fields. In this work, we show that quantum correlated light can improve the performance of such sensors, increasing both their sensitivity and their bandwidth. Specifically, we develop a silicon-chip based cavity optomechanical magnetometer that incorporates phase squeezed light to suppress optical shot noise. At frequencies where shot noise is the dominant noise source this allows a 20% improvement in magnetic field sensitivity. Furthermore, squeezed light broadens the range of frequencies at which thermal noise dominates, which has the effect of increasing the overall sensor bandwidth by 50%. These proof-of-principle results open the door to apply quantum correlated light more broadly in chip-scale sensors and devices.

physics.optics↗

arXiv2018

Deterministic phase measurements exhibiting super-sensitivity and super-resolution

Phase super-sensitivity is obtained when the sensitivity in a phase measurement goes beyond the quantum shot noise limit, whereas super-resolution is obtained when the interference fringes in an interferometer are narrower than half the input wavelength. Here we show experimentally that these two features can be simultaneously achieved using a relatively simple setup based on Gaussian states and homodyne measurement. Using 430 photons shared between a coherent- and a squeezed vacuum state, we demonstrate a 22-fold improvement in the phase resolution while we observe a 1.7-fold improvement in the sensitivity. In contrast to previous demonstrations of super-resolution and super-sensitivity, this approach is fully deterministic.

quant-ph↗

arXiv2016

Non-destructive profilometry of optical nanofibres

Single-mode optical nanofibres are a central component of a broad range of applications and emerging technologies. Their fabrication has been extensively studied over the past decade, but imaging of the final sub-micrometre products has been restricted to destructive or low-precision techniques. Here we demonstrate an optical scattering-based scanning method that uses a probe nanofibre to locally scatter the evanescent field of a sample nanofibre. The method does not damage the sample nanofibre and is easily implemented only using the same equipment as in a standard fibre puller setup. We demonstrate sub-nanometre radial resolution at video rates (0.7 nm in 10 ms) on single mode nanofibres, allowing for a complete high-precision profile to be obtained within minutes of fabrication. The method thus enables non-destructive, fast and precise characterisation of optical nanofibers, with applications ranging from optical sensors and cold atom traps to non-linear optics.

physics.optics↗

arXiv2016

A Quantum Optomechanical Interface Beyond the Resolved Sideband Limit

Mechanical oscillators which respond to radiation pressure are a promising means of transferring quantum information between light and matter. Optical--mechanical state swaps are a key operation in this setting. Existing proposals for optomechanical state swap interfaces are only effective in the resolved sideband limit. Here, we show that it is possible to fully and deterministically exchange mechanical and optical states outside of this limit, in the common case that the cavity linewidth is larger than the mechanical resonance frequency. This high-bandwidth interface opens up a significantly larger region of optomechanical parameter space, allowing generation of non-classical motional states of high-quality, low-frequency mechanical oscillators.

quant-ph↗

arXiv2014

Coherent control and feedback cooling in a remotely-coupled hybrid atom-optomechanical system

Cooling to the motional ground state is an important first step in the preparation of nonclassical states of mesoscopic mechanical oscillators. Light-mediated coupling to a remote atomic ensemble has been proposed as a method to reach the ground state for low frequency oscillators. The ground state can also be reached using optical measurement followed by feedback control. Here we investigate the possibility of enhanced cooling by combining these two approaches. The combination, in general, outperforms either individual technique, though atomic ensemble-based cooling and feedback cooling each individually dominate over large regions of parameter space.

quant-ph↗

arXiv2013

Gaussian error correction of quantum states in a correlated noisy channel

Noise is the main obstacle for the realization of fault tolerant quantum information processing and secure communication over long distances. In this work, we propose a communication protocol relying on simple linear optics that optimally protects quantum states from non-Markovian or corre- lated noise. We implement the protocol experimentally and demonstrate the near ideal protection of coherent and entangled states in an extremely noisy channel. Since all real-life channels are exhibit- ing pronounced non-Markovian behavior, the proposed protocol will have immediate implications in improving the performance of various quantum information protocols.

quant-ph↗

arXiv2013

Quantum-enhanced micro-mechanical displacement sensitivity

We report on a hitherto unexplored application of squeezed light: for quantum-enhancement of mechanical transduction sensitivity in microcavity optomechanics. Using a toroidal silica microcavity, we experimentally demonstrate measurement of the transduced phase modulation signal with a sensitivity $-0.72(\pm 0.01)$\,dB below the shot noise level. This is achieved for resonant probing in the highly under-coupled regime, by preparing the probe in a weak coherent state with phase squeezed vacuum states at sideband frequencies.

quant-ph↗

arXiv2012

Continuous variable quantum key distribution with two-mode squeezed states

Quantum key distribution (QKD) enables two remote parties to grow a shared key which they can use for unconditionally secure communication [1]. The applicable distance of a QKD protocol depends on the loss and the excess noise of the connecting quantum channel [2-10]. Several QKD schemes based on coherent states and continuous variable (CV) measurements are resilient to high loss in the channel, but strongly affected by small amounts of channel excess noise [2-6]. Here we propose and experimentally address a CV QKD protocol which uses fragile squeezed states combined with a large coherent modulation to greatly enhance the robustness to channel noise. As a proof of principle we experimentally demonstrate that the resulting QKD protocol can tolerate more noise than the benchmark set by the ideal CV coherent state protocol. Our scheme represents a very promising avenue for extending the distance for which secure communication is possible.

quant-ph↗

arXiv2012

Experimental Investigation of the Evolution of Gaussian Quantum Discord in an Open System

Gaussian quantum discord is a measure of quantum correlations in Gaussian systems. Using Gaussian discord we quantify the quantum correlations of a bipartite entangled state and a separable two-mode mixture of coherent states. We experimentally analyze the effect of noise addition and dissipation on Gaussian discord and show that the former noise degrades the discord while the latter noise for some states leads to an increase of the discord. In particular, we experimentally demonstrate the near-death of discord by noisy evolution and its revival through dissipation.

quant-ph↗