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Lasse Gresista

Publications and source records attributed to Lasse Gresista.

9 recordsLinked to original sources

Quantum Coulomb Liquids of Different Rank in the Breathing Pyrochlore Antiferromagnet

Emergent gauge fields and Coulomb liquids have long been central to the physics of frustrated pyrochlore magnets, yet their realization beyond conventional, i.e. rank-1 $U(1)$, spin ice and into fully quantum higher-rank regimes has remained elusive. Here we provide a controlled demonstration of this physics in the spin-$\tfrac{1}{2}$ quantum Heisenberg antiferromagnet on the breathing pyrochlore lattice with symmetry-allowed Dzyaloshinskii--Moriya interactions, using the pseudofermion functional renormalization group. We show that tuning the breathing asymmetry stabilizes extended quantum analogues of both rank-1 and rank-2 $U(1)$ Coulomb liquids within a single microscopic model, directly distinguished by their characteristic pinch-point morphologies in momentum space. This provides the first controlled quantum realization in three dimensions where gauge theories of different rank emerge within a single microscopic spin Hamiltonian. In addition, quantum fluctuations qualitatively reshape the classical nearest-neighbor atlas of phases, causing an incommensurate spiral instability and an extended quantum-disordered regime without dipolar order, both absent from the classical model. Our results establish the breathing pyrochlore as a timely and experimentally relevant platform where higher-rank gauge constraints, conventional magnetic order, and fluctuation-driven quantum phases compete on equal footing, opening a direct route to diagnosing emergent gauge structure in three-dimensional quantum magnets.

cond-mat.str-el

Unconventional orders in the maple-leaf ferro-antiferromagnetic Heisenberg model

Motivated by the search for unconventional orders in frustrated quantum magnets, we present a multi-method investigation into the nature of the quantum phase diagram of the spin-$1/2$ Heisenberg model on the maple-leaf lattice with three symmetry-inequivalent nearest-neighbor interactions. It has been argued that the parameter regime with antiferromagnetic couplings on hexagons $J_h$ and ferromagnetic couplings on triangles $J_t$ and dimer $J_d$ bonds, is potentially host to a cornucopia of emergent phases with unconventional orders. Our analysis indeed identifies an extended region where any conventional dipolar magnetic order is absent. A hexagonal singlet state is found in the region around $J_{d}=J_{t}=0$, while a dimerized hexagonal singlet order of a lattice nematic character appears proximate to the phase boundary with the c$120^\circ$ antiferromagnetic order. Interestingly, upon traversing the bulk of the paramagnetic (PM) region, we find a variety of distinct correlation profiles, which are qualitatively different from those of the hexagonal singlet and dimerized hexagonal singlet orders but feature no appreciable spin-nematic response, while the boundary with the ferromagnetic phase shows evidence of spin-nematic order. This PM region is thus likely host to an ensemble of nonmagnetic phases which could putatively include quantum spin liquids. Our phase diagram is built from a complementary application of state-of-the-art implementations of the cluster mean-field and pseudo-fermion functional renormalization group approaches, together with an unconstrained Luttinger-Tisza treatment of the model providing insights from the semi-classical limit.

cond-mat.str-el

Quantum effects on pyrochlore higher-rank U(1) spin liquids: Pinch-line singularities, spin nematics, and connections to oxide materials

Motivated by the magnetism of pyrochlore oxides, we consider the effect of quantum fluctuations in the most general symmetry-allowed nearest-neighbor Kramers exchange Hamiltonian on the pyrochlore lattice. At the classical level, this Hamiltonian exhibits a rich landscape of classical spin liquids and a variety of nonconventional magnetic phases. In contrast, much remains unclear for the quantum model, where quantum fluctuations have the potential to alter the classical landscape and stabilize novel magnetic phases. Employing state-of-the-art pseudo-fermion functional renormalization group calculations for the spin-$1/2$ model, we determine the quantum phase diagram at relevant cross-sections, where the classical model hosts an algebraic nodal rank-2 spin liquid and a spin nematic order. We find large regions in parameter space on which dipolar magnetic order is absent and, based on known fingerprints in the correlation functions, we suggest that this nonconventional region is composed of an ensemble of distinct phases stabilized by quantum fluctuations. Our results hint at the existence of a spin nematic phase, and we identify the quantum analog of the classical rank-2 spin liquid. Furthermore, we highlight the importance of assessing the subtle interplay of quantum and thermal fluctuations in reconciling the experimental findings on the nature of magnetic order in Yb$_2$Ti$_2$O$_7$.

cond-mat.str-el

Noncoplanar orders and quantum disordered states in maple-leaf (anti)ferromagnets

A promising route towards the realization of chiral spin liquids is the quantum melting of classically noncoplanar spin states via quantum fluctuations. In the classical realm, such noncoplanar orders can effectively be stabilized by interactions beyond nearest neighbors. Motivated by the recent synthesis of materials with a maple-leaf lattice geometry, we study the effect of cross-plaquette couplings on elementary Heisenberg antiferromagnets for this geometry (as well as their ferromagnetic counterparts). We find a rich spectrum of noncoplanar states, including a novel icosahedral order as well as incommensurate spin spirals, using large-scale Monte Carlo simulations in combination with a semi-analytical analysis. To inspect the potential quantum melting of these states, we analyze the quantum $S = 1/2$ variant of these models using pseudo-fermion functional renormalization group (pf-FRG) simulations. Notably, we indeed find extended parameter regimes lacking long-range magnetic order -- in regions classically occupied by noncoplanar orders -- which we putatively identify with the possible formation of chiral quantum spin liquids.

cond-mat.str-el

Candidate quantum disordered intermediate phase in the Heisenberg antiferromagnet on the maple-leaf lattice

Quantum antiferromagnets on geometrically frustrated lattices have long attracted interest for the formation of quantum disordered states and the possible emergence of quantum spin liquid (QSL) ground states. Here we turn to the nearest-neighbor spin-$1/2$ Heisenberg antiferromagnet on the maple-leaf lattice, which is known to relieve frustration by the formation of canted $120^{\circ}$ magnetic order or valence bond crystal order when varying the bond anisotropy. Employing a pseudo-fermion functional renormalization group approach to assess its ground state phase diagram in detail, we present evidence for a QSL regime sandwiched between these two limiting phases. The formation of such a QSL might signal proximity to a possible deconfined quantum critical point from which it emerges, and that is potentially accessible by tuning the exchange couplings. Our conclusions are based on large-scale simulations involving a careful finite-size scaling analysis of the behavior of magnetic susceptibility and spin-spin correlation functions under renormalization group flow.

cond-mat.str-el

Spin-valley magnetism on the triangular moiré lattice with SU(4) breaking interactions

The discovery of correlated insulating states in moiré heterostructures has renewed the interest in strongly-coupled electron systems where spin and valley (or layer) degrees of freedom are intertwined. In the strong-coupling limit, such systems can be effectively described by SU(4) spin-valley models akin to Kugel-Khomskii models long studied in the context of spin-orbit coupled materials. However, typical moiré heterostructures also exhibit interactions that break the SU(4) symmetry down to SU(2)${}_{\mathrm{spin}}\otimes$U(1)${}_{\mathrm{valley}}$. Here we investigate the impact of such symmetry-breaking couplings on the magnetic phase diagram for triangular superlattices considering a filling of two electrons (or holes) per moiré unit cell. We explore a broad regime of couplings -- including XXZ anisotropies, Dzyaloshinskii-Moriya exchange and on-site Hund's couplings -- using semi-classical Monte Carlo simulations. We find a multitude of classically ordered phases, including (anti-)ferromagnetic, incommensurate, and stripe order, manifesting in different sectors of the spin-valley model's parameter space. Zooming in on the regimes where quantum fluctuations are likely to have an effect, we employ pseudo-fermion functional renormalization group (pf-FRG) calculations to resolve quantum disordered ground states such as spin-valley liquids, which we indeed find for certain parameter regimes. As a concrete example, we discuss the case of trilayer graphene aligned with hexagonal boron nitride using material-specific parameters.

cond-mat.str-el

Network of chiral one-dimensional channels and localized states emerging in a moiré system

Moiré systems provide a highly tunable platform for engineering band structures and exotic correlated phases. Here, we theoretically study a model for a single layer of graphene subject to a smooth moiré electrostatic potential, induced by an insulating substrate layer. For sufficiently large moiré unit cells, we find that ultra-flat bands coexist with a triangular network of chiral one-dimensional (1D) channels. These channels mediate an effective interaction between localized modes with spin-, orbital- and valley degrees of freedom emerging from the flat bands. The form of the interaction reflects the chiralilty and 1D nature of the network. We study this interacting model within an $SU(4)$ mean-field theory, semi-classical Monte-Carlo simulations, and an $SU(4)$ spin-wave theory, focusing on commensurate order stabilized by local two-site and chiral three-site interactions. By tuning a gate voltage, one can trigger a non-coplanar phase characterized by a peculiar coexistence of three different types of order: ferromagnetic spin order in one valley, non-coplanar chiral spin order in the other valley, and 120$^\circ$ order in the remaining spin and valley-mixed degrees of freedom. Quantum and classical fluctuations have qualitatively different effects on the observed phases and can, for example, create a finite spin-chirality purely via fluctuation effects.

cond-mat.str-el

Moments and multiplets in moiré materials: A pseudo-fermion functional renormalization group for spin-valley models

The observation of strongly-correlated states in moiré systems has renewed the conceptual interest in magnetic systems with higher SU(4) spin symmetry, e.g. to describe Mott insulators where the local moments are coupled spin-valley degrees of freedom. Here, we discuss a numerical renormalization group scheme to explore the formation of spin-valley ordered and unconventional spin-valley liquid states at zero temperature based on a pseudo-fermion representation. Our generalization of the conventional pseudo-fermion functional renormalization group approach for $\mathfrak{su}$(2) spins is capable of treating diagonal and off-diagonal couplings of generic spin-valley exchange Hamiltonians in the self-conjugate representation of the $\mathfrak{su}$(4) algebra. To achieve proper numerical efficiency, we derive a number of symmetry constraints on the flow equations that significantly limit the number of ordinary differential equations to be solved. As an example system, we investigate a diagonal SU(2)$_{\textrm{spin}}$ $\otimes$ U(1)$_{\textrm{valley}}$ model on the triangular lattice which exhibits a rich phase diagram of spin and valley ordered phases.

cond-mat.str-el

Dimensional crossover for universal scaling far from equilibrium

We perform a dynamical finite-size scaling analysis of a nonequilibrium Bose gas which is confined in the transverse plane. Varying the transverse size, we establish a dimensional crossover for universal scaling properties far from equilibrium. Our results suggest that some aspects of the dynamical universal behavior of anisotropic systems can be classified in terms of fractional spatial dimensions. We discuss our findings in view of recent experimental results with quasi one-dimensional setups of quenched ultracold quantum gases.

cond-mat.quant-gas