arXiv subjects

Laura Fernández

Publications and source records attributed to Laura Fernández.

4 recordsLinked to original sources

arXiv2024

The role of rare-earth atoms in the anisotropy and antiferromagnetic exchange coupling at a hybrid metal-organic interface

Magnetic anisotropy and magnetic exchange interactions are crucial parameters that characterize the hybrid metal-organic interface, key component of an organic spintronic device. We show that the incorporation of 4$f$ RE atoms to hybrid metal-organic interfaces of CuPc/REAu$_2$ type (RE= Gd, Ho) constitutes a feasible approach towards on-demand magnetic properties and functionalities. The GdAu$_2$ and HoAu$_2$ substrates differ in their magnetic anisotropy behavior. Remarkably, the HoAu$_2$ surface boosts the inherent out-of-plane anisotropy of CuPc, owing to the match between the anisotropy axis of substrate and molecule. Furthermore, the presence of RE atoms leads to a spontaneous antiferromagnetic (AFM) exchange coupling at the interface, induced by the 3$d$-4$f$ superexchange interaction between the unpaired 3$d$ electron of CuPc and the 4$f$ electrons of the RE atoms. We show that 4$f$ RE atoms with unquenched quantum orbital momentum ($L$), as it is the case of Ho, induce an anisotropic interfacial exchange coupling.

cond-mat.mtrl-sci↗

arXiv2024

Del Visual al Auditivo: Sonorización de Escenas Guiada por Imagen

Recent advances in image, video, text and audio generative techniques, and their use by the general public, are leading to new forms of content generation. Usually, each modality was approached separately, which poses limitations. The automatic sound recording of visual sequences is one of the greatest challenges for the automatic generation of multimodal content. We present a processing flow that, starting from images extracted from videos, is able to sound them. We work with pre-trained models that employ complex encoders, contrastive learning, and multiple modalities, allowing complex representations of the sequences for their sonorization. The proposed scheme proposes different possibilities for audio mapping and text guidance. We evaluated the scheme on a dataset of frames extracted from a commercial video game and sounds extracted from the Freesound platform. Subjective tests have evidenced that the proposed scheme is able to generate and assign audios automatically and conveniently to images. Moreover, it adapts well to user preferences, and the proposed objective metrics show a high correlation with the subjective ratings.

eess.AS↗

arXiv2023

Ultraconfined plasmons in atomically thin crystalline silver nanostructures

The ability to confine light down to atomic scales is critical for the development of applications in optoelectronics and optical sensing as well as for the exploration of nanoscale quantum phenomena. Plasmons in metallic nanostructures can achieve this type of confinement, although fabrication imperfections down to the subnanometer scale hinder actual developments. Here, we demonstrate narrow plasmons in atomically thin crystalline silver nanostructures fabricated by prepatterning silicon substrates and epitaxially depositing silver films of just a few atomic layers in thickness. Combined with on-demand lateral shaping, this procedure allows for an unprecedented control over optical field confinement in the near-infrared spectral region. Specifically, we observe fundamental and higher-order plasmons featuring extreme spatial confinement and high-quality factors that reflect the crystallinity of the metal. Our approach holds potential for the design and exploitation of atomic-scale nanoplasmonic devices in optoelectronics, sensing, and quantum-physics applications.

cond-mat.mes-hall↗

arXiv2019

Plasmonics in Atomically-Thin Crystalline Silver Films

Light-matter interaction at the atomic scale rules fundamental phenomena such as photoemission and lasing, while enabling basic everyday technologies, including photovoltaics and optical communications. In this context, plasmons --the collective electron oscillations in conducting materials-- are important because they allow manipulating optical fields at the nanoscale. The advent of graphene and other two-dimensional crystals has pushed plasmons down to genuinely atomic dimensions, displaying appealing properties such as a large electrical tunability. However, plasmons in these materials are either too broad or lying at low frequencies, well below the technologically relevant near-infrared regime. Here we demonstrate sharp near-infrared plasmons in lithographically-patterned wafer-scale atomically-thin silver crystalline films. Our measured optical spectra reveal narrow plasmons (quality factor $\sim4$), further supported by a low sheet resistance comparable to bulk metal in few-atomic-layer silver films down to seven Ag(111) monolayers. Good crystal quality and plasmon narrowness are obtained despite the addition of a thin passivating dielectric, which renders our samples resilient to ambient conditions. The observation of spectrally sharp and strongly confined plasmons in atomically thin silver holds great potential for electro-optical modulation and optical sensing applications.

cond-mat.mes-hall↗