arXiv subjects

Laura Serino

Publications and source records attributed to Laura Serino.

13 recordsLinked to original sources

arXiv2026

Coherent temporal filtering of multimode parametric down-conversion using a quantum pulse gate

Spectrally pure and indistinguishable single photons are essential for quantum network platforms, where high-visibility interference underpins many quantum information protocols. However, most practical single-photon sources emit spectrally multimode states with reduced purity. Conventional spectral intensity filtering can partially improve purity but cannot select a well-defined temporal mode (TM). Here, we demonstrate coherent temporal filtering of a multimode parametric down-conversion (PDC) source using a quantum pulse gate (QPG) and benchmark its performance against conventional intensity filtering. The generated PDC photons exhibit strong spectral correlations, rendering extraction of pure heralded photons from the pair a challenge. We demonstrate that QPG filtering consistently generates heralded photons with purities above 0.90 regardless of the filter shape. Contrariwise, using spectral intensity filters yields mixed photons. Photon purities are probed with chronocyclic Q-function tomography. Furthermore, we demonstrate the versatility of QPG filtering by extracting structured TMs, including superposition of picosecond time bins. These results establish the QPG as a practical coherent filtering tool for quantum network applications.

quant-ph↗

arXiv2026

A high-performance quantum pulse gate in thin-film lithium niobate

In this work, we demonstrate a quantum pulse gate (QPG) in thin-film lithium niobate. QPGs enable the selective manipulation and detection of temporal modes of quantum light and form the basis of numerous applications in photonic quantum technologies. To date, their widespread adaption is held back by two main limitations: restricted wavelength and polarization combinations of the involved fields and low normalized conversion efficiencies. We overcome these limitations through developing a QPG in thin-film lithium niobate. We design a waveguide geometry that provides the required dispersion properties for a highly efficient type-0 sum-frequency generation.We verify our design through mapping of the phase matching intensity, and demonstrate high-quality QPG operation by measuring a temporal-mode selectivity of (96.8$\pm$1.7)% on par with existing QPGs. Thanks to the strong confinement in thin-film lithium niobate, we succeed in demonstrating an internal conversion efficiency of (89.6$\pm$0.1)% for a pump power of only 20mW in front of our sample. This yields a lower-bound estimate for the normalized conversion efficiency of (1810$\pm$10)$\mathrm{W}^{-1}\mathrm{cm}^{-2}$, three orders of magnitude higher than in previous QPGs. Our results establish thin-film lithium niobate as ideal platform for high-performance QPGs and are a major step towards practical QPGs for photonic quantum technologies.

quant-ph↗

arXiv2026

Generalised quantum interference

Hong-Ou-Mandel interference is one of the clearest signatures of quantum behaviour: two identical photons meeting at a beam splitter always leave together. Here we demonstrate that this symmetry can be broken. Using a programmable integrated photonic processor, we interfere imbalanced two-photon states on a variable beam splitter and show that the output state of quantum interference can be continuously tuned, reaching the extreme case where destructive interference suppresses bunching at one output port. The asymmetry creates a forbidden bunching channel: photons may exit together at one port or separately at both ports, but cannot emerge together at the other port.

quant-ph↗

arXiv2026

Quantum-limited detection of arrival time and carrier frequency of time-dependent signals

Precise measurements of both the arrival time and carrier frequency of light pulses are essential for time-frequency-encoded quantum technologies. Quantum mechanics, however, imposes fundamental limits on the simultaneous determination of these quantities. In this work, we derive and experimentally verify the quantum uncertainty bounds governing joint time-frequency measurements. We show that when detection is restricted to finite time windows, the problem is naturally described by a quantum rotor, rendering the commonly used Heisenberg uncertainty relation inapplicable. We further propose an optimal detection scheme that saturates these fundamental limits. By sampling the Q-function, we demonstrate the reconstruction of the Wigner function beyond the harmonic oscillator. Using an experimental implementation based on a quantum pulse gate, we confirm that the proposed scheme approaches the ultimate quantum limit for simultaneous time-frequency measurements. These results provide a new framework for joint time-frequency detection with direct implications for precision measurements and quantum information processing.

quant-ph↗

arXiv2025

Complementarity-based complementarity: the choice of mutually unbiased observables shapes quantum uncertainty relations

Quantum uncertainty relations impose fundamental limits on the joint knowledge that can be acquired from complementary observables: perfect knowledge of a quantum state in one basis implies maximal indetermination in all other mutually unbiased bases (MUBs). Uncertainty relations derived from joint properties of the MUBs are generally assumed to be uniform, irrespective of the specific observables chosen within a set. In this work, we demonstrate instead that the uncertainty relations can depend on the choice of observables. Through both experimental observation and numerical methods, we show that selecting different sets of three MUBs in a 5-dimensional quantum system results in distinct uncertainty bounds, i.e. in varying degrees of complementarity, in terms of both entropy and variance.

quant-ph↗

arXiv2025

Observing High-dimensional Bell Inequality Violations using Multi-Outcome Spectral Measurements

Violation of Bell inequalities is an essential requirement for many quantum information and communication protocols. In high-dimensional systems, Bell inequality tests face the challenge of implementing genuinely multi-outcome measurements, since the emulation of these with separate dichotomic projections opens a binarisation loophole that local hidden variable theories can exploit. Here we show that the joint spectral intensity of a two-photon entangled state contains access to the necessary multi-outcome measurements to overcome this obstacle and certify and violate a Bell inequality for high-dimensional states. This result is contrary to the belief that the joint spectral intensity is a phase-insensitive quantity and does not have sufficient information to certify entanglement or Bell-nonlocality. Using this approach, we violate the CGLMP Bell inequality up to dimension d = 8, all with negligible p-values, and for the first time close the binarisation loophole in high-dimensional Bell experiments. Guaranteeing Bell-nonlocal correlations using frequency-only measurements removes the technological hurdle of measurements in the temporal domain, thus greatly simplifying any practical implementation of future high-dimensional quantum information protocols.

quant-ph↗

arXiv2025

Experimental entropic uncertainty relations in dimensions three to five

We provide experimental validation of tight entropic uncertainty relations for the Shannon entropies of observables with mutually unbiased eigenstates in high dimensions. In particular, we address the cases of dimensions $d = 3$, $4$ and $5$ and consider from $2$ to $d+1$ mutually unbiased bases. The experiment is based on pulsed frequency bins measured with a multi-output quantum pulse gate, which can perform projective measurements on a complete high-dimensional basis in the time-frequency domain. Our results fit the theoretical predictions: the bound on the sum of the entropies is never violated and is saturated by the states that minimize the uncertainty relations.

quant-ph↗

arXiv2025

Frequency-bin interferometry for reconstructing electric fields with low intensity

Ultrafast single-photon pulses with tailored time-frequency properties are highly attractive for quantum information science, offering high-dimensional encoding and compatibility with integrated optics platforms. However, accurate characterization of such pulses, including spectral coherence, remains challenging because current methods require substantial experimental resources and complex reconstruction algorithms. Here, we introduce frequency-bin interferometry for reconstructing electric fields with low intensity (FIREFLY), a technique that directly provides spectral amplitude, phase, and coherence profiles of single-photon pulses without requiring intensive reconstruction algorithms. Our approach measures the two-point spectral correlation function of the pulse by interfering its different frequency components using a quantum pulse gate (QPG) driven by a reference pump pulse. We demonstrate its compatibility with quantum light by characterizing partially coherent pulses generated by a type-0 parametric down-conversion process. We also overcome this requirement of a known pump pulse by introducing spectral shear into our interferometric scheme using a multi-output QPG (mQPG). This enables simultaneous characterization of a single-photon-level input pulse alongside an unknown pump pulse. Notably, our method achieves theory-experiment similarity above 95\% across all retrieved profiles, which demonstrates the reliability of this scheme for quantum information applications based on time-frequency encodings.

physics.optics↗

arXiv2024

Self-guided tomography of time-frequency qudits

High-dimensional time-frequency encodings have the potential to significantly advance quantum information science; however, practical applications require precise knowledge of the encoded quantum states, which becomes increasingly challenging for larger Hilbert spaces. Self-guided tomography (SGT) has emerged as a practical and scalable technique for this purpose in the spatial domain. Here, we apply SGT to estimate time-frequency states using a multi-output quantum pulse gate. We achieve fidelities of more than 99\% for 3- and 5-dimensional states without the need for calibration or post-processing. We demonstrate the robustness of SGT against statistical and environmental noise, highlighting its efficacy in the photon-starved regime typical of quantum information applications.

quant-ph↗

arXiv2024

Programmable time-frequency mode-sorting of single photons with a multi-output quantum pulse gate

We demonstrate a high-dimensional mode-sorter for single photons based on a multi-output quantum pulse gate, which we can program to switch between different temporal-mode encodings including pulse modes, frequency bins, time bins, and their superpositions. This device can facilitate practical realizations of quantum information applications such as high-dimensional quantum key distribution, and thus enables secure communication with enhanced information capacity. We characterize the mode-sorter through a detector tomography in 3 and 5 dimensions and find a fidelity up to $0.958\pm 0.030$ at the single-photon level.

quant-ph↗

arXiv2024

Pulse characterization at the single-photon level through chronocyclic $Q$-function measurements

The characterization of the complex spectral amplitude that is, the spectrum and spectral phase, of single-photon-level light fields is a crucial capability for modern photonic quantum technologies. Since established pulse characterisation techniques are not applicable at low intensities, alternative approaches are required. Here, we demonstrate the retrieval of the complex spectral amplitude of single-photon-level light pulses through measuring their chronocyclic $Q-$function. Our approach draws inspiration from quantum state tomography by exploiting the analogy between quadrature phase space and time-frequency phase space. In the experiment, we perform time-frequency projections with a quantum pulse gate, which directly yield the chronocyclic $Q-$function. We evaluate the data with maximum likelihood estimation, which is the established technique for quantum state tomography. This yields not only an unambigious estimate of the complex spectral amplitude of the state under test that does not require any \textit{a priori} information, but also allows for, in principle, estimating the spectral-temporal coherence properties of the state. Our method accurately recovers features such as jumps in the spectral phase and is resistant against regions with zero spectral intensity, which makes it immediately beneficial also for classical pulse characterization problems.

quant-ph↗

arXiv2024

Orchestrating time and color: a programmable source of high-dimensional entanglement

High-dimensional encodings based on temporal modes (TMs) of photonic quantum states provide the foundations for a highly versatile and efficient quantum information science (QIS) framework. Here, we demonstrate a crucial building block for any QIS applications based on TMs: a programmable source of maximally entangled high-dimensional TM states. Our source is based on a parametric down-conversion process driven by a spectrally shaped pump pulse, which facilitates the generation of maximally entangled TM states with a well-defined dimensionality that can be chosen programmatically. We characterize the effective dimensionality of the generated states via measurements of second-order correlation functions and joint spectral intensities, demonstrating the generation of bi-photon TM states with a controlled dimensionality in up to 20 dimensions.

quant-ph↗

arXiv2022

Realization of a multi-output quantum pulse gate for decoding high-dimensional temporal modes of single-photon states

Temporal modes (TMs) of photons provide an appealing high-dimensional encoding basis for quantum information. While techniques to generate TM states have been established, high-dimensional decoding of single-photon TMs remains an open challenge. In this work, we experimentally demonstrate demultiplexing of five-dimensional TMs of single photons with an average fidelity of 0.96 $\pm$ 0.01, characterized via measurement tomography. This is achieved using a newly developed device, the multi-output quantum pulse gate (mQPG). We demonstrate a proof-of-principle complete decoder based on the mQPG that operates on any basis from a set of 6 five-dimensional MUBs and is therefore suitable as a receiver for high-dimensional quantum key distribution. Furthermore, we confirm the high-quality operation of the mQPG by performing resource-efficient state tomography with an average fidelity of 0.98 $\pm$ 0.02.

quant-ph↗