arXiv subjects

Laurent Jalabert

Publications and source records attributed to Laurent Jalabert.

7 recordsLinked to original sources

arXiv2026

Room-temperature 1/3 suppression of diffusive shot noise

Diffusive conductors share a universal shot noise reduction of 1/3. This result can be obtained from quantum scattering, Boltzmann-Langevin kinetics, or by symmetric simple exclusion process, but experiments have been limited to cryogenic conditions and the understanding of this universality remains incomplete. Here we show that ferrocene redox cycling in a microfluidic gap is room temperature realization of this universality. An analytical model of the current and its noise is derived and confirmed experimentally. The universal 1/3 shot noise suppression is recovered in the diffusion-limited regime, providing a bridge between mesoscopic physics and electrochemistry, opening a new route for probing molecular dynamics through room-temperature noise measurements.

cond-mat.mes-hall↗

arXiv2026

Enhancement of far-field thermal emission via polaritonic cavity modes

Controlling thermal emission is crucial for applications involving thermophotovoltaics, thermal sensing, imaging, and camouflage. While prior studies focused on the emission of thermally excited guided modes (TEGMs) inside cavities, their contribution to the far-field radiation outside cavities has remained unexplored. Here, we demonstrate a tunable far-field thermal channel enabled by TEGMs arising from the coupling of surface phonon-polaritons and cavity resonances. By combining infrared emissivity experiments with fluctuational electrodynamics simulations, we identify distinct spectral features marking the conversion of two-dimensionally confined polaritonic modes into three-dimensional radiative channels. We find that silicon cavities covered with SiO2 enhance the emissivity by up to 200% near the polaritonic spectral resonance, whereas bare silicon cavities yield only broadband enhancement. These findings provide experimental evidence of TEGMs and establish a simple cavity architecture as an effective and scalable platform for tailoring thermal radiation without complex nanofabrication.

cond-mat.mes-hall↗

arXiv2025

Ultra-High-Temperature Vacuum Prober for Electrical and Thermal Measurements

We develop an ultra-high-temperature vacuum probe station (UHT-VPS) featuring a sample holder heated by thermal radiation from a silicon carbide heater. This contactless configuration electrically isolates the sample from the high-power heating source through a vacuum gap, ensuring reliable measurements under extreme conditions. The capability of this UHT-VPS to measure electrical signals from 30 nV upward on bulk sapphire is demonstrated using the 3w/2w method. Measurements are continuously operated from 300 to 1150 K, under high vacuum, for a total of about 66 hours without readjusting the contact. They yield the linear and quadratic temperature coefficients of resistance of chromium/platinum micro-resistances, as well as the sapphire's thermal conductivity and thermal diffusivity. By recording the heater and sensor temperature signals up to 30 kHz and fitting them with theoretical models that account for the quadratic TCR of Cr/Pt microwires, we obtain values in agreement with literature data obtained by optical methods. In this temperature range, we also measure thermal conductivity, which cannot be directly accessed by optical techniques. Our system thus provides an effective solution for simultaneously retrieving the electrical and thermal properties of materials using a single set of 3w/2w data up to unprecedented temperature levels.

physics.ins-det↗

arXiv2023

Electrochemical Shot-Noise of a Redox Monolayer

Redox monolayers are the base for a wide variety of devices including high-frequency molecular diodes or biomolecular sensors. We introduce a formalism to describe the electrochemical shot-noise of such monolayer, confirmed experimentally at room temperature in liquid. The proposed method, carried out at equilibrium, avoids parasitic capacitance, increases the sensitivity and allows to obtain quantitative information such as the electronic coupling (or standard electron transfer rates), its dispersion and the number of molecules. Unlike in solid-state physics, the homogeneity in energy levels and transfer rates in the monolayer yields a Lorentzian spectrum. This first step for shot-noise studies in molecular electrochemical systems opens perspectives for quantum transport studies in liquid environment at room temperature as well as highly sensitive measurements for bioelectrochemical sensors.

cond-mat.mes-hall↗

arXiv2023

Polaritonic Waveguide Emits Super-Planckian Thermal Radiation

Classical Planck's theory of thermal radiation predicts an upper limit of the heat transfer between two bodies separated by a distance longer than the dominant radiation wavelength (far-field regime). This limit can be overcome when the dimensions of the absorbent bodies are smaller than the dominant wavelength due to hybrid electromagnetic waves, known as surface phonon-polaritons (SPhPs). Here, we experimentally demonstrate that the far-field radiative heat transfer between two non-absorbent bodies can also overcome Planck's limit, by coating them with an absorbent material to form a polaritonic waveguide. This super-Planckian far-field thermal radiation is confirmed by measuring the radiative thermal conductance between two silicon plates coated with silicon dioxide nanolayers. The observed conductance is twice higher than Planck's limit and agrees with the predictions of our model for the SPhP waveguide modes. Our findings could be applied to thermal management in microelectronics and silicon photonics.

physics.optics↗

arXiv2022

Asymmetry of tensile vs. compressive elasticity and permeability contributes to the regulation of exchanges in collagen gels

The Starling principle describes exchanges in tissues based on the balance of hydrostatic and osmotic flows. This balance neglects the coupling between mechanics and hydrodynamics, a questionable assumption in strained elastic tissues due to intravascular pressure. Here, we measure the elasticity and permeability of collagen gels under tensile and compressive stress via the comparison of the temporal evolution of pressure in an air cavity sealed at the outlet of a collagen slab with an analytical kinetic model. We observe a drop in the permeability and enhanced strain-stiffening of native collagen gels under compression, both effects being essentially lost after chemical cross-linking. Further, we prove that this asymmetric response accounts for the accumulation of compressive stress upon sinusoidal fluid injection, which modulates the material's permeability. Our results thus show that the properties of collagen gels regulate molecular exchanges and could help understand drug transport in tissues.

physics.bio-ph↗

arXiv2021

Observation of quasi-ballistic thermal transport of surface phonon-polaritons over hundreds of micrometres

Long-distance propagation of heat carriers is essential for efficient heat dissipation in microelectronics. However, in dielectric nanomaterials, the primary heat carriers - phonons - can propagate ballistically only for hundreds of nanometres, which limits their heat conduction efficiency. Theory predicts that surface phonon-polaritons (SPhPs) can overcome this limitation and conduct heat without dissipation for hundreds of micrometres. In this work, we experimentally demonstrate such long-distance heat transport by SPhPs. Using the 3$ω$ technique, we measure the in-plane thermal conductivity of SiN nanomembranes for different heater-sensor distances (100 and 200 $μ$m), membrane thicknesses (30 - 200 nm), and temperatures (300 - 400 K). We find that in contrast with thick membranes, thin nanomembranes support heat conduction by SPhPs, as evidenced by an increase in the thermal conductivity with temperature. Remarkably, the thermal conductivity measured 200 $μ$m away from the heater are consistently higher than that measured 100 $μ$m closer. This result suggests that heat conduction by SPhPs is quasi-ballistic over at least hundreds of micrometres. Thus, our findings show that SPhPs can enhance heat dissipation in polar nanomembranes and find applications in thermal management, near-field radiation, and polaritonics.

cond-mat.mes-hall↗