SearcharxivSearch

arXiv subjects

Laurin Ostermann

Publications and source records attributed to Laurin Ostermann.

At least 19 recordsLinked to original sources

The Cumulant Expansion Approach: The Good, The Bad and The Ugly

The configuration space, i.e. the Hilbert space, of compound quantum systems grows exponentially with the number of its subsystems: its dimensionality is given by the product of the dimensions of its constituents. Therefore a full quantum treatment is rarely possible analytically and can be carried out numerically for fairly small systems only. Fortunately, in order to obtain interesting physics, approximations often very well suffice. One of these approximations is given by the cumulants expansion, where expectation values of products of operators are approximated by products of expectation values of said operators, neglecting higher-order correlations. The lowest order of this approximation is widely known as the mean field approximation and used routinely throughout quantum physics. Despite its ubiquitous presence, a general criterion for applicability and convergence properties of higher order cumulants expansions remains to be found. In this paper, we discuss two problems in quantum electrodynamics and quantum information, namely the collective radiative dissipation of a dipole-dipole interacting chain of atoms and the factorization of a bi-prime by annealing in an adiabatic quantum simulator. In the first case we find smooth, convergence behavior, where the approximation performs increasingly better with higher orders, while in the latter going beyond mean field turns out useless and, even for small system sizes, we are puzzled by numerically challenging and partly non-physical solutions.

quant-ph

Selective Preparation of Collective States in Coupled Quantum Emitters Using the SUPER Excitation Scheme

The efficient preparation of collective eigenstates of subwavelength-spaced optical dipoles is a prerequisite for observing their signature radiative properties and for their applications in quantum information processing. We theoretically investigate the deterministic preparation of superradiant and subradiant states of two dipole-coupled two-level quantum emitters at deep-subwavelength separation using the Swing-UP of Quantum Emitter Population (SUPER) excitation scheme. Utilizing suitable pulse parameters for two red-detuned, time-overlapping Gaussian pulses, the SUPER scheme enables close-to-unity population inversion in the targeted collective eigenstates. Furthermore, a tunable optical phase in the SUPER scheme enables the simultaneous inversions in both pure super- and subradiant states with finite populations, thereby resulting in the preparation of hybrid collective states. These results are possible to realize with or without an optical cavity. Our approach to populating the collective eigenstates in a cavity environment paves the way for the efficient preparation of these states in the presence of environmental decoherence. Our scheme enables single-photon generation, which is measured using the second-order correlation function. We also discuss in detail possible experimental realizations, in particular using solid-state emitters and molecules.

quant-ph

Self-ordering, cooling, and lasing in an ensemble of clock atoms

Active atomic clocks are predicted to provide far better short-term stability and robustness against thermal fluctuations than typical feedback-based optical atomic clocks. However, continuous laser operation using an ensemble of clock atoms still remains an experimentally challenging task. We study spatial self-organization in a transversely driven ensemble of clock atoms inside an optical resonator and coherent light emission from the cavity. We focus on the spectral properties of the emitted light in the narrow atomic linewidth regime, where the phase coherence providing frequency stability is stored in the atomic dipoles rather than the cavity field. The atoms are off-resonantly driven by a standing-wave coherent laser transversely to the cavity axis allowing for atomic motion along the cavity axis as well as along the pump. In order to treat larger atom numbers we employ a second-order cumulant expansion which allows us to calculate the spectrum of the cavity light field. We identify the self-organization threshold where the atoms align themselves in a checkerboard pattern, thus maximizing light scattering into the cavity, which simultaneously induces cooling. For a larger driving intensity, more atoms are transferred to the excited state, reducing cooling but increasing light emission from the excited atoms. This can be enhanced via a second cavity mode at the atomic frequency spatially shifted by a quarter wavelength. For large enough atom numbers we observe laser-like emission close to the bare atomic transition frequency.

quant-ph

Subradiance and Superradiant Long Range Excitation Transport among Quantum Emitter Ensembles in a Waveguide

In contrast to free space, in waveguides the dispersive and dissipative dipole-dipole interactions among quantum emitters exhibit a periodic behavior over remarkably long distances. We propose a novel setup exploiting this long-range periodicity in order to create highly excited subradiant states and facilitate fast controlled collective energy transport amongst far-apart ensembles coupled to a waveguide. For sufficiently large ensembles collective superradiant emission into the fiber modes dominates over its free space counterpart. We show that for a large number of emitters a fast transverse coherent pulse can create almost perfect subradiant states with up to $50\%$ excitation. On the other hand, for a coherent excitation of one sub-ensemble above an overall excitation fraction of $50\%$ we find a nearly lossless and fast energy transfer to the ground state sub-ensemble. This transport can be enhanced or suppressed by controlling the positions of the ensembles relative to each other, while it can also be realized with a random position distribution. In the optimally enhanced case this fast transfer appears as superradiant emission with subsequent superabsorption, yet, without a superradiant decay after the absorption. The highly excited subradiant states as well as the superradiant excitation transfer appear as suitable building blocks in applications like active atomic clocks, quantum batteries, quantum information protocols and quantum metrology procedures such as fiber-based Ramsey schemes.

quant-ph

Temperature-Enhanced Critical Quantum Metrology

We show that the performance of critical quantum metrology protocols, counter-intuitively, can be enhanced by finite temperature. We consider a toy-model squeezing Hamiltonian, the Lipkin-Meshkov-Glick model and the paradigmatic Ising model. We show that the temperature enhancement of the quantum Fisher information can be achieved by adiabatic preparation of the critical state and by preparing it directly in the proximity of the critical point. We also find a relatively simple, however, non-optimal measurement capable of harnessing finite temperature to increase the parameter estimation sensitivity. Therefore, we argue that temperature can be considered as a resource in critical quantum metrology.

quant-ph

Demonstration and modelling of time-bin entangled photons from a quantum dot in a nanowire

Resonant excitation of the biexciton state in an InAsP quantum dot by a phase-coherent pair of picosecond pulses allows preparing time-bin entangled pairs of photons via the biexciton-exciton cascade. We show that this scheme can be implemented for a dot embedded in an InP nanowire. The underlying physical mechanisms can be represented and quantitatively analyzed by an effective three-level open system master equation. Simulation parameters including decay and intensity dependent dephasing rates are extracted from experimental data, which in turn let us predict the resulting entanglement and optimal operating conditions.

quant-ph

Cavity Sub- and Superradiance Enhanced Ramsey Spectroscopy

Ramsey spectroscopy in large, dense ensembles of ultra-cold atoms trapped in optical lattices suffers from dipole-dipole interaction induced shifts and collective superradiance limiting its precision and accuracy. We propose a novel geometry implementing fast signal readout with minimal heating for large atom numbers at lower densities via an optical cavity operated in the weak single atom but strong collective coupling regime. The key idea is controlled collective transverse $π/2$-excitation of the atoms to prepare a macroscopic collective spin protected from cavity superradiance. This requires that the two halves of the atomic ensemble are coupled to the cavity mode with opposite phase, which is naturally realized for a homogeneously filled volume covering odd and even sites of the cavity mode along the cavity axis. The origin of the superior precision can be traced back to destructive interference among sub-ensembles in the complex nonlinear collective atom field dynamics. In the same configuration we find surprising regular self-pulsing of the cavity output for suitable continuous illumination. Our simulations for large atom numbers employing a cumulant expansion are qualitatively confirmed by a full quantum treatment of smaller ensembles.

cond-mat.quant-gas

Polarization Control of Radiation and Energy Flow in Dipole-Coupled Nanorings

Collective optical excitations in dipole-coupled nanorings of sub-wavelength spaced quantum emitters exhibit extreme sub-radiance and field confinement facilitating an efficient and low-loss ring-to-ring energy transfer. We show that energy shifts, radiative lifetimes, and emission patterns of excitons and biexcitons in such rings can be tailored via the orientation of the individual dipoles. Tilting the polarization from perpendicular to tangential to the ring dramatically changes the lifetime of the symmetric exciton state from superradiance to subradiance with the radiated field acquiring orbital angular momentum. At a magic tilt angle all excitons are degenerate and the transport fidelity between two rings exhibits a minimum. Further simulations suggest that, for certain parameters, the decay decreases double-exponentially with the emitter's density. Disorder in the rings' structure can even enhance radiative lifetimes. The transport efficiency strongly depends on polarization and size, which we demonstrate by simulating a bio-inspired example of two rings with 9 and 16 dipoles as found in biological light harvesting complexes (LHC). The field distribution in the most superradiant state in a full LHC multi-ring structure shows tight sub-wavelength field confinement in the central ring, while long-lived subradiant states store energy in the outer rings.

quant-ph

A Nanoscale Coherent Light Source

Generically, a laser is composed of an optical resonator coupled to a gain medium. If the light amplification via stimulated emission dominates the mirror losses, the emitted light is coherent. Recent studies have shown that sub-wavelength sized rings of quantum emitters possess subradiant eigenmodes which mimic high-Q optical resonators. We add a continuously pumped atom as a gain medium in the ring's center creating a minimalistic coherent light source. The system behaves like a thresholdless laser, featuring a narrow linewidth well below the natural linewidth of the constituent atoms.

quant-ph

Superradiant Cooling, Trapping, and Lasing of Dipole-Interacting Clock Atoms

A cold atomic gas with an inverted population on a transition coupled to a field mode of an optical resonator constitutes a generic model of a laser. For quasi-continuous operation, external pumping, trapping and cooling of the atoms is required to confine them in order to achieve enough gain inside the resonator. As inverted atoms are high-field seekers in blue detuned light fields, tuning the cavity mode to the blue side of the atomic gain transition allows for combining lasing with stimulated cavity cooling and dipole trapping of the atoms at the antinodes of the laser field. We study such a configuration using a semiclassical description of particle motion along the cavity axis. In extension of earlier work we include free space atomic and cavity decay as well as atomic dipole-dipole interactions and their corresponding forces. We show that for a proper choice of parameters even in the bad cavity limit the atoms can create a sufficiently strong field inside the resonator such that they are trapped and cooled via the superradiant lasing action with less than one photon on average inside the cavity.

quant-ph

Subradiance in Multiply Excited States of Dipole-Coupled V-Type Atoms

We generalize the theoretical modeling of collective atomic super- and subradiance to the multilevel case including spontaneous emission from several excited states towards a common ground state. We show that in a closely packed ensemble of $N$ atoms with $N-1$ distinct excited states each, one can find a new class of non-radiating dark states,, which allows for long-term storage of $N-1$ photonic excitations. Via dipole-dipole coupling only a single atom in the ground state is sufficient in order to suppress the decay of all $N-1$ other atoms. By means of some generic geometric configurations, like a triangle of V-type atoms or a chain of atoms with a $J=0 \to J=1$ transition, we study such subradiance including dipole-dipole interactions and show that even at finite distances long lifetimes can be observed. While generally hard to prepare deterministically, we identify various possibilities for a probabilistic preparation via a phase controlled laser pump and decay.

quant-ph

Extraordinary subradiance with lossless excitation transfer in dipole-coupled nano-rings of quantum emitters

A ring of sub-wavelength spaced dipole-coupled quantum emitters possesses only few radiant but many extraordinarily subradiant collective modes. These exhibit a 3D-confined spatial radiation field pattern forming a nano-scale high-Q optical resonator. We show that tailoring the geometry, orientation and distance between two such rings allows for increasing the ratio of coherent ring-to-ring coupling versus free-space emission by several orders of magnitude. In particular we find that subradiant excitations, when delocalized over several ring sites, are effectively transported between the rings with a high fidelity.

quant-ph

Super- and subradiance of clock atoms in multimode optical waveguides

The transversely confined propagating modes of an optical fiber mediate virtually infinite range energy exchanges among atoms placed within their field, which adds to the inherent free space dipole-dipole coupling. Typically, the single atom free space decay rate largely surpasses the emission rate into the guided fiber modes. However, scaling up the atom number as well as the system size amounts to entering a collective emission regime, where fiber-induced superradiant spontaneous emission dominates over free space decay. We numerically study this super- and subradiant decay of highly excited atomic states for one or several transverse fiber modes as present in hollow core fibers. As particular excitation scenarios we compare the decay of a totally inverted state to the case of Pi/2 pulses applied transversely or along the fiber axis as in standard Ramsey or Rabi interferometry. While a mean field approach fails to correctly describe the initiation of superradiance, a second-order approximation accounting for pairwise atom-atom quantum correlations generally proves sufficient to reliably describe superradiance of ensembles from two to a few hundred particles. In contrast, a full account of subradiance requires the inclusion of all higher order quantum correlations. Considering multiple guided modes introduces a natural effective cut-off for the interaction range emerging from the dephasing of different fiber contributions.

quant-ph

QuantumOptics.jl: A Julia framework for simulating open quantum systems

We present an open source computational framework geared towards the efficient numerical investigation of open quantum systems written in the Julia programming language. Built exclusively in Julia and based on standard quantum optics notation, the toolbox offers speed comparable to low-level statically typed languages, without compromising on the accessibility and code readability found in dynamic languages. After introducing the framework, we highlight its features and showcase implementations of generic quantum models. Finally, we compare its usability and performance to two well-established and widely used numerical quantum libraries.

quant-ph

Subradiance and entanglement in atoms with several independent decay channels

Spontaneous emission of a two--level atom in free space is modified by other atoms in its vicinity leading to super- and sub-radiance. In particular, for atomic distances closer than the transition wavelength the maximally entangled antisymmetric superposition state of two individually excited atomic dipole moments possesses no total dipole moment and will not decay spontaneously at all. Such a two-atom dark state does not exist, if the atoms possess alternative decay channels towards other atomic lower energy states. However, we show here that for any atomic state with $N-1$ independent spontaneous decay channels one can always find a $N$-particle highly entangled state, which completely decouples from the free radiation field and does not decay. Moreover, we show that this state is the unique state orthogonal to the subspace spanned by the lower energy states with this property. Its sub-radiant property largely survives at finite atomic distances.

quant-ph

Selective protected state preparation of coupled dissipative quantum emitters

Inherent binary or collective interactions in ensembles of quantum emitters induce a spread in the energy and lifetime of their eigenstates. While this typically causes fast decay and dephasing, in many cases certain special entangled collective states with minimal decay can be found, which possess ideal properties for spectroscopy, precision measurements or information storage. We show that for a specific choice of laser frequency, power and geometry or a suitable configuration of control fields one can efficiently prepare these states. We demonstrate this by studying preparation schemes for strongly subradiant entangled states of a chain of dipole-dipole coupled emitters. The prepared state fidelity and its entanglement depth is further improved via spatial excitation phase engineering or tailored magnetic fields.

quant-ph

Optimized geometries for future generation optical lattice clocks

Atoms deeply trapped in magic wavelength optical lattices provide a Doppler- and collision-free dense ensemble of quantum emitters ideal for high precision spectroscopy. Thus, they are the basis of some of the best optical clock setups to date. However, despite their minute optical dipole moments the inherent long range dipole-dipole interactions in such lattices generate line shifts, dephasing and modified decay. We show that in a perfectly filled lattice these effects are resonantly enhanced depending on lattice constant, lattice geometry and excitation scheme inducing clock shifts of many atomic linewidths and reducing measurement precision via superradiance. However, under optimal conditions collective effects can be exploited to yield zero effective shifts and prolong dipole lifetimes beyond the single atom decay. In particular we identify 2D hexagonal or square lattices with lattice constants below the optical wavelength as most promising configurations for an accuracy and precision well below the independent ensemble limit. This geometry should also be an ideal basis for related applications such as superradiant lasers, precision magnetometry or long lived quantum memories.

quant-ph

Coherence and degree of time-bin entanglement from quantum dots

We report on the generation of time-bin entangled photon pairs from a semiconductor quantum dot via pulsed resonant biexciton generation. Based on theoretical modeling we optimized the duration of the excitation pulse to minimize the laser-induced dephasing and increase the biexciton-to-background single exciton occupation probability. This results in a high degree of entanglement with a concurrence of up to 0.78(6) and a 0.88(3) overlap with a maximally entangled state. Theoretical simulations also indicate a power dependent nature of the dephasing during the laser excitation that limits the coherence of the excitation process.

quant-ph