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Le Wang

Publications and source records attributed to Le Wang.

At least 73 records · Page 4Linked to original sources

Tetragonal BaCoO$_3$: A Co$^{4+}$ Ferromagnetic Mott Insulator with Inverted Spin Crossover

The interplay between crystal electric field splitting of d states and Hund's rule exchange energy in cobalt-based perovskites offers a promising avenue for inducing spin-state transitions. This study reports a new body-centered tetragonal (BCT) phase of BaCoO$_3$ (BCT-BaCoO$_3$), synthesized under high pressure (15 GPa) and high temperature (1200 °C) conditions. BCT-BaCoO$_3$ adopts a double perovskite structure of EuTiO$_3$-type (space group I4/mcm, #140), confirmed by high-resolution scanning transmission electron microscopy. X-ray photoelectron spectroscopy reveals a rare Co$^{4+}$ valence state. Magnetization and X-ray absorption measurements reveal a low-spin to high-spin transition that takes place between 200 and 300 K. While spin crossovers are relatively common among common oxides, the one observed in BCT-BaCoO$_3$ is remarkable in that it proceeds in the opposite direction from conventional spin transitions. BCT-BaCoO$_3$ exhibits a low-spin (S = 1/2) state at high temperatures and transitions to a high-spin (S = 5/2) state at low temperatures. Within the high-spin state, hard ferromagnetic order onsets at T$_C$ = 107 K. Electrical resistivity indicates weak magnetoresistance and insulating behavior. Overall, BCT-BaCoO$_3$ presents an exceptional model for the exploration of spin-state transitions and the study of Co spin states in cobalt-based perovskites.

cond-mat.mtrl-sci↗

Controllable Synthesis of Submillimeter Ultrathin 2D Ferromagnetic Cr5Te8 Nanosheets by GaTe-Assisted CVD

2D non-van der Waals (vdW) Cr5Te8 has attracted widespread research interest for its air stability and thickness-dependent magnetic properties. However, exploring new methods for growing larger-scale ultrathin 2D Cr5Te8 remains challenging. Here, we selected GaTe powder as precursor to supply Te monomers and fabricated large-scale 2D Cr5Te8 nanosheets. By optimizing the growth temperature and source-substrate distance (DSS), we successfully achieved Cr5Te8 nanosheets with lateral sizes of up to ~0.19 mm and corresponding thicknesses down to ~4.8 nm. The role of GaTe enhances the efficient Te atoms concentration, which promoted the lateral growth of Cr5Te8 nanosheets. Furthermore, our findings reveal the presence of Cr5Te8 nanosheets exhibiting serrated edges and a stacked structure like wedding cakes. Magnetic property measurement revealed the intense out-of-plane ferromagnetism in Cr5Te8, with the Curie temperature (TC) of 172 K. This work paves a way for the controllable growth of the submillimeter ultrathin 2D ferromagnetic crystalline and lays the foundation for the future synthesis of millimeter ultrathin ferromagnets.

cond-mat.mes-hall↗

Muon Spin Relaxation Study of Spin Dynamics on a Kitaev honeycomb material H$_3$LiIr$_2$O$_6$

The vacancy effect in quantum spin liquid (QSL) has been extensively studied. A finite density of random vacancies in the Kitaev model can lead to a pileup of low-energy density of states (DOS), which is generally experimentally determined by a scaling behavior of thermodynamic or magnetization quantities. Here, we report detailed muon spin relaxation ($μ$SR) results of H$_3$LiIr$_2$O$_6$, a Kitaev QSL candidate with vacancies. The absence of magnetic order is confirmed down to 80 mK, and the spin fluctuations are found to be persistent at low temperatures. Intriguingly, the time-field scaling law of longitudinal-field (LF)-$μ$SR polarization is observed down to 0.1 K. This indicates a dynamical scaling, whose critical exponent 0.46 is excellently consistent with the scaling behavior of specific heat and magnetization data. All the observations point to the finite DOS with the form $N(E) \sim E^{-0.5}$ , which is expected for the Kitaev QSL in the presence of vacancies. Our μSR study provides a dynamical fingerprint of the power-law low-energy DOS, and introduces a crucial new insight into the vacancy effect in QSL.

cond-mat.str-el↗

Multimodal LLM Enhanced Cross-lingual Cross-modal Retrieval

Cross-lingual cross-modal retrieval (CCR) aims to retrieve visually relevant content based on non-English queries, without relying on human-labeled cross-modal data pairs during training. One popular approach involves utilizing machine translation (MT) to create pseudo-parallel data pairs, establishing correspondence between visual and non-English textual data. However, aligning their representations poses challenges due to the significant semantic gap between vision and text, as well as the lower quality of non-English representations caused by pre-trained encoders and data noise. To overcome these challenges, we propose LECCR, a novel solution that incorporates the multi-modal large language model (MLLM) to improve the alignment between visual and non-English representations. Specifically, we first employ MLLM to generate detailed visual content descriptions and aggregate them into multi-view semantic slots that encapsulate different semantics. Then, we take these semantic slots as internal features and leverage them to interact with the visual features. By doing so, we enhance the semantic information within the visual features, narrowing the semantic gap between modalities and generating local visual semantics for subsequent multi-level matching. Additionally, to further enhance the alignment between visual and non-English features, we introduce softened matching under English guidance. This approach provides more comprehensive and reliable inter-modal correspondences between visual and non-English features. Extensive experiments on four CCR benchmarks, \ie Multi30K, MSCOCO, VATEX, and MSR-VTT-CN, demonstrate the effectiveness of our proposed method. Code: \url{https://github.com/LiJiaBei-7/leccr}.

cs.CV↗

Merging Parameter Estimation and Classification Using LASSO

Soft sensing is a way to indirectly obtain information of signals for which direct sensing is difficult or prohibitively expensive. It may not \textit{a priori} be evident which sensors provide useful information about the target signal, and various operating conditions often necessitate different models. In this paper, we provide a systematic method to construct a soft sensor that can deal with these issues. We propose a single estimation criterion, where the objectives are encoded in terms of model fit, model sparsity (reducing the number of different models), and model parameter coefficient sparsity (to exclude irrelevant sensors). The proposed method is tested on real-world scenarios involving prototype vehicles, demonstrating its effectiveness.

eess.SY↗

PMT: Progressive Mean Teacher via Exploring Temporal Consistency for Semi-Supervised Medical Image Segmentation

Semi-supervised learning has emerged as a widely adopted technique in the field of medical image segmentation. The existing works either focuses on the construction of consistency constraints or the generation of pseudo labels to provide high-quality supervisory signals, whose main challenge mainly comes from how to keep the continuous improvement of model capabilities. In this paper, we propose a simple yet effective semi-supervised learning framework, termed Progressive Mean Teachers (PMT), for medical image segmentation, whose goal is to generate high-fidelity pseudo labels by learning robust and diverse features in the training process. Specifically, our PMT employs a standard mean teacher to penalize the consistency of the current state and utilizes two sets of MT architectures for co-training. The two sets of MT architectures are individually updated for prolonged periods to maintain stable model diversity established through performance gaps generated by iteration differences. Additionally, a difference-driven alignment regularizer is employed to expedite the alignment of lagging models with the representation capabilities of leading models. Furthermore, a simple yet effective pseudo-label filtering algorithm is employed for facile evaluation of models and selection of high-fidelity pseudo-labels outputted when models are operating at high performance for co-training purposes. Experimental results on two datasets with different modalities, i.e., CT and MRI, demonstrate that our method outperforms the state-of-the-art medical image segmentation approaches across various dimensions. The code is available at https://github.com/Axi404/PMT.

cs.CV↗

R3D-AD: Reconstruction via Diffusion for 3D Anomaly Detection

3D anomaly detection plays a crucial role in monitoring parts for localized inherent defects in precision manufacturing. Embedding-based and reconstruction-based approaches are among the most popular and successful methods. However, there are two major challenges to the practical application of the current approaches: 1) the embedded models suffer the prohibitive computational and storage due to the memory bank structure; 2) the reconstructive models based on the MAE mechanism fail to detect anomalies in the unmasked regions. In this paper, we propose R3D-AD, reconstructing anomalous point clouds by diffusion model for precise 3D anomaly detection. Our approach capitalizes on the data distribution conversion of the diffusion process to entirely obscure the input's anomalous geometry. It step-wisely learns a strict point-level displacement behavior, which methodically corrects the aberrant points. To increase the generalization of the model, we further present a novel 3D anomaly simulation strategy named Patch-Gen to generate realistic and diverse defect shapes, which narrows the domain gap between training and testing. Our R3D-AD ensures a uniform spatial transformation, which allows straightforwardly generating anomaly results by distance comparison. Extensive experiments show that our R3D-AD outperforms previous state-of-the-art methods, achieving 73.4% Image-level AUROC on the Real3D-AD dataset and 74.9% Image-level AUROC on the Anomaly-ShapeNet dataset with an exceptional efficiency.

cs.CV↗

Adjusting for Participation Bias in Case-Control Genetic Association Studies for Rare Diseases

Collection of genotype data in case-control genetic association studies may often be incomplete for reasons related to genes themselves. This non-ignorable missingness structure, if not appropriately accounted for, can result in participation bias in association analyses. To deal with this issue, Chen et al. (2016) proposed to collect additional genetic information from family members of individuals whose genotype data were not available, and developed a maximum likelihood method for bias correction. In this study, we develop an estimating equation approach to analyzing data collected from this design that allows adjustment of covariates. It jointly estimates odds ratio parameters for genetic association and missingness, where a logistic regression model is used to relate missingness to genotype and other covariates. Our method allows correlation between genotype and covariates while using genetic information from family members to provide information on the missing genotype data. In the estimating equation for genetic association parameters, we weight the contribution of each genotyped subject to the empirical likelihood score function by the inverse probability that the genotype data are available. We evaluate large and finite sample performance of our method via simulation studies and apply it to a family-based case-control study of breast cancer.

stat.ME↗

Diffuse X-ray Explorer: a high-resolution X-ray spectroscopic sky surveyor on the China Space Station

DIffuse X-ray Explorer (DIXE) is a proposed high-resolution X-ray spectroscopic sky surveyor on the China Space Station (CSS). DIXE will focus on studying hot baryons in the Milky Way. Galactic hot baryons like the X-ray emitting Milky Way halo and eROSITA bubbles are best observed in the sky survey mode with a large field of view. DIXE will take advantage of the orbital motion of the CSS to scan a large fraction of the sky. High-resolution X-ray spectroscopy, enabled by superconducting microcalorimeters based on the transition-edge sensor (TES) technology, will probe the physical properties (e.g., temperature, density, elemental abundances, kinematics) of the Galactic hot baryons. This will complement the high-resolution imaging data obtained with the eROSITA mission. Here we present the preliminary design of DIXE. The payload consists mainly of a detector assembly and a cryogenic cooling system. The key components of the detector assembly are a microcalorimeter array and frequency-domain multiplexing readout electronics. To provide a working temperature for the detector assembly, the cooling system consists of an adiabatic demagnetization refrigerator and a mechanical cryocooler system.

astro-ph.IM↗

Near-Room-Temperature Field-Controllable Exchange Bias in 2D van der Waals Ferromagnet Fe3GaTe2

Exchange bias (EB) is a cornerstone of modern magnetic memory and sensing technologies. Its extension to the realm of two-dimensional (2D) van der Waals (vdW) magnets holds promise for revolutionary advancements in miniaturized and efficient atomic spintronic devices. However, the blocking temperature of EB in 2D vdW magnets is currently well below room temperature ~130 K. This study reports a robust EB phenomenon in Fe3GaTe2 thin-layer devices, which significantly increases the blocking temperature to a near-room-temperature record of 280 K. Both the bias direction and magnitude can be isothermally tuned by adjusting the field sweep range, in striking contrast to the conventional EB in ferromagnetic/antiferromagnetic (FM/AFM) bilayers. We propose an exchange spring model in which crystal defects with higher coercivity act as the pivotal pinning source for the observed EB phenomenon, deviating from the conventional FM/AFM interface mechanism. Cumulative growth of minor loops and multiple magnetization reversal paths are observed in field cycles below the saturation field, consistent with the hard FM defects behavior of our exchange spring model. These findings provide insights into the complex magnetic order in 2D ferromagnets and open new avenues for developing practical ultrathin vdW spintronic devices with EB-like properties at room temperature.

cond-mat.mes-hall↗

Tunable Collective Excitations in Epitaxial Perovskite Nickelates

The formation of plasmons through the collective excitation of charge density has generated intense discussions, offering insights to fundamental sciences and potential applications. While the underlying physical principles have been well-established, the effects of many-body interactions and orbital hybridization on plasmonic dynamics remain understudied. In this work, we present the observation of conventional metallic and correlated plasmons in epitaxial La1-xSrxNiO3 (LSNO) films with varying Sr doping concentrations (x = 0, 0.125, 0.25), unveiling their intriguing evolution. Unlike samples at other doping concentrations, the x = 0.125 intermediate doping sample does not exhibit the correlated plasmons despite showing high optical conductivity. Through a comprehensive experimental investigation using spectroscopic ellipsometry and X-ray absorption spectroscopy, the O2p-Ni3d orbital hybridization for LSNO with a doping concentration of x = 0.125 is found to be significantly enhanced, alongside a considerable weakening of its effective correlation U*. These factors account for the absence of correlated plasmons and the high optical conductivity observed in LSNO (0.125). Our results underscore the profound impact of orbital hybridization on the electronic structure and the formation of plasmon in strongly-correlated systems. This in turn suggest that LSNO could serve as a promising alternative material in optoelectronic devices.

cond-mat.mtrl-sci↗

Towards Generalizable Multi-Object Tracking

Multi-Object Tracking MOT encompasses various tracking scenarios, each characterized by unique traits. Effective trackers should demonstrate a high degree of generalizability across diverse scenarios. However, existing trackers struggle to accommodate all aspects or necessitate hypothesis and experimentation to customize the association information motion and or appearance for a given scenario, leading to narrowly tailored solutions with limited generalizability. In this paper, we investigate the factors that influence trackers generalization to different scenarios and concretize them into a set of tracking scenario attributes to guide the design of more generalizable trackers. Furthermore, we propose a point-wise to instance-wise relation framework for MOT, i.e., GeneralTrack, which can generalize across diverse scenarios while eliminating the need to balance motion and appearance. Thanks to its superior generalizability, our proposed GeneralTrack achieves state-of-the-art performance on multiple benchmarks and demonstrates the potential for domain generalization. https://github.com/qinzheng2000/GeneralTrack.git

cs.CV↗

Magnetic phase transitions in the triangular-lattice spin-1 dimer compound K2Ni2(SeO3)3

In our study, we conduct magnetization and heat capacity measurements to investigate field induced magnetic phase transitions within the newly synthesized compound K2Ni2(SeO3)3, a spin-1 dimer system arranged on a triangular lattice. From our first-principles simulations, we determine that the spin system in K2Ni2(SeO3)3 can be represented as a two-dimensional triangular-lattice spin-1 dimer model, including an intra-dimer exchange of J1 = 0.32 meV, an inter-dimer exchange of J2 = 0.79 meV, and an easy-axis anisotropy of D = 0.14 meV. The presence of easy-axis magnetic anisotropy explains the distinct magnetic phase diagrams observed under c-axis directional and in-plane magnetic fields. Notably, our investigation unveils a two-step phase transition with the magnetic field aligned with the c direction. Our findings yield valuable insights into the magnetic phase transitions inherent to geometrically frustrated magnetic systems featuring dimer structures.

cond-mat.str-el↗

Uncovering an Interfacial Band Resulting from Orbital Hybridization in Nickelate Heterostructures

The interaction of atomic orbitals at the interface of perovskite oxide heterostructures has been investigated for its profound impact on the band structures and electronic properties, giving rise to unique electronic states and a variety of tunable functionalities. In this study, we conducted an extensive investigation of the optical and electronic properties of epitaxial NdNiO3 thin films grown on a series of single crystal substrates. Unlike films synthesized on other substrates, NdNiO3 on SrTiO3 (NNO/STO) gives rise to a unique band structure which features an additional unoccupied band situated above the Fermi level. Our comprehensive investigation, which incorporated a wide array of experimental techniques and density functional theory calculations, revealed that the emergence of the interfacial band structure is primarily driven by the orbital hybridization between Ti 3d orbitals of the STO substrate and O 2p orbitals of the NNO thin film. Furthermore, exciton peaks have been detected in the optical spectra of the NNO/STO film, attributable to the pronounced electron-electron (e-e) and electron-hole (e-h) interactions propagating from the STO substrate into the NNO film. These findings underscore the substantial influence of interfacial orbital hybridization on the electronic structure of oxide thin-films, thereby offering key insights into tuning their interfacial properties.

cond-mat.mtrl-sci↗

Learning Discriminative Spatio-temporal Representations for Semi-supervised Action Recognition

Semi-supervised action recognition aims to improve spatio-temporal reasoning ability with a few labeled data in conjunction with a large amount of unlabeled data. Albeit recent advancements, existing powerful methods are still prone to making ambiguous predictions under scarce labeled data, embodied as the limitation of distinguishing different actions with similar spatio-temporal information. In this paper, we approach this problem by empowering the model two aspects of capability, namely discriminative spatial modeling and temporal structure modeling for learning discriminative spatio-temporal representations. Specifically, we propose an Adaptive Contrastive Learning~(ACL) strategy. It assesses the confidence of all unlabeled samples by the class prototypes of the labeled data, and adaptively selects positive-negative samples from a pseudo-labeled sample bank to construct contrastive learning. Additionally, we introduce a Multi-scale Temporal Learning~(MTL) strategy. It could highlight informative semantics from long-term clips and integrate them into the short-term clip while suppressing noisy information. Afterwards, both of these two new techniques are integrated in a unified framework to encourage the model to make accurate predictions. Extensive experiments on UCF101, HMDB51 and Kinetics400 show the superiority of our method over prior state-of-the-art approaches.

cs.CV↗

Robust Noisy Label Learning via Two-Stream Sample Distillation

Noisy label learning aims to learn robust networks under the supervision of noisy labels, which plays a critical role in deep learning. Existing work either conducts sample selection or label correction to deal with noisy labels during the model training process. In this paper, we design a simple yet effective sample selection framework, termed Two-Stream Sample Distillation (TSSD), for noisy label learning, which can extract more high-quality samples with clean labels to improve the robustness of network training. Firstly, a novel Parallel Sample Division (PSD) module is designed to generate a certain training set with sufficient reliable positive and negative samples by jointly considering the sample structure in feature space and the human prior in loss space. Secondly, a novel Meta Sample Purification (MSP) module is further designed to mine adequate semi-hard samples from the remaining uncertain training set by learning a strong meta classifier with extra golden data. As a result, more and more high-quality samples will be distilled from the noisy training set to train networks robustly in every iteration. Extensive experiments on four benchmark datasets, including CIFAR-10, CIFAR-100, Tiny-ImageNet, and Clothing-1M, show that our method has achieved state-of-the-art results over its competitors.

cs.CV↗

Surprising pressure-induced magnetic transformations from Helimagnetic order to Antiferromagnetic state in NiI2

Interlayer magnetic interactions play a pivotal role in determining the magnetic arrangement within van der Waals (vdW) magnets, and the remarkable tunability of these interactions through applied pressure further enhances their significance. Here, we investigate NiI2 flakes, a representative vdW magnet, under hydrostatic pressures up to 11 GPa. We reveal a notable increase in magnetic transition temperatures for both helimagnetic and antiferromagnetic states, and find that a reversible transition from helimagnetic to antiferromagnetic (AFM) phases at approximately 7 GPa challenges established theoretical and experimental expectations. While the increase in transition temperature aligns with pressure-enhanced overall exchange interaction strengths, we identify the significant role of the second-nearest neighbor interlayer interaction, which competes with intra-layer frustration and favors the AFM state as demonstrated in the Monte Carlo simulations. Experimental and simulated results converge on the existence of an intermediate helimagnetic ordered state in NiI2 before transitioning to the AFM state. These findings underscore the pivotal role of interlayer interactions in shaping the magnetic ground state, providing fresh perspectives for innovative applications in nanoscale magnetic device design.

cond-mat.mtrl-sci↗

Boosting Semi-Supervised Temporal Action Localization by Learning from Non-Target Classes

The crux of semi-supervised temporal action localization (SS-TAL) lies in excavating valuable information from abundant unlabeled videos. However, current approaches predominantly focus on building models that are robust to the error-prone target class (i.e, the predicted class with the highest confidence) while ignoring informative semantics within non-target classes. This paper approaches SS-TAL from a novel perspective by advocating for learning from non-target classes, transcending the conventional focus solely on the target class. The proposed approach involves partitioning the label space of the predicted class distribution into distinct subspaces: target class, positive classes, negative classes, and ambiguous classes, aiming to mine both positive and negative semantics that are absent in the target class, while excluding ambiguous classes. To this end, we first devise innovative strategies to adaptively select high-quality positive and negative classes from the label space, by modeling both the confidence and rank of a class in relation to those of the target class. Then, we introduce novel positive and negative losses designed to guide the learning process, pushing predictions closer to positive classes and away from negative classes. Finally, the positive and negative processes are integrated into a hybrid positive-negative learning framework, facilitating the utilization of non-target classes in both labeled and unlabeled videos. Experimental results on THUMOS14 and ActivityNet v1.3 demonstrate the superiority of the proposed method over prior state-of-the-art approaches.

cs.CV↗