arXiv subjects

Lee A. Rozema

Publications and source records attributed to Lee A. Rozema.

At least 37 records · Page 2Linked to original sources

arXiv2023

Semi-device-independent certification of indefinite causal order in a photonic quantum switch

We report an experimental certification of indefinite causal order that relies only on the characterization of the operations of a single party. We do so in the semi-device-independent scenario with the fewest possible assumptions of characterization of the parties' local operations in which indefinite causal order can be demonstrated with the quantum switch. To achieve this result, we introduce the concept of semi-device-independent causal inequalities and show that the correlations generated in a photonic quantum switch, in which all parties are able to collect local outcome statistics, achieve a violation of this inequality of 224 standard deviations. This result consists of the experimental demonstration of indefinite causal order with the fewest device-characterization assumptions to date.

quant-ph↗

arXiv2023

Nonlinear quantum logic with colliding graphene plasmons

Graphene has emerged as a promising platform to bring nonlinear quantum optics to the nanoscale, where a large intrinsic optical nonlinearity enables long-lived and actively tunable plasmon polaritons to strongly interact. Here we theoretically study the collision between two counter-propagating plasmons in a graphene nanoribbon, where transversal subwavelength confinement endows propagating plasmons with %large effective masses a flat band dispersion that enhances their interaction. This scenario presents interesting possibilities towards the implementation of multi-mode polaritonic gates that circumvent limitations imposed by the Shapiro no-go theorem for photonic gates in nonlinear optical fibers. As a paradigmatic example we demonstrate the feasibility of a high fidelity conditional Pi phase shift (CZ), where the gate performance is fundamentally limited only by the single-plasmon lifetime. These results open new exciting avenues towards quantum information and many-body applications with strongly-interacting polaritons.

quant-ph↗

arXiv2022

Enhanced Photonic Maxwell's Demon with Correlated Baths

Maxwell's Demon is at the heart of the interrelation between quantum information processing and thermodynamics. In this thought experiment, a demon generates a temperature gradient between two thermal baths initially at equilibrium by gaining information at the single-particle level and applying classical feed-forward operations, allowing for the extraction of work. Here we implement a photonic version of Maxwell's Demon with active feed-forward in a fibre-based system using ultrafast optical switches. We experimentally show that, if correlations exist between the two thermal baths, the Demon can generate a temperature difference over an order of magnitude larger than without correlations, and so extract more work. Our work demonstrates the great potential of photonic experiments -- which provide a unique degree of control on the system -- to access new regimes in quantum thermodynamics.

quant-ph↗

arXiv2022

Giant enhancement of third-harmonic generation in graphene-metal heterostructures

Nonlinear nanophotonics leverages engineered nanostructures to funnel light into small volumes and intensify nonlinear optical processes with spectral and spatial control. Due to its intrinsically large and electrically tunable nonlinear optical response, graphene is an especially promising nanomaterial for nonlinear optoelectronic applications. Here we report on exceptionally strong optical nonlinearities in graphene-insulator-metal heterostructures, demonstrating an enhancement by three orders of magnitude in the third-harmonic signal compared to bare graphene. Furthermore, by increasing the graphene Fermi energy through an external gate voltage, we find that graphene plasmons mediate the optical nonlinearity and modify the third-harmonic signal. Our findings show that graphene-insulator-metal is a promising heterostructure for optically-controlled and electrically-tunable nano-optoelectronic components.

cond-mat.mes-hall↗

arXiv2022

High-harmonic generation enhancement with graphene heterostructures

We investigate high-harmonic generation in graphene heterostructures consisting of metallic nanoribbons separated from a graphene sheet by either a few-nanometer layer of aluminum oxide or an atomic monolayer of hexagonal boron nitride. The nanoribbons amplify the near-field at the graphene layer relative to the externally applied pumping, thus allowing us to observe third- and fifth-harmonic generation in the carbon monolayer at modest pump powers in the mid-infrared. We study the dependence of the nonlinear signals on the ribbon width and spacer thickness, as well as pump power and polarization, and demonstrate enhancement factors relative to bare graphene reaching 1600 and 4100 for third- and fifth-harmonic generation, respectively. Our work supports the use of graphene heterostructures to selectively enhance specific nonlinear processes of interest, an essential capability for the design of nanoscale nonlinear devices.

cond-mat.mes-hall↗

arXiv2022

Inferring work by quantum superposing forward and time-reversal evolutions

The study of thermodynamic fluctuations allows one to relate the free energy difference between two equilibrium states with the work done on a system through processes far from equilibrium. This finding plays a crucial role in the quantum regime, where the definition of work becomes non-trivial. Based on these relations, here we develop a simple interferometric method allowing a direct estimation of the work distribution and the average dissipative work during a driven thermodynamic process by superposing the forward and time-reversal evolutions of the process. We show that our scheme provides useful upper bounds on the average dissipative work even without full control over the thermodynamic process, and we propose methodological variations depending on the possible experimental limitations encountered. Finally, we exemplify its applicability by an experimental proposal for implementing our method on a quantum photonics system, on which the thermodynamic process is performed through polarization rotations induced by liquid crystals acting in a discrete temporal regime.

quant-ph↗

arXiv2021

Experimental entanglement of temporal order

The study of causal relations has recently been applied to the quantum realm, leading to the discovery that not all physical processes have a definite causal structure. While indefinite causal processes have previously been experimentally shown, these proofs relied on the quantum description of the experiments. Yet, the same experimental data could also be compatible with definite causal structures within different descriptions. Here, we present the first demonstration of indefinite temporal order outside of quantum formalism. We show that our experimental outcomes are incompatible with a class of generalised probabilistic theories satisfying the assumptions of locality and definite temporal order. To this end, we derive physical constraints (in the form of a Bell-like inequality) on experimental outcomes within such a class of theories. We then experimentally invalidate these theories by violating the inequality using entangled temporal order. This provides experimental evidence that there exist correlations in nature which are incompatible with the assumptions of locality and definite temporal order.

quant-ph↗

arXiv2021

Experimental Higher-Order Interference in a Nonlinear Triple Slit

Interference between two waves is a well-known concept in physics, and its generalization to more than two waves is straight-forward. The order of interference is defined as the number of paths that interfere in a manner that cannot be reduced to patterns of a lower order. In practice, second-order interference means that in, say, a triple-slit experiment, the interference pattern when all three slits are open can be predicted from the interference patterns between all possible pairs of slits. Quantum mechanics is often said to only exhibit second-order interference. However, this is only true under specific assumptions, typically single-particles undergoing linear evolution. Here we experimentally show that nonlinear evolution can in fact lead to higher-order interference. The higher-order interference in our experiment has a simple quantum mechanical description; namely, optical coherent states interacting in a nonlinear medium. Our work shows that nonlinear evolution could open a loophole for experiments attempting to verify Born's rule by ruling out higher-order interference.

quant-ph↗

arXiv2021

Higher-order interference between multiple quantum particles interacting nonlinearly

The double-slit experiment is the most direct demonstration of interference between individual quantum objects. Since similar experiments with single particles and more slits produce interference fringes reducible to a combination of double-slit patterns it is usually argued that quantum interference occurs between pairs of trajectories, compactly denoted as second-order interference. Here we show that quantum mechanics in fact allows for interference of arbitrarily high order. This occurs naturally when one considers multiple quantum objects interacting in the presence of a nonlinearity, both of which are required to observe higher-order interference. We make this clear by treating a generalised multi-slit interferometer using second-quantisation. We then present explicit experimentally-relevant examples both with photons interacting in nonlinear media and an interfering Bose-Einstein condensate with particle-particle interactions. These examples are all perfectly described by quantum theory, and yet exhibit higher-order interference based on multiple particles interacting nonlinearly.

quant-ph↗

arXiv2021

Experimental Quantum Communication Enhancement by Superposing Trajectories

In quantum communication networks, wires represent well-defined trajectories along which quantum systems are transmitted. In spite of this, trajectories can be used as a quantum control to govern the order of different noisy communication channels, and such a control has been shown to enable the transmission of information even when quantum communication protocols through well-defined trajectories fail. This result has motivated further investigations on the role of the superposition of trajectories in enhancing communication, which revealed that the use of quantum control of parallel communication channels, or of channels in series with quantum-controlled operations, can also lead to communication advantages. Building upon these findings, here we experimentally and numerically compare different ways in which two trajectories through a pair of noisy channels can be superposed. We observe that, within the framework of quantum interferometry, the use of channels in series with quantum-controlled operations generally yields the largest advantages. Our results contribute to clarify the nature of these advantages in experimental quantum-optical scenarios, and showcase the benefit of an extension of the quantum communication paradigm in which both the information exchanged and the trajectory of the information carriers are quantum.

quant-ph↗

arXiv2018

Experimental few-copy multi-particle entanglement detection

Quantum technologies lead to a variety of applications that outperform their classical counterparts. In order to build a quantum device it must be verified that it operates below some error threshold. Recently, because of technological developments which allow for the experimental realization of quantum states with increasing complexity, these tasks must be applied to large multi-qubit states. However, due to the exponentially-increasing system size, tasks like quantum entanglement verification become hard to carry out in such cases. Here we develop a generic framework to translate any entanglement witness into a resource-efficient probabilistic scheme. We show that the confidence to detect entanglement grows exponentially with the number of individual detection events. To benchmark our findings, we experimentally verify the presence of entanglement in a photonic six-qubit cluster state generated using three single-photon sources operating at telecommunication wavelengths. We find that its presence can be certified with at least 99.74% confidence by detecting 20 copies of the quantum state. Additionally, we show that genuine six-qubit entanglement is verified with at least 99% confidence by using 112 copies of the state. Our protocol can be carried out with a remarkably low number of copies, making it a practical and applicable method to verify large-scale quantum devices.

quant-ph↗

arXiv2016

Experimental Verification of an Indefinite Causal Order

Investigating the role of causal order in quantum mechanics has recently revealed that the causal distribution of events may not be a-priori well-defined in quantum theory. While this has triggered a growing interest on the theoretical side, creating processes without a causal order is an experimental task. Here we report the first decisive demonstration of a process with an indefinite causal order. To do this, we quantify how incompatible our set-up is with a definite causal order by measuring a 'causal witness'. This mathematical object incorporates a series of measurements which are designed to yield a certain outcome only if the process under examination is not consistent with any well-defined causal order. In our experiment we perform a measurement in a superposition of causal orders - without destroying the coherence - to acquire information both inside and outside of a 'causally non-ordered process'. Using this information, we experimentally determine a causal witness, demonstrating by almost seven standard deviations that the experimentally implemented process does not have a definite causal order.

quant-ph↗

arXiv2016

Comment on Adler's "Does the Peres experiment using photons test for hyper-complex (quaternionic) quantum theories?"

In his recent article [arXiv:1604.04950], Adler questions the usefulness of the bound found in our experimental search for genuine effects of hyper-complex quantum mechanics [arXiv:1602.01624]. Our experiment was performed using a black-box (instrumentalist) approach to generalized probabilistic theories; therefore, it does not assume a priori any particular underlying mechanism. From that point of view our experimental results do indeed place meaningful bounds on possible effects of "post-quantum theories", including quaternionic quantum mechanics. In his article, Adler compares our experiment to non-relativistic and Möller formal scattering theory within quaternionic quantum mechanics. With a particular set of assumptions, he finds that quaternionic effects would likely not manifest themselves in general. Although these assumptions are justified in the non-relativistic case, a proper calculation for relativistic particles is still missing. Here, we provide a concrete relativistic example of Klein-Gordon scattering wherein the quaternionic effects persist. We note that when the Klein-Gordon equation is formulated using a Hamiltonian formalism it displays a so-called "indefinite metric", a characteristic feature of relativistic quantum wave equations. In Adler's example this is directly forbidden by his assumptions, and therefore our present example is not in contradiction to his work. In complex quantum mechanics this problem of an indefinite metric is solved in second quantization. Unfortunately, there is no known algorithm for canonical field quantization in quaternionic quantum mechanics.

quant-ph↗

arXiv2016

Experimental Test of Hyper-Complex Quantum Theories

In standard quantum mechanics, complex numbers are used to describe the wavefunction. Although complex numbers have proven sufficient to predict the results of existing experiments, there is no apparent theoretical reason to choose them over real numbers or generalizations of complex numbers, i.e. hyper-complex numbers. Experiments performed to date have proven that real numbers are insufficient, but whether or not hyper-complex numbers are required remains an open question. Quantum theories based on hyper-complex numbers are one example of a post-quantum theory, which must be put on a firm experimental foundation. Here we experimentally probe hyper-complex quantum theories, by studying one of their deviations from complex quantum theory: the non-commutativity of phases. We do so by passing single photons through a Sagnac interferometer containing two physically different phases, having refractive indices of opposite sign. By showing that the phases commute with high precision, we place limits on a particular prediction of hyper-complex quantum theories.

quant-ph↗

arXiv2014

Characterizing an Entangled-Photon Source with Classical Detectors and Measurements

Quantum state tomography (QST) is a universal tool for the design and optimization of entangled-photon sources. It typically requires single-photon detectors and coincidence measurements. Recently, it was suggested that the information provided by the QST of photon pairs generated by spontaneous parametric down-conversion could be obtained by exploiting the stimulated version of this process, namely difference frequency generation. In this protocol, so-called "stimulated-emission tomography" (SET), a seed field is injected along with the pump pulse, and the resulting stimulated emission is measured. Since the intensity of the stimulated field can be several orders of magnitude larger than the intensity of the corresponding spontaneous emission, measurements can be made with simple classical detectors. Here, we experimentally demonstrate SET and compare it with QST. We show that one can accurately reconstruct the polarization density matrix, and predict the purity and concurrence of the polarization state of photon pairs without performing any single-photon measurements.

quant-ph↗

arXiv2014

Experimental Superposition of Orders of Quantum Gates

In a quantum computer, creating superpositions of quantum bits (qubits) in different states can lead to a speed-up over classical computers [1], but quantum mechanics also allows for the superposition of quantum circuits [2]. In fact, it has recently been theoretically predicted that superimposing quantum circuits, each with a different gate order, could provide quantum computers with an even further computational advantage [3-5]. Here, we experimentally demonstrate this enhancement by applying two quantum gates in a superposition of both possible orders to determine whether the two gates commute or anti-commute. We are able to make this determination with only a single use (or query) of each gate, while all quantum circuits with a fixed order of gates would require at least two uses of one of the gates [3]. Remarkably, when the problem is scaled to N gates, creating a superposition of quantum circuits is likely to provide an exponential advantage over classical algorithms, and a linear advantage over quantum algorithms with fixed gate order [4]. The new resource that we exploit in our experiment can be interpreted as a "superposition of causal orders". We demonstrate such a superposition could allow some quantum algorithms to be implemented with an efficiency that is unlikely to be achieved on a quantum computer with a fixed gate order.

quant-ph↗

arXiv2014

Quantum Data Compression of a Qubit Ensemble

Data compression is a ubiquitous aspect of modern information technology, and the advent of quantum information raises the question of what types of compression are feasible for quantum data, where it is especially relevant given the extreme difficulty involved in creating reliable quantum memories. We present a protocol in which an ensemble of quantum bits (qubits) can in principle be perfectly compressed into exponentially fewer qubits. We then experimentally implement our algorithm, compressing three photonic qubits into two. This protocol sheds light on the subtle differences between quantum and classical information. Furthermore, since data compression stores all of the available information about the quantum state in fewer physical qubits, it could provide a vast reduction in the amount of quantum memory required to store a quantum ensemble, making even today's limited quantum memories far more powerful than previously recognized.

quant-ph↗

arXiv2014

On the Optimal Choice of Spin-Squeezed States for Detecting and Characterizing a Quantum Process

Quantum metrology uses quantum states with no classical counterpart to measure a physical quantity with extraordinary sensitivity or precision. Most metrology schemes measure a single parameter of a dynamical process by probing it with a specially designed quantum state. The success of such a scheme usually relies on the process belonging to a particular one-parameter family. If this assumption is violated, or if the goal is to measure more than one parameter, a different quantum state may perform better. In the most extreme case, we know nothing about the process and wish to learn everything. This requires quantum process tomography, which demands an informationally-complete set of probe states. It is very convenient if this set is group-covariant -- i.e., each element is generated by applying an element of the quantum system's natural symmetry group to a single fixed fiducial state. In this paper, we consider metrology with 2-photon ("biphoton") states, and report experimental studies of different states' sensitivity to small, unknown collective SU(2) rotations ("SU(2) jitter"). Maximally entangled N00N states are the most sensitive detectors of such a rotation, yet they are also among the worst at fully characterizing an a-priori unknown process. We identify (and confirm experimentally) the best SU(2)-covariant set for process tomography; these states are all less entangled than the N00N state, and are characterized by the fact that they form a 2-design.

quant-ph↗