arXiv subjects

Leen Decin

Publications and source records attributed to Leen Decin.

At least 55 records · Page 3Linked to original sources

arXiv2023

Stratospheric dayside-to-nightside circulation drives the 3-D ozone distribution on synchronously rotating rocky exoplanets

Determining the habitability and interpreting future atmospheric observations of exoplanets requires understanding the atmospheric dynamics and chemistry from a 3-D perspective. Previous studies have shown significant spatial variability in the ozone layer of synchronously rotating M-dwarf planets, assuming an Earth-like initial atmospheric composition. We use a 3-D Coupled Climate-Chemistry model to understand this distribution of ozone and identify the mechanism responsible for it. We document a previously unreported connection between the ozone production regions on the photochemically active dayside hemisphere and the nightside devoid of stellar radiation and thus photochemistry. We find that stratospheric dayside-to-nightside overturning circulation can advect ozone-rich air to the nightside. On the nightside, ozone-rich air subsides at the locations of two quasi-stationary Rossby gyres, resulting in an exchange between the stratosphere and troposphere and the accumulation of ozone at the gyre locations. We identify the hemispheric contrast in radiative heating and cooling as the main driver of this ozone circulation. Dynamically-driven chemistry also impacts other tracer species in the atmosphere (gaseous and non-gaseous phase) as long as chemical lifetimes exceed dynamical lifetimes. These findings illustrate the 3-D nature of planetary atmospheres, predicting spatial and temporal variability that will impact spectroscopic observations of exoplanet atmospheres.

astro-ph.EP↗

arXiv2023

3D simulations of AGB stellar winds -- II. Ray-tracer implementation and impact of radiation on the outflow morphology

Stars with an initial mass below ~ 8 Msun evolve through the asymptotic giant branch (AGB) phase, during which they develop strong stellar winds. Recent observations have revealed significant morphological complexities in their outflows, most likely caused by a companion. We study the impact of the radiation force on such companion-perturbed AGB outflows. We present the implementation of a ray tracer for radiative transfer in smoothed particle hydrodynamics (SPH) and compared four different descriptions of radiative transfer: the free-wind, the geometrical, the Lucy, and the attenuation approximation. For both low and high mass-loss rates, the velocity profile of the outflow is modified when going from the free-wind to the geometrical approximation, also resulting in a different morphology. In the case of a low mass-loss rate, the effect of the Lucy and attenuation approximation is negligible due to the low densities but morphological differences appear in the high mass-loss rate regime. By comparing the radiative equilibrium temperature and radiation force to full 3D radiative transfer, we show that the Lucy approximation works best. Although, close to the companion, artificial heating occurs and it fails to simulate the shadow cast by the companion. The attenuation approximation produces a lower equilibrium temperature and weaker radiation force, but it produces the shadow cast by the companion. From the predictions of the 3D radiative transfer, we also conclude that a radially directed radiation force is a reasonable assumption. The radiation force thus plays a critical role in dust-driven AGB winds, impacting the velocity profile and morphological structures. For low mass-loss rates, the geometrical approximation suffices, while high mass-loss rates require a more rigorous method, where the Lucy approximation provides the most accurate results although not accounting for all effects.

astro-ph.SR↗

arXiv2023

Photochemically-produced SO$_2$ in the atmosphere of WASP-39b

Photochemistry is a fundamental process of planetary atmospheres that regulates the atmospheric composition and stability. However, no unambiguous photochemical products have been detected in exoplanet atmospheres to date. Recent observations from the JWST Transiting Exoplanet Early Release Science Program found a spectral absorption feature at 4.05 $μ$m arising from SO$_2$ in the atmosphere of WASP-39b. WASP-39b is a 1.27-Jupiter-radii, Saturn-mass (0.28 M$_J$) gas giant exoplanet orbiting a Sun-like star with an equilibrium temperature of $\sim$1100 K. The most plausible way of generating SO$_2$ in such an atmosphere is through photochemical processes. Here we show that the SO$_2$ distribution computed by a suite of photochemical models robustly explains the 4.05 $μ$m spectral feature identified by JWST transmission observations with NIRSpec PRISM (2.7$σ$) and G395H (4.5$σ$). SO$_2$ is produced by successive oxidation of sulphur radicals freed when hydrogen sulphide (H$_2$S) is destroyed. The sensitivity of the SO$_2$ feature to the enrichment of the atmosphere by heavy elements (metallicity) suggests that it can be used as a tracer of atmospheric properties, with WASP-39b exhibiting an inferred metallicity of $\sim$10$\times$ solar. We further point out that SO$_2$ also shows observable features at ultraviolet and thermal infrared wavelengths not available from the existing observations.

astro-ph.EP↗

arXiv2023

The effect of thermal non-equilibrium on kinetic nucleation

Nucleation is considered to be the first step in dust and cloud formation in the atmospheres of asymptotic giant branch (AGB) stars, exoplanets, and brown dwarfs. In these environments dust and cloud particles grow to macroscopic sizes when gas phase species condense onto cloud condensation nuclei (CCNs). Understanding the formation processes of CCNs and dust in AGB stars is important because the species that formed in their outflows enrich the interstellar medium. Although widely used, the validity of chemical and thermal equilibrium conditions is debatable in some of these highly dynamical astrophysical environments. We aim to derive a kinetic nucleation model that includes the effects of thermal non-equilibrium by adopting different temperatures for nucleating species, and to quantify the impact of thermal non-equilibrium on kinetic nucleation. Forward and backward rate coefficients are derived as part of a collisional kinetic nucleation theory ansatz. The endothermic backward rates are derived from the law of mass action in thermal non-equilibrium. We consider elastic collisions as thermal equilibrium drivers. For homogeneous TiO2 nucleation and a gas temperature of 1250 K, we find that differences in the kinetic cluster temperatures as small as 20 K increase the formation of larger TiO2 clusters by over an order of magnitude. An increase in cluster temperature of around 20 K at gas temperatures of 1000 K can reduce the formation of a larger TiO2 cluster by over an order of magnitude. Our results confirm and quantify the prediction of previous thermal non-equilibrium studies. Small thermal non-equilibria can cause a significant change in the synthesis of larger clusters. Therefore, it is important to use kinetic nucleation models that include thermal non-equilibrium to describe the formation of clusters in environments where even small thermal non-equilibria can be present.

astro-ph.EP↗

arXiv2023

A broadband thermal emission spectrum of the ultra-hot Jupiter WASP-18b

Close-in giant exoplanets with temperatures greater than 2,000 K (''ultra-hot Jupiters'') have been the subject of extensive efforts to determine their atmospheric properties using thermal emission measurements from the Hubble and Spitzer Space Telescopes. However, previous studies have yielded inconsistent results because the small sizes of the spectral features and the limited information content of the data resulted in high sensitivity to the varying assumptions made in the treatment of instrument systematics and the atmospheric retrieval analysis. Here we present a dayside thermal emission spectrum of the ultra-hot Jupiter WASP-18b obtained with the NIRISS instrument on JWST. The data span 0.85 to 2.85 $μ$m in wavelength at an average resolving power of 400 and exhibit minimal systematics. The spectrum shows three water emission features (at $>$6$σ$ confidence) and evidence for optical opacity, possibly due to H$^-$, TiO, and VO (combined significance of 3.8$σ$). Models that fit the data require a thermal inversion, molecular dissociation as predicted by chemical equilibrium, a solar heavy element abundance (''metallicity'', M/H = 1.03$_{-0.51}^{+1.11}$ $\times$ solar), and a carbon-to-oxygen (C/O) ratio less than unity. The data also yield a dayside brightness temperature map, which shows a peak in temperature near the sub-stellar point that decreases steeply and symmetrically with longitude toward the terminators.

astro-ph.EP↗

arXiv2022

Radiative Transfer as a Bayesian Linear Regression problem

Electromagnetic radiation plays a crucial role in various physical and chemical processes. Hence, almost all astrophysical simulations require some form of radiative transfer model. Despite many innovations in radiative transfer algorithms and their implementation, realistic radiative transfer models remain very computationally expensive, such that one often has to resort to approximate descriptions. The complexity of these models makes it difficult to assess the validity of any approximation and to quantify uncertainties on the model results. This impedes scientific rigour, in particular, when comparing models to observations, or when using their results as input for other models. We present a probabilistic numerical approach to address these issues by treating radiative transfer as a Bayesian linear regression problem. This allows us to model uncertainties on the input and output of the model with the variances of the associated probability distributions. Furthermore, this approach naturally allows us to create reduced-order radiative transfer models with a quantifiable accuracy. These are approximate solutions to exact radiative transfer models, in contrast to the exact solutions to approximate models that are often used. As a first demonstration, we derive a probabilistic version of the method of characteristics, a commonly-used technique to solve radiative transfer problems.

astro-ph.IM↗

arXiv2022

Early Release Science of the exoplanet WASP-39b with JWST NIRCam

Measuring the metallicity and carbon-to-oxygen (C/O) ratio in exoplanet atmospheres is a fundamental step towards constraining the dominant chemical processes at work and, if in equilibrium, revealing planet formation histories. Transmission spectroscopy provides the necessary means by constraining the abundances of oxygen- and carbon-bearing species; however, this requires broad wavelength coverage, moderate spectral resolution, and high precision that, together, are not achievable with previous observatories. Now that JWST has commenced science operations, we are able to observe exoplanets at previously uncharted wavelengths and spectral resolutions. Here we report time-series observations of the transiting exoplanet WASP-39b using JWST's Near InfraRed Camera (NIRCam). The long-wavelength spectroscopic and short-wavelength photometric light curves span 2.0 - 4.0 $μ$m, exhibit minimal systematics, and reveal well-defined molecular absorption features in the planet's spectrum. Specifically, we detect gaseous H$_2$O in the atmosphere and place an upper limit on the abundance of CH$_4$. The otherwise prominent CO$_2$ feature at 2.8 $μ$m is largely masked by H$_2$O. The best-fit chemical equilibrium models favour an atmospheric metallicity of 1-100$\times$ solar (i.e., an enrichment of elements heavier than helium relative to the Sun) and a sub-stellar carbon-to-oxygen (C/O) ratio. The inferred high metallicity and low C/O ratio may indicate significant accretion of solid materials during planet formation or disequilibrium processes in the upper atmosphere.

astro-ph.EP↗

arXiv2022

Early Release Science of the Exoplanet WASP-39b with JWST NIRSpec G395H

Measuring the abundances of carbon and oxygen in exoplanet atmospheres is considered a crucial avenue for unlocking the formation and evolution of exoplanetary systems. Access to an exoplanet's chemical inventory requires high-precision observations, often inferred from individual molecular detections with low-resolution space-based and high-resolution ground-based facilities. Here we report the medium-resolution (R$\sim$600) transmission spectrum of an exoplanet atmosphere between 3-5 $μ$m covering multiple absorption features for the Saturn-mass exoplanet WASP-39b, obtained with JWST NIRSpec G395H. Our observations achieve 1.46x photon precision, providing an average transit depth uncertainty of 221 ppm per spectroscopic bin, and present minimal impacts from systematic effects. We detect significant absorption from CO$_2$ (28.5$σ$) and H$_2$O (21.5$σ$), and identify SO$_2$ as the source of absorption at 4.1 $μ$m (4.8$σ$). Best-fit atmospheric models range between 3 and 10x solar metallicity, with sub-solar to solar C/O ratios. These results, including the detection of SO$_2$, underscore the importance of characterising the chemistry in exoplanet atmospheres, and showcase NIRSpec G395H as an excellent mode for time series observations over this critical wavelength range.

astro-ph.EP↗

arXiv2022

Early Release Science of the exoplanet WASP-39b with JWST NIRISS

Transmission spectroscopy provides insight into the atmospheric properties and consequently the formation history, physics, and chemistry of transiting exoplanets. However, obtaining precise inferences of atmospheric properties from transmission spectra requires simultaneously measuring the strength and shape of multiple spectral absorption features from a wide range of chemical species. This has been challenging given the precision and wavelength coverage of previous observatories. Here, we present the transmission spectrum of the Saturn-mass exoplanet WASP-39b obtained using the SOSS mode of the NIRISS instrument on the JWST. This spectrum spans $0.6 - 2.8 μ$m in wavelength and reveals multiple water absorption bands, the potassium resonance doublet, as well as signatures of clouds. The precision and broad wavelength coverage of NIRISS-SOSS allows us to break model degeneracies between cloud properties and the atmospheric composition of WASP-39b, favoring a heavy element enhancement ("metallicity") of $\sim 10 - 30 \times$ the solar value, a sub-solar carbon-to-oxygen (C/O) ratio, and a solar-to-super-solar potassium-to-oxygen (K/O) ratio. The observations are best explained by wavelength-dependent, non-gray clouds with inhomogeneous coverage of the planet's terminator.

astro-ph.EP↗

arXiv2022

No evidence for radius inflation in hot Jupiters from vertical advection of heat

Understanding the radiative-dynamical coupling between upper photosphere and deeper atmosphere is a key in understanding the abnormal large radii of hot Jupiters. One needs very long integration times of 3D general circulation models (GCMs) with self consistent radiative transfer to achieve a better understanding of the feedback process between dynamics and radiation. We here present the longest 3D non-gray GCM study (86000 d) of an ultra hot Jupiter (WASP-76 b) published to this date that reached a final converged state. Furthermore, we present a method that can be used to accelerate the path towards temperature convergence in the deep atmospheric layers. We find that the final converged temperature profile is cold in the deep atmospheric layers, lacking any sign of vertical transport of potential temperature by large scale atmospheric motions. We thus conclude that the coupling between radiation and dynamics alone is not sufficient to explain the abnormal large radii of inflated hot gas giants.

astro-ph.EP↗

arXiv2022

Exploring the deep atmospheres of HD 209458b and WASP-43b using a non-gray general circulation model

Simulations with a 3D general circulation model (GCM) suggest that one potential driver behind the observed radius inflation in hot Jupiters may be the downward advection of energy from the highly irradiated photosphere into the deeper layers. Here, we compare dynamical heat transport within the non-inflated hot Jupiter WASP-43b and the canonical inflated hot Jupiter HD 209458b, with similar effective temperatures. We investigate to what extent the radiatively driven heating and cooling in the photosphere (at pressures smaller than 1 bar) influence the deeper temperature profile (at pressures between 1 to 700 bar). Our simulations with the new non-gray 3D radiation-hydrodynamical model expeRT/MITgcm show that the deep temperature profile of WASP-43b is associated with a relatively cold adiabat. The deep layers of HD 209458b, however, do not converge and remain nearly unchanged regardless of whether a cold or a hot initial state is used. Furthermore, we show that different flow structures in the deep atmospheric layers arise. There, we find that WASP-43b exhibits a deep equatorial jet, driven by the relatively fast tidally locked rotation of this planet (0.81 days), as compared to HD 209458b (3.47 days). However, by comparing simulations with different rotation periods, we find that the resulting flow structures only marginally influence the temperature evolution in the deep atmosphere, which is almost completely dominated by radiative heating and cooling. Furthermore, we find that the evolution of deeper layers can influence the 3D temperature structure in the photosphere of WASP-43b. Thus, dayside emission spectra of WASP-43b may shed more light onto the dynamical processes occurring at greater depths.

astro-ph.EP↗

arXiv2022

Lightning-induced chemistry on tidally-locked Earth-like exoplanets

Determining the habitability and interpreting atmospheric spectra of exoplanets requires understanding their atmospheric physics and chemistry. We use a 3-D Coupled Climate-Chemistry Model, the Met Office Unified Model with the UK Chemistry and Aerosols framework, to study the emergence of lightning and its chemical impact on tidally-locked Earth-like exoplanets. We simulate the atmosphere of Proxima Centauri b orbiting in the Habitable Zone of its M-dwarf star, but the results apply to similar M-dwarf orbiting planets. Our chemical network includes the Chapman ozone reactions and hydrogen oxide (HO$_{\mathrm{x}}$=H+OH+HO$_2$) and nitrogen oxide (NO$_{\mathrm{x}}$=NO+NO$_2$) catalytic cycles. We find that photochemistry driven by stellar radiation (177-850 nm) supports a global ozone layer between 20-50 km. We parameterise lightning flashes as a function of cloud-top height and the resulting production of nitric oxide (NO) from the thermal decomposition of N$_2$ and O$_2$. Rapid dayside convection over and around the substellar point results in lightning flash rates of up to 0.16 flashes km$^{-2}$yr$^{-1}$, enriching the dayside atmosphere below altitudes of 20 km in NO$_{\mathrm{x}}$. Changes in dayside ozone are determined mainly by UV irradiance and the HO$_{\mathrm{x}}$ catalytic cycle. ~45% of the planetary dayside surface remains at habitable temperatures (T$_{\mathrm{surf}}$>273.15 K) and the ozone layer reduces surface UV radiation levels to 15%. Dayside-nightside thermal gradients result in strong winds that subsequently advect NO$_{\mathrm{x}}$ towards the nightside, where the absence of photochemistry allows NO$_{\mathrm{x}}$ chemistry to involve reservoir species. Our study also emphasizes the need for accurate UV stellar spectra to understand the atmospheric chemistry of exoplanets.

astro-ph.EP↗

arXiv2022

Impact of stellar flares on the chemical composition and transmission spectra of gaseous exoplanets orbiting M dwarfs

Stellar flares of active M dwarfs can affect the atmospheric composition of close-orbiting gas giants, and can result in time-dependent transmission spectra. We aim to examine the impact of a variety of flares, differing in energy, duration, and occurrence frequency, on the composition and spectra of close-orbiting, tidally locked gaseous planets with climates dominated by equatorial superrotation. We used a series of pseudo-2D photo- and thermochemical kinetics models, which take advection by the equatorial jet stream into account, to simulate the neutral molecular composition of a gaseous planet (effective temperature 800 K) that orbits a flaring M dwarf. We then computed transmission spectra for the evening and morning limb. We find that the upper regions of the dayside and evening limb are heavily depleted in CH4 and NH3 up to several days after a flare with a total radiative energy of $ 2 \times 10^{33} $ erg. Molar fractions of C2H2 and HCN are enhanced up to a factor three on the nightside and morning limb after day-to-nightside advection of photodissociated species. CH4 depletion reduces transit depths by 100-300 parts per million (ppm) on the evening limb and C2H2 production increases the 14 micron feature up to 350 ppm on the morning limb. We find that repeated flaring drives the atmosphere to a composition that differs from its pre-flare distribution and that this translates to a permanent modification of the transmission spectrum. We show that single high-energy flares can affect the atmospheres of close-orbiting gas giants up to several days after the flare event, during which their transmission spectra are altered by several hundred ppm. Repeated flaring has important implications for future retrieval analyses of exoplanets around active stars, as the atmospheric composition and resulting spectral signatures substantially differ from models that do not include flaring.

astro-ph.EP↗

arXiv2022

Identification of carbon dioxide in an exoplanet atmosphere

Carbon dioxide (CO2) is a key chemical species that is found in a wide range of planetary atmospheres. In the context of exoplanets, CO2 is an indicator of the metal enrichment (i.e., elements heavier than helium, also called "metallicity"), and thus formation processes of the primary atmospheres of hot gas giants. It is also one of the most promising species to detect in the secondary atmospheres of terrestrial exoplanets. Previous photometric measurements of transiting planets with the Spitzer Space Telescope have given hints of the presence of CO2 but have not yielded definitive detections due to the lack of unambiguous spectroscopic identification. Here we present the detection of CO2 in the atmosphere of the gas giant exoplanet WASP-39b from transmission spectroscopy observations obtained with JWST as part of the Early Release Science Program (ERS). The data used in this study span 3.0 to 5.5 μm in wavelength and show a prominent CO2 absorption feature at 4.3 μm (26σ significance). The overall spectrum is well matched by one-dimensional, 10x solar metallicity models that assume radiative-convective-thermochemical equilibrium and have moderate cloud opacity. These models predict that the atmosphere should have water, carbon monoxide, and hydrogen sulfide in addition to CO2, but little methane. Furthermore, we also tentatively detect a small absorption feature near 4.0 μm that is not reproduced by these models.

astro-ph.EP↗

arXiv2022

Grid of Pseudo-2D Chemistry Models for Tidally-Locked Exoplanets. I. The Role of Vertical and Horizontal Mixing

The atmospheres of synchronously rotating exoplanets are intrinsically three-dimensional, and fast vertical and horizontal winds are expected to mix the atmosphere, driving the chemical composition out of equilibrium. Due to the longer computation times associated with multi-dimensional forward models, horizontal mixing has only been investigated for a few case studies. In this paper, we aim to generalize the impact of horizontal and vertical mixing on the chemistry of exoplanet atmospheres over a large parameter space. We do this by applying a sequence of post-processed forward models for a large grid of synchronously rotating gaseous exoplanets, where we vary the effective temperature (between 400 K and 2600 K), surface gravity, and rotation rate. We find that there is a dichotomy in the horizontal homogeneity of the chemical abundances. Planets with effective temperatures below 1400 K tend to have horizontally homogeneous, vertically quenched chemical compositions, while planets hotter than 1400 K exhibit large compositional day-night differences for molecules such as methane. Furthermore, we find that the planet's rotation rate impacts the planetary climate, and thus also the molecular abundances and transmission spectrum. By employing a hierarchical modelling approach, we assess the relative importance of disequilibrium chemistry on the exoplanet transmission spectrum, and conclude that the temperature has the most profound impact. Temperature differences are also the main cause of limb asymmetries, which we estimate could be observable with the James Webb Space Telescope. This work highlights the value of applying a consistent modelling setup to a broad parameter space in exploratory theoretical research.

astro-ph.EP↗

arXiv2022

3D hydrodynamical survey of the impact of a companion on the morphology and dynamics of AGB outflow

With the use of high-resolution ALMA observations, complex structures that resemble those observed in post-AGB stars and planetary nebulae are detected in the circumstellar envelopes of low-mass evolved stars. These deviations from spherical symmetry are believed to be caused primarily by the interaction with a companion star or planet. With the use of three-dimensional hydrodynamic simulations, we study the impact of a binary companion on the wind morphology and dynamics of an AGB outflow. We classifiy the wind structures and morphology that form in these simulations with the use of a classification parameter, constructed with characteristic parameters of the binary configuration. Finally we conclude that the companion alters the wind expansion velocity through the slingshot mechanism, if it is massive enough.

astro-ph.SR↗

arXiv2022

Buckyball-metal complexes as promising carriers of astronomical unidentified infrared emission bands

Infrared emission bands with wavelengths between 3-20 μm are observed in a variety of astrophysical environments [1,2]. They were discovered in the 1970s and are generally attributed to organic compounds [3,4]. However, over 40 years of research efforts still leave the source of these emission bands largely unidentified [5-7]. Here, we report the first laboratory infrared (6-25 μm) spectra of gas-phase fullerene-metal complexes, [C60-Metal]+ (Metal = Fe and V), and show with density functional theory calculations that complexes of C60 with cosmically abundant metals, including Li, Na, K, Mg, Ca, Al, V, and Fe, all have similar infrared spectral patterns. Comparison with observational infrared spectra from several fullerene-rich planetary nebulae demonstrates a strong positive linear cross-correlation. The infrared features of [C60-Metal]+ coincide with four bands attributed earlier to neutral C60 bands, and in addition also with several to date unexplained bands. Abundance and collision theory estimates furthermore indicate that [C60-Metal]+ could plausibly form and survive in astrophysical environments. Hence, [C60-Metal]+ are proposed as promising carriers, in supplement to C60, of astronomical infrared emission bands, potentially representing the largest molecular species in space other than the bare fullerenes C60, C60+, and C70. This work opens a new chapter for studying cosmic fullerene species and carbon chemistry in the Universe.

astro-ph.GA↗

arXiv2022

Route towards complete 3D hydro-chemical simulations of companion-perturbed AGB outflows

Low- and intermediate mass stars experience a significant mass loss during the last phases of their evolution, which obscures them in a vast, dusty envelope. Although it has long been thought this envelope is generally spherically symmetric in shape, recent high-resolution observations find that most of these stars exhibit complex and asymmetrical morphologies, most likely resulting from binary interaction. In order to improve our understanding about these systems, theoretical studies are needed in the form of numerical simulations. Currently, a handful of simulations exist, albeit they mainly focus on the hydrodynamics of the outflow. Hence, we here present the pathway to more detailed and accurate modelling of companion-perturbed outflows with Phantom, by discussing the missing but crucial physical and chemical processes. With these state-of-the-art simulations we aim to make a direct comparison with observations to unveil the true identity on the embedded systems.

astro-ph.SR↗