arXiv subjects

Leo Joon Il Moon

Publications and source records attributed to Leo Joon Il Moon.

6 recordsLinked to original sources

arXiv2026

Tunable Mpemba Effect in a Prethermal Many-Body Spin Network

Relaxation in an interacting system is determined not only by its initial distance from equilibrium, but also by the relaxation modes populated by the initial state. Here we experimentally observe and control the Mpemba effect, in which a state farther from equilibrium overtakes one initially closer, in an extended, disordered $^{13}$C nuclear-spin network in diamond. Field cycling allows us to prepare distinct spatial polarization profiles by independently controlling hyperpolarization and defect-mediated relaxation. We then track their evolution under Floquet driving, which stabilizes a long-lived prethermal regime. We observe reproducible Mpemba crossings and tune the crossing time over several orders of magnitude, from late-time thermalization into the prethermal plateau. Semiclassical simulations show that randomly positioned paramagnetic defects create fast-relaxing regions and defect-poor regions that support the slowest collective relaxation mode. The Mpemba crossings are set by the initial state overlap with this mode. Our results demonstrate anomalous relaxation within a prethermal many-body regime and identify disorder, transport, and mode-selective state preparation as resources for controlling relaxation in extended spin networks.

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arXiv2026

Prethermal rotating-frame solid echo in a dipolar nuclear-spin network

Floquet prethermalization can endow interacting quantum solids with long-lived, approximately conserved quantities, enabling Hamiltonian engineering and new dynamical probes. Using a hyperpolarized network of dipolar-coupled $^{13}$C nuclear spins in diamond driven by pulsed spin-locking, we access a rotating-frame prethermal plateau with quasi-conserved transverse magnetization and cycle-resolved inductive readout. Within this prethermal manifold we observe a robust \emph{rotating-frame solid echo}: after an apparent decay of the rotating-frame free-induction signal over a delay $τ$, the magnetization revives at time $2τ$ following a single $(α)_y$ pulse, with maximum amplitude near $α\simeqπ/2$. The echo envelope decays as a stretched exponential with characteristic time $T_2'\approx 13\,$ms. Analytical arguments and toy-model simulations attribute the revival to Floquet micromotion that transfers coherences between operator subspaces, so that only a subset of the many-body dephasing dynamics is inverted by the $y$ pulse. These results translate classic echo physics into the prethermal rotating frame and point to continuously interrogated prethermal spin ensembles as a versatile platform for high-throughput spectroscopy, Hamiltonian engineering, and long-duration quantum sensing.

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arXiv2026

Sensing with discrete time crystals

Prethermal discrete time crystals (PDTCs) are a nonequilibrium state of matter characterized by long-range spatiotemporal order, and exhibiting a subharmonic response stabilized by many-body interactions under periodic driving. The inherent robustness of time crystalline order to perturbations in the drive protocol makes DTCs promising for applications in quantum technologies. We exploit the susceptibility of PDTC order to deviations in its order parameter to devise highly frequency-selective quantum sensors for time-varying (AC) magnetic fields in a system of strongly-driven, dipolar-coupled 13C nuclear spins in diamond. Integrating a time-varying AC field into the PDTC allows us to exponentially increase its lifetime, with improvements of up to three orders of magnitude (44,204 cycles), and results in a strong resonant response in the time crystalline order parameter. The linewidth of our sensor is limited by the PDTC lifetime alone, as strong interspin interactions help stabilize DTC order. The sensor operates in the 0.5-50kHz range - a challenging frequency regime for sensors based on atomic vapor or electronic spins - and attains a competitive sensitivity. PDTC sensors are resilient to errors in the drive protocol and sample inhomogeneities, and are agnostic to the macroscopic details of the physical platform: the underlying physical principle applies equally to superconducting qubits, neutral atoms, and trapped ions.

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arXiv2024

Anomalously extended Floquet prethermal lifetimes and applications to long-time quantum sensing

Floquet prethermalization is observed in periodically driven quantum many-body systems where the system avoids heating and maintains a stable, non-equilibrium state, for extended periods. Here we introduce a novel quantum control method using off-resonance and short-angle excitation to significantly extend Floquet prethermal lifetimes. This is demonstrated on randomly positioned, dipolar-coupled, 13C nuclear spins in diamond, but the methodology is broadly applicable. We achieve a lifetime $T_2'~800 s at 100 K while tracking the transition to the prethermal state quasi-continuously. This corresponds to a >533,000-fold extension over the bare spin lifetime without prethermalization, and constitutes a new record both in terms of absolute lifetime as well as the total number of Floquet pulses applied (here exceeding 7 million). Using Laplace inversion, we develop a new form of noise spectroscopy that provides insights into the origin of the lifetime extension. Finally, we demonstrate applications of these extended lifetimes in long-time, reinitialization-free quantum sensing of time-varying magnetic fields continuously for ~10 minutes at room temperature. Our work facilitates new opportunities for stabilizing driven quantum systems through Floquet control, and opens novel applications for continuously interrogated, long-time responsive quantum sensors.

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arXiv2024

Experimental observation of a time rondeau crystal: Temporal Disorder in Spatiotemporal Order

Our understanding of phases of matter relies on symmetry breaking, one example being water ice whose crystalline structure breaks the continuous translation symmetry of space. Recently, breaking of time translation symmetry was observed in systems not in thermal equilibrium. The associated notion of time crystallinity has led to a surge of interest, raising the question about the extent to which highly controllable quantum simulators can generate rich and tunable temporal orders, beyond the conventional classification of order in static systems. Here, we investigate different kinds of partial temporal orders, stabilized by non-periodic yet structured drives, which we call rondeau order. Using a $^{13}$C-nuclear-spin diamond quantum simulator, we report the first experimental observation of a -- tunable degree of -- short-time disorder in a system exhibiting long-time stroboscopic order. This is based on a novel spin control architecture that allows us to implement a family of drives ranging from structureless via structured random to quasiperiodic and periodic drives. Leveraging a high throughput read-out scheme, we continuously observe the spin polarization over 105 pulses to probe rondeau order, with controllable lifetimes exceeding 4 seconds. Using the freedom in the short-time temporal disorder of rondeau order, we show the capacity to encode information in the response of observables. Our work broadens the landscape of observed nonequilibrium temporal order, paving the way for new applications harnessing driven quantum matter.

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arXiv2024

Hamiltonian-reconstruction distance as a success metric for the Variational Quantum Eigensolver

The Variational Quantum Eigensolver (VQE) is a hybrid quantum-classical algorithm for quantum simulation that can be run on near-term quantum hardware. A challenge in VQE -- as well as any other heuristic algorithm for finding ground states of Hamiltonians -- is to know how close the algorithm's output solution is to the true ground state, when the true ground state and ground-state energy are unknown. This is especially important in iterative algorithms, such as VQE, where one wants to avoid erroneous early termination. Recent developments in Hamiltonian reconstruction -- the inference of a Hamiltonian given an eigenstate -- give a metric can be used to assess the quality of a variational solution to a Hamiltonian-eigensolving problem. This metric can assess the proximity of the variational solution to the ground state without any knowledge of the true ground state or ground-state energy. In numerical simulations and in demonstrations on a cloud-based trapped-ion quantum computer, we show that for examples of both one-dimensional transverse-field-Ising (11 qubits) and two-dimensional J1-J2 transverse-field-Ising (6 qubits) spin problems, the Hamiltonian-reconstruction distance gives a helpful indication of whether VQE has yet found the ground state or not. Our experiments included cases where the energy plateaus as a function of the VQE iteration, which could have resulted in erroneous early stopping of the VQE algorithm, but where the Hamiltonian-reconstruction distance correctly suggests to continue iterating. We find that the Hamiltonian-reconstruction distance has a useful correlation with the fidelity between the VQE solution and the true ground state. Our work suggests that the Hamiltonian-reconstruction distance may be a useful tool for assessing success in VQE, including on noisy quantum processors in practice.

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