arXiv subjects

Leonid P. Rokhinson

Publications and source records attributed to Leonid P. Rokhinson.

At least 19 recordsLinked to original sources

arXiv2025

Characterization of superconducting germanide and germanosilicide films of Pd, Pt, Rh and Ir formed by solid-phase epitaxy

Facilitated by recent advances in strained Ge/SiGe quantum well (QW) growth technology, superconductor-semiconductor hybrid devices based on group IV materials have been developed, potentially augmenting the functionality of quantum circuits. The formation of highly transparent superconducting platinum germanosilicide (PtSiGe) contacts to Ge/SiGe heterostructures by solid-phase epitaxy between Pt and SiGe has recently been reported, although with a relatively low critical temperature $<1\,\mathrm{K}$. Here, we present a comparative study of the superconducting properties of Pt, Pd, Rh, and Ir germanides, along with an in-depth characterization of Ir(Si)Ge films formed by solid-phase epitaxy. For films fabricated under optimal epitaxy conditions, we report $T_\mathrm{c}=3.4\,\mathrm{K}$ ($2.6\,\mathrm{K}$ for IrGe (IrSiGe). High-resolution scanning transmission electron microscopy (HRSTEM) and energy-dispersive X-ray spectroscopy (EDX) reveal that Ir reacts with Ge substrates to form a polycrystalline IrGe layer with a sharp IrGe/Ge interface.

cond-mat.supr-con↗

arXiv2025

Towards a hybrid 3D transmon qubit with topological insulator-based Josephson junctions

Superconducting quantum circuits provide a versatile platform for studying quantum materials by leveraging precise microwave control and utilizing the tools of circuit quantum electrodynamics (QED). Hybrid circuit devices incorporating novel quantum materials could also lead to new qubit functionalities, such as gate tunability and noise resilience. Here, we report experimental progress towards a transmon-like qubit made with a superconductor-topological insulator-superconductor (S-TI-S) Josephson junction using exfoliated BiSbTeSe2. We present a design that enables us to systematically characterize the hybrid device, from DC transport of the S-TI-S junction, to RF spectroscopy, to full circuit QED control and measurement of the hybrid qubit. In addition, we utilize a high-quality-factor superconducting cavity to characterize material and fabrication-induced losses, thereby guiding our efforts to improve device quality.

cond-mat.mes-hall↗

arXiv2024

Influence of disorder on antidot vortex Majorana states in 3D topological insulators

Topological insulator/superconductor two-dimensional heterostructures are promising candidates for realizing topological superconductivity and Majorana modes. In these systems, a vortex pinned by a pre-fabricated antidot in the superconductor can host Majorana zero-energy modes (MZMs), which are exotic quasiparticles that may enable quantum information processing. However, a major challenge is to design devices that can manipulate the information encoded in these MZMs. One of the key factors is to create small and clean antidots, so the MZMs, localized in the vortex core, have a large gap to other excitations. If the antidot is too large or too disordered, the level spacing for the subgap vortex states may become smaller than temperature. In this paper, we numerically investigate the effects of disorder, chemical potential, and antidot size on the subgap vortex spectrum, using a two-dimensional effective model of the topological insulator surface. Our model allows us to simulate large system sizes with vortices up to 1.8 $μ$m in diameter (with a 6 nm lattice constant). We also compare our disorder model with the transport data from existing experiments. We find that the spectral gap can exhibit a non-monotonic behavior as a function of disorder strength, and that it can be tuned by applying a gate voltage.

cond-mat.mes-hall↗

arXiv2023

Diamagnetic mechanism of critical current non-reciprocity in multilayered superconductors

Recent excitement in observation of non-reciprocal critical current (NRC) is motivated by a suggestion that "superconducting diode effect" may be an intrinsic property of non-centrosymmetric superconductors with strong spin-orbit interactions[1]. Theoretically it has been understood that linear in the Cooper pair momentum terms, caused by the Rashba spin-orbit and Zeeman interactions or, more generally, any symmetry-allowed Lifshitz invariants[2] in uniform singlet superconductors, do not contribute to the supercurrent, although the role of higher-order terms remains unclear[3, 4]. In this work we show that critical current non-reciprocity is a generic property of multilayered superconductor structures in the presence of magnetic field-generated diamagnetic currents. In the regime of an intermediate coupling between the layers, the Josephson vortices are predicted to form at high fields and currents. We report the observation of NRC in nanowires fabricated from InAs/Al heterostructures. The effect is independent of the crystallographic orientation of the wire, ruling out an intrinsic origin of NRC. Non-monotonic NRC evolution with magnetic field is consistent with the generation of diamagnetic currents and formation of the Josephson vortices. This extrinsic NRC mechanism can be used to design novel devices for superconducting circuits.

cond-mat.supr-con↗

arXiv2022

Discovery of a high-temperature antiferromagnetic state and transport signatures of exchange interactions in a Bi2Se3/EuSe heterostructure

Spatial confinement of electronic topological surface states (TSS) in topological insulators poses a formidable challenge because TSS are protected by time-reversal symmetry. In previous works formation of a gap in the electronic spectrum of TSS has been successfully demonstrated in topological insulator/magnetic material heterostructures, where ferromagnetic exchange interactions locally lifts the time-reversal symmetry. Here we report an experimental evidence of exchange interaction between a topological insulator Bi2Se3 and a magnetic insulator EuSe. Spin-polarized neutron reflectometry reveals a reduction of the in-plane magnetic susceptibility within a 2 nm interfacial layer of EuSe, and the combination of SQUID magnetometry and Hall measurements points to the formation of an antiferromagnetic layer with at least five-fold enhancement of Néel's temperature. Abrupt resistance changes in high magnetic fields indicate interfacial exchange coupling that affects transport in a TSS. High temperature local control of TSS with zero net magnetization unlocks new opportunities for the design of electronic, spintronic and quantum computation devices, ranging from quantization of Hall conductance in zero fields to spatial localization of non-Abelian excitations in superconducting topological qubits.

cond-mat.mes-hall↗

arXiv2022

A Platform for Braiding Majorana Modes with Magnetic Skyrmions

After a decade of intense theoretical and experimental efforts, demonstrating braiding of Majorana modes remains an unsolved problem in condensed matter physics due to platform specific challenges. In this work, we propose topological superconductor -- magnetic multilayer heterostructures with on-chip microwave cavity readout as a novel platform for initializing, braiding and reading out Majorana modes. Stray fields from a skyrmion in the magnetic layers can nucleate a vortex in the topological superconducting layer. Such a vortex is known to host Majorana bound states at its core. Through analytical calculations within London and Thiele formalisms, and through micromagnetic simulations, we show that our nucleation and braiding scheme can be effectively realized with a variety of existing options for magnetic and superconducting layers. Further, we show that the coupling of the Majorana bound states to electric field of a resonator leads to an experimentally observable parity-dependent dispersive shift of the resonator frequency. Our work paves the way for realizing Majorana braiding in the near future.

cond-mat.mes-hall↗

arXiv2021

Observation of coexisting weak localization and superconducting fluctuations in strained Sn1-xInxTe thin films

Topological superconductors have attracted tremendous excitement as they are predicted to host Majorana zero modes that can be utilized for topological quantum computing. Candidate topological superconductor Sn1-xInxTe thin films (0<x<0.3) grown by molecular beam epitaxy and strained in the (111) plane are shown to host three coexisting quantum effects: localization, antilocalization and superconducting fluctuations above the critical temperature Tc. An analysis of the normal state magnetoresistance reveals these effects. Weak localization is consistently observed in superconducting samples, indicating that superconductivity originates dominantly from trivial valence band states that may be strongly spin-orbit split. A large enhancement of the conductivity is observed above Tc, indicating that quantum coherent quasiparticle effects coexist with superconducting fluctuations. Our results motivate a re-examination of the debated pairing symmetry of this material when subjected to quantum confinement and lattice strain.

cond-mat.supr-con↗

arXiv2021

Epitaxial growth and magnetic characterization of EuSe thin films with various crystalline orientations

We report different growth modes and corresponding magnetic properties of thin EuSe films grown by molecular beam epitaxy on BaF2, Pb1-xEuxSe, GaAs, and Bi2Se3 substrates. We show that EuSe growth predominantly in (001) orientation on GaAs(111) and Bi2Se3, but along (111) crystallographic direction on BaF2 (111) and Pb1-xEuxSe (111). High-resolution transmission electron microscopy measurements reveal an abrupt and highly crystalline interface for both (001) and (111) EuSe films. In agreement with previous studies, ordered magnetic phases include antiferromagnetic, ferrimagnetic, and ferromagnetic phases. In contrast to previous studies, we found strong hysteresis for the antiferromagnetic-ferrimagnetic transition. An ability to grow epitaxial films of EuSe on Bi2Se3 and of Bi2Se3 on EuSe enables further investigation of interfacial exchange interactions between various phases of an insulating metamagnetic material and a topological insulator.

cond-mat.mtrl-sci↗

arXiv2021

Transport in helical Luttinger liquids in the fractional quantum Hall regime

Domain walls in fractional quantum Hall ferromagnets are gapless helical one-dimensional channels formed at the boundaries of topologically distinct quantum Hall (QH) liquids. Naïvely, these helical domain walls (hDWs) constitute two counter-propagating chiral states with opposite spins. Coupled to an s-wave superconductor, helical channels are expected to lead to topological superconductivity with high order non-Abelian excitations. Here we investigate transport properties of hDWs in the $ν=2/3$ fractional QH regime. Experimentally we found that current carried by hDWs is substantially smaller than the prediction of the naïve model. Luttinger liquid theory of the system reveals redistribution of currents between quasiparticle charge, spin and neutral modes, and predicts the reduction of the hDW current. Inclusion of spin-non-conserving tunneling processes reconciles theory with experiment. The theory confirms emergence of spin modes required for the formation of fractional topological superconductivity.

cond-mat.mes-hall↗

arXiv2019

Highly skewed current-phase relation in superconductor-topological insulator-superconductor Josephson junctions

Three-dimensional topological insulators (TI's) in proximity with superconductors are expected to exhibit exotic phenomena such as topological superconductivity (TSC) and Majorana bound states (MBS), which may have applications in topological quantum computation. In superconductor-TI-superconductor Josephson junctions, the supercurrent versus the phase difference between the superconductors, referred to as the current-phase relation (CPR), reveals important information including the nature of the superconducting transport. Here, we study the induced superconductivity in gate-tunable Josephson junctions (JJs) made from topological insulator BiSbTeSe2 with superconducting Nb electrodes. We observe highly skewed (non-sinusoidal) CPR in these junctions. The critical current, or the magnitude of the CPR, increases with decreasing temperature down to the lowest accessible temperature (T ~ 20 mK), revealing the existence of low-energy modes in our junctions. The gate dependence shows that close to the Dirac point the CPR becomes less skewed, indicating the transport is more diffusive, most likely due to the presence of electron/hole puddles and charge inhomogeneity. Our experiments provide strong evidence that superconductivity is induced in the highly ballistic topological surface states (TSS) in our gate-tunable TI- based JJs. Furthermore, the measured CPR is in good agreement with the prediction of a model which calculates the phase dependent eigenstate energies in our system, considering the finite width of the electrodes as well as the TSS wave functions extending over the entire circumference of the TI.

cond-mat.supr-con↗

arXiv2019

Anomalous low-temperature enhancement of supercurrent in topological-insulator nanoribbon Josephson junctions: evidence for low-energy Andreev bound states

We report anomalous enhancement of the critical current at low temperatures in gate-tunable Josephson junctions made from topological insulator BiSbTeSe$_2$ nanoribbons with superconducting Nb electrodes. In contrast to conventional junctions, as a function of the decreasing temperature $T$, the increasing critical current $I_c$ exhibits a sharp upturn at a temperature $T_*$ around 20$\%$ of the junction critical temperatures for several different samples and various gate voltages. The $I_c$ vs. $T$ demonstrates a short junction behavior for $T>T_*$, but crosses over to a long junction behavior for $T<T_*$ with an exponential $T$-dependence $I_c \propto \exp\big(-k_B T/δ\big)$, where $k_B$ is the Boltzmann constant. The extracted characteristic energy-scale $δ$ is found to be an order of magnitude smaller than the induced superconducting gap of the junction. We attribute the long-junction behavior with such a small $δ$ to low-energy Andreev bound states (ABS) arising from winding of the electronic wavefunction around the circumference of the topological insulator nanoribbon (TINR). Our TINR-based Josephson junctions with low-energy ABS are promising for future topologically protected devices that may host exotic phenomena such as Majorana fermions.

cond-mat.supr-con↗

arXiv2017

Gate-tunable supercurrent and multiple Andreev reflections in a superconductor-topological insulator nanoribbon-superconductor hybrid device

We report on the observation of gate-tunable proximity-induced superconductivity and multiple Andreev reflections (MAR) in a bulk-insulating BiSbTeSe$_2$ topological insulator nanoribbon (TINR) Josephson junction (JJ) with superconducting Nb contacts. We observe a gate-tunable critical current ($I_C$) for gate voltages ($V_g$) above the charge neutrality point ($V_{CNP}$), with $I_C$ as large as 430 nA. We also observe MAR peaks in the differential conductance ($dI/dV$) versus DC voltage ($V_{dc}$) across the junction corresponding to sub-harmonic peaks (at $V_{dc} = V_n = 2Δ_{Nb}/en$, where $Δ_{Nb}$ is the superconducting gap of the Nb contacts and $n$ is the sub-harmonic order). The sub-harmonic order, $n$, exhibits a $V_g$-dependence and reaches $n = 13$ for $V_g = 40$ V, indicating the high transparency of the Nb contacts to TINR. Our observations pave the way toward exploring the possibilities of using TINR in topologically protected devices that may host exotic physics such as Majorana fermions.

cond-mat.mes-hall↗

arXiv2017

Parafermion supporting platform based on spin transitions in the fractional quantum Hall effect regime

We propose an experimentally-feasible system based on spin transitions in the fractional quantum Hall effect regime where parafermions, high-order non-abelian excitations, can be potentially realized. We provide a proof-of-concept experiments showing that in specially designed heterostructures spin transitions at a filling factor 2/3 can be induced electrostatically, allowing local control of polarization and on-demand formation of helical domain walls with fractionalized charge excitations, a pre-requisite ingredient for parafermions formation. We also present exact diagonalization numerical studies of domain walls formed between domains with different spin polarization in the fractional quantum Hall effect regime and show that they indeed possess electronic and magnetic structure needed for parafermion formation when coupled to an s-wave superconductor.

cond-mat.mes-hall↗

arXiv2017

Mesoscopic transport in electrostatically-defined spin-full channels in quantum Hall ferromagnets

In this work we use electrostatic control of quantum Hall ferromagnetic transitions in CdMnTe quantum wells to study electron transport through individual domain walls (DWs) induced at a specific location. These DWs are formed due to hybridization of two counter-propagating edge states with opposite spin polarization. Conduction through DWs is found to be symmetric under magnetic field direction reversal, consistent with the helical nature of these DWs. We observe that long domain walls are in the insulating regime with localization length 4 - 6~$μ$m. In shorter DWs the resistance saturates to a non-zero value at low temperatures. Mesoscopic resistance fluctuations in a magnetic field are investigated. The theoretical model of transport through impurity states within the gap induced by spin-orbit interactions agrees well with the experimental data. Helical DWs have required symmetry for the formation of synthetic p-wave superconductors. Achieved electrostatic control of a single helical domain wall is a milestone on the path to their reconfigurable network and ultimately to a demonstration of braiding of non-Abelian excitations.

cond-mat.mes-hall↗

arXiv2016

Electrostatic control of quantum Hall ferromagnetic transition, a step toward reconfigurable network of helical channels

Ferromagnetic transitions between quantum Hall states with different polarization at a fixed filling factor can be studied by varying the ratio of cyclotron and Zeeman energies in tilted magnetic field experiments. However, an ability to locally control such transitions at a fixed magnetic field would open a range of attractive applications, e.g. formation of a reconfigurable network of one-dimensional helical domain walls in a two-dimensional plane. Coupled to a superconductor, such domain walls can support non-Abelian excitation. In this article we report development of heterostructures where quantum Hall ferromagnetic (QHFm) transition can be controlled locally by electrostatic gating. A high mobility two-dimensional electron gas is formed in CdTe quantum wells with engineered placement of paramagnetic Mn impurities. Gate-induced electrostatic field shifts electron wavefunction in the growth direction and changes overlap between electrons in the quantum well and d-shell electrons on Mn, thus controlling the s-d exchange interaction and the field of the QHFm transition. The demonstrated shift of the QHFm transition at a filling factor $ν=2$ is large enough to allow full control of spin polarization at a fixed magnetic field.

cond-mat.mes-hall↗

arXiv2015

Induced superconductivity in high mobility two dimensional electron gas in GaAs heterostructures

Introduction of a Josephson field effect transistor (JoFET) concept sparked active research on proximity effects in semiconductors. Induced superconductivity and electrostatic control of critical current has been demonstrated in two-dimensional gases in InAs, graphene and topological insulators, and in one-dimensional systems including quantum spin Hall edges. Recently, interest in superconductor-semiconductor interfaces was renewed by the search for Majorana fermions, which were predicted to reside at the interface. More exotic non-Abelian excitations, such as parafermions (fractional Majorana fermions) or Fibonacci fermions may be formed when fractional quantum Hall edge states interface with superconductivity. In this paper we develop transparent superconducting contacts to high mobility two-dimensional electron gas (2DEG) in GaAs and demonstrate induced superconductivity across several microns. Supercurrent in a ballistic junction has been observed across 0.6 $μ$m of 2DEG, a regime previously achieved only in point contacts but essential to the formation of well separated non-Abelian states. High critical fields ($>16$ Tesla) in NbN contacts enables investigation of a long-sought regime of an interplay between superconductivity and strongly correlated states in a 2DEG at high magnetic fields.

cond-mat.mes-hall↗

arXiv2015

Magnetic field induced helical mode and topological transitions in a quasi-ballistic topological insulator nanoribbon with circumferentially quantized surface state sub-bands

A topological insulator (TI) nanowire (NW), where the core is insulating and the 2D spin-helical Dirac fermion topological surface states (TSS) are circumferentially quantized into a series of 1D sub-bands, promises novel topological physics and applications. An axial magnetic flux (Φ) through the core drives periodic topological transitions in the surface sub-bands, changing from being all doubly-degenerate with a gapped Dirac point (DP) at integer (including zero) flux quanta (Φ$_0$ = h/e, with h being the Planck constant and e the electron charge), to contain a topologically-protected, non-degenerate 1D spin helical mode with restored DP at half-integer flux quanta. The resulting magnetoconductance is predicted to exhibit Aharonov-Bohm oscillations (ABO) with maxima occurring alternatively at half-integer or integer flux quanta (referred to as π-ABO or 0-ABO), depending periodically on the Fermi wavevector (k$_F$, with period 2π/C, C being the NW circumference). Here, we report a clear observation of such k$_F$-periodic alternations between 0-ABO and π-ABO in Bi$_2$Te$_3$ TI nanoribbon (NR, a rectangular cross sectional NW) field effect devices, which exhibit quasi-ballistic transport over ~2 μm (as manifested in length-independent conductance, exponential decaying ABO amplitude with increasing temperature (T), and an 1/T dependence of the extracted phase coherence length). The conductances as functions of the gate voltage at half and zero flux quanta also exhibit clear, but anti-correlated oscillations periodic in k$_F$ (with period 2π/C, equivalently when C encloses an integer multiples of Fermi wavelength 2π/k$_F$), consistent with the circumferentially quantized surface sub-bands. We also extract the minimal Fermi energy and momentum for TSS to emerge out of the bulk valence band, in agreement with the known Bi$_2$Te$_3$ bandstructure.

cond-mat.mes-hall↗

arXiv2014

Gate Tunable Relativistic Mass and Berry$'$s phase in Topological Insulator Nanoribbon Field Effect Devices

Transport due to spin-helical massless Dirac fermion surface state is of paramount importance to realize various new physical phenomena in topological insulators, ranging from quantum anomalous Hall effect to Majorana fermions. However, one of the most important hallmarks of topological surface states, the Dirac linear band dispersion, has been difficult to reveal directly in transport measurements. Here we report experiments on Bi2Te3 nanoribbon ambipolar field effect devices on high-k SrTiO3 substrates, where we achieve a gate-tuned bulk metal-insulator transition and the topological transport regime with substantial surface state conduction. In this regime, we report two unambiguous transport evidences for gate-tunable Dirac fermions through π Berry$'$s phase in Shubnikov-de Haas oscillations and effective mass proportional to the Fermi momentum, indicating linear energy-momentum dispersion. We also measure a gate-tunable weak anti-localization (WAL) with 2 coherent conduction channels (indicating 2 decoupled surfaces) near the charge neutrality point, and a transition to weak localization (indicating a collapse of the Berry$'$s phase) when the Fermi energy approaches the bulk conduction band. The gate-tunable Dirac fermion topological surface states pave the way towards a variety of topological electronic devices.

cond-mat.mes-hall↗