arXiv subjects

Li-kun Shi

Publications and source records attributed to Li-kun Shi.

At least 19 recordsLinked to original sources

arXiv2025

High-Temperature Quantum Oscillations of a Non-equilibrium Non-Fermi Liquid

A periodically driven Fermi gas coupled to a simple boson bath reaches a non-equilibrium steady-state occupation with sharp non-analyticities at certain momenta. Here, we demonstrate that these non-analyticities behave as emergent Fermi surfaces by showing that they give rise to quantum oscillations of observables with a period controlled by the effective Fermi surface area enclosed by these non-analyticities. However, these oscillations have several striking differences with standard equilibrium quantum oscillations. For example, they remain non-analytic at finite temperatures, their amplitude can survive up to extremely high temperatures comparable to the frequency of the drive, and they can display non-monotonic temperature dependence completely at odds with standard Lifshits-Kosevich behavior.

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arXiv2025

Dissipation-Shaped Quantum Geometry in Nonlinear Transport

The theory of the intrinsic nonlinear Hall effect, a key probe of quantum geometry, is plagued by conflicting expressions for the conductivity that is independent of the dissipation strength (rate, $\Gamma^0$). We clarify the origin of this ambiguity by demonstrating that the "intrinsic" response is not universal, but is inextricably linked to the dissipation mechanism that establishes the non-equilibrium steady state (NESS). We establish a benchmark by solving the exact NESS density matrix for a generic Bloch system coupled to a featureless fermionic bath. Our exact $\Gamma^0$ conductivity decomposes into two parts: (i) a geometric contribution, $\sigma^{\text{geo}}$, whose form recovers the intraband quantum metric contribution ($\sim\partial_k g$), providing an exact derivation that clarifies inconsistencies in the literature, and (ii) a novel, purely kinetic contribution, $\sigma^{\text{kin}} \propto v^3 f^{(4)}_0$, which is absent when dissipation is modeled by white-noise disorder (e.g., a constant-$\Gamma$ Green's function model). The discrepancy in $\sigma^{\text{kin}}$ between these distinct physical mechanisms is a proof that the $\Gamma^0$ nonlinear conductivity is not a unique property of the Bloch Hamiltonian, but is contingent on the physical system-bath coupling.

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arXiv2025

Algebraic Exact Solution for Driven Landau Levels in Two-dimensional Electron Gases

Controlling quantum systems with time-dependent fields opens avenues for engineering novel states of matter and exploring non-equilibrium phenomena. Landau levels in two-dimensional electron gases (2DEGs), with their discrete energy spectrum and characteristic cyclotron dynamics, provide an important platform for realizing and studying such driven quantum systems. While exact solutions for driven Landau levels exist, they have been limited to specific gauges or representations. In this work, we present an algebraic, gauge- and representation-independent exact solution for driven Landau levels in 2DEGs subject to arbitrary time-dependent electromagnetic fields. Our approach, based on a time-dependent unitary transformation via the displacement operator, provides clear physical insights into the driven quantum dynamics. We apply this method to derive the exact Floquet states and quasienergies for periodically driven Landau levels, and we extend our analysis to the resonant driving regime, where the Floquet picture breaks down and the electron wavefunction exhibits unbounded spatial spreading. Furthermore, we calculate the instantaneous energy absorption rate, revealing distinct absorption behaviors between coherent states and Fock or thermal states, stemming from quantum interference effects.

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arXiv2024

Ultra-critical Floquet Non-Fermi Liquid

We demonstrate that periodically driven Fermions coupled to simple bosonic baths have steady state occupations of Floquet Bloch bands that generically display non-analyticties at certain momenta which resemble the Fermi surfaces of equilibrium non-Fermi liquids. Remarkably these non-equilibrium Fermi surfaces remain sharp even when the bath is at finite temperature, leading to critical power-law decaying correlations at finite temperature, a phenomenon with no analogue in equilibrium. We also show that generically there is in-gap current rectification for clean metals lacking inversion symmetry, and explain why this occurs universally regardless of the details of collisions.

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arXiv2023

The Floquet Fermi Liquid

We demonstrate the existence of a non-equilibrium "Floquet Fermi Liquid" state arising in partially filled Floquet Bloch bands weakly coupled to ideal fermionic baths, which possess a collection of "Floquet Fermi surfaces" enclosed inside each other, resembling matryoshka dolls. We elucidate several properties of these states, including their quantum oscillations under magnetic fields which feature slow beating patterns of their amplitude reflecting the different areas of the Floquet Fermi surfaces, consistent with those observed in microwave induced resistance oscillation experiments. We also investigate their specific heat and thermodynamic density of states and demonstrate how by controlling properties of the drive, such as its frequency, one can tune some of the Floquet Fermi surfaces towards non-equilibrium van-Hove singularities without changing the electron density.

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arXiv2023

The Fermi-Dirac staircase occupation of Floquet bands and current rectification inside the optical gap of metals: a rigorous perspective

We consider a model of a Bloch band subjected to an oscillating electric field and coupled to a featureless fermionic heat bath, which can be solved exactly. We demonstrate rigorously that in the limit of vanishing coupling to this bath (so that it acts as an ideal thermodynamic bath) the occupation of the Floquet band is not a simple Fermi-Dirac distribution function of the Floquet energy, but instead it becomes a ``staircase'' version of this distribution. We show that this distribution generically leads to a finite rectified electric current within the optical gap of a metal even in the limit of vanishing carrier relaxation rates, providing a rigorous demonstration that such rectification is generically possible and clarifying previous statements in the optoelectronics literature. We show that this current remains non-zero even up to the leading perturbative second order in the amplitude of electric fields, and that it approaches the standard perturbative expression of the Jerk current obtained from a simpler Boltzmann description within a relaxation time approximation when the frequencies are small compared to the bandwidth.

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arXiv2022

The Berry dipole photovoltaic demon and the thermodynamics of photo-current generation within the optical gap of metals

We dismantle the previously held misconception that it is impossible for bulk rectification mechanisms to induce a net DC electric current when the frequency of the impinging radiation lies within the optical gap of a metal in the limit of small carrier relaxation rates. We argue that generically such in-gap rectification mechanisms are irreversible and accompanied by a continuous exchange of energy with a heat bath and must also be necessarily accompanied by a small but finite absorption of radiation in order to guarantee the positivity of the net entropy production and abide by the second law of thermodynamics. We show, however, that the intra-band non-linear Hall effect arising from the Berry curvature is a special kind of in-gap rectification mechanism that behaves as a ``photo-voltaic demon'', namely it can operate as an ideal reversible and dissipationless conveyor of energy between the radiation and an external circuit. Its reversible nature allows for an interesting mode of operation as an amplifier of circularly polarized light, whose efficiency can approach 100%, and which could be technologically promising especially in the infrared frequency range.

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arXiv2022

Defect bulk-boundary correspondence of topological skyrmion phases of matter

Unpaired Majorana zero-modes are central to topological quantum computation schemes as building blocks of topological qubits, and are therefore under intense experimental and theoretical investigation. Their generalizations to parafermions and Fibonacci anyons are also of great interest, in particular for universal quantum computation schemes. In this work, we find a different generalization of Majorana zero-modes in effectively non-interacting systems, which are zero-energy bound states that exhibit a cross structure -- two straight, perpendicular lines in the complex plane -- composed of the complex number entries of the zero-mode wavefunction on a lattice, rather than a single straight line formed by complex number entries of the wavefunction on a lattice as in the case of an unpaired Majorana zero-mode. These cross zero-modes are realized for topological skyrmion phases under certain open boundary conditions when their characteristic momentum-space spin textures trap topological defects. They therefore serve as a second type of bulk-boundary correspondence for the topological skyrmion phases. In the process of characterizing this defect bulk-boundary correspondence, we develop recipes for constructing physically-relevant model Hamiltonians for topological skyrmion phases, efficient methods for computing the skyrmion number, and introduce three-dimensional topological skyrmion phases into the literature.

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arXiv2021

Polariton-drag enabled quantum geometric photocurrents in high symmetry materials

Lowered symmetry enables access to a wide set of responses not typically accessible in high symmetry materials. Prime examples are time-reversal forbidden quantum geometric photocurrent responses (e.g., linear injection and circular shift photocurrents) that are thought to vanish in non-magnetic materials. Here we argue that polariton-drag processes enable to unblock such quantum geometric photocurrents even in non-magnetic and centrosymmetric materials. Strikingly, we uncover how a cooperative effect between finite q irradiation and the Fermi surface position leads to a polariton selective photoexcitation (PSP). PSP enables to directly address carriers within tight momentum resolved windows of the Fermi surface to yield giant enhancements of quantum geometric photocurrents. This selectivity enables to directly track momentum resolved quantum geometric quantities along the Fermi surface providing a new tool to interrogate the quantum geometry of high symmetry materials.

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arXiv2020

Atomic configuration controlled photocurrent in van der Waals homostructures

Conventional photocurrents at a p-n junction depend on macroscopic built-in fields and are typically insensitive to the microscopic details of a crystal's atomic configuration. Here we demonstrate how atomic configuration can control photocurrent in van der Waals (vdW) materials. In particular, we find bulk shift photocurrents (SPC) can display a rich (atomic) configuration dependent phenomenology that range from contrasting SPC currents for different stacking arrangements in a vdW homostructure (e.g., AB vs BA stacking) to a strong light polarization dependence for SPC that align with crystallographic axes. Strikingly, we find that SPC in vdW homostructures can be directed by modest strain, yielding sizeable photocurrent magnitudes under unpolarized light irradiation and manifesting even in the absence of p-n junctions. These demonstrate that SPC are intimately linked to how the Bloch wavefunctions are embedded in real space, and enables a new macroscopic transport probe (photocurrent) of lattice-scale registration in vdW materials.

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arXiv2020

Geometric photon-drag effect and nonlinear shift current in centrosymmetric crystals

The nonlinear shift current, also known as the bulk photovoltaic current generated by linearly polarized light, has long been known to be absent in crystals with inversion symmetry. Here we argue that a non-zero shift current in centrosymmetric crystals can be activated by a photon-drag effect. Photon-drag shift current proceeds from a `shift current dipole' (a geometric quantity characterizing interband transitions) and manifests a purely transverse response in centrosymmetric crystals. This transverse nature proceeds directly from the shift-vector's pseudovector nature under mirror operation and underscores its intrinsic geometric origin. Photon-drag shift current can greatly enhanced by coupling to polaritons and provides a new and sensitive tool to interrogate the subtle interband coherences of materials with inversion symmetry previously thought to be inaccessible via photocurrent probes.

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arXiv2020

Cooperative orbital moments and edge magnetoresistance in monolayer WTe$_2$

We argue that edge electrons in monolayer WTe$_2$ can possess a "cooperative" orbital moment (COM) that critically impacts its edge magnetoresistance behavior. Arising from the cooperative action of both Rashba and Ising spin orbit coupling, COM quickly achieves large magnitudes (of order few Bohr magnetons) even for relatively small spin-orbit coupling strengths. As we explain, such large COM magnitudes arise from an unconventional cooperative spin canting of edge spins when Rashba and Ising spin orbit coupling act together. Strikingly, COM can compete with spin moments to produce an unusual anisotropic edge magnetoresistance oriented at an oblique angle. In particular, this competition produces a direction along which $\mathbf{B}$ is ineffective at gapping out the edge spectrum leaving it nearly gapless. As a result, large contrasts in gap sizes manifest as $\mathbf{B}$ is rotated granting giant anisotropic magnetoresistance of 0.1-10 million % at 10 T and low temperature.

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arXiv2019

Shift vector as the geometric origin of beam shifts

Goos-Hanchen (GH) and Imbert-Fedorov (IF) shifts are lateral and transverse displacements of a wavepacket reflecting off a surface. A dramatic real-space manifestation of wavepacket phases, they have traditionally been analyzed in a model dependent fashion. Here we argue that GH and IF shifts admit a general geometrical description and arise from a gauge invariant geometric phase. In particular, we show GH/IF shifts can be naturally captured by a shift vector, analogous to the shift vector from shift currents in the bulk photovoltaic effect. Employing Wilson loops to visualize the scattering processes contributing to the shift vector, we separate the shift into an intrinsic (depends solely on the system bulk) and an extrinsic part. This enables to establish a clear model-independent link between symmetry and the presence/absence of intrinsic and extrinsic GH/IF shifts.

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arXiv2019

Gate-tunable flat bands in van der Waals patterned dielectric superlattices

Superlattice engineering provides the means to reshape the fabric felt by quasiparticles moving in a material. Here we argue that bandstructure engineering with superlattices can be pushed to the extreme limit by stacking gapped van der Waals (vdW) materials on patterned dielectric substrates. Specifically, we find that high quality vdW patterned dielectric superlattices (PDS) realize a series of robust flat bands that can be directly switched on and off by gate voltage in situ. In contrast to existing superlattice platforms, these flat bands are realized without the need for fine tuning. Instead, the bands become flat as the gate voltage increases in magnitude. The characteristics of PDS flatbands are highly tunable: the type of flatband (single non-degenerate or dirac-cone-like), localization length, and interaction energy are sensitive to the applied gate voltage. As a result, electron-electron interactions in the PDS flatbands can become stronger than both the bandwidth and disorder broadening, providing a setting for correlated behavior such as flatband ferromagnetism. We expect PDS flatbands can be experimentally realized in a range of readily available gapped vdW materials such as monolayer transition metal dichalcogenides, e.g. WSe2.

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arXiv2019

Non-trivial quantum oscillation geometric phase shift in a trivial band

The accumulation of non-trivial geometric phases in a material's response is often a tell-tale sign of a rich underlying internal structure. Studying quantum oscillations provides one of the ways to determine these geometrical phases, such as Berry's phase, that play a central role in topological quantum materials. We report on magneto-transport measurements in ABA-trilayer graphene, the band structure of which is comprised of a weakly gapped linear Dirac band, nested within a trivial quadratic band. Here we show Shubnikov-de Haas (SdH) oscillations of the quadratic band shifted by a phase that sharply departs from the expected 2$\pi$ Berry's phase. Our analysis reveals that, surprisingly, the anomalous phase shift is non-trivial and is inherited from the non-trivial Berry's phase of the linear Dirac band due to strong filling-enforced constraints between the linear and quadratic band Fermi surfaces. Given that many topological materials contain multiple bands, our work indicates how additional bands, which are thought to obscure the analysis, can actually be exploited to tease out the subtle effects of Berry's phase.

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arXiv2018

Symmetry, spin-texture, and tunable quantum geometry in a WTe$_2$ monolayer

The spin orientation of electronic wavefunctions in crystals is an internal degree of freedom, typically insensitive to electrical knobs. We argue from a general symmetry analysis and a $\vec k \cdot \vec p$ perspective, that monolayer 1T'-WTe$_2$ possesses a gate-activated canted spin texture that produces an electrically tunable bulk band quantum geometry. In particular, we find that due to its out-of-plane asymmetry, an applied out-of-plane electric field breaks inversion symmetry to induce both in-plane and out-of-plane electric dipoles. These in-turn generate spin-orbit coupling to lift the spin degeneracy and enable a bulk band Berry curvature and magnetic moment distribution to develop. Further, due to its low symmetry, Berry curvature and magnetic moment in 1T'-WTe$_2$ possess a dipolar distribution in momentum space, and can lead to unconventional effects such as a current induced magnetization and quantum non-linear anomalous Hall effect. These render 1T'-WTe$_2$ a rich two-dimensional platform for all-electrical control over quantum geometric effects.

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arXiv2017

Plasmon geometric phase and plasmon Hall shift

The collective plasmonic modes of a metal comprise a pattern of charge density and tightly-bound electric fields that oscillate in lock-step to yield enhanced light-matter interaction. Here we show that metals with non-zero Hall conductivity host plasmons with a fine internal structure: they are characterized by a current density configuration that sharply departs from that of ordinary zero Hall conductivity metals. This non-trivial internal structure dramatically enriches the dynamics of plasmon propagation, enabling plasmon wavepackets to acquire geometric phases as they scatter. Strikingly, at boundaries these phases accumulate allowing plasmon waves that reflect off to experience a non-reciprocal parallel shift along the boundary displacing the incident and reflected plasmon trajectories. This plasmon Hall shift, tunable by Hall conductivity as well as plasmon wavelength, displays the chirality of the plasmon's current distribution and can be probed by near-field photonics techniques. Anomalous plasmon dynamics provide a real-space window into the inner structure of plasmon bands, as well as new means for directing plasmonic beams.

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arXiv2017

Large optical conductivity of Dirac semimetal Fermi arc surfaces states

Fermi arc surface states, a hallmark of topological Dirac semimetals, can host carriers that exhibit unusual dynamics distinct from that of their parent bulk. Here we find that Fermi arc carriers in intrinsic Dirac semimetals possess a strong and anisotropic light matter interaction. This is characterized by a large Fermi arc optical conductivity when light is polarized transverse to the Fermi arc; when light is polarized along the Fermi arc, Fermi arc optical conductivity is significantly muted. The large surface spectral weight is locked to the wide separation between Dirac nodes and persists as a large Drude weight of Fermi arc carriers when the system is doped. As a result, large and anisotropic Fermi arc conductivity provides a novel means of optically interrogating the topological surfaces states of Dirac semimetals.

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