arXiv subjects

Liang-Wen Pi

Publications and source records attributed to Liang-Wen Pi.

5 recordsLinked to original sources

arXiv2025

Adiabatic approach for high harmonic generation in solids induced by intense low-frequency pulses

An analytic description of high harmonic generation (HHG) in solids induced by intense low-frequency pulses is presented within an adiabatic approach, which treats laser-matter interactions nonperturbatively. We derive the analytical expression for the laser-dressed state of an electron in an arbitrary spatially periodic potential, taking into account multiband structure of the solid target. Closed-form formulas for electron current and HHG spectra are presented. Based on the developed theory, we provide an analytic explanation for key features of HHG yield and show that the interband mechanism of HHG prevails over the intraband one.

physics.optics↗

arXiv2025

Nonadiabatic effect in high order harmonic generation revealed by a fully analytical method

We propose a fully analytical method for describing high-order harmonic generation (HHG). This method is based on the strong-field approximation (SFA) and electron-trajectory theory, but utilizes the perturbation expansion on the Keldysh parameter $\gamma$. This expansion allows us to clearly differentiate the nonadiabatic and adiabatic effects on HHG. We show that the nonadiabatic effect relating to high-order expansion depends on the laser wavelength and remarkably enhances the HHG yields for cases of short wavelengths, providing deeper insights into wavelength-dependent HHG yields which are important in producing attosecond pulses. Especially, our method provides the analytical and accurate descriptions of nonadiabatic exit velocity and position of the tunneling electron at the tunnel exit. These descriptions are meaningful for constructing a fully analytical and quantitative Coulomb-included HHG model, which is crucial in HHG-based attosecond measurement.

physics.optics↗

arXiv2025

Photoionization time delays probe electron correlations

The photoelectric effect, explained by Einstein in 1905, is often regarded as a one-electron phenomenon. However, in multi-electron systems, the interaction of the escaping electron with other electrons, referred to as electron correlation, plays an important role. For example, electron correlations in photoionization of the outer $s$-subshells of rare gas atoms lead to a substantial minimum in the ionization probability, which was theoretically predicted in 1972 and experimentally confirmed using synchrotron radiation. However, recent attosecond photoionization time delay measurements in argon strongly disagree with theory, thus raising questions on the nature of electron correlations leading to this minimum. In this work, combining high-spectral resolution attosecond interferometry experiments and novel theoretical calculations allows us to identify the most essential electron correlations affecting the photoemission. The measurement of time delays gives unprecedented insight into the photoionization process, unraveling details of the atomic potential experienced by the escaping electron and capturing its dynamics.

physics.atom-ph↗

arXiv2024

Circularly polarized RABBIT applied to a Rabi-cycling atom

We utilize the reconstruction of attosecond beating by interference of two-photon transitions (RABBIT) technique to study the phase of a Rabi-cycling atom using circularly polarized extreme ultraviolet and infrared (IR) fields, where the IR field induces Rabi oscillations between the 2s and 2p states of lithium. Autler-Townes splittings are observed in sidebands of the photoelectron spectra and the relative phases of outgoing electron wave packets are retrieved from the azimuthal angle. In this RABBIT scheme, more ionization pathways beyond the usual two-photon pathways are required. Our results show that the polar-angle-integrated and polar-angle-resolved RABBIT phases have different behaviors when the XUV and IR fields have co- and counter-rotating circular polarizations, which are traced back to the different ionization channels according to the selection rules in these two cases and their competition relying on the propensity rule in laser-assisted photoionization.

physics.atom-ph↗

arXiv2017

Discontinuities in the Electromagnetic Fields of Vortex Beams in the Complex Source/Sink Model

An analytical discontinuity is reported in what was thought to be the discontinuity-free exact nonparaxial vortex beam phasor obtained within the complex source/sink model. This discontinuity appears for all odd values of the orbital angular momentum mode. Such discontinuities in the phasor lead to nonphysical discontinuities in the real electromagnetic field components. We identify the source of the discontinuities, and provide graphical evidence of the discontinuous real electric fields for the first and third orbital angular momentum modes. A simple means of avoiding these discontinuities is presented.

physics.optics↗