arXiv subjects

Libor Šmejkal

Publications and source records attributed to Libor Šmejkal.

At least 19 recordsLinked to original sources

arXiv2026

Room-temperature ferroelectric p-wave magnet

P -wave magnets exhibit odd-parity spin polarization in momentum space while retaining zero net magnetization, offering a promising route toward nonrelativistic spintronics. Previously reported p-wave magnets based on combined time-reversal and lattice-translation symmetry, Tt, have thus far exhibited ordering temperatures below the liquid-nitrogen range. Here, we demonstrate a distinct route to a pristine p-wave magnetism that does not require T t symmetry, and instead is based on incommensurate spin-spiral order. Specifically, the cycloidal magnetic structure of the multiferroic BiFeO3 (BFO) intrinsically realizes p-wave magnetism coexisting with ferroelectric polarization at room temperature. Combining symmetry analysis, density-functional-theory calculations, and circular photogalvanic-effect (CPGE) measurements, we find a large nonrelativistic spin splitting of approximately 100 meV associated with the cycloidal order. The resulting p-wave spin polarization gives rise to a characteristic CPGE response whose sign can be reversibly switched by electrically controlling the cycloid chirality. Our results establish ferroelectric BiFeO3 as a room-temperature platform for electrically switchable p-wave magnetism and provide a route toward voltage-controlled spintronic devices based on parity-breaking magnetic order.

cond-mat.mtrl-sci↗

arXiv2026

Reversible field-free superconducting diode effect controlled by an antiferromagnet

The semiconductor diode, which allows current to flow preferentially in one direction, is a fundamental building block of numerous modern electronic circuits. Its superconducting analogue---the superconducting diode effect---enables directional dissipationless current flow and may provide similar functionality in future superconducting quantum circuits. Realization of such a nonreciprocal supercurrent requires broken time-reversal symmetry. At zero applied field, this has been typically associated either with intrinsic unconventional superconductivity or extrinsic spin-split electronic states induced by magnetic proximity. Here we demonstrate a field-free superconducting diode effect in conventional superconducting Al proximitized by collinear antiferromagnetic CuMnAs, whose electronic structure breaks time-reversal symmetry without generating spin splitting. By tuning the proximity effect through an insulating AlAs interlayer and correlating the reversal of the diode polarity with the reversal of the remanent Néel state, we establish that the antiferromagnet controls the superconducting diode effect. Our results show that neither spin-split bands nor net magnetization is required for a magnetically controlled field-free superconducting diode effect, extending superconducting nonreciprocity to a broader class of collinear compensated magnets.

cond-mat.supr-con↗

arXiv2026

Time-reversal-odd Transport in Odd-Parity Magnets

Unconventional magnets combining vanishing net magnetization with spin-split electronic structures and anomalous transport have attracted considerable attention. Using spin-group symmetry analysis, we derive general conditions for odd-parity spin splitting in two- and three-dimensional coplanar noncollinear antiferromagnets. We identify a key spin-group symmetry whose relativistic counterpart forbids time-reversal-odd transport and show that breaking it allows such transport in the presence of spin-orbit coupling. Tight-binding calculations validate these symmetry arguments and demonstrate an anomalous Hall effect in a fully compensated odd-parity magnetic state without an external field. By screening a three-dimensional magnetic materials database and constructing two-dimensional heterostructures, we further identify realistic platforms exhibiting pronounced spin-orientation-dependent anomalous Hall and magneto-optical effects. Our results establish a general symmetry framework for time-reversal-odd responses in odd-parity magnets and highlight fully compensated odd-parity magnets as a promising platform for controlling anomalous transport.

cond-mat.mtrl-sci↗

arXiv2026

Fermi-surface studies of altermagnetic CrSb from Shubnikov-de Haas oscillations

Within the family of altermagnets, CrSb is a metallic, collinearly ordered material that exhibits particularly strong symmetry-induced spin splitting in its band structure. In this study, we combine electrical magnetotransport measurements up to 68 T on microfabricated single-crystalline CrSb with first-principles calculations to investigate its Fermi surface. Notably, we study the temperature and field-orientation dependence of magnetic quantum oscillations observed in the magnetoresistance. The observed frequency spectrum agrees well with results from density-functional-theory calculations. Our results confirm the predicted electronic band structure of altermagnetic CrSb and highlight the importance of high magnetic fields for accurately mapping the Fermi surfaces of unconventional emergent materials.

cond-mat.mtrl-sci↗

arXiv2026

Nonrelativistic-Ising superconductivity in p-wave magnets

We discuss a possibility of superconductivity in the p-wave magnets. These are recently discovered materials that have zero net magnetization by symmetry and finite non-relativistic spin splitting of electron bands, like in altermagnets. Similarly, the spin polarizations is collinear in the momentum space. Yet, as opposed to altermagnets, the magnetization is noncollinear in the real space, and the spin splitting obeys time-reversal symmetry in the momentum space. As a result, if such material harbors superconductivity (due to phonons, or any other mechanism), the only supported superconducting symmetry is Ising superconductivity, an exotic symmetry where any Cooper pair is a 50:50 mix of singlet and triplet. This unusual behavior is also in stark contrast to regular antiferromagnet, which can support Cooper pairs of any parity, and altermagnets, which can only support nonunitary triplet pairs. The presence of large triplet component and enhanced resilience against pair breaking is inherent to the p-wave magnets and as such is unconventional as it does not materialize in conventional spin-orbit coupling induced Ising superconductors.

cond-mat.supr-con↗

arXiv2026

Giant perpendicular Edelstein polarization in 2D compensated magnets via bichromatic Floquet driving

While unconventional $p$-wave magnets can generate nonrelativistic Edelstein polarizations, spin-group symmetries strictly forbid these responses in unconventional magnets with higher-order harmonics, such as $d$-wave altermagnets. Here, we demonstrate that combining Rashba spin-orbit coupling with bichromatic Floquet driving activates giant perpendicular Edelstein polarizations (PEPs) across 2D altermagnets and broader classes of unconventional spin-polarized magnets -- a feat monochromatic driving cannot achieve. By dynamically breaking two-fold rotational symmetry, the two-frequency drive (including bilinear, bicircular, and circular-linear configurations) induces a stray-field-free in-plane Zeeman-like field that generates orbitally dominated PEPs (0.5--1.5 $μ_{\rm B}$). This massive response is governed by universal selection rules tied to the system's magnetic parity and the second beam's harmonics. These emergent PEPs provide a powerful mechanism for perpendicular memory writing.

cond-mat.mtrl-sci↗

arXiv2026

Optical signatures of bulk g-wave altermagnetism in MnTe

For planar d-wave altermagnets, it has been shown that a spin polarization can be induced in a controlled fashion by ultrashort-pulse excitation, even though the material is magnetically compensated. Here, we theoretically analyze the response of the prototypical bulk $g$-wave altermagnet $α$-MnTe to linearly polarized ultrashort pulses. We demonstrate how the electronic spin response in $α$-MnTe exhibits different symmetry characteristics by calculating the excited electron distributions based on ab initio band structure data. These characteristics depend not only on the nodal planes of the bulk g-wave altermagnet, but also on the excitation pulse. We present a simple procedure to analyze the excited-state characteristics via two-dimensional cuts through the three-dimensional Brillouin zone, which can be used as guidance to present-day magneto-optical techniques.

cond-mat.mtrl-sci↗

arXiv2026

Emergent altermagnetism at surfaces of antiferromagnets: full symmetry classification and material identification

We demonstrate the emergence of altermagnetism at the surfaces of antiferromagnets, vastly expanding the number of material candidates with altermagnetic characteristics and establishing a route towards two-dimensional altermagnetism through surface-induced symmetry breaking. We do so by developing a surface spin group formalism that fully classifies all surface magnetic states and identifies altermagnetic surface spin groups that can arise at the surfaces of antiferromagnets. We use this formalism to identify over 150 antiferromagnetic entries from the MAGNDATA database with at least one altermagnetic surface, often times with multiple such surfaces in the same material, and clarify the role of surface roughness and terraces. We illustrate this emergent phenomenon in a realistic Lieb lattice-based minimal model and present ab initio calculations on two representative material candidates, $\text{NaMnP}$ and $\text{FeGe}_2$, exhibiting $d$-wave and $g$-wave surface altermagnetism, respectively. Our theory naturally resolves the contradiction of recent experimental reports of $d$-wave spin splitting from ARPES measurements on metallic Lieb lattice compounds such as KV$_2$Se$_2$O that have been shown to be antiferromagnetic in the bulk. Hence, we establish a new paradigm for generating effectively two-dimensional altermagnetism by functionalizing the abundant material class of collinear antiferromagnets as viable platforms for controlled surface altermagnetism.

cond-mat.mtrl-sci↗

arXiv2026

All optical excitation of spin polarization in d-wave altermagnets

The recently discovered altermagnets exhibit collinear magnetic order with zero net magnetization but with unconventional spin-polarized d/g/i-wave band structures, expanding the known paradigms of ferromagnets and antiferromagnets. In addition to novel current-driven electronic transport effects, the unconventional time-reversal symmetry breaking in these systems also makes it possible to obtain a spin response to \emph{linearly polarized} fields in the optical frequency domain. We show through ab-initio calculations of the prototypical d-wave altermagnet RuO$_2$, with a symmetry combining twofold spin rotation with fourfold lattice rotation, $[C_2\|C_{4z}]$, that there is an optical analogue of a spin splitter effect, as the coupling to a linearly polarized exciting laser field makes the d-wave character of the altermagnet directly visible. By magneto-optical measurements on RuO$_2$ films of different thicknesses ranging from $2$ to $8\,$nanometers, we demonstrate the predicted connection of the linear polarization of an ultrashort pump pulse to the sign and magnitude of the optically excited electronic spin polarization in the ultrathin RuO$_2$ films. The possibility of exciting and controlling an electronic spin polarization by linearly polarized optical pulses in a compensated system is a unique consequence of the altermagnetic material properties. Our experimental results therefore establish an optical pump-probe based protocol for detection of altermagnetic characteristics in ultrathin RuO$_2$ films, but our all-optical approach should apply more generally to materials in this altermagnetic symmetry class.

cond-mat.mtrl-sci↗

arXiv2026

Quantum-impurity sensing of altermagnetic order

Quantum sensing with individual spin defects has emerged as a versatile platform to probe microscopic properties of condensed matter systems. Here we demonstrate that quantum relaxometry with nitrogen-vacancy (NV) centers in diamond can reveal the anisotropic spin dynamics of altermagnetic insulators together with their characteristic spin polarised bands. We show that the distance and orientation dependent relaxation rate of a nearby quantum impurity encodes signatures of momentum space anisotropy in the spin diffusion response, a hallmark of altermagnetic order. This directional sensitivity is unprecedented in the landscape of quantum materials sensing, and it enables the distinction of altermagnets from conventional antiferromagnets via local, noninvasive measurements. Our results could spark new NV-sensing experiments on spin transport and symmetry breaking in altermagnets, and highlight the role of NV orientation to probe anisotropic phenomena in condensed matter systems.

cond-mat.mes-hall↗

arXiv2026

Odd-Parity-Wave Magnons and Nonrelativistic Thermal Edelstein Effect

Odd-parity-wave magnets are noncollinear compensated magnets with spin-split band structure in the absence of spin-orbit coupling and dipolar interactions. In contrast to altermagnets, their spin-polarized band structure breaks inversion symmetry, but preserves time-reversal symmetry rendering their spin texture odd in momentum space. Here, we study the spin dynamics of the magnetic texture and compute the band structure and spin polarization of magnons. We present minimal spin models of noncoplanar odd-parity-wave magnets purely stabilized by exchange interactions that host p- and f-wave spin textures for the magnetic excitations. We demonstrate that two of these models exhibit collinear spin textures, i.e., the magnon spin polarization is restricted to a global (quantization) axis independent of the momentum giving rise to single-component odd-parity-wave magnetism, previously associated primarily with coplanar ground states. Finally, the nonrelativistic magnonic thermal Edelstein effect -- a nonequilibrium magnetization induced by a temperature gradient -- is shown to exist for p-wave magnets in linear response and inherits its anisotropic angular dependence from the partial-wave character of the spin-polarized band structure. Our findings suggest that insulating odd-parity-wave magnets are promising candidates for magnon spintronics applications.

cond-mat.mes-hall↗

arXiv2026

Ferroelectric $p$-wave magnets

Couplings between ferroelectric and magnetic orders offer promising routes toward low-dissipation electronics. However, such couplings are notably rare, largely due to the poor compatibility between insulating band structures and ferromagnetism. Here, we study a different strategy: we identify previously overlooked time-reversal-symmetric $p$- and $f$-wave spin-polarized insulating electronic states in ferroelectrics with noncollinear magnetic sublattices. We show that combining spin and magnetic group theory enables a systematic classification of the origin of polar symmetry breaking. We distinguish crystallographic, exchange-, or spin-orbit-driven mechanisms. Furthermore, we identify more than 50 candidate materials. Using first-principles calculations, we demonstrate a pristine, time-reversal-symmetric $p$-wave spin-polarized electronic structure in the well-known multiferroic $\mathrm{GdMn_2O_5}$. We further show that its $p$-wave order can be switched electrically, opening alternative paths toward spintronic and multiferroic functionalities in this class of materials.

cond-mat.mtrl-sci↗

arXiv2026

Persistent altermagnetism

Persistent spin textures with collinear spin polarization are promising platforms for spintronics applications. However, their typically relativistic spin-orbit origin leads to weak spin splittings and fragile spin coherence. Here, we demonstrate a previously overlooked class of robust collinear spin polarization protected by mirror symmetry in combination with a strong exchange-driven altermagnetic order, which persists even in the presence of spin-orbit coupling. By combining first-principles calculations with a systematic classification of spin and magnetic layer groups, we identify this phenomenon-termed persistent altermagnetic spin polarization (PASP)-to occur in 158 spin layer groups and in representative materials including metallic V$_2$Te$_2$O, insulating La$_2$CuO$_4$, and semiconducting VSI$_2$. Furthermore, we theoretically demonstrate that PASP is ferroelectrically switchable in VSI$_2$. Finally, we show that this PASP switching can lead to large changes in spin-filtering conductance in a model all-altermagnetic junction. Our results open the possibility of employing PASP in all-altermagnetic magnetic memory and spin-transistor devices and establish universal principles of altermagnetism in spin-orbit-coupled monolayers.

cond-mat.mes-hall↗

arXiv2026

Microscopic origin of $p$-wave magnetism

$P$-, $f$-, or $h$-wave antialtermagnets yield large non-relativistic spin splitting with out-of-plane spin polarization in momentum space perpendicular to the coplanar non-collinear local magnetic moments. We provide a microscopic explanation of this unconventional spin polarization by linking it to a previously overlooked site-compensated spin density that orders antiparallel when projected onto opposite momenta. We verify this result both by model derivation of the out-of-plane momentum-space spin polarization being proportional to the direct-space cross product of the coplanar non-collinear spin order, as well as by ab initio calculations in the material candidate CeNiAsO. By providing a general classification and analytic expression for the spin polarization of all spinful two-site tight-binding Hamiltonians, we reveal the momentum-resolved spin polarization as a probe of the Bloch-state geometry arising from spin-site coupling. Furthermore, our approach allows for geometric distinction between ferro-, alter-, and antialtermagnets. Our results provide a quantitative guidance for quantized out-of-plane momentum-space spin polarization and large spin splitting, and construction principles for antialtermagnets.

cond-mat.mes-hall↗

arXiv2026

Topological textures and emergent altermagnetic signatures in ultrathin BiFeO3

Magnetoelectric multiferroics, materials with intrinsically coupled electric polarization and magnetic order, promise ultralow-power switching, nonvolatile memory, and energy-efficient signal transduction. Yet practical deployment demands ultrathin films down to the atomic limit, where both orders typically degrade. Maintaining both order parameters at the thinnest scales in complex oxides remains a tremendous challenge, as uncompensated bound charge drives nanoscale depolarization in most ferroelectrics, while off-stoichiometry, reduced anisotropy, and charge transfer can produce magnetic dead layers in ultrathin oxides at substrate interfaces. Here, we realize a multiferroic phase of BiFeO3 that not only sustains both order parameters at room temperature with no dead layer but also exhibits signatures of emergent altermagnetism in the four-unit-cell, ultrathin limit. First-principles calculations, spin symmetry analysis, atomic-resolution imaging, and angle-resolved magnetic imaging reveal that short-circuit electrostatic boundary conditions, together with epitaxial strain, drive a continuous second-order, thickness-driven phase transition that enables the formation of multiferroic topological textures. Moreover, the imposed boundary conditions stabilize a d-wave altermagnetic time-reversal symmetry breaking, with corresponding signatures observed in magnetic circular dichroism. Collectively, these results establish a pathway to stabilize unconventional multiferroicity at device-relevant thicknesses, reframing scaling limits for oxide electronics.

cond-mat.mtrl-sci↗

arXiv2025

Quantization of spin circular photogalvanic effect in altermagnetic Weyl semimetals

We theoretically predict a spin-current analog of the quantized circular photogalvanic effect in Weyl semimetals. This phenomenon is forbidden in antiferromagnets by symmetry but uniquely allowed in altermagnets, highlighting a novel and intrinsic characteristic of altermagnetism. To systematically explore second-order spin current responses, we classify all symmetry-allowed responses based on spin point groups. Furthermore, we provide a comprehensive classification of altermagnetic Weyl semimetals by identifying spin space groups that host symmetry-enforced Weyl points. Utilizing this classification, we construct a symmetry-guided tight-binding model and confirm our predictions. Finally, we identify Weyl crossings in a material candidate via first-principle calculations. Our work unveils a distinctive optical response of altermagnets, paving the way for a new frontier in altermagnetism.

cond-mat.mes-hall↗

arXiv2025

Orbital magnetization from parallel transport of Bloch states

Quantum geometric formulations of linear and nonlinear responses can be constructed from a single building block in the form of a gauge-invariant interband transition operator. Here, we identify a second building block for quantum geometry: a band-resolved adiabatic connection operator that captures the noncommutativity between band projectors and their momentum derivatives. The band-resolved adiabatic connection operator, first introduced in the theory of adiabatic driving, serves as a generalized angular momentum within the state manifold of single bands, and we employ it to reformulate expressions for the band-resolved orbital magnetic moment. This form provides a complementary geometric interpretation alongside the multiband separation between energetic- and quantum-state properties by the two-state Berry curvature. Our formalism allows us to present formulas valid for both nondegenerate and degenerate bands, thereby removing the limitations of the common Bloch-state formula. We illustrate our theory by calculating a large orbital magnetization emerging without spin-orbit coupling in a spin-compensated, noncoplanar anomalous Hall magnet with degenerate bands.

cond-mat.mes-hall↗

arXiv2025

Cavity-induced coherent magnetization and polaritons in altermagnets

Altermagnets feature antiparallel spin sublattices with $d$-, $g$-, or $i$-wave spin order, yielding nonrelativistic spin splitting without net magnetization. We show that embedding a two-dimensional $d$-wave altermagnet in a driven optical cavity induces a finite, tunable magnetization. Coherent photon driving couples selectively to electronic sublattices, and the resulting altermagnets' symmetry-broken spin texture yields a pronounced steady-state spin imbalance -- coherent magnetization -- absent in conventional antiferromagnets for the same lattice configuration. A mean-field Lindblad analysis reveals the dominance of quadratic over linear couplings. In the strong-coupling regime, distinct polariton signatures emerge in the steady state of induced magnetization. This work demonstrates cavity control of altermagnets for spintronic applications.

cond-mat.str-el↗