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Lihui Bai

Publications and source records attributed to Lihui Bai.

At least 19 recordsLinked to original sources

Fractional Magnonic Frequency Combs

Magnonic frequency combs (MFCs) are spectacular phenomena in microwave-driven high-quality magnets. Like the equally spaced prongs in a comb, conventional \textit{integer} MFCs are sharp resonances with an equal and constant frequency difference. Here we report \textit{fractional} MFCs in a high-quality magnetic sphere that emerges when adding a low-power, precisely detuned microwave to the main drive that compresses the frequency spacings to a rational fraction of the original comb, generating high-density spectral grids with hundreds of lines. The theoretical analysis finds that parametric three-magnon scattering is the dominant non-linear process that reproduces the observation well. This mechanism is unique to magnets: it does not exist in an optomechanical system, where the Kerr and optical nonlinearities govern comb formation at a much higher power input. Since our platform operates as a frequency ``vernier caliper" with much higher sensitivity than integer MFCs, it has application potential in precision metrology.

cond-mat.mtrl-sci

Weak Magnetic Sensing via Floquet Driving in an Active Cavity Magnon Coupled System

While significant advancements have been made in weak magnetic field detection, conventional high-sensitivity techniques are often limited by requirements for cryogenic operation or bulky setups. In this work, we develop a sensitive alternating magnetic field sensor based on a coupled system of an active microwave cavity and yttrium iron garnet (YIG), with the components implemented on printed circuit boards (PCBs). By introducing electrically tunable gain to compensate for cavity losses, we substantially improve both the quality factor and the signal intensity. Under the coupled system, Floquet modulation is induced by the alternating magnetic field, allowing for weak field detection by driving a specific hybrid mode and measuring the resulting Floquet sidebands. This miniaturized device operates at room temperature, achieving a detection limit of 121 pT/\sqrt{Hz}.

cond-mat.mes-hall

A voltage-responsive strongly dipolar-coupled macrospin network with emergent dynamics for computing

Emergent behavior, which arises from local interactions between simple elements, is pervasive in nature. It underlies the energy-efficient computing in our brains. However, realizing such dynamics in artificial materials, particularly under low-energy stimuli, remains a fundamental challenge. While dipole-dipole interactions are typically suppressed in magnetic storage, here we harness and amplify them to construct a strongly dipolar-coupled network of SmCo5 macrospins at wafer scale, which can exhibit intrinsic interaction-driven collective dynamics in response to voltage pulses. The network combines three essential ingredients: strong dipolar coupling by large single-domain macrospin, giant voltage control of coercivity over nearly 1000-fold, and disordered network topology with frustrated Ising-like energy landscape. When stimulated by 1 V pulses, the network enters a regime where interaction-driven magnetic behaviors emerge, including spontaneous demagnetization, greatly enhanced magnetization modulation, reversible freeze and resume evolution and stochastic convergence toward low-energy magnetic configurations. All these behaviors are completely absent at the single-nanomagnet level. Furthermore, by constructing micromagnetic models of the strongly dipolar-coupled macrospin networks, we show that the resulting nonlinear, high-dimensional collective dynamics, intrinsic to strongly-interacting systems, can enable accurate chaotic Mackey-Glass prediction and multiclass drone-signal classification. Our work establishes the voltage-responsive strongly-coupled SmCo5 network as a mesoscopic platform for probing emergent magnetic dynamics previously inaccessible under ambient conditions. It also suggests a fundamental distinct route towards scalable, low-voltage computing, one rooted in native physical interaction-driven collective dynamics at the network level.

cond-mat.mtrl-sci

Ultrasensitive Magnetometer based on Cusp Points of the Photon-Magnon Synchronization Mode

Ultrasensitive magnetometers based on spin resonances have led to remarkable achievements. However, the gyromagnetic ratios of these spin resonances that determine the responsivity of magnetometers to weak magnetic fields are inherently constrained by the Land$\acute{e}$ g-factor of particles, such as the electron, with a constant gyromagnetic ratio of $\gamma_e=2\pi\times28$ GHz/T. Here, we demonstrate an ultrasensitive magnetometer based on the cusp point (CP) of photon-magnon synchronization modes (PMSMs). The PMSM's gyromagnetic ratio at the CP is enhanced to $37\gamma_e$ and further amplified to $236\gamma_e$ by utilizing the sixth-order oscillating mode of the PMSM. Moreover, the emission linewidth of the PMSM can be reduced to 0.06 Hz, resulting in excellent sensitivity to weak magnetic fields. These outstanding properties position our magnetometer to potentially achieve superior sensitivity to conventional magnetometers. Our work introduces a cost-effective prototype for the next generation of magnetometry, and may advance scientific research and technologies that rely on ultrasensitive magnetic field detection.

cond-mat.mes-hall

Enhancement of Magnon Transport by Superconductor Meissner Screening

Recent experiments observe the spin-wave-Meissner-current modes in ferromagnetic insulator-superconductor heterostructures, in which the coherently excited spin waves seemingly do not decay as usual beneath the superconductor strip [Borst et al., Science 382, 430 (2023)]. We interpret this phenomenon by demonstrating that the stray magnetic field emitted by the magnetization dynamics is reflected, focused, and enhanced inside the ferromagnet by the supercurrent induced in the superconductor, such that the group velocity of spin waves is strongly enhanced. Analytical and numerical calculations based on this model predict that the coherent transport of magnons is enhanced by close to 500% for yttrium iron garnet capped by superconducting NbN with a decay length exceeding millimeters. Our finding may augment the performance of magnons in quantum information and quantum transport processing.

cond-mat.mes-hall

Variation between Antiferromagnetism and Ferrimagnetism in NiPS3 by Electron Doping

How to electrically control magnetic properties of a magnetic material is promising towards spintronic applications, where the investigation of carrier doping effects on antiferromagnetic (AFM) materials remains challenging due to their zero net magnetization. In this work, we found electron doping dependent variation of magnetic orders of a two-dimensional (2D) AFM insulator NiPS3, where doping concentration is tuned by intercalating various organic cations into the van der Waals gaps of NiPS3 without introduction of defects and impurity phases. The doped NiPS3 shows an AFM-ferrimagnetic (FIM) transition at doping level of 0.2-0.5 electrons/cell and a FIM-AFM transition at doping level of >= 0.6 electrons/cell. We propose that the found phenomenon is due to competition between Stoner exchange dominated inter-chain ferromagnetic order and super-exchange dominated inter-chain AFM order at different doping level. Our studies provide a viable way to exploit correlation between electronic structures and magnetic properties of 2D magnetic materials for realization of magnetoelectric effect.

cond-mat.mtrl-sci

Enhanced spin transfer torque in platinum/ferromagnetic-metal structures by optimizing the platinum thickness

Spin transfer torque (STT) driven by a charge current plays a key role in magnetization switching in heavy-metal/ferromagnetic-metal structures. The STT efficiency defined by the ratio between the effective field due to STT and the current density, is required to be improved to reduce energy compulsions in the STT-based spintronic devices. In this work, using the harmonic Hall measurement method, we experimentally studied the STT efficiency in platinum(Pt)/FM structures as a function of the Pt thickness. We found that the STT efficiency strongly depends on the Pt thickness and reaches a maximum value of 4.259 mT/($10^6$A/$cm^{2}$) for the 1.8-nm-thickness Pt sample. This result indicates that competition between spin Hall effect (SHE) and Rashba effect as well as spin diffusion process across the Pt layer determines the Pt thickness for the maximum STT efficiency. We demonstrated the role played by the spin diffusion besides the spin current generation mechanisms in improvement of the STT efficiency, which is helpful in designing STT-based devices.

cond-mat.mtrl-sci

Transient Response of the Cavity-Magnon-Polariton

The Rabi oscillations of a coupled spin-photon system are experimentally studied using time domain microwave transmission measurements. An external magnetic bias field is applied to control the amplitude and frequency of Rabi oscillations, which are a measure of the coherent spin-photon energy exchange and coupling strength respectively. The amplitude and frequency control is described in the time domain as the transient response of a two-level spin-photon system. This approach reveals the link between steady state and transient behaviour of the cavity-magnon-polariton, which is necessary to interpret time domain cavity-spintronic experiments. This transient model also allows us to understand and quantify the polariton mode composition, which can be controlled by the bias field.

cond-mat.mes-hall

Electrical control of spin mixing conductance in a Y$_3$Fe$_5$O$_{12}$/Platinum bilayer

We report a tunable spin mixing conductance, up to $\pm 22\%$, in a Y${}_{3}$Fe${}_{5}$O${}_{12}$/Platinum (YIG/Pt) bilayer.This control is achieved by applying a gate voltage with an ionic gate technique, which exhibits a gate-dependent ferromagnetic resonance line width. Furthermore, we observed a gate-dependent spin pumping and spin Hall angle in the Pt layer, which is also tunable up to $\pm$ 13.6\%. This work experimentally demonstrates spin current control through spin pumping and a gate voltage in a YIG/Pt bilayer, demonstrating the crucial role of the interfacial charge density for the spin transport properties in magnetic insulator/heavy metal bilayers.

cond-mat.mes-hall

Cavity mediated manipulation of distant spin currents using cavity-magnon-polariton

Using electrical detection of a strongly coupled spin-photon system comprised of a microwave cavity mode and two magnetic samples, we demonstrate the long distance manipulation of spin currents. This distant control is not limited by the spin diffusion length, instead depending on the interplay between the local and global properties of the coupled system, enabling systematic spin current control over large distance scales (several centimeters in this work). This flexibility opens the door to improved spin current generation and manipulation for cavity spintronic devices.

cond-mat.mtrl-sci

Topological Properties of a Coupled Spin-Photon System Induced by Damping

We experimentally examine the topological nature of a strongly coupled spin-photon system induced by damping. The presence of both spin and photonic losses results in a non-Hermitian system with a variety of exotic phenomena dictated by the topological structure of the eigenvalue spectra and the presence of an exceptional point (EP), where the coupled spin-photon eigenvectors coalesce. By controlling both the spin resonance frequency and the spin-photon coupling strength we observe a resonance crossing for cooperativities above one, suggesting that the boundary between weak and strong coupling should be based on the EP location rather than the cooperativity. Furthermore we observe dynamic mode switching when encircling the EP and identify the potential to engineer the topological structure of coupled spin-photon systems with additional modes. Our work therefore further highlights the role of damping within the strong coupling regime, and demonstrates the potential and great flexibility of spin-photon systems for studies of non-Hermitian physics.

cond-mat.mtrl-sci

Linking Magnon-Cavity Strong Coupling to Magnon-Polaritons through Effective Permeability

Strong coupling in cavity-magnon systems has shown great potential for use in spintronics and information processing technologies due to the low damping rates and long coherence times. Although such systems are conceptually similar to those coupled by magnon-polaritons (MPs), the link between magnon-cavity coupling and MPs has not been explicitly defined. In this work we establish such a connection by studying the frequency-wavevector dispersion of a strongly coupled magnon-cavity system, using a height-adjustable microwave cavity, and by modelling the observed behaviour through the system's effective permeability. A polariton gap between the upper and lower coupled modes of the magnon-cavity system is defined, and is seen to be dependent on the system's effective filling factor. This gap is equal to the MP polariton gap in the limit where filling factor = 1, corresponding to the removal of the microwave cavity. Thus, our work clarifies the connection between magnon-cavity and MP coupling, improving our understanding of magnon-photon interactions in coupled systems.

cond-mat.mes-hall

Indirect Coupling between Two Cavity Photon Systems via Ferromagnetic Resonance

We experimentally realize indirect coupling between two cavity modes via strong coupling with the ferromagnetic resonance in Yttrium Iron Garnet (YIG). We find that some indirectly coupled modes of our system can have a higher microwave transmission than the individual uncoupled modes. Using a coupled harmonic oscillator model, the influence of the oscillation phase difference between the two cavity modes on the nature of the indirect coupling is revealed. These indirectly coupled microwave modes can be controlled using an external magnetic field or by tuning the cavity height. This work has potential for use in controllable optical devices and information processing technologies.

cond-mat.mes-hall

Spin dynamical phase and anti-resonance in a strongly coupled magnon-photon system

We experimentally studied a strongly coupled magnon-photon system via microwave transmission measurements. An anti-resonance, i.e. the suppression of the microwave transmission, is observed, indicating a relative phase change between the magnon response and the driving microwave field. We show that this anti-resonance feature can be used to interpret the phase evolution of the coupled magnon-microwave system and apply this technique to reveal the phase evolution of magnon dark modes. Our work provides a standard procedure for the phase analysis of strongly coupled systems, enabling the phase characterization of each subsystem, and can be generally applied to other strongly coupled systems.

cond-mat.mtrl-sci

Study of the cavity-magnon-polariton transmission line shape

We experimentally and theoretically investigate the microwave transmission line shape of the cavity-magnon-polariton (CMP) created by inserting a low damping magnetic insulator into a high quality 3D microwave cavity. While fixed field measurements are found to have the expected Lorentzian characteristic, at fixed frequencies the field swept line shape is in general asymmetric. Such fixed frequency measurements demonstrate that microwave transmission can be used to access magnetic characteristics of the CMP, such as the field line width $ΔH$. By developing an effective oscillator model of the microwave transmission we show that these line shape features are general characteristics of harmonic coupling. At the same time, at the classical level the underlying physical mechanism of the CMP is electrodynamic phase correlation and a second model based on this principle also accurately reproduces the experimental line shape features. In order to understand the microscopic origin of the effective coupled oscillator model and to allow for future studies of CMP phenomena to extend into the quantum regime, we develop a third, microscopic description, based on a Green's function formalism. Using this method we calculate the transmission spectra and find good agreement with the experimental results.

cond-mat.mtrl-sci

Spin Pumping in Electrodynamically Coupled Magnon-Photon Systems

We use electrical detection, in combination with microwave transmission, to investigate both resonant and non-resonant magnon-photon coupling at room temperature. Spin pumping in a dynamically coupled magnon-photon system is found to be distinctly different from previous experiments. Characteristic coupling features such as modes anti-crossing, line width evolution, peculiar line shape, and resonance broadening are systematically measured and consistently analyzed by a theoretical model set on the foundation of classical electrodynamic coupling. Our experimental and theoretical approach pave the way for pursuing microwave coherent manipulation of pure spin current via the combination of spin pumping and magnon-photon coupling.

cond-mat.mtrl-sci

A Universal Method for Separating Spin Pumping from Spin Rectification Voltage of Ferromagnetic Resonance

We develop a method for universally resolving the important issue of separating spin pumping (SP) from spin rectification (SR) signals in bilayer spintronics devices. This method is based on the characteristic distinction of SP and SR, as revealed in their different angular and field symmetries. It applies generally for analyzing charge voltages in bilayers induced by the ferromagnetic resonance (FMR), independent of FMR line shape. Hence, it solves the outstanding problem that device specific microwave properties restrict the universal quantification of the spin Hall angle in bilayer devices via FMR experiments. Furthermore, it paves the way for directly measuring the nonlinear evolution of spin current generated by spin pumping. The spin Hall angle in a Py/Pt bilayer is thereby directly measured as 0.021$\pm$0.015 up to a large precession cone angle of about 20$^{\circ}$.

cond-mat.mtrl-sci

Electrical Detection of Direct and Alternating Spin Current Injected from a Ferromagnetic Insulator into a Ferromagnetic Metal

We report room temperature electrical detection of spin injection from a ferromagnetic insulator (YIG) into a ferromagnetic metal (Permalloy, Py). Non-equilibrium spins with both static and precessional spin polarizations are dynamically generated by the ferromagnetic resonance of YIG magnetization, and electrically detected by Py as dc and ac spin currents, respectively. The dc spin current is electrically detected via the inverse spin Hall effect of Py, while the ac spin current is converted to a dc voltage via the spin rectification effect of Py which is resonantly enhanced by dynamic exchange interaction between the ac spin current and the Py magnetization. Our results reveal a new path for developing insulator spintronics, which is distinct from the prevalent but controversial approach of using Pt as the spin current detector.

cond-mat.mtrl-sci