arXiv subjects

Lilian Childress

Publications and source records attributed to Lilian Childress.

At least 19 recordsLinked to original sources

arXiv2026

Real-time tissue-equivalent measurement of individual clinical radiotherapy pulses

We apply the precision tools of cavity-enhanced absorption sensing to clinical oncology, demonstrating a dosimeter paradigm in which a centimeter-scale volume of water serves as a tissue-equivalent sensing medium. Our proof-of-concept, all-optical scheme achieves real-time readout of clinical radiation pulses with a nominal single-pulse resolution of 90 $μ$Gy. This demonstration paves the way toward fiber-integrated, micron-scale devices for $\textit{in situ}$ universal absolute dosimetry during treatment.

physics.med-ph↗

arXiv2026

Magnetometry with Broadband Microwave Fields in Nitrogen-Vacancy Centers in Diamond

Nitrogen-vacancy (NV) centers in diamond are optically addressable and versatile light-matter interfaces with practical application in magnetic field sensing, offering the ability to operate at room temperature and reach sensitivities below pT/$\sqrt{\mathrm{Hz}}$. We propose an approach to simultaneously probe all of the magnetically sensitive states using a broadband microwave field and demonstrate that it can be used to measure the external DC magnetic field strength with sensitivities on the order of 10~pT/$\sqrt{\mathrm{Hz}}$. We develop tools for analyzing the temporal signatures in the transmitted broadband microwaves to estimate the magnetic field, comparing maximum likelihood estimation based on minimizing the Kullback-Leibler divergence to various neural network models, and both methods independently reach practical sensitivities. These results are achieved without optimizing parameters such as the bandwidth, and shape of the probing microwave field such that further improvements in sensitivity can be envisioned. Our results motivate novel implementations of NV-based magnetic sensors with the potential for vectorial magnetic field detection at 1-10 kHz update rates and improved sensitivities without requiring a bias magnetic field.

cond-mat.mes-hall↗

arXiv2026

Vector Magnetometry with Broadband Microwave Fields in Nitrogen-Vacancy Centers in Diamond

We present a novel method for full vector magnetometry using nitrogen-vacancy (NV) centers. In contrast to conventional optically detected magnetic resonance techniques, our method employs two distinct broadband microwave pulses and measures them after transmission through the NV sensor medium, thus capturing the line splitting of the ground state triplet due to the Zeeman effect. Two orthogonally polarized microwave pulses allow resolving all magnetic field components independently by reading out differently oriented NV centers. Simulated data is analyzed using deep neural networks, whose efficacy we expect to translate very well to experiments. Our method yields sensitivities between $5~\mathrm{pT}/\sqrt{\mathrm{Hz}}$ and $100~\mathrm{pT}/\sqrt{\mathrm{Hz}}$ across different magnetic field vector components, while achieving approximately $\mathrm{nT}$ accuracy at a signal-to-noise (SNR) ratio of $70~\mathrm{dB}$. By being capable of accurately measuring magnetic fields down to $25~\mathrm{μT}$, the need for a bias field beyond Earth's magnetic field is eliminated.

quant-ph↗

arXiv2026

Triple-Tone Microwave Control for Sensitivity Optimization in Compact Ensemble Nitrogen-Vacancy Magnetometers

Ensembles of nitrogen-vacancy (NV) centers in diamond are a well-established platform for quantum magnetometry under ambient conditions. One challenge arises from the hyperfine structure of the NV, which, for the common $^{14}$N isotope, results in a threefold reduction of contrast and thus sensitivity. By addressing each of the NV hyperfine transitions individually, triple-tone microwave (MW) control can mitigate this sensitivity loss. Here, we experimentally and theoretically investigate the regimes in which triple-tone excitation offers an advantage over standard single-tone MW control for two DC magnetometry protocols: pulsed optically detected magnetic resonance (ODMR) and Ramsey interferometry. We validate a master equation model of the NV dynamics against ensemble NV measurements, and use the model to explore triple-tone vs single-tone sensitivity for different MW powers and NV dephasing rates. For pulsed ODMR, triple-tone driving improves sensitivity by up to a factor of three in the low-dephasing regime, with diminishing gains when dephasing rates approach the hyperfine splitting. In contrast, for Ramsey interferometry, triple-tone excitation only improves sensitivity if MW power is limited. Our results delineate the operating regimes where triple-tone control provides a practical strategy for enhancing NV ensemble magnetometry in portable and power-limited sensors.

quant-ph↗

arXiv2025

Bias-field-free operation of nitrogen-vacancy ensembles in diamond for accurate vector magnetometry

Accurate measurement of vector magnetic fields is critical for applications including navigation, geoscience, and space exploration. Nitrogen-vacancy (NV) center spin ensembles offer a promising solution for high-sensitivity vector magnetometry, as their different orientations in the diamond lattice measure different components of the magnetic field. However, the bias magnetic field typically used to separate signals from each NV orientation introduces inaccuracy from drifts in permanent magnets or coils. Here, we present a novel bias-field-free approach that labels the NV orientations via the direction of the microwave (MW) field in a variable-pulse-duration Ramsey sequence used to manipulate the spin ensemble. Numerical simulations demonstrate the possibility to isolate each orientation's signal with sub-nT accuracy in most terrestrial fields, even without precise MW field calibration, at only a moderate cost to sensitivity. We also provide proof-of-principle experimental validation, observing relevant features that evolve as expected with applied magnetic field. Looking forward, by removing a key source of drift, the proposed protocol lays the groundwork for future deployment of NV magnetometers in high-accuracy or long-duration missions.

quant-ph↗

arXiv2024

Lifetime Reduction of Single Germanium-Vacancy Centers in Diamond via a Tunable Open Microcavity

Coupling between a single quantum emitter and an optical cavity presents a key capability for future quantum networking applications. Here, we explore interactions between individual germanium-vacancy (GeV) defects in diamond and an open microcavity at cryogenic temperatures. Exploiting the tunability of our microcavity system to characterize and select emitters, we observe a Purcell-effect-induced lifetime reduction of up to $4.5\pm0.3$, and extract coherent coupling rates up to $360\pm20$ MHz. Our results indicate that the GeV defect has favorable optical properties for cavity coupling, with a quantum efficiency of at least $0.34\pm0.05$ and likely much higher.

quant-ph↗

arXiv2024

Radiation hardness of open Fabry-Perot microcavities

High-finesse microcavities offer a platform for compact, high-precision sensing by employing high-reflectivity, low-loss mirrors to create effective optical path lengths that are orders of magnitude larger than the device geometry. Here, we investigate the radiation hardness of Fabry-Perot microcavities formed from dielectric mirrors deposited on the tips of optical fibers. The microcavities are irradiated under both conventional (~0.1 Gy/s) and ultrahigh (FLASH, ~20 Gy/s) radiotherapy dose rates. Within our measurement sensitivity of ~40 ppm loss, we observe no degradation in the mirror absorption after irradiation with over 300 Gy accumulated dose. This result highlights the excellent radiation hardness of the dielectric mirrors forming the cavities, enabling new optics-based, real-time, in-vivo, tissue-equivalent radiation dosimeters with ~10 micron spatial resolution (our motivation), as well as other applications in high-radiation environments.

physics.med-ph↗

arXiv2023

Comparing continuous and pulsed nitrogen-vacancy DC magnetometry in the optical-power-limited regime

Ensembles of nitrogen-vacancy (NV) center spins in diamond offer a robust, precise and accurate magnetic sensor. As their applications move beyond the laboratory, practical considerations including size, complexity, and power consumption become important. Here, we compare two commonly-employed NV magnetometry techniques -- continuous-wave (CW) vs pulsed magnetic resonance -- in a scenario limited by total available optical power. We develop a consistent theoretical model for the magnetic sensitivity of each protocol that incorporates NV photophysics - in particular, including the incomplete spin polarization associated with limited optical power; after comparing the models' behaviour to experiments, we use them to predict the relative DC sensitivity of CW versus pulsed operation for an optical-power-limited, shot-noise-limited NV ensemble magnetometer. We find a $\sim 2-3 \times$ gain in sensitivity for pulsed operation, which is significantly smaller than seen in power-unlimited, single-NV experiments. Our results provide a resource for practical sensor development, informing protocol choice and identifying optimal operation regimes when optical power is constrained.

quant-ph↗

arXiv2023

Single-spin spectroscopy of spontaneous and phase-locked spin torque oscillator dynamics

We employ N-$V$ magnetometry to measure the stray field dynamics of a ferromagnetic permalloy nanowire driven by spin-orbit torques. Specifically, we observe the optically detected magnetic resonance (ODMR) signatures of both spontaneous DC-driven magnetic oscillations and phase-locking to a second harmonic drive, developing a simple macrospin model that captures the salient features. We also observe signatures of dynamics beyond the macrospin model, including an additional ODMR feature (associated with a second SW mode) and one mode sapping power from another. Our results provide additional insight into N-$V$-spin wave coupling mechanisms, and represent a new modality for sub-wavelength N-$V$ scanned probe microscopy of nanoscale magnetic oscillators.

cond-mat.mes-hall↗

arXiv2023

Robust spin relaxometry with fast adaptive Bayesian estimation

Spin relaxometry with nitrogen-vacancy (NV) centers in diamond offers a spectrally selective, atomically localized, and calibrated measurement of microwave-frequency magnetic noise, presenting a versatile probe for condensed matter and biological systems. Typically, relaxation rates are estimated with curve-fitting techniques that do not provide optimal sensitivity, often leading to long acquisition times that are particularly detrimental in systems prone to drift or other dynamics of interest. Here we show that adaptive Bayesian estimation is well suited to this problem, producing dynamic relaxometry pulse sequences that rapidly find an optimal operating regime. In many situations (including the system we employ), this approach can speed the acquisition by an order of magnitude. We also present a four-signal measurement protocol that is robust to drifts in spin readout contrast, polarization, and microwave pulse fidelity while still achieving near-optimal sensitivity. The combined technique offers a practical, hardware-agnostic approach for a wide range of NV relaxometry applications.

quant-ph↗

arXiv2021

Cavity-enhanced absorption sensing with robust sideband locking

We present a simple, continuous, cavity-enhanced optical absorption measurement technique based on high-bandwidth Pound-Drever-Hall (PDH) sideband locking. The technique provides a resonant amplitude quadrature readout that can be mapped onto the cavity's internal loss rate, and is naturally compatible with weak probe beams. With a proof-of-concept 5-cm-long Fabry-Perot cavity, we measure an absorption sensitivity of $6.6 \times 10^{-11} ~\text{cm}^{-1}/\sqrt{\text{Hz}}$ at 100 kHz (roughly the cavity bandwidth) and $\sim 10^{-10}~\text{cm}^{-1}/\sqrt{\text{Hz}}$ from 30 kHz to 1 MHz, with $38~μ$W collected from the cavity's circulating power.

physics.optics↗

arXiv2021

A mechanically stable and tunable cryogenic Fabry-Perot microcavity

High-finesse, open-geometry microcavities have recently emerged as a versatile tool for enhancing interactions between photons and material systems, with a range of applications in quantum optics and quantum information science. However, mechanical vibrations pose a considerable challenge to their operation within a closed-cycle cryostat, particularly when spatial tunability and free-space optical access are required. Here, we present the design and characterization of a system that can achieve $\sim$16 pm-rms passive mechanical stability between two high-finesse mirrors while permitting both three-dimensional positioning of the cavity mode and free-space confocal imaging. The design relies on two cascaded vibration isolation stages connected by leaf springs that decouple axial and lateral motion, and incorporates tuned-mass and magnetic damping. Furthermore, we present a technique for quantifying cavity length displacements similar to or larger than the cavity linewidth, allowing in-situ measurement of vibrations with and without active feedback. Our results facilitate operation of a tunable, high-finesse cavity within a closed-cycle cryostat, representing an enabling technology for cavity coupling to a variety of solid-state systems.

physics.ins-det↗

arXiv2021

Cavity quantum electrodynamics with color centers in diamond

Coherent interfaces between optical photons and long-lived matter qubits form a key resource for a broad range of quantum technologies. Cavity quantum electrodynamics (cQED) offers a route to achieve such an interface by enhancing interactions between cavity-confined photons and individual emitters. Over the last two decades, a promising new class of emitters based on defect centers in diamond have emerged, combining long spin coherence times with atom-like optical transitions. More recently, advances in optical resonator technologies have made it feasible to realize cQED in diamond. This article reviews progress towards coupling color centers in diamond to optical resonators, focusing on approaches compatible with quantum networks. We consider the challenges for cQED with solid-state emitters and introduce the relevant properties of diamond defect centers before examining two qualitatively different resonator designs: micron-scale Fabry-Perot cavities and diamond nanophotonic cavities. For each approach, we examine the underlying theory and fabrication, discuss strengths and outstanding challenges, and highlight state-of-the-art experiments.

quant-ph↗

arXiv2020

Cavity-Enhanced Photon Emission from a Single Germanium-Vacancy Center in a Diamond Membrane

The nitrogen-vacancy center in diamond has been explored extensively as a light-matter interface for quantum information applications, however it is limited by low coherent photon emission and spectral instability. Here, we present a promising interface based on an alternate defect with superior optical properties (the germanium-vacancy) coupled to a finesse $\approx11{,}000$ fiber cavity, resulting in a $31^{+11}_{-15}$-fold increase in the spectral density of emission. This work sets the stage for cryogenic experiments, where we predict a measurable increase in the spontaneous emission rate.

quant-ph↗

arXiv2018

Charge State Dynamics During Excitation and Depletion of the Nitrogen Vacancy Center in Diamond

The charge state dynamics of the nitrogen-vacancy (NV) center in diamond play a key role in a wide range of applications, yet remain imperfectly understood. Using single ps-pulses and pulse pairs, we quantitatively investigate the charge dynamics associated with excitation and fluorescence depletion of a single NV center. Our pulsed excitation approach permits significant modeling simplifications, and allows us to extract relative rates of excitation, stimulated emission, ionization, and recombination under 531 nm and 766 nm illumination. By varying the duration between paired pulses, we can also investigate ionization and recombination out of metastable states. Our results are directly applicable to experiments employing stimulated emission-depletion imaging, and can be used to predict optimal operating regimes where excitation and stimulated emission are maximized relative to charge-state-switching processes.

quant-ph↗

arXiv2015

Efficient signal processing for time-resolved fluorescence detection of nitrogen-vacancy spins in diamond

Room-temperature fluorescence detection of the nitrogen-vacancy center electronic spin typically has low signal to noise, requiring long experiments to reveal an averaged signal. Here, we present a simple approach to analysis of time-resolved fluorescence data that permits an improvement in measurement precision through signal processing alone. Applying our technique to experimental data reveals an improvement in signal to noise equivalent to a 14% increase in photon collection efficiency. We further explore the dependence of the signal to noise ratio on excitation power, and analyze our results using a rate equation model. Our results provide a rubric for optimizing fluorescence spin detection, which has direct implications for improving precision of nitrogen-vacancy-based sensors.

quant-ph↗

arXiv2015

A Fabry-Perot Microcavity for Diamond-Based Photonics

Open Fabry-Perot microcavities represent a promising route for achieving a quantum electrodynamics (cavity-QED) platform with diamond-based emitters. In particular, they offer the opportunity to introduce high purity, minimally fabricated material into a tunable, high quality factor optical resonator. Here, we demonstrate a fiber-based microcavity incorporating a thick (> 10 μm) diamond membrane with a finesse of 17,000, corresponding to a quality factor Q ~ $10^6$. Such minimally fabricated, thick samples can contain optically stable emitters similar to those found in bulk diamond. We observe modified microcavity spectra in the presence of the membrane, and develop analytic and numerical models to describe the effect of the membrane on cavity modes, including loss and coupling to higher-order transverse modes. We estimate that a Purcell enhancement of approximately 20 should be possible for emitters within the diamond in this device, and provide evidence that better diamond surface treatments and mirror coatings could increase this value to 200 in a realistic system.

quant-ph↗

arXiv2013

High-fidelity projective readout of a solid-state spin quantum register

Initialization and readout of coupled quantum systems are essential ingredients for the implementation of quantum algorithms. If the state of a multi-qubit register can be read out in a single shot, this enables further key resources such as quantum error correction and deterministic quantum teleportation, as well as direct investigation of quantum correlations (entanglement). While spins in solids are attractive candidates for scalable quantum information processing, thus far single-shot detection has only been achieved for isolated qubits. Here, we demonstrate preparation and measurement of a multi-spin quantum register by implementing resonant optical excitation techniques originally developed in atomic physics. We achieve high-fidelity readout of the electronic spin associated with a single nitrogen-vacancy (NV) centre in diamond at low temperature, and exploit this readout to project up to three nearby nuclear spin qubits onto a well-defined state. Conversely, we can distinguish the state of the nuclear spins in a single shot by mapping it onto and subsequently measuring the electronic spin. Finally, we show compatibility with qubit control by demonstrating initialization, coherent manipulation, and single-shot readout in a single experiment on a two-qubit register, using techniques suitable for extension to larger registers. These results pave the way for the first test of Bell's inequalities on solid-state spins and the implementation of measurement-based quantum information protocols.

quant-ph↗