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Linhua Liu

Publications and source records attributed to Linhua Liu.

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Superballistic transport of thermal photons in confined many-body systems

Ballistic transport, realized when the system size is smaller than the mean free path of energy carriers, is traditionally regarded as the ultimate limit for energy transfer. Here, we predict a superballistic radiative heat transport regime that surpasses this limit in dilute chains of plasmonic nanoparticles confined within cavities. This anomalous regime exhibits superlinear scaling of the effective thermal conductivity (k ~L^1.5) and originates from the amplification of long-range interactions mediated by cavity-guided modes. Our results establish a framework for ultrafast photonic heat transport and open pathways for thermal management, information processing and energy transfer in quantum and nanoscale systems.

physics.optics

Favorable and unfavorable many-body interactions for near-field radiative heat transfer in nanoparticle networks

Near-field radiative heat transfer (NFRHT) in nanoparticle networks is complicated due to the multiple scattering of thermally excited electromagnetic wave (namely, many-body interaction, MBI). The MBI regime is analyzed using the many-body radiative heat transfer theory at the particle scale for networks of a few nanoparticles. Effect of MBI on radiative heat diffusion in networks of a large number of nanoparticles is analyzed using the normal-diffusion radiative heat transfer theory at the continuum scale. An influencing factor $\psi$ is defined to numerically figure out the border of the different many-body interaction regimes. The whole space near the two nanoparticles can be divided into four zones, non-MBI zone, enhancement zone, inhibition zone and forbidden zone, respectively. Enhancement zone is relatively smaller than the inhibition zone, so many particles can lie in the inhibiting zone that the inhibition effect of many-body interaction on NFRHT in nanoparticle networks is common in literature. Analysis on the radiative thermal energy confirms that multiple scattering caused by the inserted scatter accounts for the enhancement and inhibition of NFRHT. By arranging the nanoparticle network in aspect of structures and optical properties, the MBI can be used to modulate radiative heat diffusion characterized by the radiative effective thermal conductivity ($k_{\rm eff}$) over a wide range, from inhibition (over 55% reduction) to amplification (30 times of magnitude). To achieve a notable MBI, it is necessary to introduce particles that have resonances well-matched with those of the particles of interest, irrespective of their match with the Planckian window. This work may help for the understanding of the thermal radiation in nanoparticle networks.

physics.app-ph

Many-body interaction on near-field radiative heat transfer between two nanoparticles caused by proximate particle ensembles

Near-field radiative heat transfer (NFRHT) has received growing attention because of its high intensity far beyond the Planck's black-body limit. Insertion of a third object in proximity of the two articles can significantly influence and manipulate its NFRHT. However, for the system composed of many particles, the effect of many-body interaction (MBI) on NFRHT between arbitrary two particles is still not well understood. In this work, the MBI is studied for two particles with three typical proximate ensembles: particle chain, plane and grating. With the increasing of proximate particle size, the MBI on NFRHT will experience a radical change from inhibition to enhancement. The polarizability of the proximate particle increases with particle radius, which enhances the interaction between the proximate particles and the main particle, and then results in enhancement of NFRHT between the main particles. When twisting the proximate particle ensemble, the proximate MBI accounts for a smooth and non-oscillated twisting angle dependence of NFRHT, different from the oscillation phenomenon of NFRHT for particle gratings. This work deepens the understanding of NFRHT in dense particulate systems.

physics.optics

Extinction by plasmonic nanoparticles in dispersive and dissipative media

Extinction of small metallic spheres has been well understood through the classical Mie theory when the host medium is dispersive and transparent. However, the role of host dissipation on the particulate extinction remains a competition between the enhancing and reducing effects on the localized surface plasmonic resonance (LSPR). Here, using a generalized Mie theory, we elaborate on the specific influence mechanisms of host dissipation on the extinction efficiency factors of a plasmonic nanosphere. To this end, we isolate the dissipative effects by comparing the dispersive and dissipative host with its transparent counterpart. As a result, we identify the damping effects of host dissipation on the LSPR including the resonance widening and amplitude reducing. The resonance positions are shifted by host dissipation, which cannot be predicted by the classical Fr\"ohlich condition. Finally, we demonstrate that a wide-band extinction enhancement due to host dissipation can be realized away from the positions of LSPR.

physics.optics

Photothermal behavior for two-dimensional nanoparticle ensembles: Multiple scattering and thermal accumulation effects

Light-assisted micro-nanoscale temperature control in complex nanoparticle network attracts lots of research interests. Many efforts have been put on the optical properties of the nanoparticle networks and only a few investigations on its light-induced thermal behavior was reported. We consider two-dimensional (2D) square-lattice nanoparticle ensemble made of typical metal Ag with a radius of 5 nm. The effect of complex optical coupling and thermal accumulation on the light-induced thermal behavior in plasmonic resonance frequency (around 383 nm) is analyzed by means of the Green\textquotesingle s function approach. Regime borders of both optical coupling and thermal accumulation effects on the photothermal behavior of 2D square-lattice nanoparticle ensemble are figured out clearly and quantitatively. A dimensionless parameter $φ$ is defined as the ratio of full temperature increase to that without considering the optical coupling or thermal accumulation to quantify the optical coupling and thermal accumulation effects on photothermal behavior. The more compact the nanoparticle ensemble is, the stronger the optical coupling on thermal behavior is. When the lattice spacing increases to tens of nanoparticle radius, the optical coupling becomes insignificant. When $φ\approx 1$ (lattice spacing increases to hundreds of nanoparticle radius), the thermal accumulation effects are weak and can be neglected safely. The polarization-dependent distribution of temperature increase of nanoparticles is observed only in the compact nanoparticle ensemble, while for dilute ensemble, such polarization-dependent temperature increase distribution can not be observed anymore. This work may help for the understanding of the light-induced thermal transport in the 2D particle ensemble.

physics.optics

Photonic p-n Junction: An Ideal Near-Field Heat Flux Modulator

Using a pair of p- and n-type semiconductors separated by a nanoscale vacuum gap, we introduce an optoelectronics element prototype, "photonic p-n junction", as an analogue of the electronic p-n junction, which is demonstrated to serve as an ideal near-field heat flux modulator. The high modulation performance relies on the switch among three fundamental photon-carrier interaction modes (i.e., surface plasmon polaritons, symmetric depleted internal plasmon polaritons and symmetric accumulated surface plasmon polaritons) caused by the changes in hole and electron densities near the surfaces under a tunable bias. This prototype offers new thoughts not only for contactless thermal management at nanoscale but also for design of optoelectronics devices processing information carried by plasmon polaritons.

physics.optics

Near-field radiation assisted smart skin for spacecraft thermal control

Thermal control is of critical importance for normal operation of spacecraft. Given thermal radiation is the only means of heat dissipation in space, an efficient thermal control approach for spacecraft is to coat the radiator with a tunable-emittance "skin" that can tune its heat dissipation according to various thermal conditions. The existing schemes solely relying on far-field thermal radiation, which are based on mechanical, electrochromic or thermochromic working principles, are difficult to combine the advantages of all-solid-state structure, actively and accurate tuning, and large tuning range of heat flux. In this work, we propose a near-field radiation assisted (NFRA) smart skin for thermal control which can tune the heat rejection accurately and in a large range. It contains a metal-insulator-semiconductor (MIS) structure, where the carrier distribution in the semiconductor layer can be electrically altered. In this way, the near-field heat flux, and ultimately the skin emission power expressed using effective emittance, can be controlled as a function of the applied voltage. The variation range of the effective emittance can exceed 0.7 when adjusting the applied voltage from -10 V to 100 V with our preliminary design. This work opens a new way of smart skin design for active spacecraft thermal control.

physics.app-ph

Normal heat diffusion in many-body system via thermal photons

A normal-diffusion theory for heat transfer in many-body systems via carriers of thermal photons is developed. The thermal conductivity tensor is rigorously derived from fluctuational electrodynamics as a coefficient of diffusion term for the first time. In addition, a convection-like heat transfer behavior is revealed in systems of asymmetric distribution of particles, indicating violation of Fourier's law for such system. Considering the central role of thermal conductivity in heat transfer, this work paves a way for understanding, analysis and manipulation of heat transfer in nanoparticle system via thermal photons with many-body interactions.

physics.app-ph

Many-body effective thermal conductivity in phase-change nanoparticle chains due to near-field radiative heat transfer

In dense systems composed of numerous nanoparticles, direct simulations of near-field radiative heat transfer (NFRHT) require considerable computational resources. NFRHT for the simple one-dimensional nanoparticle chains embedded in a non-absorbing host medium is investigated from the point of view of the continuum by means of an approach combining the many-body radiative heat transfer theory and the Fourier law. Effects of the phase change of the insulator-metal transition material (VO$_2$), the complex many-body interaction (MBI) and the host medium relative permittivity on the characteristic effective thermal conductivity (ETC) are analyzed. The ETC for VO$_2$ nanoparticle chains below the transition temperature can be as high as 50 times of that above the transition temperature due to the phase change effect. The strong coupling in the insulator-phase VO$_2$ nanoparticle chain accounts for its high ETC as compared to the low ETC for the chain at the metallic phase, where there is a mismatch between the characteristic thermal frequency and resonance frequency. The strong MBI is in favor of the ETC. For SiC nanoparticle chains, the MBI even can double the ETC as compared to those without considering the MBI effect. For the dense chains, a strong MBI enhances the ETC due to the strong inter-particles couplings. When the chains go more and more dilute, the MBI can be neglected safely due to negligible couplings. The host medium relative permittivity significantly affects the inter-particles couplings, which accounts for the permittivity-dependent ETC for the VO$_2$ nanoparticle chains.

cond-mat.mes-hall

Radiative heat transfer and radiative thermal energy for 2D nanoparticle ensembles

Radiative heat transfer (RHT) and radiative thermal energy (RTE) for 2D nanoparticle ensembles are investigated in the framework of many-body radiative heat transfer theory. We consider nanoparticles made of different materials: metals (Ag), polar dielectrics (SiC) or insulator-metallic phase-change materials (VO$_2$). We start by investigating the RHT between two parallel 2D finite-size square-lattice nanoparticle ensembles, with particular attention to many-body interactions (MBI) effects. We systematically analyze the different physical regimes characterizing the RHT. When $p\ll \lambda_T$, a multiple scattering of the electromagnetic field inside the systems gives rise to a MBI regime. MBI effects manifest themselves in different ways, depending on $d$: (a) if $d > \lambda_T$, due to the pure intra-ensemble MBI inside each 2D ensemble, the total heat conductance is less affected, and the thermal conductance spectrum manifests a single peak which is nonetheless shifted with respect to the one typical of two isolated nanoparticles. (b) if $d < \lambda_T$, there is a strong simultaneous intra- and inter-ensemble MBI. In this regime there is a direct quantitative effect on the heat conductance, in addition to a qualitative effect on the thermal conductance spectrum which now manifests a new second peak. As for the RTE, to correctly describe the radiation emitted by metallic nanoparticles, we derive an expression of the Poynting vector including also magnetic contribution, in addition to the electric one. By analyzing both periodic and non-periodic ensembles, we show that the RTE emitted by a single 2D nanoparticle ensemble is sensitive to the particle distribution. As instance, we see that the RTE emitted by 2D concentric ring-configuration ensemble has an inhibition feature near the center of the ensemble.

cond-mat.mes-hall

Continuum approach based on radiation distribution function for radiative heat transfer in densely packed particulate system

The study of radiative heat transfer in particulate system is usually based on radiative transfer equation (RTE) with effective radiative properties. However, for non-random, densely and regularly packed particulate systems, the applicability of RTE is questionable due to dependent scattering and weak randomness of particle arrangement. In this paper, a new continuum approach that does not explicitly rely on the RTE is proposed for radiative heat transfer in the densely packed particulate system. The new approach is based on the generalization of the concept of radiation distribution factor (RD) at discrete scale (or particle scale) to radiation distribution function (RDF) at continuum scale. The derived governing equation is in integral form, with RDF as the continuum scale physical parameter that characterize the radiative transfer properties of the system. The characteristics of the RDF for different particulate system (randomly or regularly packed) are studied. The RDF in regularly distributed particulate system is shown to be anisotropic. The continuum approach is verified by using heat transfer simulation at the particle scale, and demonstrated to have excellent performance in predicting the temperature distribution in dense particulate system. This work provides an alternative continuum theory, which will help the analysis and understanding of radiative heat transfer in densely packed media.

physics.app-ph

Near-field radiative heat transfer between rough surfaces modeled using effective media with gradient distribution of dielectric function

Near-field radiative heat transfer (NFRHT) between rough surfaces, due to its widespread presence in engineering practice of near-field energy utilization, requires indepth studies, especially from the perspective of physical mechanism. In this paper, an effective multilayer model is built to approach the NFRHT between random rough surfaces of silicon carbide (SiC). Using the effective medium theory (EMT), the effective dielectric function of each layer is obtained, which forms a gradient distribution of dielectric function along the depth of the medium. The influence of the effective dielectric function on surface phonon polaritons (SPhPs) is analyzed, showing that the effective layers with small filling fraction of SiC feature lower SPhP resonance frequencies than SiC bulk. The coupling of SPhPs from the gradient distribution of dielectric function produces new surface modes that dominates the NFRHT. Investigation on the effect of root mean square height (RMS height, σ) reveals that the peaks of local density of states (LDOS) and spectral heat flux are red-shifted as σ increases, while the spectral heat flux below the peak frequency gets larger. This can be attributed to the coupling of SPhPs inside the rough layer. We also found the total net heat flux between rough surfaces separated by an average distance exceeds that between smooth plates and increases with increasing σ, which offer a new way to enhance NFRHT. This work provides a reference for the simulation and understanding of the NFRHT between rough surfaces.

physics.app-ph

Radiative heat transfer between metallic nanoparticle clusters in both near field and far field

Micro-nanoparticle systems have wide applications in thermal science and technology. In dense particulate system, the particle separation distance may be less than the characteristic thermal wavelength and near field effect will be significant and become a key factor to influence thermal radiation transfer in the system. In this study, radiative heat transfer (RHT) between two metallic nanoparticles clusters are explored using many-body radiative heat transfer theory implemented with the coupled electric and magnetic dipole (CEMD) approach, which effectively takes into account the contribution of magnetic polarization of metallic nanoparticles on heat exchange. As the focus, the effects of magnetic polarization and many-body interaction (MBI) on RHT were analyzed. The effects of fractal dimension and relative orientation of the clusters were also analyzed. Results show that the contribution of magnetically polarized eddy-current Joule dissipation dominates the RHT between Ag nanoparticle clusters. If only electric polarization (EP approach) is considered, the heat conductance will be underestimated as compared with the CEMD approach in both near field and far field regime. The effect of MBI on the RHT between Ag nanoparticle clusters is unobvious at room temperature, which is quite different from the SiC nanoparticle clusters. For the latter, MBI tends to suppress RHT significantly. The relative orientation has remarkable effect on radiative heat flux for clusters with lacy structure when the separation distance is in the near field. While for the separation distance in far field, both the relative orientation and the fractal dimension has a weak influence on radiative heat flux. This work will help the understanding of thermal transport in dense particulate system.

physics.app-ph

Long-distance near-field energy transport via propagating surface waves

Near-field radiative heat transfer (RHT) between two bodies can significantly exceed the far-field limit set by Planck's law due to the evanescent wave tunneling, which typically can only occur when the two bodies are separated at subwavelength distances. We show that the RHT between two SiC nanoparticles with separation distances much larger than the thermal wavelength can still exceed the far-field limit when the particles are located within a subwavelength distance away from a SiC substrate. In this configuration, the localized surface phonon polariton (SPhP) of the particles couples to the propagating SPhP of the substrate which then provides a new channel for the near-field energy transport and enhances the RHT by orders of magnitude at large distances. The enhancement is also demonstrated to appear in a chain of closely spaced SiC nanoparticles located in the near field of a SiC substrate. The findings provide a new way for the long-distance transport of near-field energy.

physics.app-ph

Radiative heat transfer in many-body systems: coupled electric and magnetic dipole approach

The many-body radiative heat transfer theory [P. Ben-Abdallah, S.-A. Biehs, and K. Joulain, Phys. Rev. Lett. 107, 114301 (2011)] only considered the contribution from the electric dipole moment. For metal particles, however, the magnetic dipole moment due to eddy current plays an important role, which can further couple with the electric dipole moment to introduce crossed terms. In this work, we develop coupled electric and magnetic dipole (CEMD) approach for the radiative heat transfer in a collection of objects in mutual interaction. Due to the coupled electric and magnetic interactions, four terms, namely the electric-electric, the electric-magnetic, the magnetic-electric and the magnetic-magnetic terms, contribute to the radiative heat flux and the local energy density. The CEMD is applied to study the radiative heat transfer between various dimers of nanoparticles. It is found that each of the four terms can dominate the radiative heat transfer depending on the position and composition of particles. Moreover, near-field many-body interactions are studied by CEMD considering both dielectric and metallic nanoparticles. The near-field radiative heat flux and local energy density can be greatly increased when the particles are in coupled resonances. Surface plasmon polariton and surface phonon polariton can be coupled to enhance the radiative heat flux.

cond-mat.other