arXiv subjects

Lino M. C. Pereira

Publications and source records attributed to Lino M. C. Pereira.

10 recordsLinked to original sources

arXiv2026

Disorder-driven symmetry suppression by van der Waals planar defects in a magnetic topological insulator

Magnetic topological insulators offer a platform to control electronic topology through magnetic order, yet reliable routes to tune their properties remain limited. Here, we show that ion irradiation allows to modify the magnetic properties and the anomalous Hall response of the van der Waals magnetic topological insulator MnBi$_2$Te$_4$. Using noble gas ion beams, intrinsic defects are introduced via collision cascades without chemical doping. We identify two distinct regimes. At low fluence, cation antisite disorder leads to a near-complete redistribution of Bi over cation sites while preserving long-range crystallographic order, accompanied by a transition from $p$-type to $n$-type transport. At high fluence, cation-anion intermixing drives the formation of a previously unreported layer-disordered phase characterized by a high density of van der Waals-specific planar defects, including swapped bilayers. Despite significant structural disorder, the system retains partial periodic order up to high displacement levels. Magnetometry and X-ray spectroscopy show that the Mn high-spin state and intralayer antiferromagnetic interactions likely persist, while macroscopic magnetic anisotropy is strongly reduced. At the same time, the magnitude of the anomalous Hall conductivity is reduced by an order of magnitude, far exceeding the change in magnetization, and its sign is modified. The observations are consistent with a suppression of the Berry curvature of the occupied states. These results establish ion irradiation as a means to tune anomalous Hall conductivity in topological insulators through defect engineering and reveal a disorder-driven approach to control symmetry and electronic structure in van der Waals magnetic materials.

cond-mat.mtrl-sci↗

arXiv2026

Spectral Fingerprints of Resonant Defect Scattering by Substitutional Mn in Graphene

Using substitutional Mn in graphene/Cu(111) as a model point defect, we combine scanning tunneling microscopy (STM) and angle-resolved photoemission spectroscopy (ARPES) to test the predicted fingerprints of resonant scattering. As the Mn concentration increases to 0.44%, the Dirac point stretching reaches 0.52 eV, while momentum broadening remains energy independent. These spectral fingerprints classify substitutional Mn as a strong resonant scatterer and establish the combination of STM and ARPES as a powerful approach to identify and characterize resonant disorder in graphene.

cond-mat.mes-hall↗

arXiv2026

Radiotracer photoluminescence for element-specific identification of color centers

We report on the implementation of a radiotracer photoluminescence spectroscopy setup at the ISOLDE radioactive ion beam facility at CERN, enabling element-specific identification of optically active defects in solids. The method combines radioactive ion implantation with optical spectroscopy, allowing the temporal evolution of photoluminescence signals to be correlated directly with nuclear decay. The setup is currently optimized for color centers in diamond and related wide-bandgap materials and enables room-temperature measurements. The system consists of an optical microscope coupled to a fiber-fed Czerny-Turner spectrometer with a liquid-nitrogen-cooled CCD detector, providing the stability required for long-duration measurements. As a proof-of-principle, radioactive $^{75}$Ga was implanted into diamond as a precursor to produce $^{75}$Ge impurities. The photoluminescence band extending from 600 nm, corresponding to the well-known GeV$^{-}$ center, exhibits an exponential decay with a half-life of $82.3^{+2.5}_{-2.3} \mathrm{min}$, in agreement with the known $β^{-}$ decay half-life of $^{75}$Ge of $82.78(4) \mathrm{min}$. This establishes a direct and unambiguous correlation between the observed spectral feature and its germanium origin. These results demonstrate the capability of the setup to perform element-specific optical spectroscopy and extend radiotracer methods to color centers in wide-bandgap materials, taking advantage of the uniquely broad range of radioactive isotopes available at ISOLDE.

physics.ins-det↗

arXiv2026

Toward nanophotonic platforms for solid-state $^{229}$Th nuclear clocks

While the $^{229}$Th nuclear isomer has recently been observed and laser-excited, converting optical nuclear manipulation into a chip-scale solid-state frequency standard remains an open challenge. Here, we present a nanophotonic platform to realize an all-solid-state nuclear clock based on the low-energy isomeric transition of $^{229}$Th embedded in high-$Q$ fluoride photonic resonators. By coupling ensembles of thorium nuclei to confined optical modes, we show that resonant field build-up in the cavity can substantially enhance the nuclear excitation rate, enabling optical interrogation at practical laser intensities. We model the nuclei-photon interaction dynamics and outline a technological roadmap toward addressing this challenge, including resonator fabrication in fluoride crystals, thorium implantation, nuclear excitation with integrated lasers, and on-chip detection of vacuum-ultraviolet photons. As an initial proof of concept, we implant a crystalline fluoride whispering-gallery-mode resonator with $^{229}$Th and assess the impact of implantation-induced damage on resonator performance. Our platform leverages recent advances in materials integration and nanophotonics to chart a realistic route toward compact and scalable nuclear frequency standards.

physics.optics↗

arXiv2023

Induced superconducting correlations in the quantum anomalous Hall insulator

Inducing Cooper pairing in a thin ferromagnetic topological insulator in the quantum anomalous Hall state (called quantum anomalous Hall insulator, QAHI) is a promising way to realize topological superconductivity with associated chiral Majorana edge states. However, finding evidence of superconducting proximity effect in a QAHI has proven to be a considerable challenge due to inherent experimental difficulties. Here we report the observation of crossed Andreev reflection (CAR) across a narrow superconducting Nb electrode contacting the chiral edge state of a QAHI, evinced by a negative nonlocal voltage measured downstream from the grounded Nb electrode. This is an unambiguous signature of induced superconducting pair correlation in the chiral edge state. Our theoretical analysis demonstrates that CAR processes of the chiral edge are not strongly dependent on the nature of the superconductivity that mediates them. Nevertheless, the characteristic length of the CAR process is found to be much longer than the superconducting correlation length in Nb, which suggests that the CAR is in fact mediated by superconductivity induced on the QAHI surface. The approach and results presented here provide a foundation for future studies of topological superconductivity and Majorana physics, as well as for the search for non-Abelian zero modes.

cond-mat.mes-hall↗

arXiv2022

Observation of the radiative decay of the ${}^{229}\mathrm{Th}$ nuclear clock isomer

The nucleus of the radioisotope thorium-229 (${}^{229}$Th) features an isomer with an exceptionally low excitation energy that enables direct laser manipulation of nuclear states. For this reason, it is a leading candidate for use in next-generation optical clocks. This nuclear clock will be a unique tool, amongst others, for tests of fundamental physics. While first indirect experimental evidence for the existence of such an extraordinary nuclear state is significantly older, the proof of existence has been delivered only recently by observing the isomer's electron conversion decay and its hyperfine structure in a laser spectroscopy study, revealing information on the isomer's excitation energy, nuclear spin and electromagnetic moments. Further studies reported the electron conversion lifetime and refined the isomer's energy. In spite of recent progress, the isomer's radiative decay, a key ingredient for the development of a nuclear clock, remained unobserved. In this Letter, we report the detection of the radiative decay of this low-energy isomer in thorium-229 (${}^{229\mathrm{m}}$Th). By performing vacuum-ultraviolet spectroscopy of ${}^{229\mathrm{m}}$Th incorporated into large-bandgap CaF${}_2$ and MgF${}_2$ crystals at the ISOLDE facility at CERN, the photon vacuum wavelength of the isomer's decay is measured as 148.71(42) nm, corresponding to an excitation energy of 8.338(24) eV. This value is in agreement with recent measurements, and decreases the uncertainty by a factor of seven. The half-life of ${}^{229\mathrm{m}}$Th embedded in MgF${}_2$ is determined to be 670(102) s. The observation of the radiative decay in a large-bandgap crystal has important consequences for the design of a future nuclear clock and the improved uncertainty of the energy eases the search for direct laser excitation of the atomic nucleus.

nucl-ex↗

arXiv2022

Magnesium-vacancy optical centers in diamond

We provide the first systematic characterization of the structural and photoluminescence properties of optically active defect centers fabricated upon implantation of 30-100 keV Mg+ ions in artificial diamond. The structural configurations of Mg-related defects were studied by the emission channeling technique for 27Mg implantations performed both at room-temperature and 800 °C, which allowed the identification of a major fraction of Mg atoms (~30-42%) in sites which are compatible with the split-vacancy structure of the MgV complex. A smaller fraction of Mg atoms (~13-17%) was found on substitutional sites. The photoluminescence emission was investigated both at the ensemble and individual defect level in a temperature range comprised between 5 K and 300 K, offering a detailed picture of the MgV-related emission properties and revealing the occurrence of previously unreported spectral features. The optical excitability of the MgV center was also studied as a function of the optical excitation wavelength enabling to identify the optimal conditions for photostable and intense emission. The results are discussed in the context of the preliminary experimental data and the theoretical models available in the literature, with appealing perspectives for the utilization of the tunable properties of the MgV center for quantum information processing applications.

cond-mat.mtrl-sci↗

arXiv2021

Current-induced breakdown of the quantum anomalous Hall effect

The quantum anomalous Hall effect (QAHE) realizes dissipationless longitudinal resistivity and quantized Hall resistance without the need of an external magnetic field. However, when reducing the device dimensions or increasing the current density, an abrupt breakdown of the dissipationless state occurs with a relatively small critical current, limiting the applications of the QAHE. We investigate the mechanism of this breakdown by studying multi-terminal devices and identified that the electric field created between opposing chiral edge states lies at the origin. We propose that electric-field-driven percolation of two-dimensional charge puddles in the gapped surface states of compensated topological-insulator films is the most likely cause of the breakdown.

cond-mat.mes-hall↗

arXiv2020

Structural and electronic properties of the pure and stable elemental 3D topological Dirac semimetal $α$-Sn

In-plane compressively strained $α$-Sn films have been theoretically predicted and experimentally proven to possess non-trivial electronic states of a 3D topological Dirac semimetal. The robustness of these states typically strongly depends on purity, homogeneity and stability of the grown material itself. By developing a reliable fabrication process, we were able to grow pure strained $α$-Sn films on InSb(100), without heating of the substrate during growth, nor using any dopants. The $α$-Sn films were grown by molecular beam epitaxy, followed by experimental verification of the achieved chemical purity and structural properties of the film's surface. Local insight into the surface morphology was provided by scanning tunneling microscopy. We detected the existence of compressive strain using Mössbauer spectroscopy and we observed a remarkable robustness of the grown samples against ambient conditions. The topological character of the samples was confirmed by angle-resolved photoemission spectroscopy, revealing the Dirac cone of the topological surface state. Scanning tunneling spectroscopy, moreover, allowed obtaining an improved insight into the electronic structure of the 3D topological Dirac semimetal $α$-Sn above the Fermi level.

cond-mat.mtrl-sci↗

arXiv2020

Probing interacting two-level systems with rare-earth ions

Two-level systems (TLS) in amorphous materials limit coherence times of a number of solid-state quantum devices. Interactions between TLS become prominent below 100 mK, but the coupling mechanism and statistical properties are still unclear. Here we determine the homogeneous linewidth of ytterbium ions (Yb$ ^{3+} $) in silica glass at 10-80 mK by using photon echo techniques as a probe of TLS. First, the homogeneous linewidth can be reduced by applying a magnetic field of 0.3 T. This effect is due to reduced magnetic interactions between adjacent Yb$ ^{3+} $. Secondly, we observe saturation of the linewidth below 50 mK to a level of approximately 30 kHz, which is much larger than the lifetime-limited value of 0.2 kHz. This saturation behavior is in conflict with the coupling to independent TLS. We show that this effect can be explained by coherently coupled TLS.

cond-mat.dis-nn↗