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Linqiang Hua

Publications and source records attributed to Linqiang Hua.

3 recordsLinked to original sources

Generation and spectroscopic characterization of continuous-wave 148.4-nm light in strontium tetraborate

Continuous-wave (CW) radiation at 148.4~nm is required to drive the $^{229}$Th isomeric transition of a solid-state nuclear clock, and frequency doubling of 296.8-nm light is its most direct source. We generate CW 148.4-nm light by random quasi-phase matching in strontium tetraborate and characterize it with a compact CaF$_2$ prism spectrometer, which reaches picowatt sensitivity without filters or a grating and reads the wavelength from the rotation angle of a solar-blind photomultiplier. The observed harmonic profile has an angular FWHM of 0.36$^{\circ}$, corresponding to a convolution-limited spectral width of about 0.6 nm rather than the intrinsic linewidth. The directly estimated output is 1.9 nW at room temperature; scaling the measured temperature dependence gives an inferred 4.8 nW at the best observed temperature. The conversion varies by an order of magnitude across the crystal and is strongly structured in temperature: between 30 $^{\circ}$C and 50 $^{\circ}$C it shows several maxima only a few degrees apart, so a small excursion moves the output from a maximum to a minimum. These measurements provide valuable information on the realization and characterization of a high-quality 148.4-nm light source, and pave the way for the future development of high-performance nuclear optical clocks.

cond-mat.mtrl-sci↗

Extreme Ultraviolet Radiation With Coherence Time Greater Than 1 s

Many atomic and molecular systems of fundamental interest possess resonance frequencies in the extreme ultraviolet (XUV) where laser technology is limited and radiation sources have traditionally lacked long-term phase coherence. Recent breakthroughs in XUV frequency comb technology have demonstrated spectroscopy with unprecedented resolution at the megahertz level, but even higher resolutions are desired for future applications in precision measurement. By characterizing heterodyne beats between two XUV comb sources, we demonstrate the capability for sub-hertz spectral resolution. This corresponds to coherence times >1 s at photon energies up to 20 eV, more than six orders of magnitude longer than previously reported. This work establishes the ability of creating highly phase-stable radiation in the XUV with performance rivaling that of visible light. Furthermore, by direct sampling of the phase of the XUV light originating from high-harmonic generation, we demonstrate precise measurements of attosecond strong-field physics.

physics.atom-ph↗

Cavity-enhanced field-free molecular alignment at a high repetition rate

Extreme ultraviolet frequency combs are a versatile tool with applications including precision measurement, strong-field physics, and solid-state physics. Here we report on an application of extreme ultraviolet frequency combs and their driving lasers for studying strong-field effects in molecular systems. We perform field-free molecular alignment and high-order harmonic generation with aligned molecules in a gas jet at a repetition rate of 154 MHz using a high-powered optical frequency comb inside a femtosecond enhancement cavity. The cavity-enhanced system provides a means to reach suitable intensities to study field-free molecular alignment and enhance the observable effects of the molecule-field interaction. We observe modulations of the driving field, arising from the nature of impulsive stimulated Raman scattering responsible for coherent molecular rotations. We foresee the impact of this work on the study of molecule-based strong-field physics, with improved precision and a more fundamental understanding of the interaction effects on both the field and molecules.

physics.optics↗