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Lisa M. DeBeer-Schmitt

Publications and source records attributed to Lisa M. DeBeer-Schmitt.

3 recordsLinked to original sources

A Fermi Surface Driven Spiral Spin Liquid

EuAg$_4$Sb$_2$ is a model material to study the interplay of electronic and spin texture degrees of freedom, exhibiting numerous multi-$q$ magnetic textures coupled with the electronic properties. It is generally understood that some combination of conduction-electron mediated interactions, frustration, and higher order interactions are responsible for complex incommensurate spin textures in centrosymmetric lanthanide materials. Here, we refine an effective model of the magnetic interactions in EuAg$_4$Sb$_2$ through measurements of diffuse magnetic neutron scattering above the ordering temperature. These diffuse measurements reveal a ring of fluctuating spin modulations that reflects a manifold of nearly degenerate propagation vectors known as a spiral spin liquid (SSL). We further identify that this approximate $U$(1) symmetric SSL emerges from magnetic interactions mediated by a quasi-2D hole pocket and exhibits critical scaling of the spatial correlations. Further, Monte Carlo simulations reveal excellent agreement with experiment and provide a comprehensive understanding of the phase diagram. This study emphasizes the connection between the rich spin textures in this material, the electronic structure, and spin liquidity$\unicode{x2014}$uncovering new insights into design principles for nano-scale spin texture materials with advantageous intertwined electronic, magnetic, and topological properties, and new mechanisms for generating the physics of spiral spin liquids.

cond-mat.str-el↗

Spin density wave and van Hove singularity in the kagome metal CeTi3Bi4

Kagome metals with van Hove singularities near the Fermi level can host intriguing quantum phenomena such as chiral loop currents, electronic nematicity, and unconventional superconductivity. However, to our best knowledge, unconventional magnetic states driven by van Hove singularities--like spin-density waves--have not been observed experimentally in kagome metals. Here, we report the magnetic and electronic structure of the layered kagome metal CeTi3Bi4, where Ti kagome electronic structure interacts with a magnetic sublattice of Ce3+ Jeff = 1/2 moments. Neutron diffraction reveals an incommensurate spin-density wave ground state of the Ce3+ moments, coexisting with commensurate antiferromagnetic order across most of the temperature-field phase diagram. The commensurate component is preferentially suppressed by thermal fluctuations and magnetic field, yielding a rich phase diagram involving an intermediate single-Q spin-density wave phase. First-principles calculations and angle-resolved photoemission spectroscopy identify van Hove singularities near the Fermi level, with the observed magnetic propagation vectors connecting their high density of states, strongly suggesting a van Hove singularity-assisted spin-density wave. These findings establish kagome metals LnTi3Bi4 as a model platform where the characteristic electronic structure of the kagome lattice plays a pivotal role in magnetic order.

cond-mat.str-el↗

Conventional Superconductivity in the Doped Kagome Superconductor Cs(V0.86Ta0.14)3Sb5 from Vortex Lattice Studies

A hallmark of unconventional superconductors is their complex electronic phase diagrams where "intertwined orders" of charge-spin-lattice degrees of freedom compete and coexist as in copper oxides and iron pnictides. While the electronic phase diagram of kagome lattice superconductor such as CsV3Sb5 also exhibits complex behavior involving coexisting and competing charge density wave order and superconductivity, much is unclear about the microscopic origin of superconductivity. Here, we study the vortex lattice (VL) in superconducting state of Cs(V0.86Ta0.14)3Sb5, where the Ta-doping suppresses charge order and enhances superconductivity. Using small-angle neutron scattering, a strictly bulk probe, we show that the VL exhibits a strikingly conventional behavior. This includes a triangular VL with a period consistent with 2e-pairing, a field dependent scattering intensity that follows a London model, and a temperature dependence consistent with a uniform superconducting gap expected for s-wave pairing. These results suggest that optimal bulk superconductivity in Cs(V1-xTax)3Sb5 arises from a conventional Bardeen-Cooper-Schrieffer electron-lattice coupling, different from spin fluctuation mediated unconventional copper and iron based superconductors.

cond-mat.supr-con↗