arXiv subjects

Liuyang Sun

Publications and source records attributed to Liuyang Sun.

5 recordsLinked to original sources

arXiv2021

Twist Angle Dependent Interlayer Exciton Lifetimes in van der Waals Heterostructures

In van der Waals (vdW) heterostructures formed by stacking two monolayers of transition metal dichalcogenides, multiple exciton resonances with highly tunable properties are formed and subject to both vertical and lateral confinement. We investigate how a unique control knob, the twist angle between the two monolayers, can be used to control the exciton dynamics. We observe that the interlayer exciton lifetimes in $\text{MoSe}_{\text{2}}$/$\text{WSe}_{\text{2}}$ twisted bilayers (TBLs) change by one order of magnitude when the twist angle is varied from 1$^\circ$ to 3.5$^\circ$. Using a low-energy continuum model, we theoretically separate two leading mechanisms that influence interlayer exciton radiative lifetimes. The shift to indirect transitions in the momentum space with an increasing twist angle and the energy modulation from the moiré potential both have a significant impact on interlayer exciton lifetimes. We further predict distinct temperature dependence of interlayer exciton lifetimes in TBLs with different twist angles, which is partially validated by experiments. While many recent studies have highlighted how the twist angle in a vdW TBL can be used to engineer the ground states and quantum phases due to many-body interaction, our studies explore its role in controlling the dynamics of optically excited states, thus, expanding the conceptual applications of "twistronics".

cond-mat.mes-hall↗

arXiv2020

Clustering with Fast, Automated and Reproducible assessment applied to longitudinal neural tracking

Across many areas, from neural tracking to database entity resolution, manual assessment of clusters by human experts presents a bottleneck in rapid development of scalable and specialized clustering methods. To solve this problem we develop C-FAR, a novel method for Fast, Automated and Reproducible assessment of multiple hierarchical clustering algorithms simultaneously. Our algorithm takes any number of hierarchical clustering trees as input, then strategically queries pairs for human feedback, and outputs an optimal clustering among those nominated by these trees. While it is applicable to large dataset in any domain that utilizes pairwise comparisons for assessment, our flagship application is the cluster aggregation step in spike-sorting, the task of assigning waveforms (spikes) in recordings to neurons. On simulated data of 96 neurons under adverse conditions, including drifting and 25\% blackout, our algorithm produces near-perfect tracking relative to the ground truth. Our runtime scales linearly in the number of input trees, making it a competitive computational tool. These results indicate that C-FAR is highly suitable as a model selection and assessment tool in clustering tasks.

stat.ML↗

arXiv2019

Moiré Potential Impedes Interlayer Exciton Diffusion in van der Waals Heterostructures

The properties of van der Waals (vdW) heterostructures are drastically altered by a tunable moiré superlattice arising from periodic variations of atomic alignment between the layers. Exciton diffusion represents an important channel of energy transport in semiconducting transition metal dichalcogenides (TMDs). While early studies performed on TMD heterobilayers have suggested that carriers and excitons exhibit long diffusion lengths, a rich variety of scenarios can exist. In a moiré crystal with a large supercell size and deep potential, interlayer excitons may be completely localized. As the moiré period reduces at a larger twist angle, excitons can tunnel between supercells and diffuse over a longer lifetime. The diffusion length should be the longest in commensurate heterostructures where the moiré superlattice is completely absent. In this study, we experimentally demonstrate that the moiré potential impedes interlayer exciton diffusion by comparing a number of WSe2/MoSe2 heterostructures prepared with chemical vapor deposition and mechanical stacking with accurately controlled twist angles. Our results provide critical guidance to developing 'twistronic' devices that explore the moiré superlattice to engineer material properties.

cond-mat.mes-hall↗

arXiv2018

Routing Valley Excitons in a Monolayer MoS2 with a Metasurface

Excitons in monolayer transition metal dichalcogenides (TMDs) are formed at K and K' points at the boundary of the Brillouin zone. They acquire a valley degree of freedom, which may be used as a complementary platform for information transport and processing. In a different context, metasurfaces consisting of engineered arrays of polarizable inclusions have enabled the manipulation of light in unprecedented ways, and found applications in imaging, optical information processing, and cloaking. Here, we demonstrate that, by coupling a MoS2 monolayer to a suitably designed metasurface consisting of asymmetric grooves, valley polarized excitons can be sorted and spatially separated even at room temperature. Emission from valley excitons is also separated in K-space, i.e., photons with opposite helicity are emitted to different directions. Our work demonstrates that metasurfaces can facilitate valley transport and establish an interface between valleytronic and photonic devices, thus addressing outstanding challenges in the nascent field of valleytronics.

cond-mat.mes-hall↗

arXiv2016

Impact of Grain Boundaries on Efficiency and Stability of Organic-Inorganic Trihalide Perovskites

Organic-inorganic perovskite solar cells have attracted tremendous attention because of their remarkably high power conversion efficiencies (PCEs). To further improve the device performance, however, it is imperative to obtain fundamental understandings on the photo-response and long-term stability down to the microscopic level. Here, we report the first quantitative nanoscale photoconductivity imaging on two methylammonium lead triiodide (MAPbI3) thin films with different PCEs by light-stimulated microwave impedance microscopy. The intrinsic photo-response is largely uniform across grains and grain boundaries, which is direct evidence on the inherently benign nature of microstructures in the perovskite thin films. In contrast, the carrier mobility and lifetime are strongly affected by bulk properties such as the sample crystallinity. As visualized by the spatial evolution of local photoconductivity, the degradation due to water diffusion through the capping layer begins with the disintegration of large grains rather than the nucleation and propagation from grain boundaries. Our findings provide new insights to improve the electro-optical properties of MAPbI3 thin films towards large-scale commercialization.

cond-mat.mtrl-sci↗