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Lora Ramunno

Publications and source records attributed to Lora Ramunno.

At least 19 recordsLinked to original sources

Quantum-dot single photon source performance with off-resonant pulse preparation schemes

The preparation of photonic qubits in the excited state is an integral part of the performance of an on-demand single photon source (SPS). Conventional resonant excitation, an excellent approach to maximize the coherence and indistinguishability of the SPS, often requires polarization filtering to remove the pump signal and isolate the qubit emission, but this results in an inherent 50\% hit to the efficiency. Recent excitation schemes strategically try to exploit pulses that excite the qubit while avoiding spectral overlap to bypass this required filtering. In this work, we compare three such pumping schemes to quantify the important SPS figures-of-merit for off-resonant quantum dot schemes, using: (i) a symmetrically detuned dichromatic pulse, (ii) a notch-filtered adiabatic rapid passage (NARP) pulse, and (iii) a swing up of the quantum emitter population (SUPER) pulse. Due to large instantaneous pulse strengths, the dichromatic pulse suffers from phonon-induced dephasing which can lower the SPS performance by up to 50\%. In contrast, the NARP and SUPER pulses are shielded from phonon coupling to differing degrees but both maintain excellent SPS performance. The SUPER pulse can lose significant efficiency if there is variance in its constituent pulses' amplitude, pulse width, or frequency, while the NARP pulse, though potentially more difficult to realize in experiments, is robust against variance in the pulse preparation.

quant-ph

Plasmonic Electro-Optic Modulators based on Epsilon-Near-Zero Materials: Comparing the Classical Drift-Diffusion and Schr\"odinger-Poisson Coupling Models

We present the design, modeling, and optimization of high-performance plasmonic electro-optic modulators leveraging voltage-gated carrier density in indium tin oxide (ITO) where the gated carrier density is modeled using both the Classical Drift-Diffusion (CDD) and Schr\"odinger-Poisson Coupling (SPC) methods. The latter ensures a more detailed and precise description of carrier distributions under various gate voltages which gains particular significance when applied to an epsilon-near-zero (ENZ) medium such as ITO. Combining the nanoscale confinement and field enhancement enabled by surface plasmon polaritons with the ENZ effect in ITO, modulator designs integrated with silicon waveguides and optimized for operation at {\lambda}0 = 1550 nm achieve a 3-dB bandwidth of 210 GHz, an insertion loss of 3 dB, and an extinction ratio of 5 dB for an overall length of < 4 {\mu}m as predicted by the SPC model. Our results illustrate trade-offs between high-speed modulator operation and low insertion loss, vs. extinction ratio, and the need for precise modelling of carrier distributions in ENZ materials.

physics.optics

Electrically tunable plasmonic metasurface as a matrix of nanoantennas

We report the fabrication and characterization of a plasmonic metasurface comprising electrically contacted sub-wavelength gold dipole nanoantennas, conformally coated by a thin hafnia film, an indium tin oxide layer and a backside mirror, forming metal-oxide-semiconductor (MOS) capacitors, for use as an electrically-tunable reflectarray or metasurface. By voltage biasing the nanoantennas through metallic connectors and leveraging the carrier refraction effect in the MOS capacitors, our measurements demonstrate phase control in reflection over a range of about 30 degrees, with a constant magnitude of reflection coefficient of 0.5, and the absence of secondary lobes. Comprehensive electromagnetic and quantum carrier models of the structure are developed and are in excellent agreement with the measurements. The metasurface holds promise for use as an optical phased array.

physics.optics

Quantum Trajectory Theory and Simulations of Nonlinear Spectra and Multi-Photon Effects in Waveguide-QED Systems with a Time-Delayed Coherent Feedback

We study the nonlinear spectra and multi-photon correlation functions for the waveguide output of a two-level system (including realistic dissipation channels) with a time-delayed coherent feedback. We compute these observables by extending a recent quantum trajectory discretized-waveguide (QTDW) approach which exploits quantum trajectory simulations and a collisional model for the waveguide to tractably simulate the dynamics. Following a description of the general technique, we show how to calculate the first and second order quantum correlation functions, in the presence of a coherent pumping field. With a short delay time, we show how feedback can be used to filter out the central peak of the Mollow triplet or switch the output between bunched and anti-bunched photons by proper choice of round trip phase. We further show how the loop length and round trip phase effects the zero-time second order quantum correlation function, an indicator of bunching or anti-bunching. New resonances introduced through the feedback loop are also shown through their appearance in the incoherent output spectrum from the waveguide. We explain these results in the context of the waiting time distributions of the system output and individual trajectories, uniquely stochastic observables that are easily accessible with the QTDW model.

quant-ph

A Finite-Difference Time-Domain approach for dispersive magnetic media

We extend the Finite-Difference Time-Domain method to treat dispersive magnetic media by incorporating magneto-optical effects through a frequency-dependent permittivity tensor. For benchmarking our method, we consider the light scattering on a magnetic sphere in the Mie regime. We first derive the analytical scattering expressions which predict a peak broadening in the scattering efficiency due to the atomic energy level splitting in the presence of a magnetic field, together with an additional rotated part in the scattered field profile due to the Faraday rotation. We show that our numerical method is able to capture the main scattering features and discuss its limitations and possible improvements in accuracy.

physics.optics

Improving On-Demand Single Photon Source Coherence and Indistinguishability Through a Time-Delayed Coherent Feedback

Single photon sources (SPSs) are an essential resource for many quantum information technologies. We demonstrate how the inclusion of time-delayed coherent feedback in a scalable waveguide system, can significantly improve the two key SPS figures of merit: coherence and indistinguishability. Our feedback protocol is simulated using a quantum trajectory discretized waveguide model which can be used to directly model Hanbury Brown and Twiss (HBT) and Hong-Ou-Mandel (HOM) interferometers. With the proper choice of the round trip phase, the non-Markovian dynamics from the time-delayed feedback improves the indistinguishability of the SPS by up to 57%. We also show how this mechanism suppresses the detrimental effects of off-chip decay and pure dephasing.

quant-ph

Inverse design of optical pulse shapes for time-varying photonics

There has been an explosion of interest in time-varying photonics due to the recent discovery and design of materials and metamaterials with strong, time-varying, nonlinear optical responses. This opens the door to novel optical phenomena including reciprocity breaking, frequency translation, and amplification that can be enhanced by optimizing the light-matter interaction. Although there has been recent interest in applying topology-based inverse design to this problem, we have decided to take a more novel approach. In this article, we will introduce a method for the inverse design of optical pulse shapes to enhance their interaction with time-varying media. We test our objective-first approach by maximizing the transmittance of optical pulses of equal intensity through time-varying media. Indeed, without requiring a change in pulse energy, we demonstrate large, broadband enhancements in the pulse energy transmission through the thin-films, including gain. Our final test includes maximizing pulse transmission through indium tin oxide, a time-varying medium when strongly pumped in its ENZ band. Through this work, we hope to inspire exploration of this new degree of freedom.

physics.optics

Understanding the nonlinear optical response of epsilon near zero materials in the time-domain

The promise of active nanophotonics technology relies on the confinement and control of light at the nanoscale. Confinement via plasmonics, dielectric resonators, and waveguides can be complemented with materials whose optical properties can be controlled using nonlinear effects. Transparent conducting oxides (TCOs) exhibit strong optical nonlinearities in their near zero permittivity spectral region, on the femtosecond time-scale. Harnessing full control over the nonlinear response requires a deeper understanding of the process. To achieve this, we develop a self-consistent time-domain model for the nonlinear optical response of TCOs and implement it into a three-dimensional finite-difference time-domain code. We compare and tune our simulation tools against recently published experimental results for intense laser irradiation of thin indium tin oxide (ITO) films. Finally, by simulating intense laser irradiation of ITO-based plasmonic metasurfaces, we demonstrate the full power of our approach. As expected, we find validating the significant enhancement of the nonlinear response of an ITO-based metasurface over bare ITO thin films. Our work thus enables quantitative nanophotonics design with epsilon-near-zero materials.

physics.optics

On the performance of optical phased array technology for beam steering

Optical phased arrays are of strong interest for beam steering in telecom and LIDAR applications. A phased array ideally requires that the field produced by each element in the array (a pixel) is fully controllable in phase and amplitude (ideally constant). This is needed to realize a phase gradient along a direction in the array, and thus beam steering in that direction. In practice, grating lobes appear if the pixel size is not sub-wavelength, which is an issue for many optical technologies. Furthermore, the phase performance of an optical pixel may not span the required $2π$ phase range, or may not produce a constant amplitude over its phase range. These limitations result in imperfections in the phase gradient, which in turn introduce undesirable secondary lobes. We discuss the effects of non-ideal pixels on beam formation, in a general and technology-agnostic manner. By examining the strength of secondary lobes with respect to the main lobe, we quantify beam steering quality, and make recommendations on the pixel performance required for beam steering within prescribed specifications. By applying appropriate compensation strategies, we show that it is possible to realize high-quality beam steering even when the pixel performance is non-ideal, with intensity of the secondary lobes be two orders of magnitude smaller than the main lobe.

eess.SP

Hyperpolarizability of plasmonic meta-atoms in metasurfaces

Plasmonic metasurfaces are promising as enablers of nanoscale nonlinear optics and flat nonlinear optical components. Nonlinear optical responses of such metasurfaces are determined by the nonlinear optical properties of individual nanostructured plasmonic meta-atoms, which are the building blocks of the metasurfaces. Unfortunately, no simple methods exist to determine the nonlinear coefficients (hyperpolarizabilities) of the meta-atoms hindering designing of nonlinear metasurfaces. Here, we develop the equivalent RLC circuit model of such meta-atoms to estimate their second-order nonlinear optical parameter i.e. the first-order hyperpolarizability in the optical spectral range. In parallel, we extract from second-harmonic generation experiments the spectrum of the 1st-order hyperpolarizabilities of individual meta-atoms consisting of asymmetrically shaped (elongated) plasmonic nanoprisms. Moreover, we verify our results using nonlinear hydrodynamic-FDTD and with calculations based on nonlinear scattering theory. All three approaches: analytical, experimental, and computational, yield results that agree very well. Our empirical RLC model can thus be used as a simple tool to enable efficient design of nonlinear plasmonic metasurfaces.

physics.optics

Mechanism of Laser Induced Filamentation in dielectrics

Laser filamentation in transparent material has a wide range of applications, from three dimensional manufacturing to biological technologies. Various experimental results showed that femtosecond laser pulse filamentation in fused silica strongly depends on laser focusing conditions. However, the physical mechanism governing each regime has not been fully understood. For the first time, single and multiple re-focusing of the laser pulse in interaction of femtosecond laser pulse with fused silica, and consequent single and multiple damage zones (filaments) have been observed in our extensive three-dimensional, high resolution FDTD (finite-difference time-domain) simulations. We show that Kerr nonlinearity plays a crucial role loose laser focusing regime, while it is not an important factor in tight laser focusing regime, where geometrical focusing becomes important. Our simulation results agree well with existing experimental findings. In addition, the improved analytical model prediction gives a reasonable estimate of the shift from Kerr nonlinearity regime to linear geometrical focusing regime.

physics.app-ph

Parallel FDTD modelling of nonlocality in plasmonics

As nanofabrication techniques become more precise, with ever smaller feature sizes, the ability to model nonlocal effects in plasmonics becomes increasingly important. While nonlocal models based on hydrodynamics have been implemented using various computational electromagnetics techniques, the finite-difference time-domain (FDTD) version has remained elusive. Here we present a comprehensive FDTD implementation of nonlocal hydrodynamics, including for parallel computing. As a sub-nanometer step size is required to resolve nonlocal effects, a parallel implementation makes the computational cost of nonlocal FDTD more affordable. We first validate our algorithms for small spherical metallic particles, and find that nonlocality smears out staircasing artifacts at metal surfaces, increasing the accuracy over local models. We find this also for a larger nanostructure with sharp extrusions. The large size of this simulation, where nonlocal effects are clearly present, highlights the importance and impact of a parallel implementation in FDTD.

physics.optics

Optical phased arrays for LIDAR: beam steering via tunable plasmonic metasurfaces

Controlling the phase and amplitude of light emitted by the elements (i.e., pixels) of an optical phased array is of paramount importance to realizing dynamic beam steering for LIDAR applications. In this paper, we propose a plasmonic pixel composed of a metallic nanoantenna covered by a thin oxide layer, and a conductive oxide, e.g., ITO, for use in a reflectarray metasurface. By considering voltage biasing of the nanoantenna via metallic connectors, and exploiting the carrier refraction effect in the metal-oxide-semiconductor capacitor in the accumulation and depletion regions, our simulations predict control of the reflection coefficient phase over a range $>330^{\circ}$ with a nearly constant magnitude. We discuss the physical mechanism underlying the optical response, the effect of the connectors, and propose strategies to maximize the magnitude of the reflection coefficient and to achieve dual-band operation. The suitability of our plasmonic pixel design for beam steering in LIDAR is demonstrated via 3D-FDTD simulations.

physics.optics

Plasmonic colours predicted by deep learning

Picosecond laser pulses have been used as a surface colouring technique for noble metals, where the colours result from plasmonic resonances in the metallic nanoparticles created and redeposited on the surface by ablation and deposition processes. This technology provides two datasets which we use to train artificial neural networks, data from the experiment itself (laser parameters vs. colours) and data from the corresponding numerical simulations (geometric parameters vs. colours). We apply deep learning to predict the colour in both cases. We also propose a method for the solution of the inverse problem -- wherein the geometric parameters and the laser parameters are predicted from colour -- using an iterative multivariable inverse design method.

physics.optics

Origin of third harmonic generation in plasmonic nanoantennas

Plasmonic nanoantennas have been recently proposed to boost nonlinear optical processes. In a metal dipole nanoantenna with a dielectric nanoparticle placed in the gap, the linear field enhancement can be exploited to enhance third harmonic emission. Since both metals and dielectrics exhibit nonlinearity, the nonlinear far-field contains contributions from each, and the impossibility of measuring these contributions separately has led to seemingly contradictory interpretations about the origin of the nonlinear emission. We determine that the origin of the third harmonic from metal-dielectric dipole nanoantennas depends on nanoantenna design, and in particular, the width. We find that the emission from gold dominates in thin threadlike nanoantennas, whereas the emission from the gap material dominates in wider nanoantennas. We also find that monopole nanoantennas perform better than dipoles having the same width, and due to their simplicity should be preferred in many applications.

physics.optics

Topographical coloured plasmonic coins

The use of metal nanostructures for colourization has attracted a great deal of interest with the recent developments in plasmonics. However, the current top-down colourization methods based on plasmonic concepts are tedious and time consuming, and thus unviable for large-scale industrial applications. Here we show a bottom-up approach where, upon picosecond laser exposure, a full colour palette independent of viewing angle can be created on noble metals. We show that colours are related to a single laser processing parameter, the total accumulated fluence, which makes this process suitable for high throughput industrial applications. Statistical image analyses of the laser irradiated surfaces reveal various distributions of nanoparticle sizes which control colour. Quantitative comparisons between experiments and large-scale finite-difference time-domain computations, demonstrate that colours are produced by selective absorption phenomena in heterogeneous nanoclusters. Plasmonic cluster resonances are thus found to play the key role in colour formation.

physics.optics

Effective Transparency in the XUV: A Pump-Probe Test of Atomistic Laser-Cluster Models

The effective transparency of rare-gas clusters, post-interaction with an extreme ultraviolet (XUV) pump pulse, is predicted by using an atomistic hybrid quantum-classical molecular dynamics model. We find there is an intensity range for which an XUV probe pulse has no lasting effect on the average charge state of a cluster after being saturated by an XUV pump pulse: the cluster is effectively transparent to the probe pulse. The intensity range for which this phenomena occurs increases with cluster size, and thus is amenable to experimental verification. We present predictions for clusters at the peak of the laser pulse profile, as well as the expected experimental time-of-flight signal integrated over the laser profile. Since our model uses only atomic photoionization rates, significant experimental deviations from our predictions would provide evidence for modified ionization potentials due to plasma effects.

physics.atm-clus

Augmented collisional ionization via excited states in XUV cluster interactions

The impact of atomic excited states is investigated via a detailed model of laser-cluster interactions, which is applied to rare gas clusters in intense femtosecond pulses in the extreme ultraviolet (XUV). This demonstrates the potential for a two-step ionization process in laser-cluster interactions, with the resulting intermediate excited states allowing for the creation of high charge states and the rapid dissemination of laser pulse energy. The consequences of this excitation mechanism are demonstrated through simulations of recent experiments in argon clusters interacting with XUV radiation, in which this two-step process is shown to play a primary role; this is consistent with our hypothesis that XUV-cluster interactions provide a unique window into the role of excited atomic states due to the relative lack of photoionization and laser field-driven phenomena. Our analysis suggests that atomic excited states may play an important role in interactions of intense radiation with materials in a variety of wavelength regimes, including potential implications for proposed studies of single molecule imaging with intense X-rays.

physics.atom-ph